Search Results (22)

Quasi-one-dimensional (quasi-1D) transition metal chalcogenides (TMCs), a subclass of low-dimensional materials, have attracted significant attention due to their unique optical and electronic properties, making them promising candidates for nonlinear photonics. In this work, NbTe₄, a quasi-1D transition metal tetrachalcogenide, was synthesized and employed for the first time as a broadband saturable absorber (SA) for pulsed laser applications. The nonlinear optical (NLO) properties of NbTe₄ were systematically characterized at 1.0 μm, 2.0 μm, and 3.0 μm, revealing saturation intensities of 59.53 GW/cm², 14 GW/cm², and 6.8 MW/cm², with corresponding modulation depths of 17.4%, 5.3%, and 21.5%. Utilizing NbTe₄-SA, passively Q-switched (PQS) pulses were successfully generated in the 1.0 μm and 2.0 μm bands, achieving pulse durations of 86 ns and 2 μs, respectively. Furthermore, stable mode-locked operation was demonstrated in an Er-doped fluoride fiber laser at 3.0 μm, yielding a pulse duration of 19 ps. These results establish NbTe₄ as a highly promising broadband SA material for next-generation ultrafast photonic devices and pave the way for the development of other quasi-1D materials in nonlinear optics. Full article

Palladium (Pd) nanocubes, a type of metallic nanostructure, have demonstrated remarkable optoelectronic properties, garnering significant attention. However, their nonlinear optical characteristics and related device applications remain underexplored. In this study, we report the fabrication of a novel saturable absorber (SA) by depositing Pd nanocubes onto a D-shaped fiber (DF). The Pd nanocubes, with an average size of 12 nm, were synthesized and integrated with a DF, resulting in a highly robust SA with broadband saturable absorption characteristics. When incorporated into Er³⁺-doped laser cavities, the Pd-DF SA enabled the generation of ultrafast pulses with a central wavelength of 1560 nm, a corresponding repetition rate of 26.7 MHz, and a temporal width of 1.85 ps. Our findings highlight the strong potential of the Pd-DF device as a versatile SA for constructing high-energy ultrafast fiber lasers. Full article

Q-switched fiber lasers have become reliable light sources for generating high-energy pulses, which can be passively modulated by saturable absorbers with excellent nonlinear optical properties. The composite combining Ag and MXene exhibits a broadband nonlinear response and high modulation depth, making it a promising candidate for saturable absorbers in pulsed lasers. Herein, we demonstrate a Q-switched Tm:Ho co-doped fiber laser centered at 2 µm, where the Ag/MXene composite serves as a saturable absorber to generate pulses. The typical spectrum, pulse train, and radio frequency spectrum of Q-switched pulses were observed, in which the 60 dB signal-to-noise ratio was higher than that of 2 µm Q-switched fiber lasers based on other materials, demonstrating the stability of the output pulses. Additionally, the long-term stability of the laser was evaluated over 2 h, where the well-maintained central wavelength and output power also indicated the robustness of the Q-switched laser. Furthermore, the influence of the pump power on the parameters of Q-switched pulses was also investigated, which is conducive to control the output characteristics of lasers. Specifically, the pulse width of the Q-switched pulse decreased, while the repetition rate, output power, and single pulse energy all increased with the increase in pump power. These experimental results demonstrate the ability of Ag/MXene as a saturable absorber and show its potential for generating high-performance pulses in ultrafast lasers. Full article

