Characteristics and Enrichment Regularity of Coalbed Methane in the No.8+9 Coal Seams of the Taiyuan Formation in the Mugua Area, Shenfu Gas Field
Abstract
1. Introduction
2. Materials and Methods
2.1. Sample Collection
2.2. Experimental Test Methods
- Coal Petrology and Coal Quality Analysis
- 2.
- Gas Content Test
- 3.
- High-Pressure Isothermal Adsorption Experiment
- 4.
- Gas Component Analysis
2.3. Data Processing and Mapping
- Drilling and Logging Data Processing
- 2.
- Plane Contour Map Drawing
- 3.
- Critical Adsorption Depth Calculation
- 4.
- Resource Abundance Calculation
3. Regional Geological Setting
4. Results and Discussion
4.1. Accumulation Conditions of Deep Coalbed Methane
4.1.1. Coal Seam Thickness and Sedimentary Control Characteristics
4.1.2. Coal Petrological and Geochemical Characteristics
- Coal Structure and Macrolithotype Characteristics
- Maceral and Proximate Analysis Characteristics
- Thermal Evolution and Coal Rank Characteristics
4.1.3. Gas-Bearing Characteristics of Coal Rocks
4.2. Enrichment Regularity of Coalbed Methane
4.2.1. Sedimentation Controls the Distribution of Source Rocks and the Basic Quality of Coal Seams
4.2.2. Thermal Evolution Degree Dominates Hydrocarbon Generation Capacity and Gas Quality
4.2.3. Temperature–Pressure Effect Controls the Present Occurrence State of Coalbed Methane
- Quantitative Calculation of Critical Adsorption Depth
- Sensitivity Analysis of Critical Adsorption Depth
- For every 0.5 °C/100 m increase in geothermal gradient, the critical adsorption depth decreases by about 100 m.
- For every 0.1% increase in Ro,max, the critical adsorption depth increases by about 50 m.
- For every 0.1 increase in pressure coefficient, the critical adsorption depth increases by about 80 m.
- Vertical Zoning Characteristics and Mechanism Explanation of “Decrease followed by Increase”
- Burial depth < 1500 m: The positive control effect of pressure is absolutely dominant, the negative effect of temperature is extremely weak, CBM is mainly stored in an adsorbed state, and the contents of dissolved and free gas are extremely low.
- 1500~1750 m: The reservoir pressure rises steadily, the negative impact of temperature on adsorption capacity is still not prominent, and the overall adsorption capacity of coal seams shows an increasing trend, forming an undersaturated CBM reservoir dominated by an adsorbed state with basically no free gas distribution.
- 1750~2000 m: Entering the critical adsorption zone, the negative effect of temperature gradually becomes dominant, and adsorbed natural gas desorbs from the coal seam surface, forming a saturated–supersaturated CBM reservoir with the coexistence of adsorbed and free gas. At this stage, hydrocarbon generation has entered the plateau period, and the hydrocarbon generation increment is limited. The gas loss caused by desorption cannot be effectively supplemented, so the gas saturation shows a fluctuating decreasing characteristic (10~130%).
- >2000 m: On the one hand, the Ro,max of coal seams is generally >1.1%, entering the peak hydrocarbon generation period, and the hydrocarbon generation amount increases significantly, making up for the gas loss caused by desorption; on the other hand, under the dominance of temperature negative effect, the adsorbed gas continues to desorb to form free gas, and the occurrence characteristic of coexistence of adsorbed and free state further pushes up the gas saturation of coal seams. Measured data show that in the burial depth interval of 2000~2200 m, the gas saturation shows a significant increasing trend with the increase in burial depth, up to 160%, with prominent saturated–supersaturated reservoir characteristics, and the development of free gas further improves the CBM development potential of this interval.
4.2.4. Preservation Conditions Control the Enrichment Degree of Coalbed Methane
- Cap Rock Sealing Conditions
- Tectonic Preservation Conditions
- Hydrodynamic Reservoir-Controlling Conditions
4.2.5. Coupling Relationship of Reservoir-Controlling Factors and Accumulation Model
- Spatiotemporal Coupling Reservoir-Controlling Mechanism of Four Factors
- Temporal Evolution Sequence
- Late Permian–Triassic (Sedimentary Diagenesis and Early Hydrocarbon Generation Stage): Sedimentation laid the spatial distribution and basic quality of coal seams, were the burial depth of coal seams gradually increased, entered the immature–low mature evolution stage, and mainly generated biogas and early pyrolysis gas.
- Jurassic–Cretaceous (Main Hydrocarbon Generation Stage): Dominated by regional metamorphism, the burial depth of coal seams reached the maximum, the thermal evolution degree entered the mature stage, and a large amount of thermogenic methane was generated, which was the main accumulation period of CBM in this area.
