Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis
Abstract
:1. Introduction
2. Methods
2.1. Simulations of the BB Aerosol Evolution
2.2. Radiative Transfer Calculations
2.2.1. Radiative Transfer Code
2.2.2. Input Parameters
2.2.3. Simulated Radiative Properties
- as AOD grows, increases, while decreases, so that ΦTOA and ΦBOA decrease (enhanced cooling effect);
- as SSA grows, and also grow and, consequently, ΦTOA decreases, while ΦBOA increases;
- as AF grows, the upward flux decreases, while the downward flux increases, so that ΦTOA and ΦBOA grow (warming effect).
3. Results
3.1. Dynamics of the Optical Characteristics of BB Aerosol
3.2. Radiative Forcing
3.3. Radiative Forcing Efficiency
4. Discussion
5. Conclusions
- -
- At the bottom of the atmosphere, the increases (that is, its absolute value becomes less) during the entire evolution process when C0 is small (10 μg/m3), which is mostly due to the dominant role of the asymmetry factor whose growth leads to an increase in the downward radiation fluxes. With much larger initial aerosol concentration increases (C0 = 100 μg/m3), the still initially increases but decreases at the second stage of the evolution;
- -
- At the top of the atmosphere, the increases (decreases by the absolute value) for the entire period of the simulation with the lowest C0 and BC/OA values due to the predominant influence of the changes in AF. As the BC/OA ratio increases, the competing effects of SSA and AF tend to compensate each other, resulting in a weaker dependence of ARFE on the photochemical age. An increase in the initial OA concentration up to C0 = 100 μg/m3 results in a more complex dependence of the ARFE on SSA and AF becomes due to the stronger effects of multiple scattering;
- -
- The dependence of the ARFE in the atmospheric column on the OA photochemical age is mirroring the corresponding dependence (taken with an opposite sign) of SSA: that is, the ARFE decreases or increases with an increase or decrease of SSA.
Author Contributions
Funding
Institutional Review Board Statement
Informed Consent Statement
Conflicts of Interest
References
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Zhuravleva, T.B.; Nasrtdinov, I.M.; Konovalov, I.B.; Golovushkin, N.A.; Beekmann, M. Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis. Atmosphere 2021, 12, 1555. https://doi.org/10.3390/atmos12121555
Zhuravleva TB, Nasrtdinov IM, Konovalov IB, Golovushkin NA, Beekmann M. Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis. Atmosphere. 2021; 12(12):1555. https://doi.org/10.3390/atmos12121555
Chicago/Turabian StyleZhuravleva, Tatiana B., Ilmir M. Nasrtdinov, Igor B. Konovalov, Nikolai A. Golovushkin, and Matthias Beekmann. 2021. "Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis" Atmosphere 12, no. 12: 1555. https://doi.org/10.3390/atmos12121555