Next Article in Journal
The Modulatory Action of Vitamin D on the Renin–Angiotensin System and the Determination of Hepatic Insulin Resistance
Next Article in Special Issue
Mechanochemical Synthesis of CuO/MgAl2O4 and MgFe2O4 Spinels for Vanillin Production from Isoeugenol and Vanillyl Alcohol
Previous Article in Journal
The Influence of Yeast Strain, β-Cyclodextrin, and Storage Time on Concentrations of Phytochemical Components, Sensory Attributes, and Antioxidative Activity of Novel Red Apple Ciders
Previous Article in Special Issue
Mechanochemical Synthesis and Characterization of CuInS2/ZnS Nanocrystals
Article Menu
Issue 13 (July-1) cover image

Export Article

Open AccessCommunication

Synthesis and Regeneration of A MXene-Based Pollutant Adsorbent by Mechanochemical Methods

1
Green Intelligence Environmental School, Yangtze Normal University, Chongqing 408100, China
2
State Key Joint Laboratory of Environment Simulation and Pollution Control (SKJLESPC), Beijing Key Laboratory of Emerging Organic Contaminants Control (BKLEOCC), Key Laboratory of Solid Waste Management and Environment Safety, School of Environment, POPs Research Center, Tsinghua University, Beijing 100084, China
*
Author to whom correspondence should be addressed.
Academic Editor: Jonathan Sperry
Molecules 2019, 24(13), 2478; https://doi.org/10.3390/molecules24132478
Received: 15 May 2019 / Revised: 5 June 2019 / Accepted: 5 June 2019 / Published: 5 July 2019
(This article belongs to the Special Issue Recent Development of Mechanochemical Synthesis)
  |  
PDF [2111 KB, uploaded 7 July 2019]
  |  

Abstract

In the present study, an adsorbent material for removal of organic contaminants in wastewater is synthetized by a green and facile mechanochemical method. It is composed of Ti3C2Tx MXene layers (obtained by mechanochemical etching of MAX phase with concentrated HF) pillared with terephthalate by rapid direct reaction. Such material shows high specific surface area (135.7 m2 g−1) and excellent adsorption capability of methylene blue (209 mg g−1) because of the larger interlayer space among MXene sheets and free carboxylate groups of terephthalate. The spent adsorbent is reutilized (with addition of sole aluminum) to synthetize the MAX phase by mechanochemical procedure, where the terephthalate and the pollutant are carbonized into the carbide. In this way, new MXene-based adsorbent can be re-synthetized for further use. View Full-Text
Keywords: MXene; mechanochemical synthesis; high energy ball milling; adsorption MXene; mechanochemical synthesis; high energy ball milling; adsorption
Figures

Graphical abstract

This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited (CC BY 4.0).
SciFeed

Share & Cite This Article

MDPI and ACS Style

Vakili, M.; Cagnetta, G.; Huang, J.; Yu, G.; Yuan, J. Synthesis and Regeneration of A MXene-Based Pollutant Adsorbent by Mechanochemical Methods. Molecules 2019, 24, 2478.

Show more citation formats Show less citations formats

Note that from the first issue of 2016, MDPI journals use article numbers instead of page numbers. See further details here.

Related Articles

Article Metrics

Article Access Statistics

1

Comments

[Return to top]
Molecules EISSN 1420-3049 Published by MDPI AG, Basel, Switzerland RSS E-Mail Table of Contents Alert
Back to Top