1. Introduction
The growth of the civil aviation industry has been rapid due to the development of the global economy and the increase in people’s living standards. However, this growth may have potential impacts on public health, the environment, and climate [
1]. Of particular concern are the carbon emissions resulting from civil aviation, which have garnered increasing attention [
2]. In recent years, carbon emissions from civil aviation have shown a trend of year-on-year growth. According to the International Air Transport Association (IATA), global civil aviation carbon emissions in 2019 (before the Corona Virus Disease 2019) were 990 million tons, accounting for 2.4% of total global carbon emissions. Civil aviation carbon emissions are expected to increase more than three times by 2050. Therefore, reducing carbon emissions from civil aviation has become an urgent issue.
According to the IATA, the total CO
2 emissions from global commercial aviation in 2019 reached 915 million tons, accounting for 2.4% of global CO
2 emissions. Additionally, 85% of the emissions come from passenger transport, reaching 778 million tons [
3]. The aviation industry urgently needs to balance the demand for green development and improve industry competitiveness. The resolution of achieving net-zero carbon emissions by the global aviation industry by 2050 was approved at the 77th IATA Annual General Meeting. The commitment of this resolution is in line with the goals of the Paris Agreement, which is to limit global temperature rise to no more than 1.5 °C. To achieve the temperature control goal, the aviation industry in 2050 will need to reduce carbon emissions by 1.8 billion tons, and 65% of the emissions will be reduced through sustainable aviation fuels. It is expected that new propulsion technologies, such as hydrogen, will reduce emissions by 13%. Efficiency improvements can contribute 3%. The remaining emissions will need to be addressed through carbon capture, utilization, and storage (11%) and offsetting (8%) [
4].
In order to reduce carbon emissions from civil aviation, International Civil Aviation Organization (ICAO) has proposed a series of emission reduction measures, which include improving aircraft fuel efficiency, adopting Sustainable Aviation Fuels (SAFS) [
5] biofuels, and improving air traffic control systems, but it cannot completely achieve carbon neutrality in the civil aviation industry [
6,
7]. In addition, some airlines have adopted their own emission reduction techniques, such as purchasing carbon offsets, adopting more environmentally friendly aircraft types, and promoting electronic passenger tickets. These measures can effectively reduce civil aviation carbon emissions, but the amount of emission reduction is relatively low.
Research shows now that the Carbon Offsetting and Reduction Scheme for International Aviation (CORSIA) program has a very limited incentive for major airlines to implement proactive mitigation measures [
8]. As a result, airlines have explored and invested in carbon capture technologies. For example, United Airlines and Occidental Petroleum are investing in a large “direct air capture of CO
2 (DAC)” plant in Texas that will operate with fans and chemicals to remove CO
2 from the air and inject it underground. The plant will utilize fans and chemicals to remove CO
2 from the air and inject it into the ground. United Airlines’ DAC technology research is driven by the company’s vow to become carbon neutral by 2050 and its belief that technology, such as efficient aircraft and sustainable biofuels, are not enough.
It is predicted that China will surpass the United States as the world’s largest civil aviation transportation market by 2030 [
3]. The need to actively explore new emission reduction options for China’s aviation transportation industry is equally important ahead of time. About 100 million tons of CO
2 were emitted in the civilian sector in China by 2020. Some studies indicate that China’s aviation carbon emissions will increase significantly from 2020–2050, with CO
2 emissions likely to increase by 1.6 to 3.9 times [
9]. As the potential for emission reduction from technology enhancement, equipment renewal, and operational optimization is approaching the “ceiling”, it is extremely difficult to achieve carbon neutrality in the air transport industry by 2050, and China’s air transport industry also needs to explore carbon capture technology to implement carbon reduction.
The DAC technology is a technology that recycles CO
2 emissions from distributed sources and is recognized as a key technology for climate change mitigation, comparable to solar, wind, batteries, and electrolyzers [
10]. The DAC technology captures CO
2 in the air by means of adsorbent. After completing the trapping, the adsorbent is regenerated by changing heat, pressure, or temperature, and the regenerated adsorbent is applied again for CO
2 trapping while the pure CO
2 is stored. The advantage of DAC technology is that it can capture CO
2 from millions of small fossil fuel-burning units and hundreds of millions of distributed sources, such as vehicles. In the International Energy Agency (IEA) 2050 net-zero emissions scenario, more than 85 million tons of CO
2 would need to be captured by the DAC technologies in 2030, capturing about 9.8 million tons of CO
2 in 2050, requiring a significant acceleration from the current approximately 0.01 MtCO
2 [
11]. There are currently 18 DAC facilities in Canada, Europe, and the United States. The first large-scale DAC unit with annual CO
2 emissions of up to one million tons is under construction with development in the US. In addition, the DAC plant has greater flexibility in terms of placement location than technologies, such as CCS or CCUS, which are primarily aimed at stationary source capture [
12,
13]. Under current technology, the levelized cost per ton of CO
2 captured from the atmosphere ranges from
$94 to
$232/ton of CO
2 [
14], and all DAC technologies have the potential to operate at less than
$200/ton [
15], with further decreases in capture costs expected in the future. Furthermore, DAC technologies can help to address unavoidable emissions and emissions from distributed sources, where 24% of transport emissions need to be reduced with the help of DAC [
16]. At the same time, DAC technology can be combined with CCS technology to capture the CO
2 leaked from the CCS technology storage [
17]. The trend of increasing CO
2 emissions from the air transportation industry is inevitable, and the rational use of DAC technology may result in “negative carbon emissions” and greatly reduce atmospheric CO
2 concentration.
