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Article

State of Health Estimation of Lithium-Ion Battery Based on Novel Health Indicators and Improved Support Vector Regression

1
School of Information and Control Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China
2
School of Architecture, Xi’an University of Architecture and Technology, Xi’an 710055, China
3
School of Mechanical and Electrical Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China
4
School of Materials Science and Engineering, Xi’an University of Architecture and Technology, Xi’an 710055, China
*
Authors to whom correspondence should be addressed.
Batteries 2025, 11(10), 347; https://doi.org/10.3390/batteries11100347
Submission received: 31 July 2025 / Revised: 15 September 2025 / Accepted: 17 September 2025 / Published: 23 September 2025

Abstract

Accurate estimation of the state of health (SOH) is a critical function of battery management system (BMS), essential for ensuring the safe and stable operation of lithium-ion batteries. To improve estimation precision, this paper proposes a novel health indicator (HI) construction method and an improved support vector regression (SVR) approach. First, the convolution operation is applied to discharge voltage data to extract new HIs that characterize battery aging; their correlations are then verified. Second, principal component analysis (PCA) is employed to reduce input dimensionality and computational burden. Third, to address the challenge of SVR parameter selection, an improved sparrow search algorithm (ISSA) is proposed for parameter optimization. Finally, the proposed method is validated using both the NASA dataset and a laboratory experimental dataset, with comparisons against existing approaches. The results show that the method achieves accurate SOH estimation under various aging conditions, demonstrating its effectiveness, robustness, and practical potential.

1. Introduction

With rapid societal development, growing requirements for energy, fossil energy shortages, and worsening environmental deterioration are becoming increasingly serious, and all countries are actively looking for clean and efficient new energy that can replace traditional oil energy [1]. According to the white paper “China’s Energy Development in the New Era”, China will vigorously develop new energy and related industries, among which the electric vehicle is an important choice for sustainable development [2]. Lithium-ion batteries, with their high energy density, long service life, low self-discharge rate, lack of memory effect, and other excellent characteristics, have found extensive applications in electric vehicles, mobile phones, and other electronic devices [3,4]. However, their performance inevitably degrades over time due to electrode reactions and environmental factors, which may impair equipment operation or even cause safety incidents [5,6]. Effective battery management system (BMS) is therefore essential, and accurate estimation of state of health (SOH) is a critical component. SOH estimation enables the tracking of battery aging and is fundamental to reliable and safe operation [7,8,9], with SOH typically defined as the ratio of current capacity to nominal capacity, i.e.,
S O H = Q c u r r e n t Q n o m i n a l × 100 %
Lately, numerous research studies have been performed on the SOH estimation of lithium-ion batteries, and the existing methodologies can be broadly distributed into three groups: direct measurement method, model-based method, and data-driven method [10,11,12]. The direct measurement method determines SOH by discharge tests, directly measuring capacity, internal resistance, or impedance. Shim et al. [13] analyzed changes in electrode properties using techniques such as impedance spectroscopy, X-ray diffraction, and atomic force microscopy, identifying causes of capacity decline. Galeotti et al. [14] applied impedance spectroscopy to four lithium-ion batteries and established a link between ohmic resistance and available capacity to estimate SOH quickly. Although this method offers high accuracy and clear principles, it is limited to laboratory settings and offline measurements.
The model-based method establishes aging mechanism models of lithium-ion batteries, expressing physical and chemical changes through equations to simulate internal reactions and degradation. Wei et al. [15] proposed an online identification battery model and used the Kalman filter and the recursive least square method to achieve dual estimation of the charging state and capacity on multiple time scales. Experimental results showed that the proposed method can estimate model parameters and the charging state and capacity in real time, with a fast convergence speed and high precision. Lyu et al. [16] introduced a novel particle filter structure by simulating the electrochemical model of the battery charge and discharge process, and the experimental verification showed that the particle filter based on the electrochemical model has higher estimation precision. However, these models are complex, require many parameters, and are difficult to construct perfectly, limiting their practical application.
Data-driven methods circumvent the complex analysis of internal aging mechanisms by directly extracting salient features from monitored battery states [17]. These approaches demonstrate high estimation accuracy and real-time capability, and they have been widely applied to SOH estimation for lithium-ion batteries. Xia et al. [18] extracted robust aging features from reconstructed voltage curves and integrated incremental capacity and differential voltage analysis with an improved BiGRU-attention model to jointly predict battery SOH and RUL. Chen et al. [19] proposed a novel deep learning framework that denoises input signals and adaptively focuses on critical multi-scale features for accurate SOH and SOC estimation under complex operating conditions. Zhao et al. [20] combined Wasserstein distance-based similarity features, voltage-position encoding, and convolutional neural networks (CNNs) to perform robust SOH estimation from incomplete charging profiles. Liu et al. [21] transformed one-dimensional charging voltage time-series data into two-dimensional representations using the Gramian angular summation field and applied ResNet for SOH estimation. Among data-driven methods, attention and transformer-based frameworks have gained wide attention in recent years. By capturing long-range dependencies and adaptively focusing on critical features, they offer strong potential for improving SOH estimation accuracy and robustness across diverse operating conditions. Gu et al. [22] and Bai et al. [23] both proposed a hybrid CNN-transformer framework for SOH prediction. They demonstrated that combining these architectures significantly improved feature representation and led to more accurate and robust SOH prediction. Zhu et al. [24] and Zhang et al. [25] both employed transformer-based architectures combined with convolutional modules to achieve multi-feature fusion and SOH prediction. By enhancing the transformer’s ability to capture local features while integrating diverse health indicators, they demonstrated an improved accuracy and robustness in lithium-ion battery SOH estimation.
In summary, although data-driven methods have made progress in SOH estimation, significant challenges remain. Existing studies often rely on health indicators (HIs) directly derived from raw voltage or capacity curves, which makes them highly sensitive to noise and external interference. Moreover, most data-driven models use parameters chosen heuristically, without systematic optimization, which weakens model generalization and prediction accuracy. As shown in Table 1, the proposed ISSA-SVR is presented alongside representative literature on recent advanced methods for comparison.
To address these gaps, this paper makes the following contributions:
  • We propose a new set of HIs extracted from voltage convolution sequences, which emphasize cycle-to-cycle morphological changes and provide robust descriptors of battery aging.
  • The extracted HIs are quantitatively analyzed for their correlation with SOH, and principal component analysis (PCA) is applied to remove redundancy and reduce model input complexity.
  • An improved sparrow search algorithm (ISSA) is developed to optimize the critical parameters of a support vector regression (SVR) model, enhancing both robustness and accuracy in SOH estimation.
In addition, the work also provides new insight into battery degradation modeling by showing that convolution-based indicators capture electrochemical aging signatures embedded in voltage profiles, and by demonstrating how metaheuristic–regression integration can effectively represent the inherently nonlinear trajectory of SOH evolution.

