2. Theoretical Model
Atomic clouds comprised of high numbers of atoms, and when driven close to electronic resonances, are optically thick. As a result, photons are scattered multiple times, undergoing a random walk inside the cloud. Such processes are described by a diffusion equation for the light intensity distribution
I, namely [
5,
6,
9,
10]:
The diffusion coefficient
quantifies photon transport, with
denoting the photon mean free path,
n the atom density, and
the photon absorption cross-section. The interval between consecutive scattering events determines the photon diffusion time
. The latter is approximately given by the lifetime of the excited state,
, with
being the transition linewidth [
7]. The coupling between the atom dynamics and photon transport originates from the dependence of the diffusion coefficient on the local density of atoms, namely,
.
Assuming local hydrodynamical equilibrium, the atom density
n and velocity field
are modelled with the usual continuity and Navier–Stokes equations:
with
being the equation of state of an ideal gas,
the optical damping rate (optical molasses), and
m the atom mass. The exchange of photons between nearby atoms and the associated momentum recoil is also at the origin of a repulsive radiation pressure force
, scaling as
and determined by the mean-field Poisson equation:
where
is the effective charge, with
denoting the absorption cross-section for re-scattered photons [
11,
12]. An effective plasma frequency,
[
13], immediately follows and allows for analogies with one-component trapped plasmas [
8]. In typical experimental conditions, the effective charge is of the order
∼
, with
e being the electron charge, and
∼
the typical atom density, resulting in a plasma frequency of
∼50–200 Hz [
14,
15]. Notice that
Q depends on the light intensity
I, providing additional coupling between the atom and photon dynamics.
The previous coupling can, in specific conditions, become unstable, leading to the nucleation of photon bubbles—a local increase in the photon number accompanied by a depletion in the atom density [
5]. The linear growth rate of the instability is given by:
Here,
is the dispersion relation of the coupled atom–light gases, with
k being the perturbation wavenumber. The coupling coefficient
depends on both the initial (equilibrium) diffusion coefficient
, and the light distribution
. The finite temperature of the atoms yields the thermal speed of sound
. From the growth rate in Equation (
5), the crossing of the instability threshold (
) requires the following conditions to be satisfied:
which, from the first relation, depend on initial local inhomogeneities in the photon distribution
. Note that the photon bubble mechanism differs from the pattern formation instability in cold atoms [
16]. In the latter, optical dipole forces, originating from far-off-resonant light and resulting from the conversion of light phase fluctuations into amplitude modulations, act on the atoms and trigger an instability in the transverse plane of the laser, whereas here we rely on quasi-resonant radiation pressure. Moreover, the pattern formation instability results from coherent photon transport, while here light is in the diffusive limit. Moreover, in contrast with the similar astrophysical instabilities, the photon bubble mechanism reported here does not require the presence of magnetic fields.
3. Experimental Results
We prepare an atomic sample of cooled
Rb atoms in a magneto-optical trap (MOT) [
17]. In a typical sample, we obtain up to
N∼
atoms at
T∼200
K and a maximum density
∼
in a near spherical cloud of about 4 mm in diameter. All the experiments are conducted with a magnetic field gradient of
∼9 G/cm. While the magnetic field has no significant influence on the observed effects, the laser detuning
strongly determines the stability of the system through the cross-sections
and
[
14]. Within the two-level atom approximation, and in the high-intensity limit relevant for our experiments (
, with
), the plasma frequency scales as
∼
, away from the resonance,
[
12,
14]. However, close to the resonance,
∼
, complications due to the Zeeman splitting of the excited manifold arise, rendering the two-level atom approximation invalid. In any case, we use
as the relevant experimental parameter, sweeping the different regions of the stability diagram. In the first part of the experiment, the trap is loaded by switching on the laser beams and the magnetic field gradient for a total duration of 3 s, long enough to ensure a steady-state number of atoms. The laser detuning during the loading step is fixed at
. It is then shifted to a different value
for a duration of 2 s, long enough so that the photon bubble instability is fully saturated and the density reaches a steady-state distribution. We then release the trap by turning off the magnetic field gradient and the trapping light. After a transient time of approximately 200
s (to ensure the absence of any residual
B field during the imaging sequence), we illuminate the trap with far-off-resonant light (
) and collect the atomic fluorescence signal with a CCD camera during an exposure time of about 300
s. As we shall demonstrate later, with
, the imaging occurs in the single-scattering regime, thus ensuring the correct retrieval of the column density distribution, a crucial feature for the subsequent interpretation of the experimental results. For each value of
, we repeat the loading and imaging sequence 255 times. The entire process is then repeated for different values of
, the parameter used to span the different instability regimes (for simplicity, the detuning
will be referred to as
from now on). Two additional CCD cameras, placed at orthogonal directions, allow us to monitor the overall shape and symmetry of the atomic sample.
