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Keywords = interdigitation phenomena

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21 pages, 11089 KiB  
Article
Acoustoelectric Effect due to an In-Depth Inhomogeneous Conductivity Change in ZnO/Fused Silica Substrates
by Cinzia Caliendo, Massimiliano Benetti, Domenico Cannatà and Farouk Laidoudi
Sensors 2024, 24(19), 6399; https://doi.org/10.3390/s24196399 - 2 Oct 2024
Viewed by 1033
Abstract
The acoustoelectric (AE) effect induced by the absorption of ultraviolet (UV) light at 365 nm in piezoelectric ZnO films was theoretically and experimentally studied. c-ZnO films 4.0 µm thick were grown by the RF reactive magnetron sputtering technique onto fused silica substrates at [...] Read more.
The acoustoelectric (AE) effect induced by the absorption of ultraviolet (UV) light at 365 nm in piezoelectric ZnO films was theoretically and experimentally studied. c-ZnO films 4.0 µm thick were grown by the RF reactive magnetron sputtering technique onto fused silica substrates at 200 °C. A surface acoustic wave (SAW) delay line was fabricated with two split-finger Al interdigital transducers (IDTs) photolithographically implemented onto the ZnO-free surface to excite and reveal the propagation of the fundamental Rayleigh wave and its third harmonic at about 39 and 104 MHz. A small area of a few square millimeters on the surface of the ZnO layer, in between the two IDTs, was illuminated by UV light at different light power values (from about 10 mW up to 1.2 W) through the back surface of the SiO2 substrate, which is optically transparent. The UV absorption caused a change of the ZnO electrical conductivity, which in turn affected the velocity and insertion loss (IL) of the two waves. It was experimentally observed that the phase velocity of the fundamental and third harmonic waves decreased with an increase in the UV power, while the IL vs. UV power behavior differed at large UV power values: the Rayleigh wave underwent a single peak in attenuation, while its third harmonic underwent a further peak. A two-dimensional finite element study was performed to simulate the waves IL and phase velocity vs. the ZnO electrical conductivity, under the assumption that the ZnO layer conductivity undergoes an in-depth inhomogeneous change according to an exponential decay law, with a penetration depth of 325 nm. The theoretical results predicted single- and double-peak IL behavior for the fundamental and harmonic wave due to volume conductivity changes, as opposed to the AE effect induced by surface conductivity changes for which a single-peak IL behavior is expected. The phenomena predicted by the theoretical models were confirmed by the experimental results. Full article
(This article belongs to the Section Physical Sensors)
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14 pages, 3490 KiB  
Article
Rapid and Sensitive Detection by Combining Electric Field Effects and Surface Plasmon Resonance: A Theoretical Study
by Qijie Qiu and Yan Xu
Micromachines 2024, 15(5), 653; https://doi.org/10.3390/mi15050653 - 15 May 2024
Cited by 3 | Viewed by 1817
Abstract
Surface plasmon resonance (SPR) has been extensively employed in biological sensing, environmental detection, as well as chemical industry. Nevertheless, the performance possessed by conventional surface plasmon resonance (SPR) biosensors can be further limited by the transport of analyte molecules to the sensing surface, [...] Read more.
Surface plasmon resonance (SPR) has been extensively employed in biological sensing, environmental detection, as well as chemical industry. Nevertheless, the performance possessed by conventional surface plasmon resonance (SPR) biosensors can be further limited by the transport of analyte molecules to the sensing surface, noteworthily when small molecules or low levels of substances are being detected. In this study, a rapid and highly sensitive SPR biosensor is introduced to enhance the ability of the target analytes’ collection by integrating AC electroosmosis (ACEO) and dielectrophoresis (DEP). Both the above-mentioned phenomena principally arise from the generation of the AC electric fields. This generation can be tailored by shaping the interdigitated electrodes (IDEs) that also serve as the SPR biomarker sensing area. The effects exerted by different parameters (e.g., the frequency and voltage of the AC electric field as well as microelectrode structures) are considered in the iSPR (interdigitated SPR) biosensor operation, and the iSPR biosensors are optimized with the sensitivity. The results of this study confirm that the iSPR can efficiently concentrate small molecules into the SPR sensing area, such that SPR reactions achieve an order of magnitude increase, and the detection time is shortened. The rapid and sensitive sensor takes on critical significance in the development of on-site diagnostics in a wide variety of human and animal health applications. Full article
(This article belongs to the Special Issue Micromachines for Dielectrophoresis, 3rd Edition)
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3 pages, 448 KiB  
Abstract
UV Light Stereoselective Limonene Sensor Using Electrospun PVP Composite Nanofibers
by Antonella Macagnano, Fabricio N. Molinari, Tiziana Mancini, Stefano Lupi and Fabrizio De Cesare
Proceedings 2024, 97(1), 131; https://doi.org/10.3390/proceedings2024097131 - 1 Apr 2024
Cited by 3 | Viewed by 1081
Abstract
This study explored the design of an innovative stereoselective S-(-)-limonene sensor according to the molecular imprinting polymer (MIP) strategy using UV light to generate in situ polymer cross-linking. A conductive composite nanofibrous fabric of polyvinylpyrrolidone (PVP), polyacrylic acid (PAA) and carbon nanotubes (MWCNTs) [...] Read more.
