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Keywords = radon and thoron exhalation rates

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12 pages, 2228 KB  
Article
The Radon Exhalation Rate and Dose Assessment of Granite Used as a Building Material in Serbia
by Fathya Shabek, Božidar Obradović, Igor Čeliković, Mirjana Đurašević, Aleksandra Samolov, Predrag Kolarž and Aco Janićijević
Atmosphere 2024, 15(12), 1495; https://doi.org/10.3390/atmos15121495 - 15 Dec 2024
Cited by 1 | Viewed by 1553
Abstract
The application of energy-saving policies in buildings could lead to a decrease in the air exchange rate in dwellings, which could consequently lead to an increase in indoor radon concentration and, therefore, to an increase in resident exposure to ionizing radiation. The aim [...] Read more.
The application of energy-saving policies in buildings could lead to a decrease in the air exchange rate in dwellings, which could consequently lead to an increase in indoor radon concentration and, therefore, to an increase in resident exposure to ionizing radiation. The aim of the research presented in this paper is to investigate radiological exposure to residents due to the usage of different granites commonly used in Serbia as a building material. From the total of 10 analysed granite samples, a wide range of radon and thoron exhalation rates were found: from <161 μBq m−2 s−1 to 5220 ± 200 μBq m−2 s−1 and from <7 mBq m−2 s−1 to 5140 ± 320 mBq m−2 s−1, respectively. Assuming a low air exchange rate of 0.2 h−1, the contribution of the measured granite material to the indoor radon concentration could go up to 150 Bq m−3. The estimated annual effective doses due to exposure to radon and thoron exhalation from the granite samples were (0.05–3.79) mSv and (<0.01–1.74) mSv, respectively. The specific activity of radionuclides ranged from 6.6 ± 0.5 Bq kg−1 to 131.8 ± 9.4 Bq kg−1 for 226Ra, from 0.5 ± 0.1 Bq kg−1 to 120.8 ± 6.5 Bq kg−1 for 232Th, and from 0.22 ± 0.01 Bq kg−1 to 1321 ± 86 Bq kg−1 for 40K. The obtained external hazard index ranged from 0.03 to 1.48, with three samples above or very close to the accepted safety limit of 1. In particular, dwellings with a low air exchange rate (causing elevated radon) could lead to an elevated risk of radiation exposure. Full article
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12 pages, 1773 KB  
Article
Seasonal Variations in Radon and Thoron Exhalation Rates from Solid Concrete Interior Walls Observed Using In Situ Measurements
by Akihiro Sakoda, Yuu Ishimori, Md. Mahamudul Hasan, Qianhao Jin and Takeshi Iimoto
Atmosphere 2024, 15(6), 701; https://doi.org/10.3390/atmos15060701 - 12 Jun 2024
Cited by 2 | Viewed by 1303
Abstract
Building materials, such as brick and concrete, are known indoor radon (222Rn) and thoron (220Rn) sources. Most radon and thoron exhalation studies are based on the laboratory testing of pieces and blocks of such materials. To discuss if laboratory [...] Read more.
Building materials, such as brick and concrete, are known indoor radon (222Rn) and thoron (220Rn) sources. Most radon and thoron exhalation studies are based on the laboratory testing of pieces and blocks of such materials. To discuss if laboratory findings can be applied to a real-world environment, we conducted intensive in situ exhalation tests on two solid concrete interior walls of an apartment in Japan for over a year. Exhalation rates of radon (JRn) and thoron (JTn) were measured using an accumulation chamber and dedicated monitors, alongside monitoring indoor air temperature (T) and absolute humidity (AHin). There were weak correlations between JRn or JTn and T or AHin at one tested wall, and moderate correlations of JRn and strong correlations of JTn with T or AHin at the other wall, meaning more or less seasonal variations. The findings aligned with previous laboratory experiments on JRn but lacked corresponding data for JTn. Additionally, a moderate or strong correlation between JRn and JTn was observed for both tested walls. Comparison with theoretical calculations revealed a new issue regarding the impact of each process of emanation and migration within concrete pores on radon and thoron exhalation. Overall, this study provides insight into parameterizing radon and thoron source inputs in modeling the spatiotemporal dynamics of indoor radon and thoron. Full article
(This article belongs to the Special Issue Environmental Radon Measurement and Radiation Exposure Assessment)
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11 pages, 5067 KB  
Article
The Determination of Radon/Thoron Exhalation Rate in an Underground Coal Mine—Preliminary Results
by Michał Bonczyk, Stanisław Chałupnik, Malgorzata Wysocka, Agata Grygier, Robert Hildebrandt and Zornitza Tosheva
Int. J. Environ. Res. Public Health 2022, 19(10), 6038; https://doi.org/10.3390/ijerph19106038 - 16 May 2022
Cited by 14 | Viewed by 2532
Abstract
The objective of this work was to perform a series of measurements of radon and thoron exhalation in the underground workings of an experimental coal mine. In the years 2012–2015, experiments on underground coal gasification were carried out in a coal mine, which [...] Read more.
