Search Results (7)

This study considers aerosol optical properties and direct radiative forcing over Harbin (126.63° E, 45.75° N), the highest latitude city in Northeast China, during 2017. Observations based on the CE-318 sun-photometer show that the annual mean values of the aerosol optical depth (AOD) at 500 nm and the Angstrom exponent (AE) at 440–870 nm over Harbin are respectively $0.26 \pm 0.20$ and $1.36 \pm 0.26$. Aerosol loading is the highest in the spring followed by winter, and the lowest loading is in autumn. ${\mathrm{AE}}_{440–870}$ is the highest in summer, second highest in winter, and lowest in autumn. The Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model is used to estimate the shortwave aerosol radiative forcing at the top of the atmosphere, on the Earth’s surface and in the atmosphere, and the annual mean values are $-16.36 \pm 18.42{ \mathrm{Wm}}^{-2}$, $-71.01 \pm 27.37{ \mathrm{Wm}}^{-2}$ and $54.65 \pm 30.62{ \mathrm{Wm}}^{-2}$, respectively, which indicate that aerosols cause climate effects of cooling the earth-atmosphere system, cooling the earth’s surface and heating the atmosphere. Four main aerosol types in Harbin are classified via AOD and AE. Specifically, clean continental, mixed type, biomass burning and urban industry, and desert dust aerosols accounted for 51%, 38%, 9%, and 2% of the total, respectively. Aerosol radiative forcing varies greatly in different seasons, and the aerosol load and type from different emission sources have an important influence on the seasonal variation of radiative forcing. Full article

Aerosol Optical Depth (AOD) and the Ångström Exponent (AE) have been calculated in the near infrared (NIR) and short-wave infrared (SWIR) spectral regions over a period of one year (May 2019–May 2020) at the high-mountain Izaña Observatory (IZO) from Fourier Transform Infrared (FTIR) solar spectra. The high-resolution FTIR measurements were carried out coincidentally with Cimel CE318-T photometric observations in the framework of the Aerosol Robotic Network (AERONET). A spectral FTIR AOD was generated using two different approaches: by means of the selection of seven narrow FTIR micro-windows (centred at 1020.90, 1238.25, 1558.25, 1636.00, 2133.40, 2192.00, and 2314.20 nm) with negligible atmospheric gaseous absorption, and by using the CE318-AERONET’s response function in the near-coincident bands (1020 nm and 1640 nm) to degrade the high-resolution FTIR spectra. The FTIR system was absolutely calibrated by means of a continuous Langley–Plot analysis over the 1-year period. An important temporal drift of the calibration constant was observed as a result of the environmental exposure of the FTIR’s external optical mirrors (linear degradation rate up to 1.75% month${}^{-1}$). The cross-validation of AERONET-FTIR databases documents an excellent agreement between both AOD products, with mean AOD differences below 0.004 and root-mean-squared errors below 0.006. A rather similar agreement was also found between AERONET and FTIR convolved bands, corroborating the suitability of low-resolution sunphotometers to retrieve high-quality AOD data in the NIR and SWIR domains. In addition, these results demonstrate that the methodology developed here is suitable to be applied to other FTIR spectrometers, such as portable and low-resolution FTIR instruments with a potentially higher spatial coverage. The spectral AOD dependence for the seven FTIR micro-windows have been also examined, observing a spectrally flat AOD behaviour for mineral dust particles (the typical atmospheric aerosols presented at IZO). A mean AE value of 0.53 ± 0.08 for pure mineral dust in the 1020–2314 nm spectral range was retrieved in this paper. A subsequent cross-validation with the MOPSMAP (Modeled optical properties of ensembles of aerosol particles) package has ensured the reliability of the FTIR dataset, with AE values between 0.36 to 0.60 for a typical mineral dust content at IZO of 100 cm${}^{-3}$ and water-soluble particle (WASO) content ranging from 600 to 6000 cm${}^{-3}$. The new database generated in this study is believed to be the first long-term time series (1-year) of aerosol properties generated consistently in the NIR and SWIR ranges from ground-based FTIR spectrometry. As a consequence, the results presented here provide a very promising tool for the validation and subsequent improvement of satellite aerosol products as well as enhance the sensitivity to large particles of the existing databases, required to improve the estimation of the aerosols’ radiative effect on climate. Full article

