1. Introduction
Water shortages are often associated with the countries located in subtropical zones, such as those in Sub-Saharan Africa [
1], the West coast of North [
2] and South America [
3], or Central Asia [
4]. The situation in these areas requires immediate action. However, the public eye tends to omit that water stress also occurs in the countries located in the North, i.e., in Europe [
5]. Moreover, compared to previous decades, less frequent precipitation during the year and more frequent heatwaves during summers only serve to worsen the situation [
6].
To minimize freshwater withdrawal, water-scarce countries have implemented various methods, i.e., rationing [
7], education on resources protection [
8], or advanced irrigation systems [
9]. They have also introduced direct solutions, such as clean water production from unconventional sources. These include desalination [
10] or direct and indirect reuse from wastewater [
11]. The latter is a promising option due to its versatility and lower cost compared with the first method [
12].
Various studies have already been done on water reuse systems applications, where a more significant number focus on use in agriculture [
13,
14]. It is already regulated by regional polices [
15], and it has been recently regulated internationally by European law [
16]. Another widely commented topic involves potable water reuse [
17,
18,
19]. This case is being studied not only as a technical, but also as a social issue [
20]. More recently, industrial water recycling has been discussed by researchers, since manufacturing processes sometimes need abundant amounts of water to operate [
21,
22,
23].
In general, cities require a large amount of water for public services such as, power and heat production, cleaning of streets and public transport fleet, sewage network flushing, greenery irrigation, landscaping, etc. However, research on water reclamation for urban purposes is not as widespread as other applications. Lee and Jepson [
24] previously reviewed the literature published on urban water reuse between 2010 and 2019, identifying 39 articles, most of which focused solely on policy-making and socio-economic issues. In South Africa, few municipalities have successfully implemented water reuse systems for urban purposes, including landscaping, sports fields irrigation and industrial purposes [
25]. Similarly, over 80% of total reclaimed water is used in China for landscaping and industrial applications [
26]. Ramaiah et al. [
27] studied the reliability of urban green space irrigation with reclaimed water. Additionally, Cherchi et al. [
28] reviewed the application of water reuse in the power production sector in the US, presenting 11 successful operating installations. Some studies have also been carried out on water reuse system modeling and planning [
29]. The environmental impacts of water reclamation techniques are defined using life cycle assessment analysis (LCA). Studies in the scope of water reuse usually are treatment technology-oriented or application-oriented. Papers that target wastewater treatment technologies [
30,
31,
32] or single processes [
33,
34] can be found. A significant number of studies address irrigation application [
35,
36] or industrial application [
37].
Most of the previous works focus on a complete analysis of a single application or a variety of methods, but analyzed one criterion. Only a few authors have investigated the topic in the scope of quality and quantity, also considering legislative issues. Municipal wastewater reuse in metropolitan areas also needs more feasibility and environmental impact studies. This paper uses a complex approach to evaluate urban water reclamation systems. It gathers all mentioned problems: the quality and quantity of the available wastewater together with current local and international policies in force, and the required infrastructure. Different application methods were considered, and deliberations were carried out to present the most optimal scenarios for the implementation of the water reuse system. Furthermore, the topic of public transport fleet cleaning was developed using comparative life cycle assessment, discussing the environmental effects of suggested solutions. It was possible to perform the analysis for this water reuse application due to the constant water demand throughout the year and fixed delivery routes. In this case, a water delivery step was considered. It is worthy of note that the delivery step is often neglected in the research, but in cases of water transport within a large metropolitan area, it has a significant contribution and should be considered. Simultaneously, there is also a lack of studies that include the comparison of results as a function of time. This provides another perspective to an overall evaluation, contrary to the independent comparison of results. Poland’s capital city, Warsaw, served as an example for this study.