2. Battery Data Analysis and Feature Extraction

In this paper, two battery datasets are used to verify the proposed SOH estimation method. One is the NASA dataset from the PCOE Research Center [26]. The other is the T1 and T2 battery dataset obtained from controlled laboratory aging experiments.

2.1. Battery Aging Dataset Description

The NASA dataset consists of 18,650 lithium-ion batteries with a nominal capacity of 2 Ah, tested under an ambient temperature of 24 °C. During the experiments, the batteries were charged at a constant current of 1.5 A until the terminal voltage reached 4.2 V, followed by constant-voltage charging until the current decreased to 20 mA. Throughout this process, terminal voltage, charging temperature, charging current, and time data were recorded. The discharge process was then performed at a constant current of 2 A until the terminal voltage reached the cut-off limit, at which point terminal voltage, discharge temperature, discharge current, time, and battery capacity were measured. The experimental information on this dataset is summarized in Table 2, and the corresponding capacity degradation curve is shown in Figure 1.
The second dataset used in this study was obtained from a laboratory charge–discharge test platform, with the experimental setup illustrated in Figure 2. The platform consists of an MHW-200 constant-temperature test chamber developed by Newell Laboratories, a battery charge–discharge test channel, and a computer system for real-time monitoring and data acquisition. The test objects are two standard 18,650-type lithium-ion cells with LiCoO2 cathodes and graphite anodes, with detailed specifications provided in Table 3. The experiments employed a constant-current charging, constant-voltage charging, and constant-current discharging protocol at an ambient temperature of 24 °C, and the corresponding data were recorded throughout the aging process. The experimental details are summarized in Table 4, and the capacity degradation curve is shown in Figure 3. Note that parameters such as ambient temperature, charge/discharge current, and voltage thresholds were precisely regulated for all experiments to isolate cycle-based aging.

2.2. Feature Extraction

Extracting appropriate HIs that accurately reflect the SOH of a battery is a critical step in data-driven methods, as it directly affects the estimation precision of the model. Using the B0018 battery as a case study, the novel HI extraction process proposed in this paper is illustrated in Figure 4. Since the charging process is generally more controlled, HIs are extracted from the discharge process. In each charge–discharge cycle, the discharge voltage decreases gradually at first and then more rapidly; with an increasing cycle number, the rate at which the terminal voltage reaches the cut-off threshold also accelerates. To capture this degradation behavior, discharge voltage was selected as the basis for HI extraction. Because raw data collection is susceptible to external noise, a convolution operation was applied to two adjacent discharge voltage sequences to enhance feature extraction. As shown in Figure 4, the convolution sequence exhibits clear trends as cycling progresses, with the span, peak value, and peak horizontal coordinate gradually all decreasing. Based on this observation and analysis, nine HIs were selected to characterize battery aging: span value, integral value, kurtosis, peak value, peak abscissa coordinate, peak slope, fuzzy entropy, energy value, and variance.
Convolution-based methods, particularly CNNs and their variants, have been widely applied in signal-processing-related areas to address problems such as noise suppression, feature extraction, and information enhancement [27,28,29,30]. The convolution operation describes the process by which two functions or sequences produce a third function or sequence by a specific integration or summation operation, expressed as
y ( n ) = ( x h ) ( n ) = m = + x ( m ) h ( n m )
The convolution operation has translation invariance, meaning that the extracted features remain valid regardless of their position in the input sequence. By focusing on local regions rather than the entire sequence, convolution provides spatial locality, which improves efficiency and makes it well suited for processing long input data. In addition, convolution acts as a smoothing and filtering mechanism. It suppresses high-frequency noise and highlights low-frequency trends that are closely related to gradual battery degradation. This allows the method to emphasize nonlinear aging patterns and makes aging-related patterns more distinguishable than in raw voltage profiles.
In addition, Pearson correlation coefficient (PCC) is utilized to evaluate the correlation between extracted HIs and battery SOH, and its expression is shown as follows:
P C C = i = 1 n ( z i z ¯ ) ( q i q ¯ ) i = 1 n ( z i z ¯ ) 2 i = 1 n ( q i q ¯ ) 2
where z and q represent HIs and SOH, respectively.
The PCC value range is within [−1, 1]. As the absolute value approaches 1, the correlation becomes stronger. PCC values for each battery are presented in Figure 5. It is notable that the worst correlation between HIs extracted in this paper and battery SOH is between 0.6 and 0.8, indicating a strong correlation between variables, and the rest are above 0.8, indicating an extremely strong correlation between variables. That is, the nine extracted HIs can effectively represent the battery degradation, which proves the rationality and effectiveness of the feature selection.

