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Article

Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal

1
Department of Physics, University of Wisconsin-Milwaukee, Milwaukee, WI 53201, USA
2
National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY 11973, USA
*
Author to whom correspondence should be addressed.
Materials 2025, 18(23), 5337; https://doi.org/10.3390/ma18235337 (registering DOI)
Submission received: 25 October 2025 / Revised: 17 November 2025 / Accepted: 24 November 2025 / Published: 26 November 2025
(This article belongs to the Section Metals and Alloys)

Abstract

We report coherent X-ray imaging of antiferromagnetic (AFM) domains and domain walls in MnBi2Te4, an intrinsic AFM topological insulator. This technique enables direct visualization of domain morphology without reconstruction algorithms, allowing us to resolve antiphase domain walls as distinct dark lines arising from the A-type AFM structure. The wall width is determined to be 550(30) nm, in good agreement with earlier magnetic force microscopy results. The temperature dependence of the AFM order parameter extracted from our images closely follows previous neutron scattering data. Remarkably, however, we find a pronounced hysteresis in the evolution of domains and domain walls: upon cooling, dynamic reorganizations occur within a narrow ∼1 K interval below TN, whereas upon warming, the domain configuration remains largely unchanged until AFM order disappears. These findings reveal a complex energy landscape in MnBi2Te4, governed by the interplay of exchange, anisotropy, and domain-wall energies, and underscore the critical role of AFM domain-wall dynamics in shaping its physical properties. These sharply defined and hysteretically evolving walls may provide a controllable AFM texture in MnBi2Te4, hinting at potential use in low-power spintronic devices based on domain-wall dynamics.
Keywords: antiferromagnetic domains; topological insulator; MnBi2Te4 antiferromagnetic domains; topological insulator; MnBi2Te4

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MDPI and ACS Style

Kim, M.G.; Boney, S.; Burgard, L.; Rutowski, L.; Mazzoli, C. Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal. Materials 2025, 18, 5337. https://doi.org/10.3390/ma18235337

AMA Style

Kim MG, Boney S, Burgard L, Rutowski L, Mazzoli C. Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal. Materials. 2025; 18(23):5337. https://doi.org/10.3390/ma18235337

Chicago/Turabian Style

Kim, Min Gyu, Starr Boney, Luke Burgard, Lillian Rutowski, and Claudio Mazzoli. 2025. "Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal" Materials 18, no. 23: 5337. https://doi.org/10.3390/ma18235337

APA Style

Kim, M. G., Boney, S., Burgard, L., Rutowski, L., & Mazzoli, C. (2025). Dynamics and Formation of Antiferromagnetic Textures in MnBi2Te4 Single Crystal. Materials, 18(23), 5337. https://doi.org/10.3390/ma18235337

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