3. Results
3.1. Opportunities for Water Reuse in Power Production
Two main surface water purification processes are coagulation and ion exchange. At the exemplary PPs, they are carried out in clarifiers and ion exchange beds, respectively. Both processes require a constant power supply and the dosing of chemical reagents such as flocculants, polyelectrolytes, lime, base or acid [
69]. Water withdrawn by PPs from the river always has to be treated prior use. The suggested solution was to maintain the current operation of water treatment plants at the facilities and only replace the water source with treated wastewater from the WWTPs.
Eight quality indicators for Vistula water and exemplary effluents (Czajka and Południe) were compared (
Table 6). It was observed that two indicators were significantly lower in treated wastewater than in river water. One was suspended solids −79% lower in Czajka effluent and 83% lower in treated wastewater from Południe. Assuming the replacement of the entire water flux with treated wastewater, the coagulation time could be shortened considerably. This would indicate a savings in power and reagent consumption, reaching as much as 80% at the coagulation step. Higher total phosphorus and nitrogen values in treated wastewater should not cause a legislative problem, since their maximum concentrations are not mentioned in the cooling water regulation. Phosphorus is also mainly removed during coagulation.
Water reclamation using ion exchange has already been successfully adopted, i.e., in Florida [
70] and India [
71]. Sulphate and chloride concentrations in analyzed WWTPs effluents were two to four times higher than in river water. The replacement of the water source would cause the quicker exhaustion of ion beds, leading to higher power and reagent consumption for regeneration. Based on the results, it is impossible to unequivocally state that the implementing of water reuse practices in power production would be economically and environmentally beneficial when only considering the provided data. Further research would have to be carried out to show which application would bring a higher reduction of power and reagents consumption—quicker coagulation or the less frequent regeneration of ion exchange beds.
3.2. Opportunities for Water Reuse in Landscaping and Street Cleaning
The possibility of tanking the water carts with treated wastewater instead of tap water was analyzed. Water quality requirements were considered, since they were recognized as the most crucial issue in reuse for landscaping and greenery irrigation, where direct human exposure to reclaimed water can occur. Currently, there are no local laws in force targeting water reuse in Poland, so the only legislation that regulates its adaptation is the one issued by the European Parliament in May 2020 [
47]. It focuses on agricultural reuse, but reuse for amenity-related and environmental purposes is also encouraged. The regulation divides crops into four classes, depending on the minimum required reclaimed water quality. Public greenery isn’t harvested, so it could be included in the lowest class D (industrial, energy and seeded crops).
Other standards that should also be considered are WHO guidelines for the safe use of wastewater. They include health-based targets for wastewater use in agriculture, divided by the type of irrigation. In the analyzed case, the most suitable type would be labor-intensive restricted irrigation. The standard parameters listed in both documents are summarized in
Table 7.
Both analyzed WWTPs effluents have much lower TSS and BOD5 than indicated in the EU Regulations. The presence and concentration of bacteria, pathogens and Helminth eggs should be defined, especially since pressurized watering with a hose causes the forming of aerosols. Due to close contact with landscaping workers and pedestrians, effluent disinfection should always be considered prior to use. Disinfection would also be necessary if wastewater was used for other landscaping purposes, like fountains or ponds. To minimize the risk of piping system clogging, it should also be checked if wastewater needs filtration to remove the remaining suspended solids.
Water reuse in street cleaning at the example location has been adapted only during the summer when used pool water was recycled. However, each pool is emptied only once per year, so this solution is not universal. In this case, according to EU Regulations, WWTP effluent could also be used for cleaning instead of tap water. An amount of 191 m
3 of water saved per day on street cleaning equals the daily freshwater demand of approx. 1340 people [
73]. This solution presents great potential with minimal investment. Similarly to water for irrigation, treated wastewater would have to be disinfected before being tanked into cleaning vehicles.
3.3. Opportunities for Water Reuse in Public Transport Fleet Cleaning
The cleaning of public transport vehicles creates yet another opportunity for water reuse implementation. Internal water reuse systems were described previously by Canales et al. [
74], Panizza and Cerisola [
75], and Hamada and Miyazaki [
76]. Since carwashes already have internal water recycling with their own pollution separation systems, WWTP effluent could be used without any tertiary treatment except disinfection to minimize the risk of bacterial exposure in forming aerosols. The daily amount of water required for the cleaning of buses, trams and metro trains in the analyzed metropolitan area is around 211 m
3, which equals the daily freshwater demand of approx. 1475 people. Such an application also has another advantage: consumption is constant and continuous throughout the year.