2.3. HI Optimization

2.3.1. PCA-Based Dimensionality Reduction Method

Considering the computational burden of the ISSA-SVR model and the presence of linear correlations among certain HIs, which leads to information redundancy, it is necessary to optimize the extracted HIs. PCA is a statistical analysis technique used for data compression and feature extraction. It uses orthogonal transformation to convert a group of correlated factors into a group of independent new factors, which can not only effectively reduce the data dimension but also retain relatively important information in the original data and reduce the complexity of the data [31,32]. The primary calculation processes of PCA are as described next.
Suppose there are n p-dimensional data x j = ( x j 1 , x j 2 , , x j p ) T , j = 1 , 2 , , n , construct a standardized sample matrix:
Z i j = x i j x ¯ j s j , i = 1 , 2 , , n ; j = 1 , 2 , , p
x ¯ j = i = 1 n x i j n , s j = i = 1 n ( x i j x ¯ j ) 2 n 1
Calculate the correlation coefficient matrix R for the standardized matrix Z :
R = Z T Z n 1
Solve the characteristic equation of the correlation coefficient matrix R to determine its principal components:
R λ I p = 0
j = 1 p λ j j = 1 p λ j δ
where δ is the threshold for the sum of the contributions of the principal components, p , which can be determined through δ .
The unit eigenvector b j o is obtained by solving the following equation:
R b = λ j b
Convert standardized variables to principal components:
U i j = z i T b j o , j = 1 , 2 , , p

2.3.2. HIs Optimization Results

The extracted HIs are optimized according to PCA, revealing the contribution percentages of individual principal components, as detailed in Table 5. The total contribution rates of the first two principal components of each battery are 98.41%, 97.70%, 97.95%, 98.46%, 99.39%, and 99.92%, respectively. Generally speaking, if the contribution rate of the principal components reaches 97%, it means that it is sufficient to describe the characteristic information contained in the original data. In other words, the first two principal components of each battery can be used as HIs reflecting the battery aging phenomenon, which significantly reduces the input size of the model and is conducive to the subsequent SOH estimation work.

3. ISSA-SVR Method

3.1. Support Vector Regression

Support vector machine (SVM) is a linear classifier based on the maximum margin principle, which identifies an optimal hyperplane for data separation [33]. For regression tasks, it is extended as support vector regression (SVR), which seeks an optimal regression hyperplane that fits the data within a narrow margin while minimizing deviations [34]. Given the nonlinear characteristics of lithium-ion battery capacity data, SVR is well-suited to SOH estimation. It reduces prediction error, is robust to outliers, and demonstrates a strong generalization ability, making it effective for nonlinear regression problems [35,36].
Assume a given sample set S = x i , y i n ( x i X = R n , y i Y = R ), where x i is the i t h input eigenvector, y i is the corresponding output vector, and n is the number of samples. Mapping the sample set from a low-dimensional space to a high-dimensional space through nonlinear mapping is defined as follows:
f ( x ) = w ϕ ( x ) + b
where x is the input data; ϕ ( x ) is the nonlinear mapping function; w is the weight; and b is the intercept.
Following the structural risk minimization principle, determining f ( x ) equates to solving an optimization task:
1 2 w 2 + C i n L ( f ( x i ) , y i )
where L is the loss function; and C is the penalty factor.
Introducing the insensitive loss function ε ( ε > 0 ) yields
L ( f ( x ) , y ) = 0 , f ( x ) y ε f ( x ) y ε , f ( x ) y > ε
Then, the SVR expression is
f ( x ) = w ϕ ( x ) + b = i n ( α i α ^ i ) K ( x i , x ) + b
where α i and α ^ i are Lagrange multipliers; and K ( x i , x ) is the kernel function, of which four main types are commonly used: linear kernel function, polynomial kernel function, sigmoid kernel function, and radial basis kernel function (RBF). Among them, RBF kernel function has fewer parameters and can realize high-dimensional mapping, and so it is the most commonly used kernel function [37]. Therefore, this paper chooses RBF as the kernel function of SVR, which is stated as follows:
K R B F ( x i , x ) = exp ( 1 2 σ 2 x i x 2 )
where σ is the width coefficient of RBF.
The penalty factor C and kernel parameter σ impact the generalization and fitting performance of the SVR model directly, but there is no effective method to guide the parameter selection, so to acquire an accurate SVR prediction model, it is essential to optimize the parameters of SVR.