In this work, we demonstrated a kind of flexibly monolithic saturable absorber (SA) with GaAs nanowires (NWs) on polyimide (PI) plastic substrate for broadband optical modulation at 1.0 and 1.5 µm, separately. The monolithic SA sample was prepared by the metalorganic vapor phase epitaxy (MOVPE) method. The crystal structure and element analysis were examined carefully by high-resolution scanning transmission electron microscopy (HRSTEM) and energy-dispersive X-ray spectroscopy (EDX). We observed a high-density distribution of NWs on the flexible substrate by scanning electron microscopy (SEM). In addition, linear and nonlinear optical properties of the sample were examined by testing the photoluminescence and absorption properties, which showed its potential application as an optical switch due to the pure semiconducting properties. After the characterizations, we experimentally demonstrated this monolithic SA for laser modulation at 1.0 and 1.5 µm, which yielded the minimum optical pulse widths of 1.531 and 6.232 µs, respectively. Our work demonstrated such a kind of monolithic flexible NW substrate-integrated device used for broadband optical modulation, which not only eased the integration process of NWs onto the fiber endface, but also proved the potential of easily integrating with more semiconducting nanomaterials (e.g., graphene, MoS₂, …) to realize monolithic active flexible photonic systems, such as a microscale phase modulator, delay-line, and so on, paving an easy avenue for the development of both active and flexible photonic devices. Full article

Two-dimensional (2D) materials have attracted considerable attention due to their potential for generating ultrafast pulsed lasers. Unfortunately, the poor stability of most layered 2D materials under air exposure leads to increased fabrication costs; this has limited their development for practical applications. In this paper, we describe the successful preparation of a novel, air-stable, and broadband saturable absorber (SA), the metal thiophosphate CrPS₄, using a simple and cost-effective liquid exfoliation method. The van der Waals crystal structure of CrPS₄ consists of chains of CrS₆ units interconnected by phosphorus. In this study, we calculated the electronic band structures of CrPS₄, revealing a direct band gap. The nonlinear saturable absorption properties, which were investigated using the P-scan technique at 1550 nm, revealed that CrPS₄-SA had a modulation depth of 12.2% and a saturation intensity of 463 MW/cm². Integration of the CrPS₄-SA into Yb-doped fiber and Er-doped fiber laser cavities led to mode-locking for the first time, resulting in the shortest pulse durations of 298 ps and 500 fs at 1 and 1.5 µm, respectively. These results indicate that CrPS₄ has great potential for broadband ultrafast photonic applications and could be developed into an excellent candidate for SA devices, providing new directions in the search for stable SA materials and for their design. Full article

This paper presents a broadband GaN microwave monolithic integrated circuit driver amplifier (MMIC DA) with compact dimensions of 1.65 mm × 0.78 mm for 5G millimeter-wave communication. The optimal impedance domain satisfying the preset goals was first acquired using the simplified load-pull procedure and small-signal simulations, followed by a weighted average method to determine the reference center matching point from which the optimal intrinsic load can be deduced. By means of de-embedding load-pull contours, modeling based on theoretical analysis, and simulation fitting for parameter identification, the nonlinear output capacitance and a series RLC model circuit approximating the input impedance response of the stabilized transistor were extracted. Under the design principle of fully absorbing the parasitic parameters of the device, explicit formulas and tabulated methods related to the Chebyshev impedance transformer were applied to construct filter-based synthesized matching networks at each stage and finally convert them into an implementable mixed-element form via the single-frequency equivalence technique. Measured on-wafer pulsed results for the proposed two-stage DA across 24–30 GHz demonstrated up to 31.1 dBm of saturated output power (P_sat) with less than 1 dB total fluctuation, 19.3 ± 1 dB of small-signal gain, and 39.8% of peak power-added efficiency (PAE) at the mid-frequency. Full article

Five novel bis-tridentate Ir(III) complexes (Ir-1–Ir-5) incorporating versatile N^N^C ligands and a N^C^N ligand (1,3-di(2-pyridyl)-4,6-dimethylbenzene) were synthesized. With the combination of experimental and theoretical methods, their steady and transient state characteristics were researched scientifically. The UV-visible absorption spectra show that the broadband charge transfer absorbance of those bis-tridentate Ir(III) complexes can reach 550 nm, all of these complexes reveal the long-lasting phosphorescent emission. Because the excited-state absorption is more powerful than the ground-state absorption, a sturdy reverse saturable absorption (RSA) process can ensue in the visible and near-infrared regions when the complexes are exposed to a 532 nm laser. Therefore, the optical power limiting (OPL) effect follows the trend: Ir-5 > Ir-4 ≈ Ir-3 > Ir-2 > Ir-1. Generally speaking, the expansion of π-conjugation and the introduction of electron donating/withdrawing groups on the N^N^C ligand could effectively elevate the OPL effect. Therefore, these octahedral bis-tridentate Ir(III) complexes might be exploited as potential OPL materials. Full article

