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Keywords = Fe-Si-Al soft magnetic powder core

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14 pages, 7361 KiB  
Article
Improving the Soft Magnetic Characteristics of Nanocrystalline Soft Magnetic Composites Through the Incorporation of Ultrafine FeSiAl Powders
by Yanyan Song, Zhi Zhang, Shaoxiong Zhou, Ruibiao Zhang, Haichen Yu and Xiantao Li
Magnetochemistry 2025, 11(4), 25; https://doi.org/10.3390/magnetochemistry11040025 - 30 Mar 2025
Cited by 1 | Viewed by 1062
Abstract
Nanocrystalline powders, characterized by a biphasic amorphous nanocrystalline structure, demonstrate outstanding soft magnetic characteristics, including reduced coercivity (Hc), enhanced effective permeability (μe), and increased resistivity. However, their high hardness, poor formability, and significant core loss (P [...] Read more.
Nanocrystalline powders, characterized by a biphasic amorphous nanocrystalline structure, demonstrate outstanding soft magnetic characteristics, including reduced coercivity (Hc), enhanced effective permeability (μe), and increased resistivity. However, their high hardness, poor formability, and significant core loss (Pcv) restrict their use in high-performance molded inductors. In this study, FeSiBCuNb/FeSiAl nanocrystalline soft magnetic composites (NSMCs) were fabricated, and the influence of varying the FeSiAl concentration on the microstructure, density, and soft magnetic characteristics of NSMCs was investigated. Then, the underlying mechanisms of these effects were explained. The results demonstrate that FeSiAl exhibits apparent deformation following compression, effectively filling the air gap between the FeSiBCuNb powder particles, thereby enhancing coupling among the magnetic particles. Consequently, the density of the NSMCs was enhanced, leading to a significant improvement in their overall soft magnetic properties. When 50 wt.% FeSiAl is added, the NSMCs display outstanding magnetic properties, including a low Hc of 4.36 Oe, a high μe of 48.7, a low Pcv of 119.35 kW/m3 at 50 mT and 100 kHz, and a high DC-bias performance of 73.29% at 100 Oe. Compared to NSMCs without FeSiAl, μe increased by 59.4% and Pcv decreased by 66.1%. Meanwhile, the incorporation of ultrafine FeSiAl powder was found to significantly improve the material properties, as the deformable FeSiAl particles effectively fill interparticle gaps during compaction, enhancing density and magnetic coupling. The 50 wt.% FeSiAl composition demonstrated exceptional properties. These advances address critical challenges in high-frequency power electronic applications and provide a practical material solution for next-generation power electronics. Full article
(This article belongs to the Section Magnetic Materials)
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14 pages, 4151 KiB  
Article
Improved Anti-Saturation Performance of Fe-Si-Al Soft Magnetic Powder Core via Adjusting the Alloy Composition
by Bowei Zhang, Zhongqiu Zou, Xuebin Zhang, Yu Han, Wei Liu and Hailin Su
Metals 2024, 14(1), 107; https://doi.org/10.3390/met14010107 - 16 Jan 2024
Cited by 2 | Viewed by 2567
Abstract
Ball-milled Fe-Si-Al soft magnetic powder cores with the particle compositions away from the classical Sendust point were prepared in this work. The influences of alloy composition on the metallographic structure, density, hardness, and resistivity of Fe-Si-Al alloy, as well as the frequency-dependent permeability, [...] Read more.
