1. Introduction
Previously, to construct necessary roads and related infrastructure, users utilized the facilities after the construction company had determined all the construction steps. However, in recent years, with the improvement in people’s quality of life, road management has transitioned to an era of identifying user services and providing related services. The road services provided currently encompass policies and technologies that consider not only user safety but also inconveniences such as fine dust, noise, and urban heat islands. This trend is evolving to offer progressive services that are friendly to both people and nature, rather than focusing solely on building new roads. According to Seoul City in South Korea (2017), the social cost of road and air pollution was estimated to be approximately KRW 0.64 trillion, with these factors constituting 50% of the road transportation fields [
1].
Suspended road dust refers to particles discharged directly into the atmosphere without a specific outlet. It is generated by pollutants accumulating on the surfaces of paved and unpaved roads, and is suspended in the atmosphere due to vehicle body turbulence and shear stress caused by tire rotation when driving a car [
2]. The air pollution process test standards define suspended road dust that is suspended in the atmosphere due to friction between the tires of vehicles driving on the road and the road surface. The EPA (AP-42 13.2.1 paved roads) indicates that suspended road dust can be defined as particles coming from various sources, deposited on the road, and then, suspended by driving vehicles [
3,
4].
Suspended road dust is just one source of particulate matter in the air, with various other contributors, including the open burning of domestic municipal solid waste [
2]. Moreover, particulate matter (PM) generated by road dust can be classified as that from exhaust emissions (EEs) or from non-exhaust emissions (NEEs) depending on the source of the emissions [
5]. EEs are formed from exhaust gas produced by the combustion of vehicle fuel and the volatilization of lubricants, whereas NEEs can be generated through the emission of dust from road surfaces such as tires, brakes, and road wear.
Research related to NEEs is gaining importance as it occurs step by step, not only from tire, road, and brake wear, but also from the suspension of road dust caused by turbulence from vehicles [
6,
7,
8,
9,
10]. According to the European Environment Agency (EEA, 2016), it was estimated that nearly 90% of total PM emissions from road traffic would come from non-emission sources by the end of 2010 [
7]. In a study on NEEs conducted abroad, D. Van der Gon et al. (2013) showed that the proportion of NEEs in the road transport sector increased from 20% to 40% from between 1990 and 2009 to between 1999 and 2010, respectively [
8]. Moreover, PM emissions from vehicular exhaust and non-exhaust sources in the megacity of Delhi show that approximately 86% of emissions are NEEs. Additionally, the total PM
10 emissions in Delhi, India (2019), were 31.5 Gg per year, with non-emission levels at 86%, which was six times higher than the emission levels (14%). The emission levels were further classified as originating from automobiles (34%), buses (23%), and heavy commercial vehicles (17%) [
9].
In studies of exhaust gas, however, engines powered by modern diesel and compressed natural gas (CNG) showed the lowest PM concentrations and toxicological responses compared to other engine types [
11]. Furthermore, there was a roughly positive relationship between transient CO, NOx, and HC emission rates and vehicle speeds, while the emission factors (EFs) decreased significantly with a speed decrease when the speed was ≤20 km/h [
12]. With the grade of the road, the emission rates of NOx and HC tended to increase, and then, decrease as acceleration increased, peaking at 0 m/s
2 without considering idling conditions. After reaching this distance, the emissions decreased as the vehicle speed continued to increase [
13]. Speed and acceleration significantly impact emission rates, increasing with increases in speed and acceleration. Emissions were minimal at 40–60 kmph and −0.5–0.5 m/s
2, but at 0 m/s, the relative pollutant fraction remained at a level of ~0.12, even at very long distances. Moreover, particles have a larger attenuation rate than gaseous pollutants, only above a particle number (PN) of ~0.6 m, and the diameters are very close to the background values. Solid particles can diffuse further in the vehicle’s transverse direction; when a car passes through a pedestrian area with a 3 m distance, pedestrians are exposed to 2.6–3-times-higher levels, according to the results of indoor experiments [
14].
