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Metals 2018, 8(1), 67; https://doi.org/10.3390/met8010067

Simple Fabrication and Characterization of an Aluminum Nanoparticle Monolayer with Well-Defined Plasmonic Resonances in the Far Ultraviolet

Instituto de Física, Universidad Nacional Autónoma de México, Circuito de la Investigación Científica s/n, Ciudad Universitaria, A.P. 20-364, Coyoacán, 04510 Ciudad de México, Mexico
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Received: 31 December 2017 / Revised: 13 January 2018 / Accepted: 16 January 2018 / Published: 18 January 2018
(This article belongs to the Special Issue Metallization of Non-Conductive Substrates)
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Abstract

Currently, aluminum plasmonics face technical challenges for the manufacture of reproducible structures by simple and low-cost techniques. In this work, we used a direct current (DC) sputtering system to grow a set of quasi-spherical aluminum nanoparticles with diameters below 10 nm. Our particles are uniformly distributed over the surface of quartz and nitrocellulose substrates. We review in detail the methodology for the determination of adequate deposition parameters to allow great reproducibility in different production runs. Likewise, we carry out an exhaustive nanostructural characterization by means of scanning and transmission electron microscopy. The latter allowed us to identify that our depositions are nanoparticle monolayers with thicknesses equal to the average particle diameter. Finally, by means of absorbance spectra we identify the presence of a very well-defined plasmonic resonance at 186 nm that is associated with the dipolar mode in particles smaller than 10 nm. Due to the sharpness of their plasmonic resonances as well as their great manufacturing simplicity and high reproducibility, our aluminum nanoparticles could be used as optical sensors. View Full-Text
Keywords: plasmonic resonances; Al nanoparticles; electron microscopy; sputtering plasmonic resonances; Al nanoparticles; electron microscopy; sputtering
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This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited (CC BY 4.0).
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Aguilar-Del-Valle, M.D.P.; Cruz-Manjarrez, H.D.J.; Rodríguez-Gómez, A. Simple Fabrication and Characterization of an Aluminum Nanoparticle Monolayer with Well-Defined Plasmonic Resonances in the Far Ultraviolet. Metals 2018, 8, 67.

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