This study explored the design of an innovative stereoselective S-(-)-limonene sensor according to the molecular imprinting polymer (MIP) strategy using UV light to generate in situ polymer cross-linking. A conductive composite nanofibrous fabric of polyvinylpyrrolidone (PVP), polyacrylic acid (PAA) and carbon nanotubes (MWCNTs) was deposited on purpose in a single step by electrospinning onto interdigital microelectrodes. The nanostructured layer was investigated by microscopy (SEM, TEM, AFM) and infrared transmission measurements (FTIR). The resulting sensing features (carried out in environmental air) seemed to be mainly dependent on the peculiarity of the nanostructure and the phenomena occurring at the interfaces between the cross-linked PVP–PAA/cavity shape and MWCNTs. Furthermore, the specificity of the host–guest interaction was proven by the sensitivity, selectivity and stereoselectivity of the sensor when exposed to similar monoterpenes ((±)-α-pinene and (±)-linalool) and the enantiomer of limonene (R(+)), respectively. Full article
(This article belongs to the Proceedings of XXXV EUROSENSORS Conference)
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9 pages, 1850 KiB  
Communication
Swirl-like Acoustofluidic Stirring Facilitates Microscale Reactions in Sessile Droplets
by Huaize Lan, Jingui Qian, Yansong Liu, Shanshan Lu, Bowei Zhang, Liang Huang, Xuefeng Hu and Wei Zhang
Micromachines 2023, 14(4), 837; https://doi.org/10.3390/mi14040837 - 12 Apr 2023
Cited by 4 | Viewed by 2212
Abstract
Sessile droplets play a crucial role in the microreactors of biochemical samples. Acoustofluidics provide a non-contact and label-free method for manipulating particles, cells, and chemical analytes in droplets. In the present study, we propose a micro-stirring application based on acoustic swirls in sessile [...] Read more.
Sessile droplets play a crucial role in the microreactors of biochemical samples. Acoustofluidics provide a non-contact and label-free method for manipulating particles, cells, and chemical analytes in droplets. In the present study, we propose a micro-stirring application based on acoustic swirls in sessile droplets. The acoustic swirls are formed inside the droplets by asymmetric coupling of surface acoustic waves (SAWs). With the merits of the slanted design of the interdigital electrode, the excitation position of SAWs is selective by sweeping in wide frequency ranges, allowing for the droplet position to be customized within the aperture region. We verify the reasonable existence of acoustic swirls in sessile droplets by a combination of simulations and experiments. The different periphery of the droplet meeting with SAWs will produce acoustic streaming phenomena with different intensities. The experiments demonstrate that acoustic swirls formed after SAWs encountering droplet boundaries will be more obvious. The acoustic swirls have strong stirring abilities to rapidly dissolve the yeast cell powder granules. Therefore, acoustic swirls are expected to be an effective means for rapid stirring of biomolecules and chemicals, providing a new approach to micro-stirring in biomedicine and chemistry. Full article
(This article belongs to the Special Issue Acoustofluidics for Chemical, Biological, and Medical Applications)
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10 pages, 2508 KiB  
Article
Particle-Induced Electrostatic Repulsion within an Electric Curtain Operating below the Paschen Limit
by Stuart J. Williams, Joseph D. Schneider, Benjamin C. King and Nicolas G. Green
Micromachines 2022, 13(2), 288; https://doi.org/10.3390/mi13020288 - 11 Feb 2022
Cited by 5 | Viewed by 3328
Abstract
The electric curtain is a platform developed to lift and transport charged particles in air. Its premise is the manipulation of charged particles; however, fewer investigations isolate dielectric forces that are observed at lower voltages (i.e., less than the Paschen limit). This work [...] Read more.
The electric curtain is a platform developed to lift and transport charged particles in air. Its premise is the manipulation of charged particles; however, fewer investigations isolate dielectric forces that are observed at lower voltages (i.e., less than the Paschen limit). This work focuses on observations of simultaneous dielectrophoretic and electrostatic forces. The electric curtain was a printed circuit board with interdigitated electrodes (0.020 inch width and spacing) coated with a layer of polypropylene, where a standing wave or travelling wave AC signal was applied (50 Hz) to produce an electric field below the Paschen limit. Soda lime glass beads (180–212 µm) demonstrated oscillatory rolling via dielectrophoretic forces. In addition, several particles simultaneously experienced rapid projectile repulsion, a behavior consistent with electrostatic phenomena. This second result is discussed as a particle-induced local increase in the electric field, with simulations demonstrating that a particle in close proximity to the curtain’s surface produces a local field enhancement of over 2.5 times. The significance of this is that individual particles themselves can trigger electrostatic repulsion in an otherwise dielectric system. These results could be used for advanced applications where particles themselves provided triggered responses, perhaps for selective sorting of micrometer particles in air. Full article
(This article belongs to the Special Issue Micromachines for Dielectrophoresis, Volume II)
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15 pages, 3461 KiB  
Article
Modeling a Dielectrophoretic Microfluidic Device with Vertical Interdigitated Transducer Electrodes for Separation of Microparticles Based on Size
by Fadi Alnaimat, Bobby Mathew and Ali Hilal-Alnaqbi
Micromachines 2020, 11(6), 563; https://doi.org/10.3390/mi11060563 - 31 May 2020
Cited by 10 | Viewed by 3617
Abstract
This article conceptualizes and mathematically models a dielectrophoretic microfluidic device with two sets of interdigitated transducer vertical electrodes for separation of a binary heterogeneous mixture of particles based on size; each set of electrodes is located on the sidewalls and independently controllable. To [...] Read more.