However, most studies related to exhaust gas have measured the concentration of carbon dioxide or PM, by conducting indoor experiments. But there has been a lack of research considering the various patterns that may occur in the city center or examining the effects of the difference in concentration occurring when a vehicle is actually driving at a constant speed [
11,
12]. Therefore, through this study, we tried to make this differentiation ourselves by identifying the dust concentration level that pedestrians passing by a road may be exposed to, the effective distance between the vehicles, and the correlation with silt loading and suspended road dust. Also, studies of suspended road dust rely on empirical methods by analyzing them according to traffic and environmental conditions at the time of measurement or selecting partial measurement areas [
2,
15]. In this study, the assertion is made that external factors can be more effectively minimized by measuring pollution levels within specific road sections while maintaining consistent conditions. In a previous study, a dust meter was permanently installed to assess the degree of pollution occurring when a vehicle passed. However, limitations arose in understanding pollution levels based on vehicle separation distance, as dust that accumulated on the road surface or that was generated by varying wind speeds was measured simultaneously. In contrast, this study aimed to uphold consistent conditions as much as possible, discerning the pollution levels generated when a vehicle passed at different separation distances. The findings of this study propose a nuanced approach, emphasizing the significance of considering variations in the distance of vehicle passage. During this period, only a single measurement vehicle was employed to determine the level of suspended road dust, revealing the limitation of addressing diverse driving patterns present in urban areas. Consequently, a hypothesis was formulated regarding the relationship between the generation of suspended road dust and the characteristics of dust emission, with the aim of exploring the quantitative correlation. To assess the impact of suspended road dust generated by vehicle movement on urban roads, this study introduced three pertinent impact conditions. Firstly, the study delved into the effect of exhaust gas produced during vehicle operation. Secondly, factors such as dust load and suspended road dust, akin to PM
10 content, were measured. Finally, the factors under consideration excluded exhaust gas—the primary cause of road dust occurrence—due to the fixed measurement position behind the front tire, with a focus on the direct suspension impact. Employing this methodology, it is posited that road dust on urban roads can serve as foundational data for estimating suspended road dust through correction coefficients.
Additionally, the quantity of silt dust per unit area collected on the pavement is denoted as sL, with dust particles known to be <75 μm in size (PM
75). However, as the suspended road dust concentration in this study focuses on PM
10, representing fine dust, it is imperative to measure and analyze both the size and percentage (%) of the dust. Though applied to PM
10 content within silt, if road dust particles are assumed to be typical spherical soil particles (density: approximately 2.5 g/cm³; dynamic shape coefficient: around 1.6), they can be considered similar. Hence, the PM
10 content of the particle diameter measured by a particle size analyzer can be deemed as the same mass fraction (mass %) when measuring the same particle, corresponding to the volume fraction (volume%) in the silt [
2,
15].
3. Results
3.1. Relationship between Suspended Road Dust and Silt Loading
The spatial contamination distribution of the sL value, measured through tests on A~C sites, is estimated to exhibit various values for each collection point. Consequently, the sL value was measured, and the spatial contamination distribution was further analyzed using the results of measuring debris on the surface at one-second intervals through a TRAKER-based mobile laboratory system. All selected data were measured under the same conditions, ensuring consistency not only at the starting point but also during acceleration, constant speed, and at the endpoint within the measurement section. The concentration of suspended road dust according to the sL value was measured in accordance with the 50 km/h operation guidelines.
As a result, the average concentration of suspended road dust was calculated for each sL collection section measured within the 100 m section by converting the travel distance from the starting point using GPS coordinates acquired through a mobile laboratory. The pollution level changes were then analyzed. The suspended road dust concentration, based on the average sL of the entire A–C site section, exhibited a high correlation, as shown in
Figure 5, with the suspended road dust concentration increasing in accordance with the amount of sL.
Figure 5.
Relationship between silt loading and dust in measurement sections.
Figure 5.
Relationship between silt loading and dust in measurement sections.
