Compactibility and Fibre Volume Fraction Limits of Unidirectional Discontinuous Carbon Fibre Thermoset Prepreg Laminates
Abstract
1. Introduction
- (i)
- Fibre reorientation and nesting at low pressures;
- (ii)
- Bending and local rearrangement at intermediate pressures;
- (iii)
- Fibre deformation (up to fibre breakage) and matrix-dominated compression at high pressures.
2. Materials and Methods
2.1. Materials
2.2. Mesoscopic FOD Analysis Method
2.3. Specimen Manufacturing and Testing
3. Results
3.1. FOD Analysis Results
3.2. Derivation of Pressure over FVC Curves
3.3. Data Extension to Distinct Process Parameters
3.4. Comparing FVC-FOD Results with Previous Work
4. Conclusions
- ▪
- Continuous CF laminates exhibit significantly higher compactibility under moderate pressures compared to UD staple CF tapes. Efficient intra-ply filament nesting enables rapid densification, even for biaxial stackings, whereas fibre discontinuity and misalignment limit packing efficiency in staple systems.
- ▪
- The compaction response of staple CF laminates is strongly governed by FOD. Both mesoscopic image analysis and mechanical compaction trials indicate that higher nominal alignment (HS) is associated with increased scatter in FVC. This behaviour is attributed to spatial inhomogeneities introduced during the carding and alignment process, leading to locally over- and under-aligned regions.
- ▪
- Extrapolation of the compaction curves demonstrates that aerospace-grade FVC values (~60%) would require consolidation pressures approaching 90 bar for the investigated material system. Such pressure levels exceed typical autoclave capabilities, indicating that pressure increase alone is not a viable route for achieving structural-grade FVC in current UD staple CF prepregs.
Author Contributions
Funding
Data Availability Statement
Acknowledgments
Conflicts of Interest
References
- Such, M.; Ward, C.; Potter, K.D. Aligned Discontinuous Fibre Composites: A Short History. J. Multifunct. Compos. 2014, 2, 155–168. [Google Scholar] [CrossRef]
- Baz, S.; Ausheyks, L.; Reichert, O.; Dinkelmann, A.; Finckh, H.; Hehl, J.; Poeppel, A.; Gresser, G.T. Recycling of long carbon fibers, Part I: Development of a high aligned RCF-sliver for a binder tape manufacturing process. In Proceedings of the ECCM 2018—18th European Conference on Composite Materials, Athens, Greece, 24–28 June 2018. [Google Scholar]
- Goergen, C.; Baz, S.; Mitschang, P.; Gresser, G.T.; Heitmann, U. Plastically deformable thanks to staple fibers. Kunststoffe Int. 2016, 5, 25–28. [Google Scholar]
- Hasan, M.M.B.; Hengstermann, M.; Dilo, R.; Abdkader, A.; Cherif, C. Investigations on the manufacturing and mechanical properties of spun yarns made from staple CF for thermoset composites. Autex Res. J. 2017, 17, 395–404. [Google Scholar] [CrossRef]
- Xiao, B.; Zaima, T.; Shindo, K.; Kohira, T.; Morisawa, J.; Wan, Y.; Yin, G.; Ohsawa, I.; Takahashi, J. Characterization and elastic property modeling of discontinuous carbon fiber reinforced thermoplastics prepared by a carding and stretching system using treated carbon fibers. Compos.–A Appl. Sci. Manuf. 2019, 126, 105598. [Google Scholar] [CrossRef]
- Manis, F.; Stegschuster, G.; Wölling, J.; Schlichter, S. Influences on textile and mechanical properties of recycled carbon fiber nonwovens produced by carding. J. Compos. Sci. 2021, 5, 209. [Google Scholar] [CrossRef]
- Khurshid, M.F.; Abdkader, A.; Cherif, C. Processing of waste carbon and polyamide fibres for high-performance thermoplastic composites: Influence of carding parameters on fibre orientation, fibre length and sliver cohesion force. J. Text. Inst. 2020, 111, 1277–1287. [Google Scholar] [CrossRef]
