Using Radiometric Measurements to Separate Dust and Smoke Radiative Effects during a Combined Smoke–Dust Event †
Abstract
:1. Introduction
2. Data and Methodology
- With a step of 0.05, we created all possible combinations of dust AOD, waso AOD, and soot AOD.
- For the UVSPEC simulations, we used the following extinction coefficient profiles:
- waso: climatological urban from OPAC [14].
- soot: maximum invariant concentration between 0.5 and 1.5 km that drops to 20% of the maximum at the surface and at 2 km (estimated roughly from the ceilometer).
- dust: homogeneous concentration from 0 to 2 km.
Deviations from the exact profiles are not expected to induce large uncertainties in the results of the radiative transfer simulations (e.g., [16]). - Using the methodology developed by Siomos et al., [17] we calculated the mass concentrations that correspond to each AOD combination, assuming a relative humidity of 50%, and then scaled the profiles.
- For each combination, we performed UVSPEC simulations of the GHI and then compared model outputs with the pyranometer measurements.
- Finally, we considered that the combination for which the simulated GHI is closer to the measured represents the composition of the mixture.
3. Results and Discussion
- -
- Attenuation of the GHI assuming that only one of each of the assumed aerosol types (1. waso, 2. soot, 3. dust) is present.
- -
- The summary of the attenuation that has been estimated individually for each aerosol type (1 + 2 + 3).
- -
- Attenuation of the GHI assuming that all aerosol species are simultaneously present (all).
- -
- Attenuation of the GHI that has been estimated using the optical properties provided by AERONET.
4. Summary and Conclusions
Author Contributions
Funding
Institutional Review Board Statement
Informed Consent Statement
Data Availability Statement
Conflicts of Interest
References
- IPCC. Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change; Stocker, T.F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S.K., Boschung, J., Nauels, A., Xia, Y., Eds.; IPCC: Geneva, Switzerland, 2013. [Google Scholar]
- Koulouri, E.; Saarikoski, S.; Theodosi, C.; Markaki, Z.; Gerasopoulos, E.; Kouvarakis, G.; Mäkelä, T.; Hillamo, R.; Mihalopoulos, N. Chemical composition and sources of fine and coarse aerosol particles in the Eastern Mediterranean. Atmos. Environ. 2008, 42, 6542–6550. [Google Scholar] [CrossRef]
- Denjean, C.; Cassola, F.; Mazzino, A.; Triquet, S.; Chevaillier, S.; Grand, N.; Bourrianne, T.; Momboisse, G.; Sellegri, K.; Schwarzenbock, A.; et al. Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean. Atmos. Chem. Phys. 2016, 16, 1081–1104. [Google Scholar] [CrossRef]
- Abdelkader, M.; Metzger, S.; Mamouri, R.E.; Astitha, M.; Barrie, L.; Levin, Z.; Lelieveld, J. Dust–air pollution dynamics over the eastern Mediterranean. Atmos. Chem. Phys. 2015, 15, 9173–9189. [Google Scholar] [CrossRef]
- Monteiro, A.; Basart, S.; Kazadzis, S.; Votsis, A.; Gkikas, A.; Vandenbussche, S.; Tobias, A.; Gama, C.; García-Pando, C.P.; Terradellas, E.; et al. Multi-sectoral impact assessment of an extreme African dust episode in the Eastern Mediterranean in March 2018. Sci. Total Environ. 2022, 843, 156861. [Google Scholar] [CrossRef] [PubMed]
- Papachristopoulou, K.; Fountoulakis, I.; Gkikas, A.; Kosmopoulos, P.G.; Nastos, P.T.; Hatzaki, M.; Kazadzis, S. 15-Year Analysis of Direct Effects of Total and Dust Aerosols in Solar Radiation/Energy over the Mediterranean Basin. Remote Sens. 2022, 14, 1535. [Google Scholar] [CrossRef]
- Castagna, J.; Senatore, A.; Bencardino, M.; Mendicino, G. Concurrent Influence of Different Natural Sources on the Particulate Matter in the Central Mediterranean Region during a Wildfire Season. Atmosphere 2021, 12, 144. [Google Scholar] [CrossRef]