The correlation coefficient calculated under these conditions for all sL data at sites A~C, including 3 m and 25 m, was 0.76, indicating a high correlation. However, it should be noted that the characteristics of the test road (road surface condition), the silt characteristics of the section (particle diameter distribution), and the characteristics of the measuring device of the mobile laboratory can all influence the results. Additionally, uncertainties in the experimental method, such as differences in dust particle size when measuring the sL of the conventional and mobile laboratory by sL, are also considered. Nonetheless, sL can effectively represent the range of suspended road dust, making it a valuable evaluation method.
When the sections collected at 3 m and 25 m were separately analyzed, as shown in
Figure 6, both the 3 m and 25 m dust collections indicated that sL influenced suspended road dust. Therefore, sL is considered to be the most influential factor in suspended road dust levels. However, it appears that an increase in sL correlates with an increase in suspended road dust, suggesting that if the levels of sL and suspended road dust are similar, the two sample collection sections are expected to be similar.
However, it was observed that the change in the concentration of suspended road dust was minimal based on the deviation in the dust load presented earlier in the section where dust was collected over 3 m. This is judged to be the result of errors caused by human factors, such as the cleaning direction, because dust in a wide section is collected at once when it is collected over 25 m. The maximum sL value for each site was different, within 100 mg/m
2. Upon analyzing the concentration of suspended road dust according to sL, the concentration of suspended road dust increased by up to 5 µg/m
3 based on 50 km/h for every 100 mg/m
2 increase [
15]. Additionally, according to the U.S. Desert Research Institute (DRI), which developed TRAKER, there is a difference of 10 µg/m
3 [
15,
18].
Figure 6.
Comparison between 3 m and 25 m sampling methods in measurement sections.
Figure 6.
Comparison between 3 m and 25 m sampling methods in measurement sections.
For an accurate comparison, the average value of the concentration of suspended road dust was calculated for each sL collection section measured within the 100 m section by converting the travel distance from the starting point using GPS coordinates acquired through a mobile laboratory to analyze the pollution level changes. The suspended road dust concentration according to the average sL of the entire A~C site section measured showed a high correlation, as shown in
Figure 7 and
Figure 8, and the suspended road dust concentration increased according to the amount of sL. The correlation coefficients are 0.51 and 0.56, respectively.
Figure 7.
Relationship between silt loading and dust in 3 m sampling method.
Figure 7.
Relationship between silt loading and dust in 3 m sampling method.
Figure 8.
Relationship between silt loading and dust in 25 m sampling method.
Figure 8.
Relationship between silt loading and dust in 25 m sampling method.
3.2. Effective Distance in terms of Exhaust Gas Based on Distance Interval
Table 6 shows the silt loading on the residential road (Site C) to examine the effects of exhaust gas. In this case, a sampling method of 25 m with 400 m suspended road dust was used based on the previous results. Subsequently, when driving starts at the beginning point, the concentration of PM
10 increases in accordance with the concentration of sL until returning to the starting point. The distribution by weight concentration was examined based on the particle size of the collected sL to assess the size distribution of suspended road dust emanating from the rear tire during driving.
The highest sL value in the experimental section was 0.011 g/m
2, which was lower than the average dust load of 0.05 g/m
2 in the urban city [
15]. Since there was no significant difference between continuous sections, it is found that there will be no significant variation in the concentration of suspended road dust due to the dust load. This is attributed to the fact that the silt on the road was washed away by more than 1 mm of rain the day before each measurement, and it is judged to be the result of more than 0.025 mm of rainfall, as suggested by the EPA [
16].
As shown in
Figure 9, the measurement results indicate that the concentration of suspended road dust was higher when the vehicle was maintained at a 10 m distance in comparison to when only one measuring vehicle passed (mobile laboratory), with an average increase of about 50%. Additionally, when driving at a 20 m distance from the front car, the concentration of suspended road dust was most similar to when only one measuring vehicle passed, and at 50 m, it was found to be lower than the distance of 20 m. All suspended road dust concentrations were higher than the background dust concentration, indicating no errors in the measurement equipment used to measure suspended road dust.