Ball-milled Fe-Si-Al soft magnetic powder cores with the particle compositions away from the classical Sendust point were prepared in this work. The influences of alloy composition on the metallographic structure, density, hardness, and resistivity of Fe-Si-Al alloy, as well as the frequency-dependent permeability, loss, and the anti-saturation performance of Fe-Si-Al powder cores, were investigated systematically. It was found that the hardness of Fe-Si-Al alloy increases with the Si mass ratio and the saturation magnetization (Ms) increases with the Fe mass ratio. The alloy hardness affects the particle size after the ball-milling process and, thus, influences the porosity of the powder core. Together with adjusting the demagnetization field by controlling the particle size and the core’s porosity, changing the alloy composition to drive K and λ deviating from zero can effectively improve the anti-saturation performance of Fe-Si-Al powder cores at the expense of hysteresis loss, to some extent. In this work, good comprehensive magnetic properties were obtained in the Fe85.5-Si12-Al2.5 powder core. Its effective permeability percentage at 100 Oe and Ms were 59.12% and 132.23 emu/g, respectively, which are higher than those of the classical Sendust core. This work provides a feasible idea for optimizing the overall performance of the high-power magnetic device. Full article
(This article belongs to the Special Issue Soft Magnetic Composites: Manufacture, Properties and Applications)
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14 pages, 4524 KiB  
Article
Enhanced Magnetic Properties and Thermal Conductivity of FeSiCr Soft Magnetic Composite with Al2O3 Insulation Layer Prepared by Sol-Gel Process
by Qintian Xie, Hongya Yu, Han Yuan, Guangze Han, Xi Chen and Zhongwu Liu
Metals 2023, 13(4), 813; https://doi.org/10.3390/met13040813 - 21 Apr 2023
Cited by 9 | Viewed by 2520
Abstract
FeSiCr soft magnetic composites (SMCs) were fabricated by the sol-gel method, and an Al2O3/resin composite layer was employed as the insulation coating. By the decomposition of boehmite (AlOOH) gel into Al2O3 in the temperature range of [...] Read more.
FeSiCr soft magnetic composites (SMCs) were fabricated by the sol-gel method, and an Al2O3/resin composite layer was employed as the insulation coating. By the decomposition of boehmite (AlOOH) gel into Al2O3 in the temperature range of 606–707 °C, a uniform Al2O3 layer could be formed on the FeSiCr powder surface. The Al2O3 insulation coating not only effectively reduced the core loss, increased the resistivity, and improved the quality factor, but it also increased the thermal conductivity of SMCs. The best overall properties with saturation magnetization Ms = 188 emu/g, effective permeability μe = 39, resistivity ρ = 8.28 × 105 Ω·cm, quality factor Q = 94 at 1 MHz, and core loss = 1173 mW/cm3 at 200 kHz and 50 mT were obtained when the SMC was prepared with powders coated by 0.5 wt.% Al2O3 and resin. The optimized SMC exhibited the lowest core loss with 27% reduction compared to the resin only-insulated sample and 71% reduction compared to the sample without insulation treatment. Importantly, the thermal conductivity of the SMCs is 5.3 W/m·K at room temperature, which is higher than that of the samples prepared by phosphating and SiO2 coating owing to the presence of a high thermal conductive Al2O3 layer. The high thermal conductivity is beneficial to enhancing the high temperature performance, lifetime, and reliability of SMCs. This work is expected to be a valuable reference for the design and fabrication of SMCs to be applied in high-temperature and high-frequency environments. Full article
(This article belongs to the Special Issue Advances in Metal-Containing Magnetic Materials)
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11 pages, 3677 KiB  
Article
Study of the Soft Magnetic Properties of FeSiAl Magnetic Powder Cores by Compounding with Different Content of Epoxy Resin
by Zhengqu Zhu, Jiaqi Liu, Huan Zhao, Jing Pang, Pu Wang and Jiaquan Zhang
Materials 2023, 16(3), 1270; https://doi.org/10.3390/ma16031270 - 2 Feb 2023
Cited by 17 | Viewed by 3021
Abstract
FeSiAl is a commonly used soft magnetic material because of its high resistivity, low core loss, and low cost. In order to systematically study the effect of epoxy resin (EP) on the insulated coating and pressing effect of FeSiAl magnetic powders, six groups [...] Read more.