Since the primary purpose of water reuse is natural environment protection, an LCA was carried out to evaluate which of the two proposed reused water delivery solutions would have a lower environmental impact. It was primarily assumed that water network construction would be less impactful than daily delivery by lorries over an extended period of time, since once built it no longer generates significant emissions. The analysis aimed to calculate how many days it would take for the piping system to become less impactful than tank lorry delivery. The results of the calculations were analyzed in 10 environmental impact categories (
Table 8). The impactful period represents the number of days after which the environmental impact of tank lorry delivery will be higher than the impact of water network construction.
Depending on the indicator, the impactful period for water network construction was between 11 days for freshwater aquatic ecotoxicity to 9.5 years for terrestrial ecotoxicity. However, the median value showed that after 73 days of operation, the water network would already have a lower environmental impact than daily delivery by tank lorries. These results show that the water network construction would undoubtedly be a better solution for reused water delivery to public transport depots. Although no other processes were included in the analysis, it could be assumed that the water network would become less impactful than lorry delivery in less than a year. Considering that this solution would be implemented permanently, the piping system should be chosen as a preferred solution.
3.4. Final Proposal of Urban Water Reuse—Case Study
Eventually, a proposal for a complex urban water reuse system was evaluated, covering all purposes mentioned in previous sections. It was observed that the daily effluent from the bigger WWTP, Czajka, could cover the total daily water demand for the bigger PP, Siekierki, with a surplus of 71,232 m3/d. This creates an opportunity for closing the loop in the power production sector in the city and still leaving the remaining effluent to be used for other purposes. However, the distance between Czajka and Siekierki is almost 20 km, and there is a 2-m incline in the elevation towards Siekierki PP. Considering the required average water flow of more than 300,000 m3/d between the facilities, the piping system could be the only option to transport such considerable amounts daily.
To diversify the water reuse management, two scenarios were evaluated. Both of them would require construction of: a tertiary treatment system of treated wastewater at WWTPs, including filtration and disinfection, reclaimed water network connecting WWTPs with corresponding public transport depots, as well as a reclaimed water tanking station at Czajka WWTP for water carts and street cleaning vehicles. Additionally, one scenario would cover the total water demand for power production, but would also require extensive investments. Furthermore, it would include the following:
construction of a connecting channel (approx. 500 m long) between Południe WWTP and Siekierki PP, using the entire Południe effluent, excluding the amount required for its own needs and the public transport depots supply,
construction of a long conduit (approx. 20 km) between Czajka WWTP and Siekierki PP, delivering the remaining water required for power production,
Such a management system would allow for satisfying the entire water demand for two exemplary PPs (Siekierki and Żerań), and the entire demand for landscaping, street cleaning and public transport fleet washing purposes. It would lead to the management of the total Południe WWTP effluent and 89% of the effluent from Czajka, lowering the wastewater discharge to the Vistula River by even 91% each year (
Figure 3). However, such a solution would require enormous investment costs to build an extensive piping system between Czajka and Siekierki. Additionally, it would have to be checked if this drastic reduction of effluent discharge wouldn’t be a risk for maintaining the environmental flow requirements.
The second scenario assumed lower investment costs in comparison to the first one, and higher effluent discharge back to the river. The proposed solution included the following:
construction of a shorter conduit (approx. 8–10 km long) between Czajka WWTP and Żerań PP,
construction of a connecting channel (approx. 500 m long) between Południe WWTP and Siekierki PP,
Such a management system would allow for satisfying the entire Żerań PP and 18% of the Siekierki PP water demand, as well as for the total demand for landscaping, street cleaning and public transport fleet washing purposes. It would lead to the management of the entire Południe WWTP effluent and 22% of the effluent from Czajka, lowering the wastewater discharge to the Vistula River by 16% each year (
Figure 4).
