1. Introduction
Two-dimensional (2D) materials are among the most interesting topics of research in condensed matter physics these days, both theoretical and applied. The rise of graphene marks the beginning of this new era [
1]. We can cite several novel 2D materials such as graphene and its derivatives, germanene, phosphorene, hesagonal boron nitride, transition metal dichalcogenides, and other 2D heterobilayers [
2]. Nevertheless, we cannot forget the recently obtained ultrahigh-mobility systems based on GaAl. Among the different physical properties studied in these materials, the electronic ones are the most important due to their impact on the future of nanoelectronics, spintronics, and potentially quantum computing. Thus, it is really worth doing a thorough research study on ultrahigh-mobility (
) two-dimensional electron systems (2DESs) and their electronic properties, such as magnetotransport. Different theoretical contributions have recently shown up, studying these high-mobility materials [
3,
4,
5,
6,
7,
8,
9,
10]. One of the most challenging demonstrates that 2DESs, under low magnetic fields (
B) and temperatures (
T), turn into a structure of Schrödinger cat states (SCSs) [
11,
12,
13,
14], a quantum superposition of coherent states [
3] of the quantum harmonic oscillator. The initial idea of coherent states [
11,
12,
13,
14,
15,
16,
17] was introduced by Schrödinger [
15], describing minimum-uncertainty constant-shape Gaussian wave packets of the quantum harmonic oscillator.
It is also worth mentioning that when irradiated under
B, those 2DESs give rise to the very well known phenomenon of microwave-induced resistance oscillations [
9,
10]. MIROs are among the most striking radiation–matter interaction effects discovered in the last two decades. We studied this effect based on
the microwave-driven electron orbit model [
3,
5,
6,
7,
8]. In this model, electron orbits (electrons under
B) are driven by radiation, performing a harmonic motion with the frequency of radiation. During this back and forth motion, electrons suffer elastic scattering due to charged impurities. One remarkable result that we found [
3,
5,
6,
7,
8] is that the time it takes the scattered electron to get from the initial to the final coherent state or evolution time,
, equals the cyclotron period,
[
3]. The rest of scattering processes at different times,
, can be ignored.
Other physical effects obtained in the dark for these materials remain to be fully explained. In this way, experimental results [
18,
19,
20] obtained with ultraclean (
) samples show the unexpected and striking effect of an almost complete magnetoresistance collapse at low
T (
K) and low
B (
), observed under irradiation and in the dark and well-known as
giant negative magnetoresistance [
21,
22,
23,
24,
25,
26,
27,
28,
29,
30] (GNM). Interestingly enough, and as observed in the same experiments, this collapse can be reversed with external parameters: with increasing
T, the set up of an in-plane
B (
) with increasing intensity can also be altered with the electron density (
) via an external metallic gate. Thus, in these experiments, longitudinal magnetoresistance (
) vs.
B has mainly been measured, as well as its variations with different physical properties, temperature, parallel magnetic fields, and electron density. According to experimentalists, in the case of ultrahigh samples, the layer structure is complex and made up of different layers. Nevertheless, the active layer, i.e., where the two-dimensional electron gas is located, is a 30 nm GaAs quantum well.
The motivation for the present work is to develop a microscopical model to explain the experimental evidence, based on coherent states and Schródinger cat states of the quantum harmonic oscillator. Thus, we approach the giant negative magnetoresistance effect based on the description of ultrahigh-mobility two-dimensional electron systems in terms of Schrödinger cat states (superposition of coherent states of the quantum harmonic oscillator). Therefore, in this article we present a theoretical model for this striking effect and the influence of external physical properties and investigate how we can make good use of them to tune GNM and use it to our advantage. In our theoretical approach we devise a phenomenological model to explain those experimental results. On the one hand, we base our study on the quantum superposition of coherent states that give rise to SCSs. Thus, the electronic structure of a ultrahigh-mobility 2DES would be mainly composed of SCSs that oscillate with a frequency double (
) that expected considering the applied field. Under these states, charged impurity scattering (elastic scattering) is seriously diminished and
drops. On the other hand, we focus on sample disorder as responsible for the cat states’ destruction to give rise to standard coherent states. Samples with lower mobility (
) would have an electronic structure based on coherent states [
3], where scattering fully takes place, giving rise to
recovery.