3.2. Sparrow Search Algorithm

The sparrow search algorithm (SSA), proposed by Xue and Shen in 2020, is a population-based metaheuristic with a strong optimization ability, fast convergence, and high robustness compared to many other swarm algorithms [38]. Inspired by the foraging and anti-predation behavior of sparrows, the population is divided into three roles: discoverers, joiners, and scouters. Discoverers, with higher energy reserves, guide the search for food sources, while joiners follow their paths. A small proportion act as scouters, issuing warnings when threats appear. Although individual roles may change during the search process, the proportions of discoverers and joiners remain constant. The main steps of SSA are summarized as follows:
Step 1: Population initialization.
X = l b + r a n d ( u b l b )
where u b and l b symbolize the maximum and minimum position boundaries of the population, respectively.
Step 2: Update the discoverer position.
x i , j t + 1 = x i , j t exp ( i α i t e r max ) , R 2 < S T x i , j t + Q L , R 2 S T
where α is a random number of [0, 1]; i t e r max is the maximum iteration quantity; Q is a random number obeying a normal distribution; R 2 is a random number of [0, 1] and denotes the warning value; S T is a random number of [0.5, 1] and denotes the safety value; and L is a one-row, j -dimensional, all-1 matrix.
Step 3: Update the joiner position.
x i , j t + 1 = Q exp ( x w o r s t t x i , j t i 2 ) , i > n 2 x p t + 1 + x i , j t x p t + 1 A + L , o t h e r w i s e
where A is a 1 × d matrix with elements randomly assigned 1 or −1; and A + = A T ( A A T ) 1 .
Step 4: Scouter and early warning.
x i , j t + 1 = x b e s t t + β ( x i , j t x b e s t t ) , f i f g x i , j t + K ( x i , j t x w o r s t t f i f w + ε ) , f i = f g
where β is a random number obeying a normal distribution with mean 0 and variance 1; K is a random number of [−1, 1], with the positive and negative indicating the orientation the sparrow is moving, and the size indicating the step control parameter; f i denotes the current individual fitness value; and f g denotes the current minimum fitness value.
Step 5: Calculate the fitness value and adjust the sparrow location.
Step 6: Verify if the stopping criterion is fulfilled—if so, output the optimal sparrow position; otherwise, return to step 2.

3.3. Improved Sparrow Search Algorithm

The traditional SSA can effectively search small solution spaces and often finds good local optima due to its strong local search ability. It is simple, easy to understand, and straightforward to implement. However, it suffers from slow convergence, a weak global search capability, and a tendency to become trapped in local minima. To address these limitations, this paper proposes an improved SSA (ISSA), which enhances population diversity and global exploration, enabling the algorithm to escape local optima and achieve higher convergence accuracy.
Chaotic mapping is introduced to initialize the population due to its advantages over random initialization. The original SSA often suffers from low population diversity, while chaotic mapping exhibits high complexity and stochasticity as a nonlinear process. Using them instead of conventional random methods can yield more stochastic sequences, leading to a more uniform population distribution, improved ergodicity, and enhanced global search ability [39]. Thus, Bernoulli mapping is employed to initialize the population, given by
z k + 1 = z k / ( 1 ρ ) , z k ( 0 , 1 ρ ] ( z k 1 + ρ ) / ρ , z k ( 1 ρ , 1 )
where k is the number of chaotic iterations; and ρ is a control parameter.
The sine–cosine algorithm (SCA) is introduced to enhance the discoverer position update in the SSA. In the SSA, the discoverer guides joiners toward food sources. However, if the discoverer becomes trapped in a local optimum, it may lead numerous joiners to converge prematurely, causing population stagnation and increasing the risk of local convergence. The SCA, proposed by Mirjalili in 2016 [40], is a stochastic optimization method that utilizes sine and cosine functions for an oscillatory search. It is characterized by simplicity, few parameters, and ease of implementation. In this work, the SCA is incorporated to modify Equation (17) in the SSA, enabling balanced global exploration and local exploitation through adaptive sine–cosine oscillations. The improved equation is as follows:
x i , j t + 1 = w x i , j t + r 1 sin ( r 2 ) r 3 x b e s t t x i , j t , R 2 < S T w x i , j t + r 1 cos ( r 2 ) r 3 x b e s t t x i , j t , R 2 S T
w = e t i t e r max 1 e 1
r 1 = a ( 1 t T )
where a is a constant, usually set to 1 or 2; t is the number of current iterations; T is the maximum number of iterations; and r 2 , r 3 are random numbers of [0, 2π], which control the travel distance of sparrows and the effect of the optimal individual on the last position of sparrows, respectively. The improved expression can maintain the individual diversity and enhance the global search capability of the algorithm by applying the oscillation change characteristic of the sine–cosine model to the particle position.
To mitigate premature convergence and limited diversity caused by joiners closely following discoverers in the SSA, a spiral search strategy from the whale optimization algorithm [41] is introduced. This dynamic update mechanism enhances movement flexibility, thereby improving population diversity, search efficiency, and optimization accuracy [42]. Accordingly, Equation (18) in the SSA is modified as follows:
x i , j t + 1 = cos ( 2 π l ) Q exp ( x w o r s t t x i , j t i 2 + z l ) , i > n 2 x p t + 1 + x i , j t x p t + 1 A + L e z l cos ( 2 π l ) , o t h e r w i s e
z = e k cos [ π ( 1 i i max ) ]
where k is the change coefficient; and l is a uniformly distributed random number in [−1, 1].
Owing to its stability and strong approximation properties, Gaussian perturbation exhibits an excellent local search performance. Applying this strategy to global-best individuals in the SSA facilitates an escape from local optima and enhances global exploration. The Gaussian perturbation is defined as follows:
x g b e s t t = x b e s t t ( 1 + G a u s s i a n ( u , σ 2 ) )
where x b e s t t is the current global optimal individual; x g b e s t t is the global optimal entity after Gaussian perturbation; u is the mean value of a Gaussian distribution; and σ is the standard deviation of the distribution.

