Search Results (9)

Extreme weather events are happening more frequently as a result of global climate change. Dust storms broke out in the spring of 2017 in China and drastically impacted the local air quality. In this study, a variety of data, including aerosol vertical profiles, surface particle concentration, meteorological parameters, and MODIS–derived aerosol optical depth, as well as backward trajectory analysis, were employed to analyze two dust events from April to May in Beijing. The dust plumes were mainly concentrated below 0.8 km, with peak PM10 values of 1000 μg·m⁻³ and 300 μg·m⁻³ in the two cases. The aerosols showed different vertical distribution characteristics. The pure dust in case 1 from 4 to 5 May 2017 had a longer duration (2 days) and presented a larger aerosol extinction coefficient (2.27 km⁻¹ at 355 nm and 1.25 km⁻¹ at 532 nm) than that of the mixed dust in case 2 on 17 April 2017 (2.01 km⁻¹ at 355 nm and 1.33 km⁻¹ at 532 nm). The particle depolarization ratio (PDR) remained constant (0.24 ± 0.03 in case 1) from the surface to 0.8 km in height. In contrast, the PDR profile in the mixed dust (case 2) layer was split into two regions—large values exceeding 0.15 above 0.6 km and small values of 0.11 ± 0.03 below 0.6 km. The influence of meteorological information on aerosol distribution was also investigated, and wind was predominant through the observing period. The pure dust in case 1 was mainly from Mongolia, with strong northwest winds, while the near-surface mixed pollution was caused by the combination of long-transported sand and local emission. Furthermore, lidar-derived profiles of dust mass concentrations in the two cases were presented. This study reveals the vertical characteristics of dust aerosols in the production and dissipation of localized dust events and confirms the efficacy of thorough observations with multiple approaches from the ground to space to monitor dust events in real time. Full article

The vertical aerosol layering of the troposphere is poorly documented in mountainous regions, particularly in the Alpine valleys, which are influenced by valley and mountain winds. To improve our knowledge of particulate matter trapped in the Annecy valley, synergetic measurements performed by a ground-based meteorological Raman lidar and a Rayleigh-Mie lidar aboard an ultralight aircraft were implemented as part of the Lacustrine-Water vApor Isotope inVentory Experiment (L-WAIVE) over Lake Annecy. These observations were complemented by satellite observations and Lagrangian modeling. The vertical profiles of aerosol optical properties (e.g., aerosol extinction coefficient (AEC), lidar ratio (LR), particle linear depolarization ratio (PDR)) are derived from lidar measurements at 355 nm during the period between 13 and 22 June 2019. The background aerosol content with an aerosol optical thickness (AOT) of 0.10 ± 0.05, corresponding to local–regional conditions influenced by anthropogenic pollution, has been characterized over the entirety of Lake Annecy thanks to the mobile ultralight payload. The aerosol optical properties are shown to be particularly variable over time in the atmospheric column, with mean LRs (PDRs) varying between 40 ± 8 and 115 ± 15 sr (2 ± 1 and 35 ± 2%). Those conditions can be disturbed by air masses that have recirculated over the valley, as well as by contributions from neighboring valleys. We have observed an important disruption in the atmospheric aerosol profiles by the arrival of an exceptionally dry air mass (RH ~ 30%), containing aerosols identified as coming from the Great Western Erg (AOT ~ 0.5, LR = 65 ± 10 sr, PDR = 20–35%) in the Sahara. These desert dust particles are shown to influence the entire atmospheric column in the Annecy valley. Such an experimental approach, coupling upward and downward lidar and spaceborne observation/Lagrangian modelling, was shown to be of significant interest for the long-term monitoring of the evolution of aerosol loads over deep valleys. It allows a better understanding of the influence of dust storms in the presence of severe convective weather processes. Full article