The above are the opportunities of DAC technology in the carbon-neutral background, meanwhile DAC technology development faces significant challenges in the future. Carbon capture technologies require high water resources [
18], and DAC technology is no different. Assessed from a whole life cycle perspective, the DAC technology does not have advantages over renewable energy in terms of land use and material consumption, and the energy consumption will increase about five times [
19]. In fact, the life cycle water consumption, material consumption, and land use of DAC systems are also of concern, and preliminary estimates of water consumption of DAC technologies range from 0 to 50 Gt/GtCO
2, and the utilization of renewable energy sources such as photovoltaic and wind power to drive DAC systems will lead to a significant increase in their life cycle land use area [
20]. The current study concluded that DAC technology development could not be achieved without strong policy support [
21].
The possibility of deploying DAC systems at airports is worthy of further study due to the relatively high carbon emissions from the LTO. The LTO cycle is a closed working process of aircraft landing from a high altitude at airport and taking off from an airport to a high altitude. It is defined as a height of 915 m from the surface to the top of the atmospheric boundary layer of airport aircraft. LTO cycle is a closed working process of aircraft landing from a high altitude to an airport and taking off from an airport to a high altitude. It is defined as a height of 915 m from the surface to the top of the atmospheric boundary layer [
22]. The current research based on the LTO cycle focuses on the accounting and management of emissions around airports [
23]. The emission is calculated with the type and number of aircraft, engine type, number of passengers, and using emission factors from the International Civil Aviation Organization engine exhaust emission database [
24]. The main focus was on the study of pollutants such as nitrogen oxides, carbon monoxide, and hydrocarbons with aviation particles at airports during the LTO phase [
25,
26]. Moreover, studying more airport-specific LTO pollutant emissions, ref. [
27] measured the total count concentration of 10 to 1000 nm particles, particle size distribution, and mass concentration of PM2.5 on the parking apron adjacent to the runway of Tianjin International Airport, China. Ref. [
28] conducted an in-depth analysis of pollutant emissions during the aircraft take-off and landing cycle at Nanjing Lukou Airport (NKG). Ref. [
29] presented ground-based, stratospheric aircraft engine emissions from flights departing at Los Angeles International Airport. Ref. [
30] employed airline flight data to evaluate emissions from Turkish Airlines during the LTO phase. Studies related to CO
2 emissions during the LTO cycle of airports have been gradually paid attention to in recent years [
31]. Aircraft emissions from the LTO cycles at Chania Airport (Crete), Greece, were estimated for the year 2016, adopting the International Civil Aviation Organization (ICAO) methodology and using daily data from air traffic [
32]. Developed a methodology using flight data and Daily Aircraft Movement Records (DAMR) data to estimate CO
2 emission levels for different phases of flight within the LTO cycle [
33]. An improved method is proposed to estimate aircraft emissions from LTO cycles [
34]. However, the above studies are limited to accounting for pollutant and carbon emissions from airport LTO cycles and do not propose breakthrough emission reduction solutions.
However, the above studies are restricted to the accounting of pollutants and carbon emissions from LTO cycles in airports and do not propose breakthrough emission reduction solutions. In fact, the research on the deployment of DAC technology in civil aviation is only at the stage of a theoretical feasibility study, and there is a lack of research on the direct deployment of DAC technology in airports. This study will carry out a preliminary exploration of the deployment of DAC systems in airports, taking a large international airport in China as an example.
Based on the demand for carbon capture systems in the aviation industry and the advantages of DAC systems themselves, this study will explore the potential of deploying DAC systems in airports. The following three main questions will be addressed: (1) What is the amount of CO2 emissions in the LTO phase at major airports in China? (2) What are the factors influencing the deployment of DAC devices at airports? (3) Which airports are suitable for DAC deployment demonstration projects?