We base this study on previous results by the authors, where high-mobility two-dimensional electron systems under low or moderate magnetic fields could be described as made up of coherent states of the quantum harmonic oscillator. Schrödinger cat states are fragile states that rise when coherent states associate. They turn up in 2D ultraclean samples and, as a consequence, they present very low dissipation, i.e., at low
T and
B. Another important property is that they show quantum interference at certain values of position and time where their probability density peaks (see below). However when disorder rises with increasing
T or
, SCSs are gradually destroyed, becoming mere coherent states. In between these two limiting situations, we propose that the electronic structure of the 2D samples is made up of an ensemble of SCSs and individual coherent states. The intensity of the
drop will depend on what kind of states are predominant in these ultraclean samples. At low
T or low
, SCSs would prevail. In the opposite scenario, at high
T or high
, coherent states would be the majority. Thus,
T and
would be the physical properties that allow us to turn, gradually and continuously, a cat state-based sample into a coherent one and vice versa. Thus,
T and/or
could be used as external tuning physical properties to control the electronic structure of 2DESs and make them SCSs or coherent states at will. We also study GNM as a function of electron density and contrast it against experimental results [
24]. We determine that GNM is not as affected by
as by
T and
.
According to our model, the GNM effect itself is explained based on two physical origins as follows. The energy difference between Landau states in SCSs is
and this makes the Landau levels involved in scattering totally misaligned. As a result, magnetoresistance based on quasi-elastic scattering plummets. This would be one of physical causes of GNM. Another reason would be that the
Schrödinger cat states, when involved in scattering processes, undergo a destructive process that makes the scattering rate vanish, and in turn,
vanishes too [
4]. The Aharonov–Bohm effect plays an essential role in the latter, transforming even Schrödinger cat states into odd ones when a phase shift of
is added [
4]. Nevertheless, there is still a remanent part of
Schrödinger cat states that would be responsible for the experimentally obtained low intensity MIRO. We conclude that ultrahigh-mobility 2DESs, under low
B and
T, are made up of a structure Schrödinger cat states and thus can become a promising bosonic mode-based platform for quantum computing [
31,
32] that could be controlled by external parameters such as
T or
.
2. Theoretical Model
Even and odd coherent states are quantum superpositions of two coherent states of equal amplitude but separated in phase by
radians (see
Figure 1):
where
for even coherent states and,
for odd coherent states. The plus sign corresponds to the even states and the minus to the odd ones. The even and odd coherent states can be obtained from the quantum harmonic oscillator ground state with the action of the even and odd displacement operators [
11],
.
and
Thus,
. The corresponding expansions of the even coherent state, including the time evolution, read
and for the odd coherent state,
Thus, even coherent states are a superposition of even eigenstates of the quantum harmonic oscillator, and the states energy is given by
. The odd ones are superpositions of odd eigenstates, and the energy is
. Interestingly enough, only every other Landau level is populated in both of them, and thus, the energy difference between populated levels is
. This latter point is key to explain GNM. Yet, for genuine coherent states,
.
The wave function for even and odd coherent states thus reads [
11,
12,
13,
14,
17]
where
is the ground state wave function of the quantum harmonic oscillator,
is the guiding center of the quantum oscillator, and
and
are the position and momentum mean values, respectively [
17]:
and
where we have determined that
.
For experimental values [
24],
is large (low
B), and the coherent states
and
can then be considered macroscopically distinguishable [
11,
12,
13,
14,
17]. Thus, the two Gaussian wave packets are located at macroscopically separated points. They classically oscillate with the frequency
, if we consider every Gaussian packet independently. Then, electrons are simultaneously localized in both spatially separated wave packets at macroscopic distances of the order of the low
B cyclotron radius. Then, the above superpositions are known as
Schrödinger cat states [
12,
13]. The normalization constants are
. These cat states are mainly used in quantum optics and have recently become relevant in quantum computing as a promising platform to implement qbits [
33].
