Search Results (7)

TEM₀₀-mode operation is a requirement in many laser-based applications due to the small divergence and high-power density of the emitted laser beam. A solar laser scheme was designed and numerically studied with the goal of increasing the solar-to-laser power conversion efficiency in the TEM₀₀-mode operation. The collection and primary concentration of sunlight was performed via twelve sets of folding mirrors and Fresnel lenses, toward a laser head composed of a fused silica torus volume and seven Ce:Nd:YAG rods, in a side-pump configuration. With this scheme, TEM₀₀-mode laser power totaling 212.39 W could potentially be produced from seven beams, with six of them being 32.60 W each and with $M_x^2$ = 1.00,$M_y^2$ = 1.01 quality factors. Notably, 35.40 W/m² collection efficiency and, most importantly, 3.73% solar-to-laser power conversion efficiency were numerically achieved. The latter efficiency value represents a 1.81-time improvement over the experimental record, established with a prototype that had a single Ce:Nd:YAG rod in an end-side pump configuration. Full article

Low-cost, lightweight, and easily available Fresnel lenses are a more alluring choice for solar laser power production, when compared to the costly and complex heliostat-parabolic mirror systems. Therefore, a seven-rod solar laser head was designed and numerically studied to enhance the efficiency in TEM₀₀-mode laser power production, employing six Fresnel lenses with 10 m² total collection area for collection and concentration of sunlight. Six folding mirrors redirected the solar rays towards the laser head, composed of six fused silica aspheric lenses and rectangular compound parabolic concentrators paired together for further concentration, and a cylindrical cavity, in which seven Nd:YAG rods were mounted and side-pumped. With conventional rods, total TEM₀₀-mode laser power reached 139.89 W, which is equivalent to 13.99 W/m² collection efficiency and 1.47% solar-to-TEM₀₀-mode laser power conversion efficiency. More importantly, by implementing rods with grooved sidewalls, the total laser power was increased to 153.29 W, corresponding to 15.33 W/m² collection and 1.61% conversion efficiencies. The side-pumping configuration and the good thermal performance may ensure that the seven-grooved-rod system has better scalability than other previously proposed schemes. Full article

Aside from the industry-standard Gaussian intensity profile, top hat and non-conventional laser beam shapes, such as doughnut-shaped profile, are ever more required. The top hat laser beam profile is well-known for uniformly irradiating the target material, significantly reducing the heat-affected zones, typical of Gaussian laser irradiation, whereas the doughnut-shaped laser beam has attracted much interest for its use in trapping particles at the nanoscale and improving mechanical performance during laser-based 3D metal printing. Solar-pumped lasers can be a cost-effective and more sustainable alternative to accomplish these useful laser beam distributions. The sunlight was collected and concentrated by six primary Fresnel lenses, six folding mirror collectors, further compressed with six secondary fused silica concentrators, and symmetrically distributed by six twisted light guides around a 5.5 mm diameter, 35 mm length Nd:YAG rod inside a cylindrical cavity. A top hat laser beam profile (M_x² = 1.25, M_y² = 1.00) was computed through both ZEMAX^® and LASCAD^® analysis, with 9.4 W/m² TEM₀₀ mode laser power collection and 0.99% solar-to-TEM₀₀ mode power conversion efficiencies. By using a 5.8 mm laser rod diameter, a doughnut-shaped solar laser beam profile (M_x² = 1.90, M_y² = 1.00) was observed. The 9.8 W/m² TEM₀₀ mode laser power collection and 1.03% solar-to-TEM₀₀ mode power conversion efficiencies were also attained, corresponding to an increase of 2.2 and 1.9 times, respectively, compared to the state-of-the-art experimental records. As far as we know, the first numerical simulation of doughnut-shaped and top hat solar laser beam profiles is reported here, significantly contributing to the understanding of the formation of such beam profiles. Full article

High-resolution scanning transmission electron microscopy (STEM) images of human tooth enamel crystals, mainly in the high-angle annular dark-field (STEM-HAADF) mode, are presented in this work along the [1000], [10-11]. and [1-210] directions. These images allow knowing some structural details at the nanometric level of the human tooth enamel crystals and of the central dark line (CDL) observed at their centers. The transmission electron microscopy (TEM) and high-resolution TEM (HRTEM) images of the CDL showed the Fresnel contrast. In the STEM bright-field (STEM-BF) and annular-dark-field (STEM-ADF) images, the CDL was observed as an unstrain hydroxyapatite (HAP)-like zone but surrounded by a strained zone. In the STEM-HAADF images, the CDL appeared with a weak contrast, and its contrasts’ thickness was registered between 3 and 8 Å. The arrangement obtained in the STEM-HAADF images by identifying the bright points with the Ca atoms produced the superposition of the HAP atomic sites, mainly along the [0001] direction. The findings provide further information on the structure details at the center of enamel crystals, which favors the anisotropic carious dissolution at the CDL. Full article

