Development of the RF-MEAM Interatomic Potential for the Fe-C System to Study the Temperature-Dependent Elastic Properties
Abstract
:1. Introduction
2. Materials and Methods
2.1. Ground State DFT Calculation
2.2. Low-Convergence AIMD Calculation
2.3. High-Convergence DFT Calculation
2.4. Potential Parameter Fitting
2.5. Potential Selection and Validation
3. Results and Discussion
3.1. Parameters for AIMD Calculations
3.2. Ground State Elastic Calculation
3.3. Finite-Temperature Elasticity Calculation
4. Conclusions
Supplementary Materials
Author Contributions
Funding
Institutional Review Board Statement
Informed Consent Statement
Data Availability Statement
Acknowledgments
Conflicts of Interest
References
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Fe-C Structure | k-Points (Gamma) | No. of Atoms | Supercell |
---|---|---|---|
B1 | 7 × 15 × 15 | 128 | 4 × 2 × 2 |
B2 | 9 × 12 × 16 | 120 | 5 × 4 × 3 |
B3 | 7 × 15 × 15 | 128 | 4 × 2 × 2 |
Cementite | 23 × 10 × 7 | 64 | 1 × 2 × 2 |
L12 | 10 × 15 × 15 | 48 | 3 × 2 × 2 |
Fe-C Structure | k-Points (Gamma) | No. of Atoms | Supercell |
---|---|---|---|
B1 | 15 × 15 × 15 | 64 | 2 × 2 × 2 |
B2 | 16 × 16 × 16 | 54 | 3 × 3 × 3 |
B3 | 15 × 15 × 15 | 64 | 2 × 2 × 2 |
Cementite | 23 × 10 × 7 | 64 | 1 × 2 × 2 |
L12 | 10 × 15 × 15 | 48 | 3 × 2 × 2 |
Structure | V (Å) | B (GPa) | B’ | |||
---|---|---|---|---|---|---|
RF-MEAM | Literature | RF-MEAM | Literature | RF-MEAM | Literature | |
B1 (FeC) | 65 | 338 | 5.28 | |||
B2 (FeC) | 16 | 302 | 4.12 | |||
B3 (FeC) | 78 | 222 | 4.50 | |||
Cementite (Fe3C) | 155 | 252 | 4.05 | |||
O-FeC | 94 | , () | 288 | , | 3.10 | , |
Elastic Constants (GPa) | Fe3C-Cementite | FeC-B1 | O-FeC | ||||||
---|---|---|---|---|---|---|---|---|---|
This Study | Literature | This Study | Literature | This Study | Literature | ||||
RF-MEAM | DFT | DFT/MEAM | RF-MEAM | DFT | DFT/MEAM | RF-MEAM | DFT | DFT/MEAM | |
C11 | 399 | 296 | 585 | 584 | 399 | 344 | |||
C22 | 459 | 392 | - | - | - | 469 | 428 | 445c | |
C33 | 364 | 330 | - | - | - | 444 | 423 | ||
C12 | 236 | 137 | 214 | 205 | 238 | 166 | |||
C13 | 210 | 181 | - | - | - | 245 | 170 | ||
C23 | 204 | 155 | - | - | - | 255 | 182 | ||
C44 | 116 | 131 | 125 | 82 | 106 | 95 | |||
C55 | 40 | 19 | - | - | - | 98 | 89 | ||
C66 | 119 | 135 | - | - | - | 81 | 66 | ||
- | |||||||||
B | 280 | 218 | 338 | 331 | 310 | 247 | |||
G | 93 | 93 | 149 | 125 | 95 | 95 | |||
Y | 252 | 245 | 390 | 334 | 259 | 253 |
T(K) | FeC-0.2% | FeC-0.4% | ||||
---|---|---|---|---|---|---|
B (GPa) | G (GPa) | E (GPa) | B (GPa) | G (GPa) | E (GPa) | |
73 | 215 | 81 | 217 | 214 | 80 | 214 |
144 | 211 | 79 | 211 | 210 | 79 | 210 |
200 | 206 | 77 | 206 | 204 | 78 | 207 |
294 | 202 | 76 | 203 | 202 | 76 | 203 |
422 | 195 | 74 | 196 | 194 | 72 | 192 |
533 | 186 | 70 | 187 | 185 | 70 | 186 |
589 | 186 | 69 | 184 | 183 | 67 | 179 |
644 | 179 | 67 | 179 | 180 | 65 | 173 |
700 | 173 | 64 | 172 | 174 | 60 | 162 |
811 | 167 | 53 | 144 | 169 | 52 | 141 |
866 | 165 | 49 | 134 | 162 | 50 | 135 |
922 | - | - | - | 154 | 42 | 116 |
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Risal, S.; Singh, N.; Duff, A.I.; Yao, Y.; Sun, L.; Risal, S.; Zhu, W. Development of the RF-MEAM Interatomic Potential for the Fe-C System to Study the Temperature-Dependent Elastic Properties. Materials 2023, 16, 3779. https://doi.org/10.3390/ma16103779
Risal S, Singh N, Duff AI, Yao Y, Sun L, Risal S, Zhu W. Development of the RF-MEAM Interatomic Potential for the Fe-C System to Study the Temperature-Dependent Elastic Properties. Materials. 2023; 16(10):3779. https://doi.org/10.3390/ma16103779
Chicago/Turabian StyleRisal, Sandesh, Navdeep Singh, Andrew Ian Duff, Yan Yao, Li Sun, Samprash Risal, and Weihang Zhu. 2023. "Development of the RF-MEAM Interatomic Potential for the Fe-C System to Study the Temperature-Dependent Elastic Properties" Materials 16, no. 10: 3779. https://doi.org/10.3390/ma16103779