Based on the Langley method and the EuroSkyRad (ESR) pack retrieval scheme, we carried out the retrieval of the aerosol properties for the CE–318 sunphotometer observation data from March 2012 to February 2014 in Kunming, China, and we explored the possible mechanisms of the seasonal variations. The seasonal variation of the aerosol optical depth (AOD) was unimodal and reached a maximum in summer. The retrieval analysis of the Angstrom exponent (α) showed the aerosol types were continental, biomass burning (BB), and urban/industrial (UI); the content of the desert dust (DD) was low, and it may have contained a sea–salt (SS) aerosol due to the influence of the summer monsoon. All the aerosol particle spectra in different seasons showed a bimodal structure. The maximum and submaximal values were located near 0.2 μm and 4 μm, respectively, and the concentration of the aerosol volume was the highest in summer. In summer, aerosol particles have a strong scattering power but a weak absorption power; this pattern is the opposite in winter. The synergistic effect of the East Asian monsoon and the South Asian monsoon seasonal oscillations can have an important impact on the variation of the aerosol properties. The oscillation variation characteristic of the total vertical columnar water vapor (CWV) and the monsoon index was completely consistent. The aerosol types and sources in the Yunnan–Kweichow Plateau and the optical radiation properties were closely related to the monsoon circulation activities during different seasons and were different from other regions in China. Full article

The visible infrared imaging radiometer suite (VIIRS) environmental data record aerosol product (VIIRS_EDR) and the aqua-moderate resolution imaging spectroradiometer (MYD04) collection 6 (C6) aerosol optical depth (AOD) products are validated against the Cimel sun–photometer (CE318) AOD measurements during different air quality conditions over the Yangtze river basin (YRB) from 2 May 2012 to 31 December 2016. For VIIRS_EDR, the AOD observations are obtained from the scientific data set (SDS) “aerosol optical depth at 550 nm” at 6 km resolution, and for aqua-MODIS, the AOD observations are obtained from the SDS “image optical depth land and ocean” at 3 km (DT3K) and 10 km (DT10K) resolutions, “deep blue aerosol optical depth 550 land” at 10 km resolution (DB10K), and “AOD 550 dark target deep blue combined” at 10 km resolution (DTB10K). Results show that the high-quality (QF = 3) DTB10K performs the best against the CE318 AOD observations, along with a higher R (0.85) and more retrievals within the expected error (EE) ± (0.05 + 15%) (55%). Besides, there is a 10% overestimation, but the positive bias does not exhibit obvious seasonal variations. Similarly, the DT3K and DT10K products overestimate AOD retrievals by 23% and 15%, respectively, all over the year, but the positive biases become larger in spring and summer. For the DB10K AOD retrievals, there is an overestimation (underestimation) in autumn and winter (spring and summer). Compared to the aqua-MODIS AOD products, the VIIRS_EDR AOD retrievals are less correlated (R = 0.73) and only 44% of the retrievals fall within EE. Meanwhile, the VIIRS_EDR shows larger bias than the aqua-MODIS C6 retrievals, and tends to overestimate AOD retrievals in summer and underestimate in winter. Additionally, there is an underestimation for the VIIRS_EDR AOD retrievals over the regions during high aerosol loadings. These indicate that the VIIRS_EDR retrieval algorithm needs to be improved in further applications over the YRB. Full article

The airborne Atmosphere Multi-angle Polarization Radiometer (AMPR) was employed to perform airborne measurements over North China between 2012 and 2016. Seven flights and synchronous ground-based observations were acquired. These data were used to test the sensor’s measurements and associated aerosol retrieval algorithm. According to the AMPR measurements, a successive surface-atmosphere decoupling based algorithm was developed to retrieve the aerosol optical depth (AOD). It works via an iteration method, and the lookup table was employed in the aerosol inversion. Throughout the results of the AMPR retrievals, the surface polarized reflectances derived from air- and ground-based instruments were well matched; the measured and simulated reflectances at the aircraft level, which were simulated based on in situ sun photometer observed aerosol properties, were in good agreement; and the AOD measurements were validated against the automatic sun-photometer (CE318) at the nearest time and location. The AOD results were close; the average deviation was less than 0.03. The MODIS AODs were also employed to test the AMPR retrievals, and they showed the same trend. These results illustrate that (i) the successive surface-atmosphere decoupling method in the retrieved program completed its mission and (ii) the aerosol retrieval method has its rationality and potential ability in the regionally accurate remote sensing of aerosol. Full article