FeSiAl is a commonly used soft magnetic material because of its high resistivity, low core loss, and low cost. In order to systematically study the effect of epoxy resin (EP) on the insulated coating and pressing effect of FeSiAl magnetic powders, six groups of composite powders and their corresponding soft magnetic powder cores (SMPCs) were prepared by changing the content of EP, and the soft magnetic properties of the powders and SMPCs were characterized. The results showed that FeSiAl powders exhibited good sphericity and morphology. The Ms of FeSiAl/EP composite powders was between 117.4–124.8 emu·g−1 after adding (0.3, 0.5, 0.7, 1, 1.5, and 2 wt. %) EP. The permeability μe of SMPCs increased first and then decreased with the increase in EP content. Among them, when the EP content was 1 wt. %, the corresponding SMPCs had the highest μe and excellent DC bias performance (63%, 100 Oe). In the whole test frequency range (50~1000 kHz), SMPCs with 1 wt. % EP content had the lowest core loss (1733.9 mW·cm−3 at 20 mT and 1000 kHz). After that, the loss separation study in the low-frequency range (50~250 kHz) was conducted, and the hysteresis loss and eddy current loss of SMPCs with 1 wt. % EP content were also the lowest. In addition, SMPCs also exhibited the best overall performance when the EP content was 1 wt. %. The results of this study can guide the design of composite insulation coating schemes and promote the development of soft magnetic materials for medium and high frequency applications. Full article
(This article belongs to the Special Issue Soft Magnetic Materials and Their Application)
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10 pages, 2808 KiB  
Article
Enhanced Magnetic Properties of FeSiAl Soft Magnetic Composites Prepared by Utilizing PSA as Resin Insulating Layer
by Hao Lu, Yaqiang Dong, Xincai Liu, Zhonghao Liu, Yue Wu, Haijie Zhang, Aina He, Jiawei Li and Xinmin Wang
Polymers 2021, 13(9), 1350; https://doi.org/10.3390/polym13091350 - 21 Apr 2021
Cited by 40 | Viewed by 3676
Abstract
Thermosetting organic resins are widely applied as insulating coatings for soft magnetic powder cores (SMPCs) because of their high electrical resistivity. However, their poor thermal stability and thermal decomposition lead to a decrease in electrical resistivity, thus limiting the annealing temperature of SMPCs. [...] Read more.
Thermosetting organic resins are widely applied as insulating coatings for soft magnetic powder cores (SMPCs) because of their high electrical resistivity. However, their poor thermal stability and thermal decomposition lead to a decrease in electrical resistivity, thus limiting the annealing temperature of SMPCs. The large amount of internal stress generated by soft magnetic composites during pressing must be mitigated at high temperatures; therefore, it is especially important to find organic resins with excellent thermal stabilities. In this study, we prepared SMPCs using poly-silicon-containing arylacetylene resin, an organic resin resistant to high temperatures, as an insulating layer. With 2 wt % PSA as an insulating layer and annealed at 700 °C for 1 h, the FeSiAl SMPCs achieved the best magnetic properties, including the lowest core loss of 184 mW/cm3 (measured at 0.1 T and 50 kHz) and highest permeability of 96. Full article
(This article belongs to the Section Polymer Composites and Nanocomposites)
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12 pages, 4978 KiB  
Article
Thermal Conductivity and Electromagnetic Interference (EMI) Absorbing Properties of Composite Sheets Composed of Dry Processed Core–Shell Structured Fillers and Silicone Polymers
by Hyun-Seok Choi, Ji-Won Park, Kyung-Sub Lee, Sang-Woo Kim and Su-Jeong Suh
Polymers 2020, 12(10), 2318; https://doi.org/10.3390/polym12102318 - 10 Oct 2020
Cited by 4 | Viewed by 3707
Abstract
This paper proposes dual-functional sheets (DFSs) that simultaneously have high thermal conductivity (TC) and electromagnetic interference (EMI) absorbing properties, making them suitable for use in mobile electronics. By adopting a simple but highly efficient dry process for manufacturing core–shell structured fillers (CSSFs) and [...] Read more.
This paper proposes dual-functional sheets (DFSs) that simultaneously have high thermal conductivity (TC) and electromagnetic interference (EMI) absorbing properties, making them suitable for use in mobile electronics. By adopting a simple but highly efficient dry process for manufacturing core–shell structured fillers (CSSFs) and formulating a close-packed filler composition, the DFSs show high performance, TC of 5.1 W m−1 K−1, and a −4 dB inter-decoupling ratio (IDR) at a 1 GHz frequency. Especially, the DFSs show a high dielectric breakdown voltage (BDV) of 3 kV mm−1, which is beneficial for application in most electronic devices. The DFSs consist of two kinds of CSSFs that are blended in accordance with the close-packing rule, Horsfield’s packing model, and with polydimethylsiloxane (PDMS) polymers. The core materials are soft magnetic Fe-12.5%Cr and Fe-6.5%Si alloy powders of different sizes, and Al2O3 ceramic powders of a 1-μm diameter are used as the shell material. The high performance of the DFS is supposed to originate from the thick and stable shell layer and the maximized filler loading capability owing to the close-packed structure. Full article
(This article belongs to the Special Issue Next-Generation Convergence Industry and Adhesives)
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