Interface interactions in 2D vertically stacked heterostructures play an important role in optoelectronic applications, and photodetectors based on graphene/InSe heterostructures show promising performance nowadays. However, nonlinear optical property studies based on the graphene/InSe heterostructure are insufficient. Here, we fabricated a graphene/InSe heterostructure by mechanical exfoliation and investigated the optically induced charge transfer between graphene/InSe heterostructures by taking photoluminescence and pump–probe measurements. The large built-in electric field at the interface was confirmed by Kelvin probe force microscopy. Furthermore, due to the efficient interfacial carrier transfer driven by the built-in electric potential (~286 meV) and broadband nonlinear absorption, the application of the graphene/InSe heterostructure in a mode-locked laser was realized. Our work not only provides a deeper understanding of the dipole orientation-related interface interactions on the photoexcited charge transfer of graphene/InSe heterostructures, but also enriches the saturable absorber family for ultrafast photonics application. Full article

Owing to its broadband absorption, ultrafast recovery time, and excellent saturable absorption feature, graphene has been recognized as one of the best candidates as a high-performance saturable absorber (SA). However, the low absorption efficiency and reduced modulation depth severely limit the application of graphene-based SA in ultrafast fiber lasers. In this paper, a single-layer graphene saturable absorber mirror (SG-SAM) was coated by a quarter-wave SiO₂ passivated layer, and a significantly enhanced modulation depth and reduced saturation intensity were obtained simultaneously compared to the SG-SAM without the SiO₂ coating layer. In addition, long-term operational stability was found in the device due to the excellent isolation and protection of the graphene absorption layer from the external environment by the SiO₂ layer. The high performance of the SAM was further confirmed by the construction of a ring-cavity EDF laser generating mode-locked pulses with a central wavelength of 1563.7 nm, a repetition rate of 34.17 MHz, and a pulse width of 830 fs. Full article

Metal nanomaterials have promising applications in ultrafast photonics due to their broadband operation, large third-order nonlinear susceptibility, and ultrafast recovery time. We realized a Q-switched pulsed erbium-doped fiber laser based on a silver nanoplate polyvinyl alcohol film as a saturable absorber. This film, with a modulation depth of 15.7%, was integrated into a fiber laser by means of a sandwich structure. We obtained Q-switched pulses in the 1.5-μm band, which plays an important role in telecommunications and atmospheric detection. Stable Q-switched pulses were obtained at the pump power of 135 mW, with a single pulse energy of 33.8 nJ, a pulse width of 2.3 μs, a repetition rate of 62.4 kHz, and a signal-to-noise ratio of about 45 dB. When increasing the pump power up to a maximum value of 246 mW, the maximum single pulse energy of 57.8 nJ was achieved. This study first demonstrates the potential of silver nanoplates as saturable absorbers in generating stable laser pulses with high energy. Full article

The principal objective of this study is to employ non-destructive broadband dielectric spectroscopy/impedance spectroscopy and machine learning techniques to estimate the moisture content in FRP composites under hygrothermal aging. Here, classification and regression machine learning models that can accurately predict the current moisture saturation state are developed using the frequency domain dielectric response of the composite, in conjunction with the time domain hygrothermal aging effect. First, to categorize the composites based on the present state of the absorbed moisture supervised classification learning models (i.e., quadratic discriminant analysis (QDA), support vector machine (SVM), and artificial neural network-based multilayer perceptron (MLP) classifier) have been developed. Later, to accurately estimate the relative moisture absorption from the dielectric data, supervised regression models (i.e., multiple linear regression (MLR), decision tree regression (DTR), and multi-layer perceptron (MLP) regression) have been developed, which can effectively estimate the relative moisture absorption from the dielectric response of the material with an R¬2 value greater than 0.95. The physics behind the hygrothermal aging of the composites has then been interpreted by comparing the model attributes to see which characteristics most strongly influence the predictions. Full article