- Cenozoic (Adjustment and Preservation Stage): The basin was uplifted as a whole, the burial depth of coal seams decreased somewhat, the temperature-pressure field was adjusted, and the 1750 m critical adsorption zone was formed; the stable structural environment and closed hydrodynamic conditions ensured the effective preservation of CBM and finally formed the present accumulation pattern.
- Spatial Coupling Characteristics
- 2.
- Classification and Key Parameters of Accumulation Models
- 3.
- Geological Verification of Accumulation Model
5. Conclusions
- (1)
- The geological accumulation basis of medium-rank deep CBM in the study area has been clarified. The No.8+9 coal seams of the Taiyuan Formation are typical medium-rank humic coal seams, with a main burial depth > 1500 m, a thickness ranging from 7.0 to 21.3 m, and an average thickness of 15.1 m, and the coal structure is dominated by primary structure (accounting for 78%); the maximum vitrinite reflectance (Ro,max) is distributed from 0.90% to 1.39% with an average of 1.08%, the organic matter is mainly Type III kerogen, the average gas content is 10.01 m3/t, and the average proportion of desorbed gas in the total gas content reaches 83.91%, with high-quality “source–reservoir integration” accumulation conditions and good exploration and development potential of deep CBM.
- (2)
- The “spatiotemporal synergistic coupling of four factors” reservoir-controlling mechanism of deep CBM in the study area has been revealed. Among them, sedimentation is the material basis of accumulation, and the tidal flat–lagoon facies form the core development zone of high-quality coal seams; regional metamorphism dominates the hydrocarbon generation process, hydrocarbon generation scale, and gas quality of coal seams; temperature–pressure coupling controls the occurrence state of “adsorbed + free gas” of CBM in coal seams deeper than 1750 m; high-quality mudstone cap rocks, a stable compressional structural background, and closed stagnant hydrodynamic conditions constitute the three major preservation guarantees for CBM enrichment; and the organic matching in space and dynamic synergy in time of the four factors jointly determine the final enrichment degree of CBM.
- (3)
- Two types of deep CBM accumulation models in the study area have been established, clarifying the key parameters and exploration potential of each model:
- Source–reservoir integration + multi-factor synergistic enrichment type: Developed in the tidal flat–lagoon facies belt, with coal seam thickness > 12 m, Ro,max > 1.0%, and gas content > 10 m3/t, the four reservoir-controlling factors are highly coupled, with excellent gas-bearing property and recoverability, being the most favorable exploration target area in the area;
- Source–reservoir limited + insufficient accumulation condition type: Developed in the delta front/tidal flat edge facies belt, with coal seam thickness < 8 m, Ro,max < 1.0%, and gas content < 8 m3/t, this model shows obvious shortcomings in accumulation conditions and limited exploration and development potential.
Author Contributions
Funding
Data Availability Statement
Conflicts of Interest
Abbreviations
| CBM | Coalbed Methane |
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| Volume Fraction of Maceral Components | Ash Mass Fraction | Ro,max | ||||||
|---|---|---|---|---|---|---|---|---|
| Vitrinite | Inertinite | Liptinite | Organic Components | Clay Minerals | Sulfide Minerals | |||
| Range | 62.10~86.35 | 13.55~37.80 | 0.10~0.15 | 88.25~94.35 | 4.55~7.50 | 0.10~4.25 | 11.12~23.07 | 0.9~1.39 |
| Mean Value | 70.99 | 28.90 | 0.11 | 92.73 | 6.13 | 1.15 | 16.26 | 1.08 |
| Classification Standard | Low-Rank Coal Ro,max/% | Medium-Rank Coal Ro,max/% | High-Rank Coal Ro,max/% |
|---|---|---|---|
| GB/T 5751-2009 | <0.65 | 0.65~2.0 | ≥2.0 |
| ASTM D388-22 | <0.5 | 0.5~2.0 | ≥2.0 |