Starting from lower values of
and going further into resonance, we observe the transition from a stable phase, persistent for
and previously investigated in [
15], into a regime where the photon bubble instability is triggered—see
Figure 1. Note that, while the use of the laser intensity as a control parameter is mainly relevant in setting the number of atoms in the trap [
11,
15], the detuning from resonance is the appropriate knob to probe the different dynamical regimes [
14]. To diagnose the instability, we perform fluorescence imaging on the atomic sample to retrieve the column density distribution of the trap, which, in the case of near-spherical symmetry, contains the full information about the real atom density profile. The latter is obtained by computing the inverse Abel transform, as described in
Appendix A.
From the onset of the instability, a localised central region of strong radiation trapping grows. At the same time, such an increase in the local photon density is responsible for atom expulsion due to radiation pressure forces—a single photon bubble is formed at the centre of the atomic sample. As the atoms are scattered away from the centre of the bubble, the light diffusion coefficient increases due to a depleted medium. At some point, the increased diffusion losses inhibit any further growth, corresponding to the saturation of the instability as the photon bubble reaches its final state. We begin by noticing that, under near-saturation conditions, the diffusion term
in Equation (
5) dominates over both the effective plasma frequency
and thermal dispersion
. Saturation occurs when growth is no longer sustainable due to a depleted medium and the consequent increase in photon losses, at which point the growth rate vanishes. This limit can be described as
, with
being the diffusion coefficient at saturation level. Here, we have also defined
, with
and
L being the final photon density distribution and size of the bubble, respectively. The saturated diffusion coefficient can be written as a correction to the initial value
, due to a depletion of the atomic density
(with
), such that
. Putting all this together, we arrive at the atomic density depletion fraction:
Since the diffusion coefficient has always a finite value, total atomic depletion should not be expected in any situation. Recall that the diffusion coefficient is given by
, with
being the photon mean free path. The photon scattering cross-section is determined by
, with
being the on-resonance cross-section and
g being a degeneracy factor that depends on the specific atomic transition [
18]. We can then rewrite Equation (
7) in terms of the photon detuning
as:
with
being the diffusion coefficient at resonance. This relation can be fitted to the experimental results—see
Figure 1—which correctly describes both the onset, the unstable phase at
, and the final state of instability in the form of quasi-static photon bubbles (QSB).
At this point, we shall elucidate the validity of the diffusion approximation in Equation (
1). The photon mean free path has been carefully measured to be of the order of
300
m for resonant light [
7]. For
, where a high depletion fraction is observed, we estimate
∼700
m and, thus,
, with
w∼4 mm being the diameter of the atomic sample, thereby ensuing the validity of the diffusion approximation. Moreover, and to further consolidate the experimental observations as evidence of photon bubbles, notice that their spatial extent is expected to be of the order
ℓ, namely,
, in good agreement with the structures depicted in
Figure 1. In addition, for
, one obtains
ℓ∼20 mm, thus ensuring the single-scattering regime during the imaging sequence.
The atom density profiles observed in the QSB regime, which persist approximately for
, are not described by the usual Wieman model [
11], which predicts a flattened density in the case of moderate optical thickness and does not account for the effects associated with the diffusive nature of light. For smaller values of
(i.e., closer to resonance), a dramatic change of the dynamics of the coupled atom–light gases is observed. In this regime, the instability leads to the growth of structures beyond the limit that is sustainable for the depleted atomic medium. At this point, the central photon bubble collapses, or bursts, followed by a re-establishment of the local atom density that again re-triggers the instability. Such processes are at the origin of a low-frequency turbulent regime, the photon bubble turbulence (PBT), which we shall now describe in greater detail.