This article conceptualizes and mathematically models a dielectrophoretic microfluidic device with two sets of interdigitated transducer vertical electrodes for separation of a binary heterogeneous mixture of particles based on size; each set of electrodes is located on the sidewalls and independently controllable. To achieve separation in the proposed microfluidic device, the small microparticles are subjected to positive dielectrophoresis and the big microparticles do not experience dielectrophoresis. The mathematical model consists of equations describing the motion of each microparticle, fluid flow profile, and electric voltage and field profiles, and they are solved numerically. The equations of motion take into account the influence of phenomena, such as inertia, drag, dielectrophoresis, gravity, and buoyancy. The model is used for a parametric study to understand the influence of parameters on the performance of the microfluidic device. The parameters studied include applied electric voltages, electrode dimensions, volumetric flow rate, and number of electrodes. The separation efficiency of the big and small microparticles is found to be independent of and dependent on all parameters, respectively. On the other hand, the separation purity of the big and small microparticles is found to be dependent on and independent of all parameters, respectively. The mathematical model is useful in designing the proposed microfluidic device with the desired level of separation efficiency and separation purity. Full article
(This article belongs to the Special Issue Particles Separation in Microfluidic Devices)
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11 pages, 428 KiB  
Article
Dependence of Optical and Microstructure Properties of Thiol-Capped Silver Nanoparticles Embedded in Polymeric Matrix
by Angela Longo, Gianfranco Carotenuto, Mariano Palomba and Sergio De Nicola
Polymers 2011, 3(4), 1794-1804; https://doi.org/10.3390/polym3041794 - 13 Oct 2011
Cited by 21 | Viewed by 8380
Abstract
Thiol-capped silver nanoparticles were prepared by in situ thermal decomposition of different silver(I)-thiolates precursors in a polymeric matrix. Depending on the structure of the organic coating, contact-free distribution of metal nanoparticles or nanoparticles aggregates were achieved. The structure and morphology of nanocomposites was [...] Read more.
Thiol-capped silver nanoparticles were prepared by in situ thermal decomposition of different silver(I)-thiolates precursors in a polymeric matrix. Depending on the structure of the organic coating, contact-free distribution of metal nanoparticles or nanoparticles aggregates were achieved. The structure and morphology of nanocomposites was analyzed by Transmission Electron Microscopy (TEM), and X-Ray Diffraction (XRD). Nanoparticles’ interaction was investigated by differential scanning calorimetry (DSC), and UV-Visible spectroscopy. In particular, only silver nanoparticles coated by n-alkyl thiols aggregated, while a contact-free dispersion was obtained by cyclohexyl thiol-capped silver nanoparticles. Full article
(This article belongs to the Special Issue Polymers for Optical Applications)
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16 pages, 1183 KiB  
Article
Planar Array Sensor for High-speed Component Distribution Imaging in Fluid Flow Applications
by Marco Jose Da Silva, Tobias Sühnel, Eckhard Schleicher, Roman Vaibar, Dirk Lucas and Uwe Hampel
Sensors 2007, 7(10), 2430-2445; https://doi.org/10.3390/s7102430 - 19 Oct 2007
Cited by 31 | Viewed by 13348
Abstract
A novel planar array sensor based on electrical conductivity measurements ispresented which may be applied to visualize surface fluid distributions. The sensor ismanufactured using printed-circuit board fabrication technology and comprises of 64 x 64interdigital sensing structures. An associated electronics measures the electricalconductivity of [...] Read more.
A novel planar array sensor based on electrical conductivity measurements ispresented which may be applied to visualize surface fluid distributions. The sensor ismanufactured using printed-circuit board fabrication technology and comprises of 64 x 64interdigital sensing structures. An associated electronics measures the electricalconductivity of the fluid over each individual sensing structure in a multiplexed manner byapplying a bipolar excitation voltage and by measuring the electrical current flowing from adriver electrode to a sensing electrode. After interrogating all sensing structures, a two-dimensional image of the conductivity distribution over a surface is obtained which in turnrepresents fluid distributions over sensor’s surface. The employed electronics can acquire upto 2500 frames per second thus being able to monitor fast transient phenomena. The systemhas been evaluated regarding measurement accuracy and depth sensitivity. Furthermore, theapplication of the sensor in the investigation of two different flow applications is presented. Full article
(This article belongs to the Special Issue Intelligent Sensors)
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