| ISO 11760-2018 | <0.6 | 0.6~2.0 | ≥2.0 |
| Well No. | Number of Samples | Air-Dry Basis Gas Content (cm3/g) | Gas Content Composition (%) | ||||||
|---|---|---|---|---|---|---|---|---|---|
| Desorbed Gas | Lost Gas | Residual Gas | |||||||
| Range | Avg. | Range | Avg. | Range | Avg. | Range | Avg. | ||
| M1-11 | 6 | 8.38~11.07 | 9.34 | 83.73~87.81 | 85.39 | 6.61~10.77 | 8.98 | 5.51~5.79 | 5.63 |
| M1-21 | 7 | 9.85~11.81 | 10.71 | 85.99~89.75 | 87.49 | 4.68~8.45 | 6.97 | 5.24~6.12 | 5.54 |
| T-M34 | 7 | 12.07~16.49 | 14.57 | 86.05~87.92 | 86.97 | 5.87~7.71 | 6.82 | 6.04~6.45 | 6.21 |
| T-M64 | 17 | 4.34~16.70 | 10.45 | 55.66~81.25 | 72.30 | 12.87~37.97 | 21.67 | 5.53~6.53 | 6.03 |
| T-M64-8 | 23 | 4.12~10.51 | 7.43 | 74.85~83.93 | 79.00 | 9.63~19.44 | 15.09 | 5.29~6.77 | 5.91 |
| T-M84 | 18 | 4.32~9.98 | 7.17 | 67.97~86.57 | 81.39 | 7.47~26.56 | 12.21 | 5.46~7.24 | 6.40 |
| T-M94 | 18 | 5.91~17.25 | 10.59 | 83.95~89.08 | 86.21 | 5.53~10.91 | 8.33 | 5.14~5.66 | 5.46 |
| M-36 | 20 | 10.19~19.94 | 14.60 | 83.36~89.89 | 85.20 | 6.77~10.42 | 8.64 | 3.34~6.60 | 6.16 |
| M-67-7 | 8 | 6.20~8.93 | 7.75 | 82.55~88.30 | 85.52 | 7.48~11.29 | 9.06 | 2.96~8.38 | 5.42 |
| M-87 | 15 | 7.52~11.84 | 9.11 | 82.87~87.17 | 85.76 | 6.66~11.45 | 8.34 | 5.59~6.18 | 5.91 |
| M-97 | 14 | 9.53~14.61 | 11.67 | 82.63~84.89 | 83.37 | 9.23~11.98 | 10.84 | 4.95~6.14 | 5.79 |
| M-08 | 14 | 4.88~8.26 | 6.67 | 86.73~91.02 | 88.26 | 2.90~7.51 | 5.84 | 5.57~6.22 | 5.90 |
| Average Value | 10.01 | 83.91 | 8.44 | 5.86 | |||||
| Well No. | Depth/m | Ro,max/% | Experimental Temperature/°C | Langmuir Volume VL/(cm3/g) | Langmuir Pressure PL/MPa |
|---|---|---|---|---|---|
| T-M34 | 1913~1915 | 1.05 | 40 | 14.55 | 2.31 |
| T-M34 | 1913~1915 | 1.05 | 60 | 12.17 | 2.05 |
| T-M34 | 1913~1915 | 1.05 | 80 | 10.32 | 1.91 |
| T-M34 | 1913~1915 | 1.05 | 100 | 8.76 | 1.78 |
| M-36 | 2056~2058 | 1.12 | 80 | 11.24 | 1.85 |
| M-97 | 1892~1894 | 1.02 | 80 | 9.87 | 1.93 |
| Accumulation Model | Sedimentary Facies Belt | Coal Seam Thickness/m | Vitrinite Content/% | Ro,max/% | Gas Content/(m3/t) | Desorbed Gas Proportion/% | Resource Abundance/(104 m3/km2) | Structural Belt | Hydrodynamic Condition | Development Potential |
|---|---|---|---|---|---|---|---|---|---|---|
| Source–reservoir integration + multi-factor synergistic enrichment type | Tidal flat–lagoon facies | >12 | >70 | 1.0~1.3 | >10 | >83 | >4.0 | Zone III | Stagnant zone | Excellent |
| Source–reservoir limited + insufficient accumulation condition type | Delta front/tidal flat edge | <8 | <60 | <1.0 | <8 | <80 | 1.0~3.0 | Zone I | Weak runoff zone | Limited |
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Share and Cite
Zhao, G.; Guo, G.; Du, J.; Zhang, Z.; Mei, X.; Sun, L.; Tang, C.; Tang, H.; He, J. Characteristics and Enrichment Regularity of Coalbed Methane in the No.8+9 Coal Seams of the Taiyuan Formation in the Mugua Area, Shenfu Gas Field. Processes 2026, 14, 1637. https://doi.org/10.3390/pr14101637
Zhao G, Guo G, Du J, Zhang Z, Mei X, Sun L, Tang C, Tang H, He J. Characteristics and Enrichment Regularity of Coalbed Methane in the No.8+9 Coal Seams of the Taiyuan Formation in the Mugua Area, Shenfu Gas Field. Processes. 2026; 14(10):1637. https://doi.org/10.3390/pr14101637
Chicago/Turabian StyleZhao, Gang, Guangshan Guo, Jia Du, Zihan Zhang, Xiaohan Mei, Leiming Sun, Chuanjiang Tang, Haozhen Tang, and Jiang He. 2026. "Characteristics and Enrichment Regularity of Coalbed Methane in the No.8+9 Coal Seams of the Taiyuan Formation in the Mugua Area, Shenfu Gas Field" Processes 14, no. 10: 1637. https://doi.org/10.3390/pr14101637
APA StyleZhao, G., Guo, G., Du, J., Zhang, Z., Mei, X., Sun, L., Tang, C., Tang, H., & He, J. (2026). Characteristics and Enrichment Regularity of Coalbed Methane in the No.8+9 Coal Seams of the Taiyuan Formation in the Mugua Area, Shenfu Gas Field. Processes, 14(10), 1637. https://doi.org/10.3390/pr14101637