We investigate the PBT regime by bringing the driving beams very close to the atomic resonance, typically
. A CCD camera working at 350 fps collects the fluorescence signal from the trap, resolving the spatio-temporal properties of the turbulent regime—see
Figure 2. We begin to investigate the low-frequency nature of turbulence by measuring the frequency power spectrum of the spatially resolved fluorescence time signal—see
Figure 2. The total signal is nearly constant, corresponding to an approximately fixed number of atoms in the trap. Additionally, for a lower laser detuning,
(QSB regime), low-amplitude isolated frequency peaks are observed. It has previously been described that, in a similar region of experimental parameters, the atomic cloud undergoes a supercritical Hopf bifurcation into an unstable regime of large-amplitude self-sustained oscillations [
14]. In that case, nevertheless, the instability is expected for clouds with large radii, typically greater than 4 mm, and with a number of atoms of the order of
, features which safely distinguish it from the one reported here. Moreover, the unstable behaviour in Ref. [
14] originates at the edge of the cloud, while the photon bubble instability is triggered in its central region. Regardless, the same authors also describe the transition from over-damped to under-damped behaviour prior to the instability threshold (lower number of atoms), which is consistent with the low-amplitude breathing oscillations of the bubbles and the red line spectrum in
Figure 2. When tuning the beams closer to resonance (
), a complex dynamical regime takes place—black line in
Figure 2—with the frequency spectrum exhibiting broad-band components at low frequencies, as expected in dissipative weak turbulent systems [
19] and originating from the complex dynamics associated with the growth and collapse of (dynamical) photon bubbles, as we shall demonstrate.
We now turn to the spatial power spectrum of the atom density fluctuations—see
Figure 2—as described in detail in
Appendix B. In the fully developed case (
), the fast
decay at high wavenumbers indicates the existence of quasi-coherent structures with well-defined scale lengths, and not self-similar (fractal) structures at different scales. This is easily understood in terms of the auto-correlation function, the conjugate quantity of the power spectrum, defined as
. For a scaling of the form
∼
, similar to a squared Lorentzian function, such as we experimentally observe, where
a is a regularisation at
(related with the inverse of the typical scale), the auto-correlation function takes the form
∼
, evidencing the existence of well-defined spatial structures of typical size
a (photon bubbles).
In order to make the above phenomenological arguments more accurate, we shall at this point resort to the photon bubble model. From the fluid equations, we derive the power spectrum of the density fluctuations (of both the atom and light gases) and in the case of dynamical spherical bubbles as
:
as derived in
Appendix C. Here,
essentially defines the inverse of the bubble size and, for
, the spectrum decays as
, as observed in the experiment. To further clarify the consistency of the model, we numerically fitted the theoretical power spectrum to the experimental results—see
Figure 2—where a good agreement is observed. The spectrum attains its maximum near
∼
∼3 mm
, corresponding to the typical bubble length
∼
∼2 mm. For lower wavenumbers
, the theoretical curve slightly diverges from the experimental data. This may be attributed to finite-size effects, given that the typical bubble size is just slightly smaller than the diameter of the system (about 4 mm). The
decay observed here is close to the Kolmogorov scaling, which, in the case of homogeneous and isotropic turbulence, gives a
inertial range in the spectrum of density fluctuations. As we have shown, however, and despite the closeness with the Kolmogorov scaling, the spectrum observed here is of a distinct physical origin, related to the complex dynamics associated with the growth and collapse of photon bubbles. The observations reported here are compatible with the ones in Ref. [
6], where the quasi-coherent structures—emerging from a realisation-average procedure—have been successfully associated to a fully developed photon bubble turbulence regime. Here, we recover the same spatial local structure, and we investigate the full dynamical evolution of the system. Moreover, unlike what has been reported in [
6], where a sharp transition from a stable to a turbulent regime had been observed, here, the transition into the fully developed phase is continuous—see
Figure 2. Nevertheless, the fully turbulent phase is only observable in a narrow range of experimental parameters. For
, for instance, the number of atoms in the trap is significantly lower, reducing the overall optical thickness and strongly suppressing the diffusive nature of light.
Regarding the low-frequency nature of the turbulent regime, we can inquire about the temporal dynamical scale associated with the inverse of the typical bubble length,
. Going back to Equation (
5), and considering a temperature
200
K,
∼
100 s
and a diffusion coefficient at resonance of
∼
m
/s [
7], we can compute the corresponding growth rate
∼10 s
. Here, we also used the condition that the damping term
from the optical molasses is not the dominant term at the centre of the cloud, corresponding to the region where the bubble nucleates, and that the initial perturbations of the light intensity distribution occur at a scale much smaller than the final bubble size, namely,
. The initially fast instability growth is gradually reduced as the light intensity increases and the atom density decreases during the bubble growth. As such, slower time scales are associated with higher energies (larger structures), which is at the origin of the observed (temporal) power spectrum. The same instability mechanism is at the origin of both the previously reported regime of quasi-static photon bubbles (QSB) and the turbulent (PBT) phase. In summary, strong radiation trapping affects the collective atomic dynamics and leads to the growth of photon bubbles. While in the QSB phase, the atomic medium is able the support the saturation of the instability, in the PTB regime, photon losses due to the depleted medium lead to the burst and decay of the bubbles, with such continuous processes being at the origin of the low-frequency turbulent regime described here.