The longer the separation distance of the vehicle, the lower the concentration of suspended road dust, suggesting a lower level of influence of exhaust gas at separation distances of 20 m or more. At a separation distance of 10 m, the concentration was about five times higher than the background concentration generated when the measuring vehicle was driven, indicating the effectiveness of exhaust gas.
Although the background dust concentration increased at a separation distance of 20 m, it was judged that there was no significant difference because the increase was within 5 µg/m³. Since there was no significant effect on the background concentration at a separation distance of 50 m, this study aimed to determine the effect of the suspended road dust concentration at a separation distance of 20 m.
Figure 9.
Results of suspended road dust measurements with different distances of intervals.
Figure 9.
Results of suspended road dust measurements with different distances of intervals.
When driving through a 10 m separation distance, the dust concentrations measured at the front inlets of the vehicles were compared and analyzed together, as shown in
Figure 10, to determine the impact of exhaust gas with the short-distance separation.
Upon analyzing the deviation in the suspended road dust concentration over time when driving at 10 m, it was observed that the suspended road dust concentration was approximately two or up to three times higher when driving at a separation distance of 10 m in all cases. At this time, the sL was very low, indicating that the effects of sL did not occur in these results. The difference between the 10 m driving result and the dust concentration when only one measuring vehicle passed is the result of the combination with the suspended road dust concentration due to exhaust gas generated during driving. It is judged that no data error occurs because it was driven in a certain section at a constant speed. Therefore, the separation distance between the front and the rear of the vehicle is considered an important factor. When measuring the dust concentration by driving around the urban area, the section where the dust concentration increases is found to have a high sL on the road. Therefore, it is judged that these factors need to be considered through a measurement vehicle managed by the local government.
Figure 10.
Effects of exhaust gas with 10 m space based on suspended road dust from measurement vehicles.
Figure 10.
Effects of exhaust gas with 10 m space based on suspended road dust from measurement vehicles.
Table 7 shows the results obtained when the change in the concentration of suspended road dust according to the separation distance is converted to a correction coefficient. The longer the distance based on the amount of dust passing through one measuring vehicle, the lower the concentration of suspended road dust. At a distance of 10 m, it is judged that the emission value is high due to dust suspended from the road surface and exhaust gas emissions generated by the vehicle in front of it.
In addition, in the case of 20 m, the separation distance of 20 m presented above is judged to be a distance that can minimize the effect on the exhaust gas concentration because the mobile laboratory has the most similar characteristics to the dust concentration passing through one. It can be interpreted that some dust suspended on the road when vehicles are 50 m apart will not accumulate again and will undergo some loss if it is suspended or if the concentration of suspended road dust is measured by leaving the lane.
3.3. Suspended Road Dust Based on Number of Vehicle Patterns
The result of measuring the concentration of suspended road dust according to vehicle driving behavior is shown in
Figure 11, and it was found that the concentration of suspended road dust increases when two cars are in parallel with another method (two cars in front, three cars in front). It is judged that dust suspended from the vehicle immediately in front of the measuring vehicle spreads into the air once more by the vehicle next to it, increasing the concentration of dust inhaled by the measuring vehicle.
Currently, the measurement of a mobile laboratory proposed by the Ministry of Environment in South Korea measures suspended road dust at the end of the road for stability of the operation. However, in the case of the suspended road dust concentration derived from this study, it was up to four times higher than when only the measurement vehicle was driven, so it is believed that more damage could occur in pedestrians walking on the side of the road. In addition, if two cars are in the front, suspended road dust in the air by the first vehicle continues to be suspended by the vehicle behind it, but it is believed to be gradually lower than the dust predicted in the dust load because it can spread into the air during the diffusion process.
Figure 11.
Results of suspended road dust with different distances of intervals.
Figure 11.
Results of suspended road dust with different distances of intervals.