- Krauklis, A.E.; Karl, C.W.; Gagani, A.I.; Jørgensen, J.K. Composite material recycling technology—State-of-the-art and sustainable development for the 2020s. J. Compos. Sci. 2021, 5, 28. [Google Scholar] [CrossRef]
- Zhang, J.; Chevali, V.S.; Wang, H.; Wang, C.H. Current status of carbon fibre and carbon fibre composites recycling. Compos. B Eng. 2020, 193, 108053. [Google Scholar] [CrossRef]
- Mehdipour, M.; Dogan, S.; Tabrizi, A.T.; Bafqi, M.S.S.; Beylergil, B.; Yildiz, M.; Okan, B.S. Engineering interfacial thermal transport through comparative analysis of electrospraying and dip coating of silanized h-BN for thermo-mechanical enhancement of CF/Epoxy composites. Compos.–A Appl. Sci. Manuf. 2025, 199, 109264. [Google Scholar] [CrossRef]
- Tutunchi, A.; Ghodrati, T.; Taghizadeh Tabrizi, A.; Osouli-Bostanabad, K. Enhancing the Mechanical Properties of CF-Reinforced Epoxy Composites through Chemically Surface Modification of Carbon Fibers via Novel Two-Step Approach by Addition of Epichlorohydrin. Funct. Compos. Struct. 2024, 6, 035005. [Google Scholar] [CrossRef]
- Laurencin, T.; Dumont, P.J.J.; Orgéas, L.; Corre, S.L.; Martoïa, F.; Rolland du Roscoat, S.; Laure, P. 3D real time and in situ observation of the fibre orientation during the plane strain flow of concentrated fibre suspensions. J. Nonnewton. Fluid Mech. 2023, 312, 104978. [Google Scholar] [CrossRef]
- Belliveau, R.; Léger, É.; Landry, B.; LaPlante, G. Measuring fibre orientation and predicting elastic properties of discontinuous long fibre thermoplastic composites. J. Compos. Mater. 2021, 55, 321–330. [Google Scholar] [CrossRef]
- Sebaey, T.A.; Catalanotti, G.; O’Dowd, N.P. A microscale integrated approach to measure and model fibre misalignment in fibre-reinforced composites. Compos. Sci. Technol. 2019, 183, 107793. [Google Scholar] [CrossRef]
- Zweifel, L.; Kupski, J.; Dransfeld, C.; Caglar, B.; Baz, S.; Cessario, D.; Gresser, G.T.; Brauner, C. Multiscale Characterisation of Staple Carbon Fibre-Reinforced Polymers. J. Compos. Sci. 2023, 7, 465. [Google Scholar] [CrossRef]
- Salaberger, D.; Kannappan, K.A.; Kastner, J.; Reussner, J.; Auinger, T. Evaluation of computed tomography data from fibre reinforced polymers to determine fibre length distribution. Int. Polym. Process. 2011, 26, 283–291. [Google Scholar] [CrossRef]
- Melenka, G.W.; Gholami, A. Fiber identification of braided composites using micro-computed tomography. Compos. Commun. 2021, 27, 100813. [Google Scholar] [CrossRef]
- Maksimcuka, J.; Obata, A.; Sampson, W.W.; Blanc, R.; Gao, C.; Withers, P.J.; Tsigkou, O.; Kasuga, T.; Lee, P.D.; Poologasundarampillai, G. X-ray tomographic imaging of tensile deformation modes of electrospun biodegradable polyester fibers. Front. Mater. 2017, 4, 43. [Google Scholar] [CrossRef]
- Diaz, A.; Guizar-Sicairos, M.; Poeppel, A.; Menzel, A.; Bunk, O. Characterization of carbon fibers using X-ray phase nanotomography. Carbon 2014, 67, 98–103. [Google Scholar] [CrossRef][Green Version]
- Gomarasca, S.; Peeters, D.M.J.; Atli-Veltin, B.; Dransfeld, C. Characterising microstructural organisation in unidirectional composites. Compos. Sci. Technol. 2021, 215, 109030. [Google Scholar] [CrossRef]
- Katuin, N.; Peeters, D.M.J.; Dransfeld, C.A. Method for the microstructural characterisation of unidirectional composite tapes. J. Compos. Sci. 2021, 5, 275. [Google Scholar] [CrossRef]
- Nikishkov, Y.; Seon, G.; Makeev, A. Structural analysis of composites with porosity defects based on X-ray computed tomography. J. Compos. Mater. 2014, 48, 2131–2144. [Google Scholar] [CrossRef]
