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Nanomaterials
Volume 16
Issue 2
10.3390/nano16020124
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Article

Self-Assembling Conjugated Organic Materials with a Silazane Anchor Group: Synthesis, Self-Organization, and Semiconductor Properties

by
Elizaveta A. Bobrova
1,2,
Maxim S. Skorotetсky
1,
Bogdan S. Kuleshov
1,
Victoria P. Gaidarzhi
1,
Askold A. Trul
1,
Elena V. Agina
1,
Oleg V. Borshchev
1,* and
Sergey A. Ponomarenko
1,*
1
Enikolopov Institute of Synthetic Polymer Materials of the Russian Academy of Sciences, Profsoyuznaya Str. 70, 117393 Moscow, Russia
2
Moscow Center for Advanced Studies, Kulakova Str. 20, 123592 Moscow, Russia
*
Authors to whom correspondence should be addressed.
Nanomaterials 2026, 16(2), 124; https://doi.org/10.3390/nano16020124 (registering DOI)
Submission received: 27 November 2025 / Revised: 6 January 2026 / Accepted: 13 January 2026 / Published: 16 January 2026
(This article belongs to the Section Nanofabrication and Nanomanufacturing)
Versions Notes

Abstract

An efficient synthetic method for the preparation of self-assembling conjugated organic materials with a silazane anchor group based on direct hydrosilylation reaction is reported. A novel organic semiconductor molecule, NH(Si-Und-BTBT-Hex)2, consisting of a polar silazane anchor group linked through undecylenic (Und) aliphatic spacers to conjugated blocks based on benzothieno[3,2-b][1]benzothiophene (BTBT) and solubilizing hexyl (Hex) end groups, was synthesized. Its self-organization on the air-water interface and solid substrates into ultrathin layers obtained by the Langmuir–Schaefer or Langmuir–Blodgett methods was investigated. Monolayer organic field-effect transistors manufactured from NH(Si-Und-BTBT-Hex)2 showed operation in the p-type mode.
Keywords: organic semiconductor; silazane group; hydrosilylation; self-organization; monolayer; Langmuir–Blodgett; Langmuir–Schaefer organic semiconductor; silazane group; hydrosilylation; self-organization; monolayer; Langmuir–Blodgett; Langmuir–Schaefer

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MDPI and ACS Style

Bobrova, E.A.; Skorotetсky, M.S.; Kuleshov, B.S.; Gaidarzhi, V.P.; Trul, A.A.; Agina, E.V.; Borshchev, O.V.; Ponomarenko, S.A. Self-Assembling Conjugated Organic Materials with a Silazane Anchor Group: Synthesis, Self-Organization, and Semiconductor Properties. Nanomaterials 2026, 16, 124. https://doi.org/10.3390/nano16020124

AMA Style

Bobrova EA, Skorotetсky MS, Kuleshov BS, Gaidarzhi VP, Trul AA, Agina EV, Borshchev OV, Ponomarenko SA. Self-Assembling Conjugated Organic Materials with a Silazane Anchor Group: Synthesis, Self-Organization, and Semiconductor Properties. Nanomaterials. 2026; 16(2):124. https://doi.org/10.3390/nano16020124

Chicago/Turabian Style

Bobrova, Elizaveta A., Maxim S. Skorotetсky, Bogdan S. Kuleshov, Victoria P. Gaidarzhi, Askold A. Trul, Elena V. Agina, Oleg V. Borshchev, and Sergey A. Ponomarenko. 2026. "Self-Assembling Conjugated Organic Materials with a Silazane Anchor Group: Synthesis, Self-Organization, and Semiconductor Properties" Nanomaterials 16, no. 2: 124. https://doi.org/10.3390/nano16020124

APA Style

Bobrova, E. A., Skorotetсky, M. S., Kuleshov, B. S., Gaidarzhi, V. P., Trul, A. A., Agina, E. V., Borshchev, O. V., & Ponomarenko, S. A. (2026). Self-Assembling Conjugated Organic Materials with a Silazane Anchor Group: Synthesis, Self-Organization, and Semiconductor Properties. Nanomaterials, 16(2), 124. https://doi.org/10.3390/nano16020124

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