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Multiferroic Hysteresis Loop
Open AccessFeature PaperArticle

Multiferroic Core-Shell Nanofibers, Assembly in a Magnetic Field, and Studies on Magneto-Electric Interactions

Physics Department, Oakland University, Rochester, MI 48309, USA
College of Electrical and Information Engineering, Zhengzhou University of Light Industry, Zhengzhou 450002, China
Faculty of Radiophysics, Electronics and Computer Systems, Taras Shevchenko National University of Kyiv, Kyiv 01601, Ukraine
Institute of Electronic and Information Systems, Novgorod State University, Veliky Novgorod 173003, Russia
Author to whom correspondence should be addressed.
Materials 2018, 11(1), 18;
Received: 2 December 2017 / Revised: 18 December 2017 / Accepted: 20 December 2017 / Published: 23 December 2017
Ferromagnetic–ferroelectric nanocomposites are of interest for realizing strong strain-mediated coupling between electric and magnetic subsystems due to a high surface area-to-volume ratio. This report is on the synthesis of nickel ferrite (NFO)–barium titanate (BTO) core–shell nanofibers, magnetic field assisted assembly into superstructures, and studies on magneto-electric (ME) interactions. Electrospinning techniques were used to prepare coaxial fibers of 0.5–1.5 micron in diameter. The core–shell structure of annealed fibers was confirmed by electron microscopy and scanning probe microscopy. The fibers were assembled into discs and films in a uniform magnetic field or in a field gradient. Studies on ME coupling in the assembled films and discs were done by magnetic field (H)-induced polarization, magneto–dielectric effects at low frequencies and at 16–24 GHz, and low-frequency ME voltage coefficients (MEVC). We measured ~2–7% change in remnant polarization and in the permittivity for H = 7 kOe, and a MEVC of 0.4 mV/cm Oe at 30 Hz. A model has been developed for low-frequency ME effects in an assembly of fibers and takes into account dipole–dipole interactions between the fibers and fiber discontinuity. Theoretical estimates for the low-frequency MEVC have been compared with the data. These results indicate strong ME coupling in superstructures of the core–shell fibers. View Full-Text
Keywords: magneto-electric; ferromagnetic; ferroelectric; multiferroic; composites magneto-electric; ferromagnetic; ferroelectric; multiferroic; composites
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MDPI and ACS Style

Sreenivasulu, G.; Zhang, J.; Zhang, R.; Popov, M.; Petrov, V.; Srinivasan, G. Multiferroic Core-Shell Nanofibers, Assembly in a Magnetic Field, and Studies on Magneto-Electric Interactions. Materials 2018, 11, 18.

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