3.4. ISSA-SVR

In this paper, the ISSA is employed to optimize the penalty factor C and kernel parameter σ in SVR, so as to enhance the estimation precision of the model. Compared with the original SSA, the ISSA can not only effectively prevent the SSA from falling into local optima but also enhance the rate of convergence and optimization precision of the SSA. In the ISSA-SVR model, the mean square error (MSE) is taken as its fitness function, and its expression is as follows:
f i t n e s s = M S E = 1 N i = 1 N ( y i y ^ i ) 2
where N is the number of training samples; y i is the actual value of the i t h training sample; and y ^ i is the predicted value of the i t h training sample. The main parameters of the ISSA-SVR are described in Table 6.
ISSA-SVR steps are described as follows:
(1)
Data preprocessing: Normalized processing of input data, specifically expressed as
x n o r m = x i x min x max x min
where x n o r m denotes the normalized data; x i denotes the original data; and x min and x max are the minimum and maximum values of the original data, respectively.
(2)
Initialization: Set parameters such as population size, maximum iteration threshold, quantity of discoverers, boundaries for initial value ranges, and dimension of independent variables.
(3)
Population Initialization: Initialize individual positions using Bernoulli chaotic mapping (Equation (20)).
(4)
Fitness Evaluation and Ranking: Compute each individual’s fitness via the objective function (Equation (27)), and then rank all individuals and assign the best as discoverers, others as joiners.
(5)
Position Update: Update the position of the discoverers based on Equations (21)–(23); update the position of the joiners based on Equations (24) and (25); update the individual positions of the scouter and early warning based on Equation (19).
(6)
Fitness Update: Recompute fitness values and update the best and worst fitness records and their positions.
(7)
Gaussian Perturbation: Apply Gaussian mutation (Equation (26)) to the global-best individual to avoid local optima.
(8)
Termination Check: Output results if the stopping criterion is met; otherwise, return to Step 4.
The pseudo-code for the ISSA-SVR algorithm (Algorithm 1) is shown below.
Algorithm 1. ISSA-SVR
Inputs: Population size p o p , the maximum iterations M , the number of discoverers P N , the number of scouters S N
Outputs: global optimal location b e s t x , global optimal fitness f g
1. Initialize population individual positions according to the Bernoulli mapping based on Equation (20).
2. for t = 1: M do
 a.
Calculate the fitness value of an individual and find the minimum fitness value f g and maximum fitness value f w based on Equation (27);
 b.
Rank Individuals, select the top PN individuals as discoverers the rest as joiners;
 c.
Update the position of the discoverers (Equations (21)–(23)), joiners (Equations (24) and (25)) and scouters (Equation (19)).
 d.
Calculate the current individual fitness value and update f g , f w , b e s t x .
 e.
Apply Gaussian perturbation to global best solution based on Equation (26).
3. End for
4. Return  b e s t x and f g
The block diagram of the proposed SOH estimation approach is displayed in Figure 6. As illustrated in the figure, the suggested approach is roughly separated into four components: data acquisition, feature extraction and processing, model training and SOH estimation, and error analysis. Firstly, discharge voltage data from the NASA battery dataset and the actual laboratory battery dataset are collected. Secondly, convolution operations are carried out on adjacent voltage sequences, respectively, and nine HIs are extracted from the resulting convolution sequences, and the correlation between them and the battery capacity are verified. To diminish the computational burden of the model, PCA is utilized to optimize dimensionality reduction in the extracted HIs. Then, ISSA is employed to optimize parameters in the SVR model, and HIs after dimensionality reduction and battery capacity data are divided into the training set and the testing set. The training set is utilized to train the ISSA-SVR model offline, and the testing set is utilized to test the SOH estimation accuracy of the model online. Finally, four error indicators are employed to assess the estimation performance of the suggested approach.

