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Keywords = uranium tail sand

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11 pages, 4025 KiB  
Article
Experimental Research on Permeability and Effective Radon Reduction of Chemical Solidification of Uranium Tailings
by Jindong Wang and Shuai Zhang
Atmosphere 2024, 15(12), 1493; https://doi.org/10.3390/atmos15121493 - 14 Dec 2024
Viewed by 973
Abstract
To be able to study the permeability coefficient and radon reduction effect of three materials before and after the solidification of uranium tailings. Firstly, uranium tailings, blast furnace slag, lime, fly ash and cement were selected as raw materials for the experiment. Three [...] Read more.
To be able to study the permeability coefficient and radon reduction effect of three materials before and after the solidification of uranium tailings. Firstly, uranium tailings, blast furnace slag, lime, fly ash and cement were selected as raw materials for the experiment. Three solidified materials were mixed with 7.5%, 10% and 12.5% of equal proportions of cement. The curing samples of nine kinds of solidified bodies were prepared after curing. Subsequently, the permeability coefficient was determined through the utilization of X-ray diffraction (XRD) and scanning electron microscopy (SEM). And cumulative radon concentrations in uranium tailings and samples were measured by RAD7. Thus, the radon exhalation rate of the original sample and the sample were determined. The experimental results show that the permeability coefficient of nine samples decreased with the quadratic function with the increase in the amount of curing agent. Microscopic scanning results show that there is a positive correlation among the radon exhalation rate, permeability coefficient and cementation degree. The best material for solidifying uranium tailings and radon insulation was blast furnace slag, followed by fly ash. Full article
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14 pages, 16751 KiB  
Article
Characterization of Seismic Dynamic Response of Uranium Tailings Dams Based on Discrete Element Method
by Ming Lan, Hongyu Huang and Yan He
Appl. Sci. 2024, 14(18), 8389; https://doi.org/10.3390/app14188389 - 18 Sep 2024
Cited by 1 | Viewed by 1068
Abstract
Tailings dams play a critical role in ensuring the safety of mining operations. However, earthquakes can cause breaches in these dams, resulting in significant casualties and property damage. This study investigates the dynamic response characteristics of uranium tailings dams subjected to seismic loading, [...] Read more.
Tailings dams play a critical role in ensuring the safety of mining operations. However, earthquakes can cause breaches in these dams, resulting in significant casualties and property damage. This study investigates the dynamic response characteristics of uranium tailings dams subjected to seismic loading, employing the discrete element method. It specifically analyzes how seismic wave amplitude, frequency, and the friction angle of tailings sand affect the dams’ dynamic response. The results reveal that the peak ground acceleration ratio (PGAR) exhibits an increasing–decreasing–increasing pattern with elevation. When the friction angle of the tailings sand exceeds 35°, the overall stability of the dam improves. Conversely, a friction angle below 25° significantly increases the risk of dam failure. Additionally, the dam shows a reduced dynamic response to seismic waves with frequencies exceeding 15 Hz. At lower frequencies, deformation and damage are primarily concentrated on the slope face, while at higher frequencies, damage is predominantly located at the bottom of the model. These findings provide a theoretical foundation and reference for the safe operation of tailings dams, highlighting their practical significance. Full article
(This article belongs to the Special Issue Recent Advances in Rock Mass Engineering)
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27 pages, 11053 KiB  
Article
Column-Test Data Analyses and Geochemical Modeling to Determine Uranium Reactive Transport Parameters at a Former Uranium Mill Site (Grand Junction, Colorado)
by Raymond H. Johnson, Aaron D. Tigar and C. Doc Richardson
Minerals 2022, 12(4), 438; https://doi.org/10.3390/min12040438 - 31 Mar 2022
Cited by 8 | Viewed by 2760
Abstract
The long-term release of uranium from residual sources at former uranium mill sites was often not considered in prior conceptual and numerical models, as contaminant removal focused on meeting radiological standards. To determine the reactive transport parameters, column tests were completed with various [...] Read more.