The article concerns the rarely described magnetic domain structure of Heusler alloys in the case of a single crystal [100]-oriented Co-Ni-Ga alloy. The structure of the magnetic domains of the alloy was compared in two states: in the quenched and additionally aged state. Ageing led to precipitation of the spherical phase γ’ nanoparticles (Co-rich, FCC lattice with a = 0.359 nm). Lorentz transmission electron microscopy observation methods combined with cooling and in situ heating of the sample in the transmission electron microscope in the temperature range from 140 K to 300 K were combined to observe the magnetic domain structure. Significant differences in the dimensions and morphology of magnetic domain boundaries have been demonstrated. The quenched sample showed no change in stripe domain structure when the aged sample showed significant development of branching magnetic structures. This may be due to a change in the chemical composition of the matrix resulting from a decrease in cobalt and nickel content at the expense of precipitations. Full article

The terahertz time-domain spectroscopy (THz-TDS) technique has been used to obtain transmission THz-radiation spectra of polymer nanocomposites containing a controlled amount of exfoliated graphene. Graphene nanocomposites (1 wt%) that were used in this work were based on poly(ethylene terephthalate-ethylene dilinoleate) (PET-DLA) matrix and were prepared via a kilo-scale (suitable for research and development, and prototyping) in-situ polymerization. This was followed by compression molding into 0.3-mm-thick and 0.9-mm-thick foils. Transmission electron microscopy (TEM) and Raman studies were used to confirm that the graphene nanoflakes dispersed in a polymer matrix consisted of a few-layer graphene. The THz-radiation transients were generated and detected using a low-temperature–grown GaAs photoconductive emitter and detector, both excited by 100-fs-wide, 800-nm-wavelength optical pulses, generated at a 76-MHz repetition rate by a Ti:Sapphire laser. Time-domain signals transmitted through the nitrogen, neat polymer reference, and 1-wt% graphene-polymer nanocomposite samples were recorded and subsequently converted into the spectral domain by means of a fast Fourier transformation. The spectral range of our spectrometer was up to 4 THz, and measurements were taken at room temperature in a dry nitrogen environment. We collected a family of spectra and, based on Fresnel equations, performed a numerical analysis, that allowed us to extract the THz-frequency-range refractive index and absorption coefficient and their dependences on the sample composition and graphene content. Using the Clausius-Mossotti relation, we also managed to estimate the graphene effective dielectric constant to be equal to ~7 ± 2. Finally, we extracted from our experimental data complex conductivity spectra of graphene nanocomposites and successfully fitted them to the Drude-Smith model, demonstrating that our graphene nanoflakes were isolated in their polymer matrix and exhibited highly localized electron backscattering with a femtosecond relaxation time. Our results shed new light on how the incorporation of exfoliated graphene nanoflakes modifies polymer electrical properties in the THz-frequency range. Importantly, they demonstrate that the complex conductivity analysis is a very efficient, macroscopic and non-destructive (contrary to TEM) tool for the characterization of the dispersion of a graphene nanofiller within a copolyester matrix. Full article

We report on high-order harmonic (HHG) two-source interferometry (TSI) in molecular gases. We used a 0-\(\pi\) phase plate to create two bright spots at the focus of a lens by converting a Gaussian laser beam into a TEM please define \(_{01}\) Transverse Electromagnetic Mode. The two bright foci produce two synchronized HHG sources. One of them is used to probe on-going dynamics in the generating medium, while the other serves to heterodyne the signal. The interference of the emissions in the far–field gives access to the phase difference between the two sources. In self–probing HHG phase spectroscopy, one of the two sources is used as a reference while the other one probes some on goin dynamics in the generating medium. We first compute overlap integrals to investigate the mode conversion efficiency. We then establish a clear relation between the laser phase-front curvature and the far-field overlap of the two HHG beams. Both Fresnel diffraction calculations and an experimental lens position scan are used to reveal variations of the phase front inclination in each source. We show that this arrangement offers \(\frac{\lambda_{XUV}}{100}\) precision, enabling extremely sensitive phase measurements. Finally, we use this compact setup for TSI and measure phase variations across the molecular alignment revival of nitrogen and in vibrating sulfur hexafluoride. In both gases, the phase variations change sign around the ionization threshold of the investigated molecule. Full article