4. Experimental Results and Analysis

4.1. Error Evaluation Indicator

To more accurately evaluate the performance of the proposed SOH estimation approach, several error metrics are employed, including mean square error (MSE), root mean square error (RMSE), mean absolute error (MAE), and mean absolute percentage error (MAPE). Their mathematical expressions are given as follows:
M S E = 1 n i = 1 n ( y ^ i y i ) 2
R M S E = 1 n i = 1 n ( y ^ i y i ) 2
M A E = 1 n i = 1 n y ^ i y i
M A P E = 1 n i = 1 n y ^ i y i y i
where y i is the true value of SOH under the i t h cycle; y ^ i is the SOH estimate value under the i t h cycle; and n is the total number of cycles evaluated by SOH.

4.2. Ablation Experiments

To verify the effectiveness of the proposed modules in ISSA-SVR, we conducted ablation experiments on both PCA-based dimensionality reduction and the ISSA refinements, namely, Bernoulli chaotic mapping (BM), the SCA, spiral search (PSA), and Gaussian perturbation (GP). For PCA, Table 7 and Table 8 show that removing PCA increases both the training time and MSE, confirming that dimensionality reduction significantly improves computational efficiency and predictive accuracy. For the ISSA refinements, Table 9 and Table 10 show that the complete ISSA-SVR consistently achieves the fastest convergence and lowest error, while removing individual modules leads to a degraded performance, with the most notable deterioration observed when SCA and PSA are excluded. These findings demonstrate that PCA effectively reduces redundancy in high-dimensional data, while the ISSA refinements collectively enhance the convergence speed, accuracy, and robustness, thereby validating the necessity of each proposed component.

4.3. Estimation Results and Analysis

Based on the NASA battery dataset and the laboratory battery dataset, this section analyzes and discusses the estimation performance of the proposed ISSA-SVR method. To evaluate robustness under different data conditions, 50%, 60%, and 70% of each dataset is used as a training set, and the results are compared against SVR, SSA-SVR, and PSO-SVR under the same training protocols. The SOH estimation results of the four models for each battery are displayed in Figure 7, Figure 8, Figure 9, Figure 10, Figure 11 and Figure 12. As shown in the figures, under different training modes, the SOH estimation performance improves as the training set proportion increases. For the same training ratio, the SVR model shows a poor generalization ability and the largest prediction errors. Although SSA-SVR and PSO-SVR improve the estimation accuracy to some extent, their overall performance remains suboptimal. In contrast, the proposed ISSA-SVR achieves the highest accuracy and the closest alignment with the actual SOH degradation curve, confirming its precision and robustness in SOH estimation.
The error metrics of different models across various batteries are shown in Table 11 and Table 12 below. It can be observed that the values of MSE, RMSE, MAE, and MAPE of the proposed approach are all within 4%, with MSE consistently below 0.1%, demonstrating its strong performance in SOH estimation. Taking the B0005 battery of the 50% training set as an example, the MSE value of the ISSA-SVR method reduces the MSE by 77.78%, 73.33%, and 50.00% compared with SVR, SSA-SVR, and PSO-SVR, respectively. Similarly, the RMSE value is reduced by 50.71%, 45.99%, and 24.28%; the MAE value reduced by 50.00%, 45.32%, and 24.27%; and the MAPE value reduced by 50.00%, 45.27%, and 24.15%, respectively. These results indicate that the proposed ISSA-SVR maintains high stability across different battery datasets and provides superior accuracy and generalization compared with alternative methods.

5. Discussion

Accurate estimation of lithium-ion battery SOH is essential for safe and reliable operation. This paper proposes an ISSA-SVR framework that combines convolution-based health indicator extraction, PCA-based dimensionality reduction, and improved sparrow search optimization for SVR parameter tuning. Convolution operations on discharge voltage sequences enable the extraction of nine degradation-related HIs, while PCA reduces redundancy and lowers computational complexity. The ISSA enhances parameter optimization by improving the global search capability and avoiding local optima, thereby strengthening estimation accuracy. Validation on two datasets under different training ratios demonstrates that the proposed method achieves error indicators within 4%, confirming its robustness, stability, and practical potential under diverse aging conditions. Future work will not only focus on validating this methodology on large-format prismatic or pouch cells but will also expand to investigate the model’s performance under practical, dynamic operating conditions, including partial charge/discharge cycles, inherent sensor noise, and irregular load profiles.

Author Contributions

R.L.: Methodology, Writing—Original Draft, Conceptualization, Validation. N.H.: Writing—Review and Editing, Investigation, Methodology, Resources, Funding Acquisition. F.C.: Investigation, Supervision, Project Administration. All authors have read and agreed to the published version of the manuscript.

Funding

This research was funded by the National Natural Science Foundation of China (Grant No. 61903291).

Data Availability Statement

The datasets used and/or analyzed during the current study are available from the corresponding author on reasonable request.

Conflicts of Interest

The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.

