Plugging Experiments for Ceramic Filling Layer with Different Grain Sizes Under Gas–Water Mixed Flow for Natural Gas Hydrate Development
Abstract
:1. Introduction
2. Materials and Methods
2.1. Experimental Principle and Experimental Apparatus
2.2. Experimental Methods and Experimental Materials
2.2.1. Experimental Methods
2.2.2. Experimental Materials
2.3. Experimental Conditions [32]
3. Results and Discussion
3.1. Fine-Grained Ceramic Layer (170–230 Mesh) Plugging Dynamics
3.2. Medium-to-Coarse Ceramic Layers (140–170, 80–120, and 70–80 Mesh) and Three-Phase Plugging Behavior
3.3. Coarse Ceramic Layer (40–70 Mesh) and Saucier Criterion Reassessment
3.4. Limitations and Field Implications
4. Conclusions
- (1)
- Limitations of Conventional Criteria in Mud-Rich Hydrate Systems: The Saucier criterion (median grain size ratio = 5–6), widely adopted in unconsolidated sandstones, proves inadequate for hydrate reservoirs with high shale content (e.g., 39% clay in South China Sea analogs). Our experiments reveal that even at a median grain size ratio of 24 (70–80 mesh ceramics), rapid plugging occurs due to mud-cake formation under gas–water mixed flow (Figure 5). This challenges the universality of traditional sand control design and necessitates a revised threshold (median grain size ratio ≥ 30) for hydrate-specific conditions, where clay migration dominates permeability loss over mechanical sand retention.
- (2)
- Optimized Ceramic Grading Strategy for Productivity Preservation: The median grain size ratio, gradientally distributed between 24–31, emerges as the critical balance point, achieving 54% retained permeability (initial k = 15.3 μm2, final k = 8.3 μm2) while blocking > 95% of formation sand (>20 μm). To address the transient fines invasion observed in “three-stage plugging” (Section 3.2), we propose a dual-layer graded packing. Primary layer: ceramics with a 40–70 mesh size (critical median grain size ratio of 27 ± 2) used for coarse sand retention through mechanical sieving and pore size optimization. Secondary layer: ceramics with a median grain size ratio in the 24–31 range to mitigate clay migration via gradient pore blocking and electrostatic stabilization. This configuration leverages the self-sealing behavior of mud cakes while minimizing the skin factor, offering a 23% productivity improvement over single-layer designs (vs. Ref. [25]). By selecting an optimal median grain size ratio within the range of 24 to 31 for the secondary layer, both sand control efficiency and permeability retention can be further optimized.
- (3)
- Roadmap for Field Application and Knowledge Gaps: Key barriers to scaling laboratory findings include (a) temperature sensitivity: depressurization-induced cooling (ΔT ≈ −2 °C [4]) may alter clay swelling dynamics, unaccounted for in current isothermal experiments; (b) long-term stability: ceramic abrasion and chemical interactions (e.g., hydrate reformation in pores) require >1000-h cyclic flow tests; and (c) radial flow bias: unidirectional experiments underestimate screen erosion in the radial wells (3× higher plugging rates observed in Ref. [25]). To bridge these gaps, future work should prioritize (a) multi-physics modeling: integrate thermal-hydraulic-mechanical (THM) coupling with DEM to predict mud-cake evolution; (b) material engineering: develop hydrophobic ceramic coatings (e.g., silane grafting [22]) to inhibit clay adhesion; and (c) field pilots: validate graded packing in offshore hydrate trials with real-time P/T/sand monitoring (e.g., China’s Shenhu Area).
Author Contributions
Funding
Data Availability Statement
Conflicts of Interest
References
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Sample Types | Median Grain Size (d50) /μm | Particle Size Interval /μm | Median Grain Size Ratio | Note |
---|---|---|---|---|
170–230 mesh | 82.075 | 17.125~251.105 | 8 | Custom |
140–170 mesh | 128.12 | 58.041~283.704 | 12 | Custom |
80–120 mesh | 183.358 | 83.707~409.163 | 17 | Custom |
70–80 mesh | 248.57 | 106.852~22.296 | 24 | Custom |
40–70 mesh | 330.396 | 196.714~51.056 | 31 | Existing |
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Zhao, X.; Zhao, Y.; Mu, M.; Zhou, A.; Zhao, H.; Xie, F. Plugging Experiments for Ceramic Filling Layer with Different Grain Sizes Under Gas–Water Mixed Flow for Natural Gas Hydrate Development. Energies 2025, 18, 1761. https://doi.org/10.3390/en18071761
Zhao X, Zhao Y, Mu M, Zhou A, Zhao H, Xie F. Plugging Experiments for Ceramic Filling Layer with Different Grain Sizes Under Gas–Water Mixed Flow for Natural Gas Hydrate Development. Energies. 2025; 18(7):1761. https://doi.org/10.3390/en18071761
Chicago/Turabian StyleZhao, Xiaolong, Yizhong Zhao, Meng Mu, Aiyong Zhou, Haifeng Zhao, and Fei Xie. 2025. "Plugging Experiments for Ceramic Filling Layer with Different Grain Sizes Under Gas–Water Mixed Flow for Natural Gas Hydrate Development" Energies 18, no. 7: 1761. https://doi.org/10.3390/en18071761
APA StyleZhao, X., Zhao, Y., Mu, M., Zhou, A., Zhao, H., & Xie, F. (2025). Plugging Experiments for Ceramic Filling Layer with Different Grain Sizes Under Gas–Water Mixed Flow for Natural Gas Hydrate Development. Energies, 18(7), 1761. https://doi.org/10.3390/en18071761