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Conventional bolt–shotcrete support technology is usually single-layered, which does not meet the requirements of strength and stiffness for roadway support. Therefore, in this paper, new combined support technology, including a multiple-layered staggered dense arrangement of bolts, multiple-layered laying of steel meshes, multiple-layered pouring of shotcrete, strengthening support of long cables, and full cross-section grouting, is proposed. Specifically, the following new combined support technology process is proposed: first layer of shotcrete (80 mm), first layer of mesh, first layer of bolt, second layer of shotcrete (50 mm), second layer of mesh, second layer of bolt, reinforced cable, third layer of shotcrete (50 mm), and grouting. The results show the following: (1) In the system of a superimposed coupling strengthening bearing arch, compared to a cable bearing arch, changing the support parameters of the bolt bearing arch can significantly vary the bearing capacity. A range of bolt spacing between 0.4 m and 0.7 m is more conducive for a high performance of the bearing capacity of the superimposed coupling strengthening bearing arch. (2) With the increase in the single-layer shotcrete thickness (from 50 mm to 100 mm), the bearing capacity of the shotcrete structure increased rapidly in the form of a power function. (3) After the multi-level bolt–shotcrete support structure was adopted, the ring peak zone of the deviatoric stress of the surrounding rock at the roadway intersection was largely transferred to the shallow part, and the plastic zone of the surrounding rock of the roadway was reduced by 43.3~52.3% compared to that of the conventional bolt–shotcrete support. The field practice model showed that the final roof-to-floor and rib-to-rib convergences of the roadway intersection were 114 mm and 91 mm after 26 days, respectively. The rock mass above the depth of 3 m of the roadway’s roof and sides was complete, the lithology was dense, and there was no obvious crack. The new technology achieves effective control of a deep roadway intersection with a large cross-section. Full article