4. Discussion
This study tackled the subject of water reuse which has not been developed on a broader scale as yet. It aimed to evaluate the universal urban water reuse system proposal. Two urban water reclamation systems proposed in this paper could allow for the reuse of 91 or 33 per cent of treated wastewater. Takeuchi and Tanaka [
77] have reported that in Japan only 1.3% of treated wastewater is recycled and used for various urban purposes, from which 22% is used for landscape irrigation. Based on data available from Shanghai and Beijing, Bauer et al. [
78] have calculated that the reclaimed water demand for city purposes (streets cleaning and greenery irrigation) of 104,000 P.E. would constitute for 202% of its actual production. Street cleaning purposes would have the biggest contribution and require 119% of the actual water production.
Reuse for municipality purposes is very versatile, but simultaneously this situation creates various implementation obstacles and challenges. Reclaimed water characterizes with different composition than the surface water used by power plants. Higher concentrations of ammonia, phosphorus or hydrogen sulfide can cause corrosion in the metallic parts. Nutrients and residual organic matter can also lead to biofilm formation, causing components fouling [
28]. Water treatment plants that serve power production facilities are designed to treat the water of specific quality occurring locally. In case of water source replacement with treated wastewater, it would be necessary to adjust the components or possibly add other treatment processes to ensure the desired nutrient and residual organic matter removal rate. Considering literature reports, the removal of these compounds at power plants is usually carried out in biofilters [
79] or membrane bioreactors [
22]. What is interesting is that ion exchange was proven to be an efficient alternative to biological processes. Zeolite resins regenerated with NaCl allow for the removal and recovery of nutrients [
80,
81]. This solution should be considered while implementing water reuse at power plants already operating with ion exchange processes. Current components would have to be adjusted to facilitate nutrient removal, but it would also require lower investment than the construction of biological reactors. In this study, the daily demands for power production of 421,093 and 146,087 m
3/d of reclaimed water were analysed. Cherchi et al. [
28] have reported 60 power plants in the US that have successfully implemented the usage of reclaimed water, from which approx. 50% consume at least 5000 m
3 per day and 20% consume more than 46,000 m
3 per day. Li et al. [
82] have conducted a study on a nuclear plant where consumption exceeds 208,000 m
3/d.
The results of the study indicated that there was approx. an 80 percent lower concentration of suspended solids in reclaimed water than in surface water. This situation is advantageous in terms of electricity and reagent consumption, but it may also be a premise for the adjustment of the coagulation process at PP. A low concentration may impede the formation of flocks, therefore new, enhanced coagulation techniques should be acknowledged. Some previous studies describe the micro-coagulation advantage over conventional coagulation processes in water reuse [
83]. It requires lower coagulant doses, shorter retention times and generates a smaller environmental footprint.
The usage of reclaimed water for greenery irrigation and landscaping is one of the most popular practices in urban water reuse [
26,
84]. The remaining nitrogen and phosphorus in WWTP effluent can lead to eutrophication and marine life degradation when discharged back into a water body [
85]. It has been determined multiple times that the WWTP effluent is more beneficial for land plants than water flora [
14,
86]. It was specified by Wang et al. [
87] that domestic wastewater can increase crop yield, but industrial wastewater has rather adverse effects and should not be considered. This research considered the water reuse in the irrigation of public landscape in the quality criterion only. Woltersdorf et al. [
88] have also included the quantity criterion, and calculated that in a small municipal area of 1400 P.E., the amount of reclaimed water would be sufficient to fully irrigate and fertilize 1ha of public greenery or cover 39% of the crop requirements for water, 100% for nitrogen and 29% for phosphorus.