In order to establish the physics of our theory on GNM, it is essential to calculate the probability density of the wave function,
which is given by
where the last term is responsible for the quantum interference. Thus, both types of superpositions are composed of two Gaussian wave packets oscillating back and forth harmonically with a phase difference of
radians. When they cross, quantum interference rises. Then, acute peaks are obtained in the probability density when
and
. Thus, we expect that electron scattering will take place mainly at these points, and this is a very important point in our model. In addition, the system as a whole oscillates with double frequency,
, although every Gaussian wave packet individually oscillates with
as we said above.
We consider the quasi-elastic scattering between Schrödinger cat states due to charged impurities. We schematically depict this kind of scattering in
Figure 2. In the upper panel, we exhibit the schematic diagram of scattering process between coherent states
and
. The scattering is quasi-elastic because the scattering source is based on charged impurities. The probability density for both coherent states is a constant-shaped Gaussian wave packet, and the scattering process evolution time is the cyclotron period, i.e.,
(see
Figure 3 and
Figure 4). In the lower panel, we observe the same as in the upper panel, but for the Schrödinger cat state case. The energy difference between populated states is
, and every other state is then populated as in the upper panel case. The schematic diagram of the lower panel corresponds to the scattering process between even Schrödinger cat states.
The longitudinal conductivity
is calculated with a semiclassical Boltzmann model [
34,
35,
36], and accordingly,
where
E is the energy,
is the density of initial Landau states, and
is the scattering rate of electrons with charged impurities.
is at the heart of the physics of our theory explaining GNM. We obtain
by the usual tensor relationships [
34,
35,
36],
, where
and
,
being the 2D electron density.
is the distance between the initial,
, and final,
, scattering-involved state guiding centers.
[
34,
35,
36] is given by Fermi’s golden rule:
where
is the number of charged impurities,
and
are the wave functions corresponding to the initial and final cat states, respectively, and
is the scattering potential for charged impurities [
34,
35,
36].
, and
is the
x-component of
, the electron momentum change during the scattering event. The
matrix element is given by [
34,
35,
36]
where the scattering integral
is [
4]
where
,
, and
.
t is the initial scattering time, and
is the final scattering time [
4]. As above, in the ± sign, “+” corresponds to magnetoresistance held by even Schrödinger cat states and “−” to odd Schrödinger cat states. As we said above, according to the probability density, the scattering processes are more likely to take place at the probability peaks. This is equivalent to having a small effective oscillation amplitude, i.e.,
and
. Thus, for instance, in the case of
, we get [
4]
Remarkably enough, due to the large value of
, the above expression turns out to be negligible (real exponentials tend to zero [
3]), except when
or
. Then, the latter values act similarly as selection rules for the scattering process to take place and contribute to magnetoresistance. After lengthy algebra, we obtain the final expression [
4]:
Thus, for the even Schrödinger cat states, we obtain
, whereas for the odd ones,
. We also obtain, that when one of the scattering-involved cat states, initial or final, is odd, the scattering integral is zero too [
4].
The latter results, in terms of scattering integrals, are very important. Firstly, a good number of scattering processes that could contribute to magnetoresistance are canceled, and secondly, the remnant magnetoresistance that still persist is being held only by even SCSs. The latter point explains one of the two physical reasons justifying GNM according to our model. The second is as follows.
We develop the Dirac delta in
,
as a sum of Lorentzian functions and, with the use of the Poisson sum rules, obtain an expression for SCSs that reads
where
is the Landau level width. Recall that the energy difference between Landau levels for a SCS is
. On the other hand, for the case of coherent states [
4], where
,
In the former case (coherent state scattering) the scattering jumps between initial and final Landau levels are aligned (see
Figure 4a). Thus, there are a lot of states available, which fully contribute to the current and magnetoresistance. Recall that the charged impurity scattering is elastic. However, for the latter case (SCS scattering), Landau levels are misaligned due to the energy difference between levels (see
Figure 4b). As a result, there are hardly any final states in the scattering jump to contribute to the current. Thus, the predominant presence of SCSs in ultrahigh-mobility 2DESs explains why the current plummets.
