Fully Printed Wearable Electrode Textile for Electrotherapy Application ^†

Abstract

Electrotherapy is a common therapeutic treatment used in pain relief. This paper presents the materials and fabrication methods used to manufacture an electrode textile for electrotherapy application. The Young’s modulus of the electrode is 0.22 MPa. The electrode textile consists of conductive tracks sandwiched between an interface layer and an encapsulation layer, and an electrode layer printed directly on top of the conductive grid patterns. The interface, conductive silver, and encapsulation layers were directly printed on fabric using screen printing. The electrode layer was printed using stencil printing. The electrode textile can survive 10,000 bending cycles around a cylinder with a diameter of 30 mm and 20 washes in a commercial washing machine.

Published: 18 January 2021

1. Introduction

Electrotherapy is a common therapeutic treatment which applies 0–100 milliampere current through electrodes placed on the skin to stimulate the nerve and interfere with the transmission of pain signals. It can be used in pain relief for knee osteoarthritis which will affect 8.3 million people in the UK by 2035 [1].

An electrotherapy device consists of two parts including an electronic control unit to control the current parameters and electrodes to deliver the current. Traditional electrotherapy devices use gel electrodes which are not compatible with textiles [2]. It is recommended gel electrodes are kept in sealed bags after use to maintain the moisture level. The standard lifetime for the gel electrodes is only 2–4 weeks due to the drying out of the electrode and the electrode contamination.

In previous work, a novel dry electrode (Fabink E-0002) was developed by the University of Southampton research group [3]. The soft and tacky (but not sticky) novel electrode combines the advantages of the dry electrode (e.g., easy to use, easy to maintain) and gel electrode (e.g., good skin contact, no hot spots) [4]. This work presents the fabrication process of an electrode textile, and its mechanical property and durability during bending and washing.

2. Materials

The polyester/cotton (A1656, plain weaving, 165 μm thick) used in this study was purchased from Whaleys Bradford Ltd. (Bradford, UK). The functional pastes for screen printing listed in

Table 1. Pastes and their functionality.

Pastes	Functionality
Fabink UV-IF-1004	Standard interface to create smooth surface on various fabrics
Fabink UV-IF-1039	Waterproof interface and encapsulation suitable for various fabrics
Fabink TC-C4007	Silver ink for printing flexible conductive layer on top of the interface layer
Fabink E-0002	Carbon rubber paste for soft and tacky (but not sticky) electrode
Binder material of the novel electrode paste	Rubber to protect silver tracks and improve the electrode–fabric adhesion

were supplied by Smart Fabric Inks Ltd. (Southampton, UK).

3. Methods

3.1. Tensile Test

The equipment used for the tensile test was the Tinius Olsen H25KS tensometer. As shown in Figure 1, the electrode sample was clamped in a vertical direction using two grips. The tensile force on the grips was recorded during the test. The tensile stress was calculated by the software as a part of the testing system.

3.2. Printing Method

A DEK248 semi-automatic screen printer shown in Figure 2a was used to print the interface, conductive silver, and encapsulation layers. Screens were supplied by MCI Precision Screens Ltd. (Melbourn, UK). Figure 2b shows the schematic diagram of stencil printing which was used to fabricate the electrode layer. The paste was placed in a 6 cm × 6 cm × 2 mm aluminum frame and casted using a squeegee to form a smooth surface.

4. Results and Discussion

4.1. Tensile Test

Figure 3 shows the tensile stress–strain curve of the electrode. The stress increases with strain from 0 to until the sample was broken. Young’s modulus is calculated as the slope of the linear fitting line, where the value is 0.22 MPa. The elongation is 355%.

For reference, the Young’s modulus of the skin is between 0.42 MPa and 0.85 MPa [5]. The electrode is softer than skin and provides good conformability without constraining body movement or causing discomfort during movement.

4.2. Electrode Textile

4.2.1. Fabrication Process

An electrode textile was fabricated by printing the five layers in the following order:

(1)

Interface layer to create a smooth and flexible surface on which the silver paste can be printed (Figure 4a). The interface layer was formed using two prints of Fabink IF-UV-1039 followed one print of Fabink IF-UV-1004. The Fabink IF-UV-1039 provides a waterproof layer and the Fabink UV-IF-1004 creates a smooth surface with good adhesion to the silver layer. Ultraviolet (UV) curing was applied after each print by exposing the sample to a UV cabinet supplied by UV Light Technology Ltd. (Birmingham, UK). The UV curing time was 60 s for Fabink IF-UV-1039 and 30 s for Fabink IF-UV1004.

(2)

Conductive silver layer to create the conductive tracks and conductive grid patterns shown in Figure 4b. The conductive layer was formed using one print of Fabink TC-C4007. The paste was cured in a box oven at 130 °C for 25 min.

(3)

Encapsulation layer printing to create a protective layer for the conductive tracks (Figure 4c). The encapsulation layer was formed using one print of Fabink IF-UV1004 followed by two prints of Fabink IF-UV-1039. Curing time was the same as those used in the interface layer.

(4)

Carbon rubber layer to provide an interface between the conductive pads and the skin (Figure 4d). The electrode layer was directly printed on top of conductive grid patterns using stencil printing. The electrode paste was cured in a box oven at 80 °C for 30 min.

(5)

Rubber layer printing around the electrode edges and silver tracks to provide electrode adhesion to the fabric and protect the conductive tracks (Figure 4e). The rubber layer was printed by hand with a syringe and cured in a box oven at 80 °C for 20 min.

4.2.2. Durability Test

The electrode textile was tested on a bending machine (Figure 5a). The diameter of the cylinder was 30 mm. The resistance change during the bending test is shown in Figure 5b. The initial resistance was 223.4 ± 51 Ω. After 5,000 bending cycles, the samples resistance was 393.7 ± 86 Ω. After 10,000 bending cycles, the samples resistance values varied from 500 Ω to 1,500 Ω.

The electrode textile was placed in a wash basket and washed with a lab coat in a commercial washing machine WME7247 supplied by Beko plc (UK). The washing time was 49 min with a spin speed at 1,000 round per minute and water temperature at 30 °C. The initial resistance of electrode textile samples was 248.3 ± 46 Ω. After 20 washes, the sample’s resistance was 342.9 ± 52 Ω. The resistance of the sample increased around 100 Ω after 20 washing cycles. The increasing resistance will increase the power consumption in electrotherapy application. However, functionality was still achieved after 20 washes.

5. Conclusions and Future Work

This paper presents the fabrication process of an electrode textile used in electrotherapy for pain relief. The Young’s modulus of the dry electrode was 0.22 MPa which is softer than human skin providing good conformability and comfort in wearable applications. The electrode could be stretched to 355% before it broke. The electrode textile survived 10,000 bending cycles at a diameter of 30 mm cylinder and 20 washes in a commercial washing machine. The electrode textile will be tested in wearable electrotherapy applications to reduce knee joint pain.