In this study, a combination of ground-based particulate matter measurements in synergy with space-borne CALIOP lidar recordings, meteorological observations, and reanalysis models have been used to study atmospheric air pollution over Amman, Jordan. The measurement was conducted over a 24-month period spanning from January 2018 to the end of December 2019. The CALIOP aerosol profiles and aerosol layer products version 4.21, level 2, with 5 km horizontal resolution were used to evaluate the vertical structure of the atmospheric constituent over the Amman region. The particle depolarization ratio (PDR) was extracted from CALIOP recordings and has been utilized to classify the type of atmospheric aerosols. This method reveals that the atmosphere above Amman mostly contains three different aerosol types including coarse-mode dust, fine-mode dust (polluted dust), and non-dust aerosols (pollution). Aerosols with 0 < ${\delta }_{\mathrm{p}}\le$ 0.075 are categorized as pollution, aerosols with 0.075 < ${\delta }_{\mathrm{p}}\le$ 0.20 as polluted dust, and aerosols with 0.20 < ${\delta }_{\mathrm{p}}\le$ 0.40 are classified as dust. Both the one- and two-step POlarization-LIdar PHOtometer Networking (POLIPHON) approaches have been applied to the CALIOP aerosol profile product to retrieve the vertical profile of the optical and micro-physical properties of each aerosol type. Lofted-layer top heights and layer thickness in the atmosphere above Amman during the study period were also extracted from the CALIOP aerosol layer products. The highest frequency of occurrence was observed for layers with a top height of 0.5 to 2.5 km with a second smaller peak at 3.5 km. The maximum frequency of the lofted layers (40% of cases) were observed with layer thickness below 0.5 km. For layers with a top height lower than 500 m above ground level, the atmosphere was mostly impacted by polluted dust and pollution aerosols. On the other hand, for layers with a top height above 2500 m agl, the atmosphere was contaminated by depolarizing dust particles. Full article

This study investigates the seasonal variation of dust aerosol vertical distribution using polarized Micropulse lidar (MPL) measurements at the Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) observatory from January 2013 to September 2017. For the first time, multi-year aerosol backscatter coefficients are retrieved at the ARM NSA site from MPL measurements and are consistent with co-located high spectral resolution lidar (HSRL) measurements. The high-quality aerosol backscatter coefficient retrievals are used to derive the particle depolarization ratio (PDR) at the wavelength of 532 nm, which is used to identify the presence of dust aerosols. The annual cycles of the vertical distributions of dust backscatter coefficient and PDR and dust aerosol optical depth (DAOD) show that aerosol loading has a maximum in late winter and early spring but a minimum in late summer and early autumn. Vertically, dust aerosol occurs in the entire troposphere in spring and winter and in the low and middle troposphere in summer and autumn. Because dust aerosols are effective ice nuclei, the seasonality of dust aerosol vertical distribution has important implications for the Arctic climate through aerosol–cloud–radiation interactions, primarily through impacting mixed-phase cloud processes. Full article

While pollen is expected to impact public human health and the Earth’s climate more and more in the coming decades, lidar remote sensing of pollen has become an important developing research field. To differentiate among the pollen taxa, a polarization lidar is an interesting tool since pollen exhibit non-spherical complex shapes. A key attribute is thus the lidar particle depolarization ratio (PDR) of pollen, which is however difficult to quantify as pollen are large and complex-shaped particles, far beyond the reach of light scattering numerical simulations. In this paper, a laboratory π-polarimeter is used to accurately evaluate the PDR of pure pollen, for the first time at the lidar exact backscattering angle of 180.0°. We hence reveal the lidar PDR of pure ragweed, ash, birch, pine, cypress and spruce pollens at 355 and 532 nm lidar wavelengths, as presented at the ELC 2021 conference. A striking result is the spectral dependence of the lidar PDR, highlighting the importance of dual-wavelength (or more) polarization lidars to identify pollen taxa. These spectral and polarimetric fingerprints of pure pollen, as they are accurate, can be used by the lidar community to invert multi-wavelength lidar polarization measurements involving pollen. Full article

The vertical structure of dust properties in desert sources is crucial for evaluating their long-range transportation and radiative forcing. To investigate vertical profiles of dust optical properties in the Taklimakan Desert, we conducted ground-based polarization Raman lidar measurements in Tazhong (83.39°E, 38.58°N, 1103 m above sea level), located at the center of the Taklimakan Desert in the summer of 2019. The lidar system developed by Lanzhou University for continuous network observation is capable of measuring polarization at 532 and 355 nm and detecting Raman signals at 387, 407, and 607 nm. The results indicate that dust aerosols in the central Taklimakan Desert were regularly lifted over 6 km during the summer with a mass concentration of 400–1000 µg m⁻³, while the majority of the dust remained restricted within 2 km. Moreover, the height of the boundary layer can reach 5–6 km in the afternoon under the strong convention. Above 3 km, dust is composed of finer particles with an effective radius (Reff.) less than 3 μm and a Ångström exponent (AE) related to the extinction coefficient (AEE)_532,355 greater than 4; below 3 km, however, dust is dominated by coarser particles. In addition, the particle depolarization ratios (PDR) of Taklimakan dust are 0.32 ± 0.06 at 532 nm and 0.27 ± 0.04 at 355 nm, while the lidar ratios (LRs) are 49 ± 19 sr at 532 nm and 43 ± 12 sr at 355 nm. This study firstly provides information on dust vertical structure and its optical properties in the center of the desert, which may aid in further evaluating their associated impacts on the climate and ecosystem. Full article

