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Appl. Sci. 2018, 8(3), 318;

Imaging Electron Dynamics with Ultrashort Light Pulses: A Theory Perspective

Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, D-22607 Hamburg, Germany
The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, D-22761 Hamburg, Germany
Received: 12 January 2018 / Revised: 13 February 2018 / Accepted: 14 February 2018 / Published: 25 February 2018
(This article belongs to the Special Issue Extreme Time Scale Photonics)
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A wide range of ultrafast phenomena in various atomic, molecular and condense matter systems is governed by electron dynamics. Therefore, the ability to image electronic motion in real space and real time would provide a deeper understanding of such processes and guide developments of tools to control them. Ultrashort light pulses, which can provide unprecedented time resolution approaching subfemtosecond time scale, are perspective to achieve real-time imaging of electron dynamics. This task is challenging not only from an experimental view, but also from a theory perspective, since standard theories describing light-matter interaction in a stationary regime can provide erroneous results in an ultrafast case as demonstrated by several theoretical studies. We review the theoretical framework based on quantum electrodynamics, which has been shown to be necessary for an accurate description of time-resolved imaging of electron dynamics with ultrashort light pulses. We compare the results of theoretical studies of time-resolved nonresonant and resonant X-ray scattering, and time- and angle-resolved photoelectron spectroscopy and show that the corresponding time-resolved signals encode analogous information about electron dynamics. Thereby, the information about an electronic system provided by these time-resolved techniques is different from the information provided by their time-independent analogues. View Full-Text
Keywords: ultrafast light-matter interaction; electron dynamics; time-resolved imaging ultrafast light-matter interaction; electron dynamics; time-resolved imaging

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Popova-Gorelova, D. Imaging Electron Dynamics with Ultrashort Light Pulses: A Theory Perspective. Appl. Sci. 2018, 8, 318.

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