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Figure 1. Capacity degradation curves of four batteries in NASA dataset.
Figure 1. Capacity degradation curves of four batteries in NASA dataset.
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Figure 2. Lab battery testing platform.
Figure 2. Lab battery testing platform.
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Figure 3. Capacity degradation curves of two batteries in laboratory dataset.
Figure 3. Capacity degradation curves of two batteries in laboratory dataset.
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Figure 4. HI extraction process.
Figure 4. HI extraction process.
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Figure 5. Pearson correlation coefficient results for each battery.
Figure 5. Pearson correlation coefficient results for each battery.
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Figure 6. SOH estimation framework of the proposed method.
Figure 6. SOH estimation framework of the proposed method.
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Figure 7. SOH estimation results for B0005. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 7. SOH estimation results for B0005. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Figure 8. SOH estimation results for B0006. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 8. SOH estimation results for B0006. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Figure 9. SOH estimation results for B0007. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 9. SOH estimation results for B0007. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Figure 10. SOH estimation results for B0018. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 10. SOH estimation results for B0018. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Figure 11. SOH estimation results for T3. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 11. SOH estimation results for T3. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Figure 12. SOH estimation results for T4. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
Figure 12. SOH estimation results for T4. (a) Estimates based on 50% training set. (b) Estimates based on 60% training set. (c) Estimates based on 70% training set.
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Table 1. Comparison of ISSA-SVR with recent studies.
Table 1. Comparison of ISSA-SVR with recent studies.
ReferenceMethodDatasetKey Technique
Wu et al. (2023) [1]PCA–PSO–BP neural networkNASADimensionality reduction + hybrid optimization
Ma et al. (2022) [3]Improved LSTM + HI extractionNASA + MITDeep learning with handcrafted HIs
Xia et al. (2023) [18]BiGRU + incremental capacity and DV featuresCALCE + SandiaBiFRU + attention
Zhu et al. (2024) [24]Sparse self-attentive transformerNASA + CALCEMulti-feature fusion + attention + convolution
Chen et al. (2025) [19]Multi-scale channel attention networkLabMulti-feature extraction + attention-based hybrid network
Zhang et al. (2025) [25]Improved transformer with DCCCALCEMulti-feature extraction + transformer
This workISSA–SVRNASA + LabConvolution-based HI + PCA + ISSA optimization
Table 2. Battery experiment data information.
Table 2. Battery experiment data information.
LabelTemperature/°CCharging Current/ADischarge Current/ACut-Off Voltage/V
B5241.522.7
B62.5
B72.2
B182.5
Table 3. Specifications of experimental batteries.
Table 3. Specifications of experimental batteries.
BatteryCapacity (Ah)Nominal Voltage (V)Working Voltage (V)Internal Resistance (mΩ)Weight (g)Dimension (mm)
T133.72.7–4.2124618 × 65
T22.63.72.7–4.2124618 × 65
Table 4. Battery experiment procedures.
Table 4. Battery experiment procedures.
StepStep NameWork TimeVoltage/VCurrent/mACut-Off Voltage/VCut-Off Current/mA
1Constant-current—constant-voltage charging/4.21500/20
2Constant-current discharging//20002.7/
3Rest5 min// /
4CycleStart step: 1//
5End/////
Table 5. Contribution rates of each principal component.
Table 5. Contribution rates of each principal component.
Battery
B0005B0006B0007B0018T3T4
M194.31%94.07%91.94%93.13%93.88%96.91%
M24.10%3.63%6.01%5.06%5.51%3.01%
M31.42%1.88%1.80%1.66%0.61%0.07%
M40.11%0.26%0.14%0.15%<0.01%<0.01%
M50.06%0.15%0.11%<0.01%<0.01%<0.01%
M6<0.01%<0.01%<0.01%<0.01%<0.01%<0.01%
M7<0.01%<0.01%<0.01%<0.01%<0.01%<0.01%
M8<0.01%<0.01%<0.01%<0.01%<0.01%<0.01%
M9<0.01%<0.01%<0.01%<0.01%<0.01%<0.01%
Table 6. ISSA-SVR parameters.
Table 6. ISSA-SVR parameters.
ParameterMeaningValue
N Population size100
T Max. iterations20
k Number of chaotic iterations100
ρ Control parameter0.7
C Penalty16
γ RBF width0.01
Table 7. Results of ablation experiments of PCA on B0005 dataset.
Table 7. Results of ablation experiments of PCA on B0005 dataset.