- Nikishkov, Y.; Airoldi, L.; Makeev, A. Measurement of voids in composites by X-ray Computed Tomography. Compos. Sci. Technol. 2013, 89, 89–97. [Google Scholar] [CrossRef]
- Yu, H.; Potter, K.D.; Wisnom, M.R. A novel manufacturing method for aligned discontinuous fibre composites (High Performance-Discontinuous Fibre method). Compos.–A Appl. Sci. Manuf. 2014, 65, 175–185. [Google Scholar] [CrossRef]
- Sharma, B.N.; Naragani, D.; Nguyen, B.N.; Tucker, C.L.; Sangid, M.D. Uncertainty quantification of fiber orientation distribution measurements for long-fiber-reinforced thermoplastic composites. J. Compos. Mater. 2018, 52, 1781–1797. [Google Scholar] [CrossRef]
- Longana, M.L.; Ong, N.; Yu, H.N.; Potter, K.D. Multiple closed loop recycling of carbon fibre composites with the HiPerDiF (High Performance Discontinuous Fibre) method. Compos. Struct. 2016, 153, 271–277. [Google Scholar] [CrossRef]
- Yarlagadda, S.; Deitzel, J.; Heider, D.; Tierney, J.; Gillespie, J.W. Tailorable Universal Feedstock for Forming (TUFF): Overview and performance. In Proceedings of the International SAMPE Technical Conference, Charlotte, NC, USA, 20–23 May 2019. [Google Scholar]
- Yamanaka, A.; Terada, M.; Ichiki, M.; Kimoto, Y.; Shiraki, K.; Nagata, M.; Shimamoto, D.; Hotta, Y. Evaluation of fiber orientation by x-ray diffraction on carbon fiber reinforced polyamide 6. J. Fiber Sci. Technol. 2020, 76, 199–207. [Google Scholar] [CrossRef]
- Yang, X.; Ju, B.F.; Kersemans, M. Assessment of the 3D ply-by-ply fiber structure in impacted CFRP by means of planar Ultrasound Computed Tomography (pU-CT). Compos. Struct. 2022, 279, 114745. [Google Scholar] [CrossRef]
- Pelivanov, I.; Ambroziński, Ł.; Khomenko, A.; Koricho, E.G.; Cloud, G.L.; Haq, M.; O’Donnell, M. High resolution imaging of impacted CFRP composites with a fiber-optic laser-ultrasound scanner. Photoacoustics 2016, 4, 55–64. [Google Scholar] [CrossRef]
- Dong, L.; Hang, H.; Park, J.G.; Mio, W.; Liang, R. Detecting Carbon Nanotube Orientation with Topological Analysis of Scanning Electron Micrographs. Nanomaterials 2022, 12, 1251. [Google Scholar] [CrossRef]
- Alavi, S.H.; Ruiz, V.; Krasieva, T.; Botvinick, E.L.; Kheradvar, A. Characterizing the collagen fiber orientation in pericardial leaflets under mechanical loading conditions. Ann. Biomed. Eng. 2013, 41, 547–561. [Google Scholar] [CrossRef] [PubMed]
- Huntley, S.J.; Rendall, T.; Longana, M.L.; Pozegic, T.; Potter, K.D.; Hamerton, I. Validation of a Smoothed Particle Hydrodynamics Model for a Highly Aligned Discontinuous Fibre Composites Manufacturing Process. Compos. Sci. Technol. 2020, 196, 108152. [Google Scholar] [CrossRef]
- Kirupanantham, G. Characterisation of Discontinuous Carbon Fibre Preforms for Automotive Applications. Ph.D. Thesis, University of Nottingham, Nottingham, UK, 2013. [Google Scholar]
- Cox, H.L. The elasticity and strength of paper and other fibrous materials. Br. J. Appl. Phys. 1952, 3, 72–79. [Google Scholar] [CrossRef]
- Edwards, H.; Evans, N.P. A method for the production of high quality aligned short fibre mats and their composites. In Proceedings of the Advances in Composite Materials, 3rd International Conference on Composite Materials, Paris, France, 26–29 August 1980; pp. 1620–1635. [Google Scholar]
- Eom, Y.; Boogh, L.; Michaud, V.; Manson, J.-A. A Structure and Property Based Process Window for Void Free Thermoset Composites. Polym. Compos. 2001, 22, 22–31. [Google Scholar] [CrossRef]
- Hubert, P.; Poursartip, A. Method for the direct measurement of the fibre bed compaction curve of composite prepregs. Compos.–A Appl. Sci. Manuf. 2001, 32, 179–187. [Google Scholar] [CrossRef]