Another problem that may occur during irrigation with treated wastewater is an unpleasant odor caused by compounds present in the effluent, such as hydrogen sulfide or volatile organic compounds [
89], because this parameter isn’t usually altered at the WWTPs [
90]. Before the reclaimed water could be tanked into water carts, besides disinfection, it would be necessary to implement the odor removal processes. Popular techniques include ozonation or adsorption [
91]. An appropriately designed ozonation process could serve for both disinfection and odor removal. Certain studies also observed the degradation of soil in public parks when reclaimed water was used for irrigation [
92,
93].
Legislative procedures may take a lot of time, especially when it concerns implementing a new technology that has not been widely tested inside the country’s territory. The lack of local regulations on water reuse may additionally prolong the process. Although the research on this subject started a few decades ago, only six countries in Europe have adopted some local policies in water reclamation: Spain [
94], France [
95,
96], Italy [
97], Portugal [
98], Greece [
99] and Cyprus [
100], where only the Greek government issued more than one document by 2022. This fact highlights the necessity to elaborate more legislative acts targeting the issue and to update those published more than a few years ago. Regulations in Europe describe various urban purposes, however only landscape irrigation of public areas is included in all of them. Other purposes include:
street cleaning (Greece, Italy, Spain),
the irrigation of ornamental flowers without contact of reclaimed water with the product (France, Greece, Italy, Spain),
cooling towers (Greece and Italy),
the industrial washing of vehicles (Italy, Spain).
Maximum values in reclaimed water have been defined for parameters such as various bacteria species, F-specific bacteriophages, Helminth eggs, TSS, TDS, turbidity, BOD, COD, pH, heavy metals, electrical conductivity, or chlorine [
84]. The local and national governments of the countries that haven’t issued any water reuse policies yet could use existing regulations as guidelines. Already adapted practices serve as examples to dispel doubts.
Another problem that makes it harder to obtain specific permits and agreements for urban water reuse, where, for example, irrigated plants come into contact with the citizens, is the so-called “yuck factor”. This refers to the negative attitude and public perception towards the reuse of municipal wastewater [
101]. In many cities, it is still believed that such practices expose residents to the risk of infections caused by bacteria and viruses that may be found in the WWTP effluent [
102]. The organoleptic properties of reused water are often also a concern. However, many studies have already been conducted, showing no bacteriological risk if the wastewater is disinfected appropriately prior to use [
103]. Moreover, as previously mentioned, treated wastewater may benefit irrigated plants more than tap water. If water reuse is planned to be implemented in the city, educational campaigns should be included in the plan to assure the citizens that these solutions are safe and have been tested multiple times for many years.
While designing the water reuse management plan, it is essential to include the environmental flow requirements. Sometimes the main emphasis is put on human needs [
104] and systems that allow for the reusing of as much wastewater as possible. However, to maintain sustainable water resource management, environmental requirements cannot be neglected. Some parts of treated wastewater has to be discharged back into the aquatic ecosystem to provide plants and animals with enough water and nutrients to survive without stress.
This study included the comparative LCA analysis of reclaimed water delivery by road lorry transportation and water distribution network (PVC pipes). A CML scenario was used as the calculation methodology. The global warming potential emission equaled 16 kg CO
2 per ton of transported water on a total distance of 289 km. Abbas and Handler [
105] have previously reported that the delivery of 1 ton of wood by large lorries generates 33.2 kg CO
2 at a distance of 300 km and 27.7 kg CO
2 at a distance of 250 km. Amores et al. [
106] have calculated the environmental impact of reclaimed water distribution networks made from PVC pipes, using the CML scenario method. Hajibabaei et al. [
107] and Sanjuan-Delmás et al. [
108] used the same methodology to calculate the environmental impact of PVC pipes production and the construction of a drinking water distribution network. The results for 1 km of constructed network in the aforementioned studies have been compiled with the results of this study in
Table 9. All four studies have reported the lowest environmental impact for ozone layer depletion and the highest for global warming.
Further research should be carried out to evaluate the in-depth environmental impact analysis and feasibility study of urban water reuse. Future studies should be interdisciplinary and focus on the combination of social, economic, environmental and technological aspects.