Next Article in Journal
Estimation of the Personal Deposited Dose of Particulate Matter and Particle-Bound Metals Using Data from Selected European Cities
Next Article in Special Issue
Diurnal and Seasonal Variations of Carbon Dioxide (CO2) Concentration in Urban, Suburban, and Rural Areas around Tokyo
Previous Article in Journal
Simulation of Severe Dust Events over Egypt Using Tuned Dust Schemes in Weather Research Forecast (WRF-Chem)
Previous Article in Special Issue
Global Atmospheric CO2 Concentrations Simulated by GEOS-Chem: Comparison with GOSAT, Carbon Tracker and Ground-Based Measurements
Open AccessArticle

An Approach to Estimate Atmospheric Greenhouse Gas Total Columns Mole Fraction from Partial Column Sampling

Climate & Ecosystem Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA
Author to whom correspondence should be addressed.
Atmosphere 2018, 9(7), 247;
Received: 17 April 2018 / Revised: 22 June 2018 / Accepted: 28 June 2018 / Published: 1 July 2018
(This article belongs to the Special Issue Greenhouse Gases: Measurements and Analysis)
This study presents a new conceptual approach to estimate total column mole fractions of CO2 and CH4 using partial column data. It provides a link between airborne in situ and remote sensing observations of greenhouse gases. The method relies on in situ observations, external ancillary sources of information (e.g., atmospheric transport models), and a regression kriging framework. We evaluate our new approach using National Oceanic and Atmospheric Administration’s (NOAA’s) AirCore program—in situ vertical profiles of CO2 and CH4 collected from weather balloons. Our paper shows that under the specific conditions of this study and assumption of unbiasedness, airborne observations up to 6500–9500 m altitude are required to achieve comparable total column CO2 mole fraction uncertainty as the Total Carbon Column Observing Network (TCCON) network provides, given as a precision of the ratio between observed and true total column-integrated mole fraction, assuming 400 ppm XCO2 (2σ, e.g., 0.8 ppm). If properly calibrated, our approach could be applied to vertical profiles of CO2 collected from aircraft using a few flask samples, while retaining similar uncertainty level. Our total column CH4 estimates, by contrast, are less accurate than TCCON’s. Aircrafts are not as spatially constrained as TCCON ground stations, so our approach adds value to aircraft-based vertical profiles for evaluating remote sensing platforms. View Full-Text
Keywords: total column; validation; TCCON; satellite; airborne measurements; kriging total column; validation; TCCON; satellite; airborne measurements; kriging
Show Figures

Figure 1

MDPI and ACS Style

Tadić, J.M.; Biraud, S.C. An Approach to Estimate Atmospheric Greenhouse Gas Total Columns Mole Fraction from Partial Column Sampling. Atmosphere 2018, 9, 247.

Show more citation formats Show less citations formats
Note that from the first issue of 2016, MDPI journals use article numbers instead of page numbers. See further details here.

Article Access Map by Country/Region

Back to TopTop