The objective of this work was to perform a series of measurements of radon and thoron exhalation in the underground workings of an experimental coal mine. In the years 2012–2015, experiments on underground coal gasification were carried out in a coal mine, which caused, among other effects, damage to rock mass. Afterward, periodic increases in the concentration of potential alpha energy (PAEC) of radon decay products in the air were found, which could pose a hazard to miners. The question posed was whether the gasification experiment resulted in the increased migration of radon and thoron. If so, did it increase the radiation hazard to miners? The adaptation of the existing instrumentation to the specific conditions was conducted, and a series of measurements were made. It was found that the measured values of radon and thoron exhalation rates ranged from 3.0 up to 38 Bq·m−2·h−1 for radon and from 500 up to 2000 Bq·m−2·h−1 for thoron. Full article
(This article belongs to the Special Issue Environmental Radioactivity Monitoring and Measurements: Radon)
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18 pages, 74987 KB  
Article
A Study of Natural Radioactivity Levels and Radon/Thoron Release Potential of Bedrock and Soil in Southeastern Ireland
by Mirsina Mousavi Aghdam, Quentin Crowley, Carlos Rocha, Valentina Dentoni, Stefania Da Pelo, Stephanie Long and Maxime Savatier
Int. J. Environ. Res. Public Health 2021, 18(5), 2709; https://doi.org/10.3390/ijerph18052709 - 8 Mar 2021
Cited by 17 | Viewed by 4840
Abstract
Radon (222Rn) and thoron (220Rn) account for almost two-thirds of the annual average radiation dose received by the Irish population. A detailed study of natural radioactivity levels and radon and thoron exhalation rates was carried out in a legislatively [...] Read more.
Radon (222Rn) and thoron (220Rn) account for almost two-thirds of the annual average radiation dose received by the Irish population. A detailed study of natural radioactivity levels and radon and thoron exhalation rates was carried out in a legislatively designated “high radon” area, as based on existing indoor radon measurements. Indoor radon concentrations, airborne radiometric data and stream sediment geochemistry were collated, and a set of soil samples were taken from the study area. The exhalation rates of radon (E222Rn) and thoron (E220Rn) for collected samples were determined in the laboratory. The resultant data were classified based on geological and soil type parameters. Geological boundaries were found to be robust classifiers for radon exhalation rates and radon-related variables, whilst soil type classification better differentiates thoron exhalation rates and correlated variables. Linear models were developed to predict the radon and thoron exhalation rates of the study area. Distribution maps of radon and thoron exhalation rates (range: E222Rn [0.15–1.84] and E220Rn [475–3029] Bq m−2 h−1) and annual effective dose (with a mean value of 0.84 mSv y−1) are presented. For some parts of the study area, the calculated annual effective dose exceeds the recommended level of 1 mSv y−1, illustrating a significant radiation risk. Airborne radiometric data were found to be a powerful and fast tool for the prediction of geogenic radon and thoron risk. This robust method can be used for other areas where airborne radiometric data are available. Full article
(This article belongs to the Special Issue Environmental Radioactivity Monitoring and Measurements: Radon)
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11 pages, 2852 KB  
Article
Long-Term Measurements of Radon and Thoron Exhalation Rates from the Ground Using the Vertical Distributions of Their Activity Concentrations
by Oumar Bobbo Modibo, Yuki Tamakuma, Takahito Suzuki, Ryohei Yamada, Weihai Zhuo, Chutima Kranrod, Kazuki Iwaoka, Naofumi Akata, Masahiro Hosoda and Shinji Tokonami
Int. J. Environ. Res. Public Health 2021, 18(4), 1489; https://doi.org/10.3390/ijerph18041489 - 4 Feb 2021
Cited by 17 | Viewed by 3827
Abstract
A long-term measurement technique of radon exhalation rate was previously developed using a passive type radon and thoron discriminative monitor and a ventilated type accumulation chamber. In the present study, this technique was applied to evaluate the thoron exhalation rate as well, and [...] Read more.
A long-term measurement technique of radon exhalation rate was previously developed using a passive type radon and thoron discriminative monitor and a ventilated type accumulation chamber. In the present study, this technique was applied to evaluate the thoron exhalation rate as well, and long-term measurements of radon and thoron exhalation rates were conducted for four years in Gifu Prefecture. The ventilated type accumulation chamber (0.8 × 0.8 × 1.0 m3) with an open bottom was embedded 15 cm into the ground. The vertical distributions of radon and thoron activity concentrations from the ground were obtained using passive type radon-thoron discriminative monitors (RADUETs). The RADUETs were placed at 1, 3, 10, 30, and 80 cm above the ground inside the accumulation chamber. The measurements were conducted from autumn 2014 to autumn 2018. These long-term results were found to be in good agreement with the values obtained by another methodology. The radon exhalation rates from the ground showed a clearly seasonal variation. Similar to findings of previous studies, radon exhalation rates from summer to autumn were relatively higher than those from winter to spring. In contrast, thoron exhalation rates were not found to show seasonal variation. Full article
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