Previous studies have shown that dust aerosols may accelerate the melting of snow and glaciers over the Tibetan Plateau. To investigate the vertical structure of dust aerosols, we conducted a ground-based observation by using multi-wavelength polarization lidar which is designed for continuous network measurements. In this study, we used the lidar observation from September to October 2020 at the Ruoqiang site (39.0°N, 88.2°E; 894 m ASL), located at the junction of the Taklimakan Desert–Tibetan Plateau. Our results showed that dust aerosols can be lifted up to 5 km from the ground, which is comparable with the elevation of the Tibetan Plateau in autumn with a mass concentration of 400–900 μg m⁻³. Moreover, the particle depolarization ratio (PDR) of the lifted dust aerosols at 532 nm and 355 nm are 0.34 ± 0.03 and 0.25 ± 0.04, respectively, indicating the high degree of non-sphericity in shape. In addition, extinction-related Ångström exponents are very small (0.11 ± 0.24), implying the large values in size. Based on ground-based lidar observation, this study proved that coarse non-spherical Taklimakan dust with high concentration can be transported to the Tibetan Plateau, suggesting its possible impacts on the regional climate and ecosystem. Full article

Ground-based measurements were carried out during field campaigns in April–June of 2010, 2011 and 2012 over northwestern China at Minqin, the Semi-Arid Climate and Environment Observatory of Lanzhou University (SACOL) and Dunhuang. In this study, three dust cases were examined, and the statistical results of dust occurrence, along with physical and optical properties, were analyzed. The results show that both lofted dust layers and near-surface dust layers were characterized by extinction coefficients of 0.25–1.05 km⁻¹ and high particle depolarization ratios (PDRs) of 0.25–0.40 at 527 nm wavelength. During the three campaigns, the frequencies of dust occurrence retrieved from the lidar observations were all higher than 88%, and the highest frequency was in April. The vertical distributions revealed that the maximum height of dust layers typically reached 7.8–9 km or higher. The high intensity of dust layers mostly occurred within the planetary boundary layer (PBL). The monthly averaged PDRs decreased from April to June, which implies a dust load reduction. A comparison of the relationship between the aerosol optical depth at 500 nm (AOD₅₀₀) and the Angstrom exponent at 440–870 nm (AE_440–870) confirms that there is a more complex mixture of dust aerosols with other types of aerosols when the effects of human activities become significant. Full article

In June 2013, a ground-based mobile lidar performed the ~10,000 km ride from Paris to Ulan-Ude, near Lake Baikal, profiling aerosol optical properties in the cities visited along the journey and allowing the first comparison of urban aerosols optical properties across Eurasia. The lidar instrument was equipped with N₂-Raman and depolarization channels, enabling the retrieval of the 355-nm extinction-to-backscatter ratio (also called Lidar Ratio (LR)) and the linear Particle Depolarization Ratio (PDR) in the urban planetary boundary or residual layer over 11 cities. The optical properties of pollution particles were found to be homogeneous all along the journey: no longitude dependence was observed for the LR, with most values falling within the 67–96 sr range. There exists only a slight increase of PDR between cities in Europe and Russia, which we attribute to a higher fraction of coarse terrigenous particles lifted from bad-tarmac roads and unvegetated terrains, which resulted, for instance, in a +1.7% increase between the megalopolises of Paris and Moscow. A few lower LR values (38 to 50 sr) were encountered above two medium size Siberian cities and in an isolated plume, suggesting that the relative weight of terrigenous aerosols in the mix may increase in smaller cities. Space-borne observations from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), retrieved during summer 2013 above the same Russian cities, confirmed the prevalence of aerosols classified as “polluted dust”. Finally, we encountered one special feature in the Russian aerosol mix as we observed with good confidence an unusual aerosol layer displaying both a very high LR (96 sr) and a very high PDR (20%), even though both features make it difficult to identify the aerosol type. Full article