Recent Advancement on the Optical Properties of Two-Dimensional Molybdenum Disulfide (MoS2) Thin Films
Abstract
:1. Introduction
2. Crystal Structure
3. Electronic Band Structure: Optical and Optoelectronic Properties
1.929 ± 0.005 | 2.136 ±.008 |
1.845 ± 0.008 | 2.053 ± 0.01 |
1.88 | 2.06 |
1.9255 | 2.137 |
1.92 | 2.124 |
1.9449 | 2.1376 |
1.90 | 2.10 |
1.91 | 2.11 |
1.82 | 1.95 |
1.78 | 1.96 |
1.88 | 2.03 |
1.85 | 1.98 |
4. Lattice Dynamic: Raman Scattering and IR Absorption
C3v(S) | D3h(Mo) | D6h(MoS2(Γ)) | Transformation Properties | Activity | Vibration Direction | Atoms Involved | Frequency(cm−1) |
---|---|---|---|---|---|---|---|
A1 | A1’ | A1g | (αxx + αyy,αzz) | Raman | Out | S | 409 |
A2’ | B1u | - | Inactive | Out | S | 403 | |
A2 | A1’’ | B2g1 | - | Inactive | Out | Mo + S | 475 |
B2g2 | - | Inactive | Out | Mo + S | 56 | ||
A2’’ | A2u1 | Tz | IR(E) | Out | Mo + S | 470 | |
A2u2 | Tz | Acoustic | Out | Mo + S | - | ||
E | E’ | E2g1 | (αxx - αyy,αzz) | Raman | In | Mo + S | 383 |
E1u1 | (Tx,Ty) | IR(E) | In | Mo + S | 384 | ||
E2g2 | (αxx - αyy,αzz) | Raman | In | Mo + S | 34 | ||
E1u2 | (Tx,Ty) | Acoustic | In | Mo + S | - | ||
E’’ | E1g | (αyz,αzx) | Raman | In | S | 286 | |
E2u | - | Inactive | In | S | 297 |
Laser (nm) | E2g1 Mode Frequency (cm−1) | A1g Mode Frequency (cm−1) | |||||||||
---|---|---|---|---|---|---|---|---|---|---|---|
1 L | 2 L | 3 L | 4 L | bulk | 1 L | 2 L | 3 L | 4 L | bulk | ||
325 | 384.2 | 382.8 | 382.8 | 382.7 | 382.5 | 404.9 | 405.5 | 406.3 | 407 | 407.8 | |
488 | 384.7 | 383.3 | 383.2 | 382.9 | 383 | 402.8 | 405.5 | 406.5 | 407.4 | 408 | |
514.5# | 384.3 | 383.2 | 382.7 | 382.3 | 382 | 403 | 404.8 | 405.8 | 406.7 | 407.8 | |
514.5* | 386.1 | 383.1 | - | 383.7 | 383.3 | 404.7 | 406.8 | - | 408 | 408.6 | |
532 | 384.7 | 382.5 | 382.4 | 382.4 | 383 | 402.7 | 404.9 | 405.7 | 406.7 | 407.8 | |
632.8 | 385 | 383.8 | 383.3 | 382.9 | 381.5 | 403.8 | 404.8 | 405 | 406 | 406.6 | |
632.8* | 386.4 | 383.1 | - | 383.3 | 382.8 | 405 | 406.2 | - | 407.3 | 408.3 |
5. Resonant Raman Scattering
Phonon Frequency (cm−1) | ||||
---|---|---|---|---|
Γ[80,85,86] | M[97] | M[84] | K[84] | |
409 | 397 | 412 | 408 | |
E2g1 | 383 | 373 | 370 | 345 |
E1g | 287 | 294 | 330 | 336 |
309 | ||||
E2g2 | 34 | - | 233(LA) | 241(LA) |
160(ZA) | 192(ZA) | |||
LA | - | 234 | 235 | 241 |
- Difference process:
- Combination process: ,
6. Conclusions
Acknowledgements
Conflicts of Interest
References
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Ye, M.; Winslow, D.; Zhang, D.; Pandey, R.; Yap, Y.K. Recent Advancement on the Optical Properties of Two-Dimensional Molybdenum Disulfide (MoS2) Thin Films. Photonics 2015, 2, 288-307. https://doi.org/10.3390/photonics2010288
Ye M, Winslow D, Zhang D, Pandey R, Yap YK. Recent Advancement on the Optical Properties of Two-Dimensional Molybdenum Disulfide (MoS2) Thin Films. Photonics. 2015; 2(1):288-307. https://doi.org/10.3390/photonics2010288
Chicago/Turabian StyleYe, Mingxiao, Dustin Winslow, Dongyan Zhang, Ravindra Pandey, and Yoke Khin Yap. 2015. "Recent Advancement on the Optical Properties of Two-Dimensional Molybdenum Disulfide (MoS2) Thin Films" Photonics 2, no. 1: 288-307. https://doi.org/10.3390/photonics2010288