We experimentally demonstrate a passively Q-switched wavelength tunable 2.8 μm erbium-doped fiber laser. Fe₃O₄ nanoparticles deposited on a gold mirror are used as a saturable absorber (SA). Stable Q-switched pulses within the tunable range of 2710–2810 nm are obtained. At the wavelength of 2760 nm, a maximum Q-switched output power of 188 mW is achieved with a repetition rate of 115.8 kHz and a pulse width of 1.3 μs. The corresponding pulse energy is 1.68 μJ. This demonstration shows the ability of Fe₃O₄ to function as a broadband mid-infrared SA. Full article

Mode-locking is an ultra-short pulse laser generation technique. The range of pulse duration may vary from picoseconds to femtoseconds. Yttrium Oxide (Y₂O₃) based saturable absorber (SA) was appropriately revealed in the mode-locked method within the 1.55-micron regime. Y₂O₃ is perfect for strength, melting point, and chemical stability and can be used as a laminated insulator due to its properties. Moreover, Y₂O₃ also owns broadband service, switching speed, and engineering features. The Y₂O₃-PVA film was produced by combining the 50 mg Y₂O₃ powder into a 50 mL polyvinyl alcohol (PVA) solution and stirring it at room temperature for about 24 h. A mode-locked pulse was recorded with the integrated Y₂O₃-PVA SA in the erbium-doped fiber laser (EDFL) cavity, and the output spectrum optical spectrum analyzer displayed was around 1560.66 nm. In addition to the sustained mode-locked pulse, a nearly constant repetition rate of 1.01 MHz at a specific pump power begins from 175.87 mW to 228.04 mW while the pulse duration is 4.15 ps. Lastly, the mode-locked pulse had been evaluated, which showed the peak power started from 4.94 kW to 6.07 kW. Full article

Ti₃C₂ nanosheet is a newly discovered two-dimensional (2D) clan. It turns out to have encouraging applications for electromagnetic shielding and energy storage. Here, Ag@ Ti₃C₂ hybrids are precisely synthesized by using the one-step solution processing method. Also, their ultrafast broadband nonlinear optical responses in the visible region are studied systematically through nanosecond open-aperture Z-scan and transient absorption techniques. The mechanism of two-photon absorption (TPA) is disclosed in the visible region (409–532 nm). When the laser energy is low and the wavelength is longer than 400 nm, nonlinear absorption cannot happen. Meanwhile, as the laser energy increases, two photons will be absorbed by the electrons in the valence band and the electrons will jump to the conduction band. The process is named as two-photon absorption which will make the specimen show reverse saturable absorption (RSA) properties. What is more, the ultrafast carrier dynamics of the specimen are studied by using the transient absorption. The result shows that the decay contains two phases: the fast and then the slow one. The two phases first come from electron–phonon and then from phonon–phonon interactions, respectively. The electron transfer and charge carrier trapping processes are further verified by the outcomes of similar measurements on Ag@ Ti₃C₂ hybrids. Besides, the two decay processes increase together with the pump fluence. These results show that Ti₃C₂ nanosheet has potential applications in broadband optical limiter. Full article

We demonstrate a passively mode-locked fiber laser using aqueous DNA solution as a saturable absorber (SA), with broadband pulse laser emission from 1 to 1.5 µm. The mode-locked laser with erbium-doped fiber as the gain material has a center wavelength of 1563 nm, a 3 dB bandwidth of 3.9 nm, and a pulse width of 822 fs, whereas the laser with ytterbium-doped fiber as the gain material and an identical DNA aqueous SA has a center wavelength of 1037 nm, a 3 dB bandwidth of 5.04 nm, and a pulse width of 250 ps. The proposed laser, which is simple and cost effective to fabricate, exhibits excellent long-term stability as well as thermal stability during high-power operation. This mode-locked laser scheme with a liquid-phase DNA component has the potential to provide in-depth understanding of the optical nonlinearity and usefulness of DNA. Full article