The first Visible Infrared Imaging Radiometer Suite (VIIRS) was launched on Suomi National Polar-orbiting Partnership (S-NPP) satellite in late 2011. Similar to the Moderate resolution Imaging Spectroradiometer (MODIS), VIIRS observes top-of-atmosphere spectral reflectance and is potentially suitable for retrieval of the aerosol optical depth (AOD). The VIIRS Environmental Data Record data (VIIRS_EDR) is produced operationally by NOAA, and is based on the MODIS atmospheric correction algorithm. The “MODIS-like” VIIRS data (VIIRS_ML) are being produced experimentally at NASA, from a version of the “dark-target” algorithm that is applied to MODIS. In this study, the AOD and aerosol model types from these two VIIRS retrieval algorithms over the North China Plain (NCP) are evaluated using the ground-based CE318 Sunphotometer (CE318) measurements during 2 May 2012–31 March 2014 at three sites. These sites represent three different surface types: urban (Beijing), suburban (XiangHe) and rural (Xinglong). Firstly, we evaluate the retrieved spectral AOD. For the three sites, VIIRS_EDR AOD at 550 nm shows a positive mean bias (MB) of 0.04–0.06 and the correlation of 0.83–0.86, with the largest MB (0.10–0.15) observed in Beijing. In contrast, VIIRS_ML AOD at 550 nm has overall higher positive MB of 0.13–0.14 and a higher correlation (0.93–0.94) with CE318 AOD. Secondly, we evaluate the aerosol model types assumed by each algorithm, as well as the aerosol optical properties used in the AOD retrievals. The aerosol model used in VIIRS_EDR algorithm shows that dust and clean urban models were the dominant model types during the evaluation period. The overall accuracy rate of the aerosol model used in VIIRS_ML over NCP three sites (0.48) is higher than that of VIIRS_EDR (0.27). The differences in Single Scattering Albedo (SSA) at 670 nm between VIIRS_ML and CE318 are mostly less than 0.015, but high seasonal differences are found especially over the Xinglong site. The values of SSA from VIIRS_EDR are higher than that observed by CE318 over all sites and all assumed aerosol modes, with a positive bias of 0.02–0.04 for fine mode, 0.06–0.12 for coarse mode and 0.03–0.05 for bi-mode at 440 nm. The overestimation of SSA but positive AOD MB of VIIRS_EDR indicate that other factors (e.g., surface reflectance characterization or cloud contamination) are important sources of error in the VIIRS_EDR algorithm, and their effects on aerosol retrievals may override the effects from non-ideality in these aerosol models. Full article

In situ observation of the aerosol optical properties is important to the validations of satellite and modeling results; however, the operational measurements can be affected by some objective factors. An experiment study has been performed in order to analyze the error in retrievals of aerosol optical properties from sunphotometer measurements caused by a variety of in situ objective factors. The standard instrument relative error analysis method was used to determine the relative error of aerosol optical depth (AOD) and Ångström exponent (AE) under the effects of five factors: spider web inside the collimator (F1); collimator bending (F2); dust inside the optical head (F3); incrustation scale inside the optical head (F4); and dust and incrustation scale inside the optical head (F5). The results showed that the five factors caused error for AOD retrieved at 1020, 870, 670 and 440 nm, with the maximum error occurring at 870 nm due to the more sensitive measurement signals. The error ranges of AOD derived from the direct solar measurements in the four bands were −0.34%–8.77%, −6.22%–9.68%, −0.05%–2.52%, −0.96%–3.48% and 5.42%–13.38% for F1, F2, F3, F4 and F5, respectively. The maximum error occurred under the influence of F5 with an average error value of 10%, while the minimum occurred owing to F3 with an average error value of 1%. All of the AEs retrieved from the experimental instruments were smaller than that from the reference instrument. The AE error values were 15.19%, 25.57%, 4.56%, 4.41% and 8.83% for F1, F2, F3, F4 and F5, respectively. The average AE retrieval error value was 11.7%. Full article