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Review
Peer-Review Record

Ceramic-Polymer Composite Membranes for Water and Wastewater Treatment: Bridging the Big Gap between Ceramics and Polymers

Molecules 2021, 26(11), 3331; https://doi.org/10.3390/molecules26113331
by Masashi Kotobuki, Qilin Gu, Lei Zhang and John Wang *
Reviewer 1: Anonymous
Reviewer 2: Anonymous
Molecules 2021, 26(11), 3331; https://doi.org/10.3390/molecules26113331
Submission received: 4 May 2021 / Revised: 25 May 2021 / Accepted: 30 May 2021 / Published: 1 June 2021
(This article belongs to the Special Issue Recent Advances in Porous Materials)

Round 1

Reviewer 1 Report

This review paper thoroughly overviews three types of ceramic-polymer composite membranes. And by looking into strategies to improve the compatibility among ceramic and polymeric components, the manuscript conclude the perspectives and challenges for the future development of the composite membranes. This review maybe provide great interest and inspiration to broad readers about ceramic-polymer composite membranes. But before this manuscript can be considered for publication, the following questions need to be addressed.

1. In the Abstract,“in the past decade, great progress has been made in improving the compatibility between ceramics and polymers, while the synergy between them has been among the main pursuits, especially in the development of the high performing nanocomposite membranes for water and wastewater treatment at lowered manufacturing cost”suggested to be deleted.

2. The classification of ceramic-polymer composite membrane((i) ceramics in polymer membranes, (ii) thin-film nano-composite (TFN) membranes, and (iii) ceramic-supported polymer membranes) is not very clear, it is suggested to modify.

3. Where is Figure 3?

4. Fig. 2. 4, 5, 6, 7, 8,10 is too rough, please redraw it.

5. In table 8, suggests adding some data support in "Improved Properties”.

6. Explain the mechanism of Figure 5 in detail

7. “3.1.2. Surface functionalization” and “3.2.2 Surface functionalization” are same.

8. In Figure 9, if there are any Reference cited to? If so, please add it.

9. It is suggested to add the latest references in recent years

10. Finally, please modify the format of the manuscript

Author Response

  1. In the Abstract,“in the past decade, great progress has been made in improving the compatibility between ceramics and polymers, while the synergy between them has been among the main pursuits, especially in the development of the high performing nanocomposite membranes for water and wastewater treatment at lowered manufacturing cost”suggested to be deleted.

Thank the reviewer for the valuable suggestion. The sentence was deleted.

  1. The classification of ceramic-polymer composite membrane((i) ceramics in polymer membranes, (ii) thin-film nano-composite (TFN) membranes, and (iii) ceramic-supported polymer membranes) is not very clear, it is suggested to modify.

Thank the reviewer for the valuable suggestion. To clarify the classification of membrane structure types, Figure 2 is added.

 

  1. Where is Figure 3?

Figure 3 (Figure 2 in the revised manuscript) is added.

 

  1. Fig. 2. 4, 5, 6, 7, 8,10 is too rough, please redraw it.

Those figures have been redrawn.

 

  1. In table 8, suggests adding some data support in "Improved Properties”.

Thank the reviewer for the suggestion. Data (Fig. 4) and explanation is added.

 

  1. Explain the mechanism of Figure 5 in detail

More explanations for Figure 5 are added.

 

  1. “3.1.2. Surface functionalization” and “3.2.2 Surface functionalization” are same.

They have been changed into “4.1.2. Surface functionalization on ceramic nanoparticles”, “4.2.2 Surface modification of polymer matrixes”

  1. In Figure 9, if there are any Reference cited to? If so, please add it.

Yes, citation is added.

 

  1. It is suggested to add the latest references in recent years

Recent papers have been added.

 

  1. Finally, please modify the format of the manuscript

The manuscript has been formatted using the template.

Author Response File: Author Response.pdf

Reviewer 2 Report

This is a review paper without scientific achievements. It should be presented in that way. Moreover, I would like to see the improving effect of the combined membranes.

I saw some formatting problems, e.g. t Figure 2 (maybe my reader made the problem.)

The article is too long.

Author Response

Please see the attachment

Author Response File: Author Response.pdf

Round 2

Reviewer 1 Report

 Authors made considerable modifications in the manuscript as suggested by reviewers. Now the paper can be accepted for publication in the present form.

Reviewer 2 Report

I accept the revised version

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