The long-term release of uranium from residual sources at former uranium mill sites was often not considered in prior conceptual and numerical models, as contaminant removal focused on meeting radiological standards. To determine the reactive transport parameters, column tests were completed with various influent waters (deionized water, site groundwater, and local river water) on sediment from identified areas with elevated uranium on the solid phase in (1) vadose-zone (VZ) sediments, (2) saturated-zone sediments with higher organic carbon content, and (3) both vadose- and saturated-zone sediments with additional gypsum content. The gypsum was precipitated when low-pH, high-sulfate, tailings fluids or acidic waste disposal water were buffered by natural aquifer calcite dissolution. In general, the resulting uranium release was higher in the sediments with greater uranium concentrations. However, the addition of deionized water (DI) to the VZ sediments delayed the uranium release until higher-alkalinity groundwater was added. Higher-alkalinity river water continued to remove uranium from the VZ sediments for an extended number of pore volumes, with the uranium being above typical standards. Thus, river flooding is more efficient at removing uranium from VZ sediments than precipitation events (DI water in column tests). Organic carbon provides a stronger uranium sorption surface, which can be explained with geochemical modeling or a larger constant sorption coefficient (Kd). Without organic carbon, the typical sorption in sands and gravels is easily measurable, but sorption is stronger at lower, water-phase uranium concentrations. This effect can be simulated with geochemical modeling, but not with a constant Kd. Areas with gypsum create situations in which geochemical sorption is more difficult to simulate, which is likely due to the presence of uranium within mineral coatings. All the above mechanisms for uranium release must be considered when evaluating remedial strategies. Column testing provides initial input parameters that can be used in future reactive transport modeling to evaluate long-term uranium release rates and concentrations. Full article
(This article belongs to the Special Issue Environmentally Sound In-Situ Recovery Mining of Uranium)
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11 pages, 2784 KiB  
Article
Occurrence and Distribution of Uranium in a Hydrological Cycle around a Uranium Mill Tailings Pond, Southern China
by Wenjie Ma, Bai Gao, Yadan Guo, Zhanxue Sun, Yanhong Zhang, Gongxin Chen, Xiaojie Zhu and Chunyan Zhang
Int. J. Environ. Res. Public Health 2020, 17(3), 773; https://doi.org/10.3390/ijerph17030773 - 26 Jan 2020
Cited by 26 | Viewed by 5900
Abstract
Uranium (U) mining activities, which lead to contamination in soils and waters (i.e., leachate from U mill tailings), cause serious environmental problems. However, limited research works have been conducted on U pollution associated with a whole soil-water system. In this study, a total [...] Read more.
Uranium (U) mining activities, which lead to contamination in soils and waters (i.e., leachate from U mill tailings), cause serious environmental problems. However, limited research works have been conducted on U pollution associated with a whole soil-water system. In this study, a total of 110 samples including 96 solid and 14 water samples were collected to investigate the characteristics of U distribution in a natural soil-water system near a U mining tailings pond. Results showed that U concentrations ranged from 0.09 ± 0.02 mg/kg to 2.56 × 104± 23 mg/kg in solid samples, and varied greatly in different locations. For tailings sand samples, the highest U concentration (2.56× 104 ± 23 mg/kg) occurred at the depth of 80 cm underground, whereas, for paddy soil samples, the highest U concentration (5.22 ± 0.04 mg/kg) was found at surface layers. Geo-accumulation index and potential ecological hazard index were calculated to assess the hazard of U in the soils. The calculation results showed that half of the soil sampling sites were moderately polluted. For groundwater samples, U concentrations ranged from 0.55 ± 0.04 mg/L to 3.36 ± 0.02 mg/L with a mean value of 2.36 ± 0.36 mg/L, which was significantly lower than that of percolating waters (ranging from 4.56 ± 0.02 mg/L to 12.05 ± 0.04 mg/L, mean 7.91 ± 0.98 mg/L). The results of this study suggest that the distribution of U concentrations in a soil-water system was closely associated with hydrological cycles and U concentrations decreased with circulation path. Full article
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13 pages, 6077 KiB  
Article
Laboratory Experimental Laws for the Radon Exhalation of Similar Uranium Samples with Low-Frequency Vibrations
by Zi-qi Cai, Xiang-yang Li, Bo Lei, Jing-fan Yuan, Chang-shou Hong and Hong Wang
Sustainability 2018, 10(8), 2937; https://doi.org/10.3390/su10082937 - 18 Aug 2018
Cited by 9 | Viewed by 4242
Abstract
It is the fact that there are lots of hazard incidents in underground uranium mines caused by radon but in-suit uranium samples were difficult to collect. Based on closed chamber method, three similar samples in different sealed ways were made in a laboratory [...] Read more.
It is the fact that there are lots of hazard incidents in underground uranium mines caused by radon but in-suit uranium samples were difficult to collect. Based on closed chamber method, three similar samples in different sealed ways were made in a laboratory with different material rations, namely uranium tailings, quartz sand, cement, iron powder and silicon powder to measure the radon concentrations with and without low-frequency vibrations, which was used by the experimental device for low-frequency vibration diffusion of radon. The results showed that the radon exhalation coming from the similar samples was influenced by the low frequency vibration; the results are presented as two-stage variations compared with the blank group. The radon exhalation increased with the rising vibration frequency when the frequency was 50 to 70 Hz, but fell slowly after reaching the peak radon exhalation rate. Analyses of the relations between the rock damage degree, changes in porosity and the occurrence of an inflection point in the radon exhalation rate in the samples found that they also increased when the frequency was between 0 to 80 in sample 3. The maximum porosity of the third samples was about 4.8% with a low-frequency vibration 60 Hz, while the maximum damage degree was about 0.07 at 50 Hz. Full article
(This article belongs to the Special Issue Nuclear Safety, Emergency, Security: Theory and Technology)
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