In summarizing the results of vehicle behavior at the same separation distance, it is observed that when two cars are parallel with the car in front, suspended road dust diffuses, resulting in a high concentration of dust. This is translated into a correction coefficient based on the concentration of suspended road dust generated by the vehicle’s driving behavior, as presented in
Table 8. A higher coefficient in front of the vehicle corresponds to a lower concentration of suspended road dust. It is inferred that driving in front of the vehicle causes dust to be suspended in the air, and this dust continues to remain airborne as the following vehicle further disperses it, reducing the concentration of tire-derived dust. Additionally, when two vehicles drive in parallel, the dust suspended from the front vehicle is relatively high, as it is further dispersed by the adjacent vehicle. Consequently, it is noted that the current mobile laboratory measurement, although taken at the end of the road, may underestimate the dust concentration measured by the vehicle.
3.4. Suspended road dust According to PM10 Content
The characteristics of tire-surface suspended road dust and dust emissions were measured for the three types of asphalt pavement applied in Yongin City, and
Table 9 is a summary of the measured suspended road dust data. First, the suspended road dust tends to increase as the vehicle’s driving speed increases. In the case of the starting point, since the vehicle is not driving, it is the same as the background dust concentration of the current measurement section, which is similar to the dust concentration suggested by the Observatory of Meteorological Administration of South Korea [
20].
In general, since PM
10 concentration is used when measuring suspended road dust through a mobile laboratory, it is necessary to distinguish the total PM
10 concentration from the dust load to examine the hypothesis in this study established between the amount of sL and the suspended road dust. Additionally, as described in
Table 10, in the case of sL and PM
10 content related to dust emission, the residential road showed the lowest at 47.8 mg/m
2, and PM
10 content was also low, indicating the lowest value for the suspended road dust concentration according to speed. In the case of commercial roads, the sL value was the highest at 229.1 mg/m
2, and in the case of industrial roads, the average PM
10 content was 6.81%, which was high according to the section.
So, it was considered that there was an impact on the difference in PM10 content for each measurement road in analyzing the characteristics of the sL. Therefore, by analyzing the results of suspended road dust on residential roads, industrial roads, and commercial roads in Yongin, it is confirmed how the change in PM10 content (%) affects the suspended road dust, and the measurement shows that the suspended road dust concentration changes according to the ratio of PM10 content (%). The suspended road dust measured on the residential road in Yongin City shows a low sL value from 0.04 g/m2 to 0.07 g/m2, but it is shown that suspended road dust is higher than that on the industrial road, which increases when driving with high levels of PM10 content.
The concentration of suspended road dust, based on travel distance, exhibited variations in pollution depending on the driving direction, even on the same sample road across all three sections (A~C) on which we collected sL. Moreover, there is a positive correlation between sL and the concentration of suspended road dust, with higher sL values corresponding to elevated dust concentrations.
For the measured industrial road in Yongin, as described in
Figure 12, the sL value was about twice as high as for the Site A (residential) section; it was found that suspended road dust increased after about 2 to 3 s when PM
10 content showed a high level. When a higher value of PM
10 content appears in a spot, there is an increased value of suspended road dust, and the effects of PM
10 on silt can lead to a high level of suspended road dust. Therefore, PM
10 content (%) in sL is judged to be a major factor in determining the concentration of suspended road dust.
Figure 12.
Effects of exhaust gas with 10 m space based on suspended road dust from measurement vehicles.
Figure 12.
Effects of exhaust gas with 10 m space based on suspended road dust from measurement vehicles.
Based on these results,
Figure 13 shows the relationship between suspended road dust and PM
10 content in silt within the entire measured section. The PM
10 content and suspended road dust concentration in the silt were found to increase similarly, but the deviation was large on the commercial road where the silt content was high.
However, if the PM
10 content in sL is too high with a value of 0.1 g/m
2, there is no significant difference in the suspended road dust concentration that affects the change in the sL value. This is because the effect of sL in creating suspended road dust is higher than that of PM
10 content. The sL value of 0.1 g/m
2 is the highest average value in South Korea in urban areas [
15].