- Servais, C.; Michaud, V.; Mansons, J.-A. The Packing Stress of Impregnated Fiber Mats. Polym. Compos. 2001, 22, 298–311. [Google Scholar] [CrossRef]
- Merhi, D.; Comte, E.; Michaud, V.; Mansons, J.A. Correlation Between Sizing Formulation and Compressive Behavior of Concentrated Glass Bundle Suspensions. Polym. Compos. 2005, 26, 370–376. [Google Scholar] [CrossRef]
- May, D.; Kühn, F.; Etchells, M.; Fauster, E.; Endruweit, A.; Lira, C. A reference specimen for compaction tests of fiber reinforcements. Adv. Manuf. Polym. Compos. Sci. 2019, 5, 230–233. [Google Scholar] [CrossRef]
- Sousa, P.; Lomov, S.; Ivens, J. Methodology of dry and wet compressibility measurement. Compos.–A Appl. Sci. Manuf. 2020, 128, 105672. [Google Scholar] [CrossRef]
- Bender, M.; Fauser, E. Novel test-rig for compaction behaviour analysis of textile reinforcements for improved RTM-process replication. Adv. Manuf. Polym. Compos. Sci. 2023, 9, 2263828. [Google Scholar] [CrossRef]
- Grieder, S.; Zhilyaev, I.; Küng, M.; Brauner, C.; Akermann, M.; Bosshard, J.; Inderkum, P.; Francisco, J.; Willemin, Y.; Eichenhofer, M. Consolidation of Additive Manufactured Continuous Carbon Fiber Reinforced Polyamide 12 Composites and the Development of Process-Related Numerical Simulation Methods. Polymers 2022, 14, 3429. [Google Scholar] [CrossRef]
- Walker, L. Development of Prepreg and Processing Technologies for recycled Carbon Fibre Based Textiles. Master’s Thesis, FHNW University of Applied Sciences and Arts Northwestern Switzerland, Windisch, Switzerland, 2021. [Google Scholar]








| Layup | Binder + Sizing Portion [m%] | Dry Areal Weight [g/m2] | |
|---|---|---|---|
| UD staple CF—LS | [0]12 | 11.05 | 80 |
| UD staple CF—HS | [0]12 | 11.05 | 80 |
| UD continuous CF | [0]12 | 5.34 | 83.5 |
| Bi-axial continuous CF | [0, 90]3s | 5.34 | 83.5 |
| P [bar] | FVC [%] | |
|---|---|---|
| Vacuum processing/LS | 0.8 | 27.4 |
| Autoclave processing/LS | 6.8 | 38.8 |
| Aerospace grade/LS | n/a | 60.0 |
| Vacuum processing/HS | 0.8 | 29.1 |
| Autoclave processing/HS | 6.8 | 42.6 |
| Aerospace grade/HS | ~90 | 60.0 |
Disclaimer/Publisher’s Note: The statements, opinions and data contained in all publications are solely those of the individual author(s) and contributor(s) and not of MDPI and/or the editor(s). MDPI and/or the editor(s) disclaim responsibility for any injury to people or property resulting from any ideas, methods, instructions or products referred to in the content. |
© 2026 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license.
Share and Cite
Preinfalck, M.; Kupski, J.; Hajikazemi, M.; Brauner, C.; Baz, S.; Gresser, G.T. Compactibility and Fibre Volume Fraction Limits of Unidirectional Discontinuous Carbon Fibre Thermoset Prepreg Laminates. Polymers 2026, 18, 1472. https://doi.org/10.3390/polym18121472
Preinfalck M, Kupski J, Hajikazemi M, Brauner C, Baz S, Gresser GT. Compactibility and Fibre Volume Fraction Limits of Unidirectional Discontinuous Carbon Fibre Thermoset Prepreg Laminates. Polymers. 2026; 18(12):1472. https://doi.org/10.3390/polym18121472
Chicago/Turabian StylePreinfalck, Miriam, Julian Kupski, Mohammad Hajikazemi, Christian Brauner, Stephan Baz, and Götz T. Gresser. 2026. "Compactibility and Fibre Volume Fraction Limits of Unidirectional Discontinuous Carbon Fibre Thermoset Prepreg Laminates" Polymers 18, no. 12: 1472. https://doi.org/10.3390/polym18121472
APA StylePreinfalck, M., Kupski, J., Hajikazemi, M., Brauner, C., Baz, S., & Gresser, G. T. (2026). Compactibility and Fibre Volume Fraction Limits of Unidirectional Discontinuous Carbon Fibre Thermoset Prepreg Laminates. Polymers, 18(12), 1472. https://doi.org/10.3390/polym18121472