In our phenomenological model, the former expression for
corresponds to a ultrahigh-mobility 2DES; i.e., it is mainly made up of SCSs. The latter is for a lower-mobility 2DES, i.e., the coherent states are predominant. In between these two scenarios, we propose a general expression for
:
where
is phenomenological
-dependent parameter, which is defined below. The electron-charged impurity (elastic) scattering jump between SCSs is graphically represented in the schematic diagram of
Figure 4b; the scattering is not efficient due to the lack of final states in an elastic jump. The scattering between genuine coherent states is represented in
Figure 4a; now the scattering is fully efficient in terms of available final states.
3. Results
The effect of increasing
T and
on electrons causes them to interact with more intensity with lattice ions, producing a stronger emission of acoustic phonons and the subsequent
increase or Landau level widening. Following Ando et al. [
35], acoustic phonon scattering (
) is linearly proportional to
T. Then
. This has to be reflected in a rise in
, which in our model is expressed as
. Where
is the LL width for
K, and
eV [
19] corresponds to the LL width of an ultrahigh-mobility 2D sample. We calculate
and
according to Ando et al. [
35]. Now we define
, where
eV is the LL width for a lower-mobility sample [
37] (
). In our simulations,
T ranges from
K to 1 K, and
K.
The action of is to force an extra oscillating motion in a perpendicular direction to the main B. This would make the interaction of the orbiting electron with the lattice ions stronger and, similarly as with T, emit more acoustic phonons. Thus, the effect of would be to produce more disorder in the sample, giving rise to extra LL widening.
The relation between
and
is determined as follows [
38]: As we have indicated above, the presence of in-plane
B alters the electron trajectory in its orbit, increasing the frequency and the number of oscillations in the
z-direction. Now the frequency of the
z-oscillating motion is
. This makes the electron trajectory longer, increasing the total orbit length and eventually the damping. This increase in the orbit length is proportionally equivalent to the increase in the number of oscillations in the
z-direction. Thus, we introduce the ratio of frequencies after and before connecting
as a correction factor for the damping factor
. The final damping parameter
is
where
is the effective length of the electron wave function when we consider a parabolic potential for the
z-confinement [
35,
38]. Now, proceeding similarly as before, the increase in LL width is
, where, in this case,
.
ranges from 0. T to 1.0 T, and for every case,
is calculated the same as
T.
In
Figure 5, we exhibit calculated results for
vs.
B as a function of
T, ranging from
K to 1 K. At
K, the curve shows a surprisingly strong
collapse or giant negative magnetoresistance. As
T rises, the GNM effect disappears little by little, and it is totally wiped out when
K. As explained above, as
T increases, the disorder of the sample increases too, and the predominant SCSs are progressively destroyed to become individual coherent states. This is reflected in the model with the Dirac delta
that is gradually turned from Equation (
16) into Equation (
17), being represented in the process by Equation (
18). In the curve of
K, the 2DES would be mainly made up of SCSs, while in the curve of
K, the 2DES would be formed by genuine coherent states. The abrupt collapse is present in the dark and under radiation. The calculated results exhibited in
Figure 5 are in qualitative agreement with available experimental results [
21,
22,
24].
In the lower panel of
Figure 6, we present the effect of
on magnetoresistance. Here we present calculated results for
vs.
B for different values of
ranging from 0T to 1T. As
increases, the effect becomes smaller and smaller, and with 1T, it has nearly disappeared. As in
Figure 5, here we find good agreement, at least qualitatively, with experiments [
21,
22,
24].
In
Figure 7, we exhibit the effect of electron density on
. The electron density goes from
to
. As in experiments, we observe that the strong GNM gets more pronounced as
decreases. The explanation can be straightforwardly established from our model if we consider the tensor relations between
and
. Thus,
. The general effect is not as important as with
T and
. Thus, in our opinion,
via an external gate voltage would not be fully effective when it comes to tuning the transition from SCSs to coherent states in ultrahigh-mobility samples. The calculated results exhibited in
Figure 7 are in good agreement with experiments [
22,
24].