At this time, if the sL value is low, the concentration of suspended road dust that can occur may be small, but if the PM10 content is high, the amount of suspended road dust increases because the tire contains a lot of PM10 particles in the silt. However, if the amount of dust is large, additional consideration should be taken because there is an error in the amount of dust actually collected through the inlet and the amount of dust inhaled during driving when the measuring vehicle drives on the road. It is believed that this study can be used to present a correction factor without the need for 1:1 matching of the suspended road dust concentration over the time that dust is collected when estimating the suspended road dust concentration according to sL.
The criteria for separating sL and PM10 content in this study were chosen based on the mechanism of suspended dust for sL on asphalt pavement. In the case of hot mix asphalt (HMA), deposited dust stays on the surface as an impermeable pavement and can be promptly suspended by a moving vehicle or wind. Consequently, even with the same dust load, the concentration of suspended road dust can vary depending on the PM10 content level present in the silt.
Figure 13.
Suspended road dust based on sL* PM10 content on different types of road.
Figure 13.
Suspended road dust based on sL* PM10 content on different types of road.
4. Discussion
This study focuses on suspended road dust, defined as particles created due to vehicle-induced turbulence and shear stress on road surfaces. NEE has become increasingly significant in recent years. However, the results of suspended road dust analyses are based on experiments with one mobile laboratory that cannot reflect the driving patterns that occur in urban areas. Therefore, this study aims to find coefficients based on the effects of exhaust gas with interval distance and the number of vehicles. Moreover, since sL reflects particles under 75 µm, this study attempts to identify factors for calculating PM10 content.
- (1)
SL is a primary determinant of suspended road dust concentration; higher sL values correspond to increased dust levels, with an average correlation of 0.76. Moreover, suspended road dust increases by up to 5 µg/m3 based on a 50 km/h driving speed for every 0.01 g/m2 increase in sL, highlighting the dominance of sL in determining dust concentration.
- (2)
Regarding the effective distance in terms of exhaust gas, maintaining a separation distance of 20 m proved effective in minimizing the impact of exhaust gas emissions on suspended concentrations. At a 10 m distance, the concentration was five times higher than the observatory background and two times higher (75 µg/m3 -> 150 µg/m3) with one measurement vehicle pass. This emphasizes the importance of a safe driving distance in relation to exhaust gas.
- (3)
As the number of vehicles in front increases, influenced by vehicle patterns, dust accumulated on the road is dispersed in the air by the movement of vehicles. The measured concentration of scattered dust decreases because it is unable to reaccumulate due to subsequent passing vehicles. When driving in front of a vehicle, dust is suspended in the air, and this suspension continues as the following vehicle disperses it, consequently lowering the concentration of dust from the tire. Additionally, when two vehicles drive in parallel, the dust suspended from the front vehicle is relatively high as it is once again dispersed by the adjacent vehicle.
- (4)
PM10 content levels were measured across different road types, with the industrial road exhibiting the highest average at 6.81%. The concentration of suspended road dust on residential roads, characterized by low sL, was notably influenced by the PM10 content (%).
However, if the PM10 content in sL is too high, there is no significant difference in the suspended road dust concentration that affects the change in the sL value. This is because the effects of sL are higher than those of PM10 content in making suspended road dust. The characteristics of PM10 concentration differences were measured in urban areas to expand upon existing studies of the suspended road dust model. This experiment aims to achieve a comprehensive understanding of road dust and coefficients for many driving patterns and exhaust gases in urban areas. Through this, we understand the long-term trends of NEE in monitoring and predicting how road dust may occur in urban areas. In addition, by including the PM10 content analysis, the effect of particle composition on suspended road dust was revealed to provide a new perspective, enhancing our understanding of the approach methodology and the precision of the measurement methodology. In this study, we demonstrate the necessity of refining the measurement protocol for road dust emission and present an innovative methodology for assessing PM10 and suspended road dust in silt.