MethodISSA-SVRw/o PCA
Training time(s)8089
MSE0.000420.00071
Table 8. Results of ablation experiments of PCA on T3 dataset.
Table 8. Results of ablation experiments of PCA on T3 dataset.
MethodISSA-SVRw/o PCA
Training time(s)110125
MSE0.000070.00015
Table 9. Results of ablation experiments of ISSA modules on B0005 dataset.
Table 9. Results of ablation experiments of ISSA modules on B0005 dataset.
MethodISSA-SVRw/o BMw/o SCAw/o PSAw/o GP
Convergence iterations4549574945
MSE0.000420.000500.000570.000480.00049
Table 10. Results of ablation experiments of ISSA modules on T3 dataset.
Table 10. Results of ablation experiments of ISSA modules on T3 dataset.
MethodISSA-SVRw/o BMw/o SCAw/o PSAw/o GP
Convergence iterations3443523939
MSE0.000070.000090.000130.000110.00008
Table 11. Comparison of error indicators of four models based on the NASA dataset.
Table 11. Comparison of error indicators of four models based on the NASA dataset.
BatteryMethodMSERMSEMAEMAPE
B0005 (50%)ISSA-SVR0.00040.02090.01810.0267
SSA-SVR0.00150.03870.03310.0488
PSO-SVR0.00080.02760.02390.0352
SVR0.00180.04240.03620.0534
B0005 (60%)ISSA-SVR0.000030.00550.00460.0068
SSA-SVR0.00050.02320.01670.0252
PSO-SVR0.00070.02580.01830.0277
SVR0.00100.03200.02320.0350
B0005 (70%)ISSA-SVR0.000020.00410.00310.0046
SSA-SVR0.00020.01250.01060.0158
PSO-SVR0.00020.01450.01140.0173
SVR0.00040.01930.01540.0233
B0006 (50%)ISSA-SVR0.00080.02850.02490.0387
SSA-SVR0.00230.04750.04130.0645
PSO-SVR0.00240.04920.04290.0669
SVR0.00300.05490.04790.0747
B0006 (60%)ISSA-SVR0.00060.02440.02240.0353
SSA-SVR0.00140.03700.03380.0533
PSO-SVR0.00210.04590.04200.0662
SVR0.00270.05230.04390.0701
B0006 (70%)ISSA-SVR0.00030.01710.01560.0250
SSA-SVR0.00050.02160.01900.0306
PSO-SVR0.00100.03200.02670.0434
SVR0.00150.03890.02900.0476
B0007 (50%)ISSA-SVR0.00030.01710.01400.0191
SSA-SVR0.00060.02370.01710.0236
PSO-SVR0.00080.02860.02360.0322
SVR0.00080.02890.02290.0314
B0007 (60%)ISSA-SVR0.000020.00390.00290.0039
SSA-SVR0.00020.01240.00890.0124
PSO-SVR0.00080.02860.02360.0322
SVR0.00030.01600.01160.0161
B0007 (70%)ISSA-SVR0.000010.00370.00270.0037
SSA-SVR0.00010.01010.00800.0111
PSO-SVR0.00020.01290.00930.0130
SVR0.00020.01280.01000.0140
B0018 (50%)ISSA-SVR0.00060.02490.01550.0222
SSA-SVR0.00310.05600.04620.0661
PSO-SVR0.00320.05700.02820.0405
SVR0.00380.01680.03290.0473
B0018 (60%)ISSA-SVR0.000080.00900.00610.0087
SSA-SVR0.00220.04680.03840.0550
PSO-SVR0.00260.05100.03200.0465
SVR0.00310.05560.03670.0533
B0018 (70%)ISSA-SVR0.000070.00820.00520.0074
SSA-SVR0.00120.03420.02770.0402
PSO-SVR0.00140.03780.03080.0447
SVR0.00150.03910.03140.0457
Table 12. Comparison of error indicators of four models based on the laboratory dataset.
Table 12. Comparison of error indicators of four models based on the laboratory dataset.
BatteryMethodMSERMSEMAEMAPE
T3 (50%)ISSA-SVR0.000070.00820.00700.0086
SSA-SVR0.00030.01680.01500.0184
PSO-SVR0.00030.01730.01100.0136
SVR0.00060.02420.01570.0196
T3 (60%)ISSA-SVR0.000020.00460.00410.0051
SSA-SVR0.00010.01090.00820.0102
PSO-SVR0.00010.01150.00880.0110
SVR0.00050.02130.01590.0199
T3 (70%)ISSA-SVR0.000010.00350.00300.0037
SSA-SVR0.000030.00550.00420.0053
PSO-SVR0.000050.00720.00580.0072
SVR0.00030.01690.01080.0136
T4 (50%)ISSA-SVR0.00020.01240.00970.0130
SSA-SVR0.00030.01790.01350.0182
PSO-SVR0.00050.02190.01610.0218
SVR0.00080.02860.02160.0291
T4 (60%)ISSA-SVR0.00010.01010.00920.0124
SSA-SVR0.00020.01550.01250.0170
PSO-SVR0.00030.01860.01470.0200
SVR0.00040.02000.01430.0198
T4 (70%)ISSA-SVR0.000040.00590.00480.0066
SSA-SVR0.00010.01150.00940.0130
PSO-SVR0.00020.01280.01090.0150
SVR0.00020.01370.01050.0147
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Li, R.; He, N.; Cheng, F. State of Health Estimation of Lithium-Ion Battery Based on Novel Health Indicators and Improved Support Vector Regression. Batteries 2025, 11, 347. https://doi.org/10.3390/batteries11100347

AMA Style

Li R, He N, Cheng F. State of Health Estimation of Lithium-Ion Battery Based on Novel Health Indicators and Improved Support Vector Regression. Batteries. 2025; 11(10):347. https://doi.org/10.3390/batteries11100347

Chicago/Turabian Style

Li, Ruoxia, Ning He, and Fuan Cheng. 2025. "State of Health Estimation of Lithium-Ion Battery Based on Novel Health Indicators and Improved Support Vector Regression" Batteries 11, no. 10: 347. https://doi.org/10.3390/batteries11100347

APA Style

Li, R., He, N., & Cheng, F. (2025). State of Health Estimation of Lithium-Ion Battery Based on Novel Health Indicators and Improved Support Vector Regression. Batteries, 11(10), 347. https://doi.org/10.3390/batteries11100347

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