- Gómez-Amo, J.L.; Estellés, V.; Marcos, C.; Segura, S.; Esteve, A.R.; Pedrós, R.; Utrillas, M.P.; Martínez-Lozano, J.A. Impact of dust and smoke mixing on column-integrated aerosol properties from observations during a severe wildfire episode over Valencia (Spain). Sci. Total Environ. 2017, 599–600, 2121–2134. [Google Scholar] [CrossRef]
- Salgueiro, V.; Costa, M.J.; Guerrero-Rascado, J.L.; Couto, F.T.; Bortoli, D. Characterization of forest fire and Saharan desert dust aerosols over south-western Europe using a multi-wavelength Raman lidar and Sun-photometer. Atmos. Environ. 2021, 252, 118346. [Google Scholar] [CrossRef]
- Masoom, A.; Fountoulakis, I.; Kazadzis, S.; Raptis, I.-P.; Kampouri, A.; Psiloglou, B.; Kouklaki, D.; Papachristopoulou, K.; Marinou, E.; Solomos, S.; et al. Investigation of the effects of the Greek extreme wildfires of August 2021 on air quality and spectral solar irradiance. EGUsphere 2023, 2023, 1–42. [Google Scholar] [CrossRef]
- Giles, D.M.; Sinyuk, A.; Sorokin, M.G.; Schafer, J.S.; Smirnov, A.; Slutsker, I.; Eck, T.F.; Holben, B.N.; Lewis, J.R.; Campbell, J.R.; et al. Advancements in the Aerosol Robotic Network (AERONET) Version 3 database—Automated near-real-time quality control algorithm with improved cloud screening for Sun photometer aerosol optical depth (AOD) measurements. Atmos. Meas. Tech. 2019, 12, 169–209. [Google Scholar] [CrossRef]
- Kazadzis, S.; Founda, D.; Psiloglou, B.E.; Kambezidis, H.; Mihalopoulos, N.; Sanchez-Lorenzo, A.; Meleti, C.; Raptis, P.I.; Pierros, F.; Nabat, P. Long-term series and trends in surface solar radiation in Athens, Greece. Atmos. Chem. Phys. 2018, 18, 2395–2411. [Google Scholar] [CrossRef]
- Emde, C.; Buras-Schnell, R.; Kylling, A.; Mayer, B.; Gasteiger, J.; Hamann, U.; Kylling, J.; Richter, B.; Pause, C.; Dowling, T.; et al. The libRadtran software package for radiative transfer calculations (version 2.0.1). Geosci. Model Dev. 2016, 9, 1647–1672. [Google Scholar] [CrossRef]
- Hess, M.; Koepke, P.; Schult, I. Optical Properties of Aerosols and Clouds: The Software Package OPAC. Bull. Am. Meteorol. Soc. 1998, 79, 831–844. [Google Scholar] [CrossRef]
- Mamouri, R.-E.; Ansmann, A. Potential of polarization/Raman lidar to separate fine dust, coarse dust, maritime, and anthropogenic aerosol profiles. Atmos. Meas. Tech. 2017, 10, 3403–3427. [Google Scholar] [CrossRef]
- Fountoulakis, I.; Papachristopoulou, K.; Proestakis, E.; Amiridis, V.; Kontoes, C.; Kazadzis, S. Effect of Aerosol Vertical Distribution on the Modeling of Solar Radiation. Remote Sens. 2022, 14, 1143. [Google Scholar] [CrossRef]
- Siomos, N.; Fountoulakis, I.; Gkertsi, F.; Voudouri, K.A.; Michailidis, K.; Garane, K.; Karagkiozidis, D.; Karanikolas, A.; Natsis, A.; Koukouli, M.E.; et al. A technique to retrieve vertical concentration profiles of individual aerosol species based on the synergy of lidar and spectrophotometer measurements. In Proceedings of the COMECAP 2021, Ioannina, Greece, 26–29 September 2021. [Google Scholar] [CrossRef]
- Siomos, N.; Fountoulakis, I.; Natsis, A.; Drosoglou, T.; Bais, A. Automated Aerosol Classification from Spectral UV Measurements Using Machine Learning Clustering. Remote Sens. 2020, 12, 965. [Google Scholar] [CrossRef]
- Dubovik, O.; Lapyonok, T.; Litvinov, P.; Herman, M.; Fuertes, D.; Ducos, F.; Lopatin, A.; Chaikovsky, A.; Torres, B.; Derimian, Y.; et al. GRASP: A versatile algorithm for characterizing the atmosphere. SPIE Newsroom 2014. [Google Scholar] [CrossRef]
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Fountoulakis, I.; Siomos, N.; Raptis, I.-P.; Eleftheratos, K.; Kouklaki, D.; Psiloglou, B.E.; Amiridis, V.; Kazadzis, S. Using Radiometric Measurements to Separate Dust and Smoke Radiative Effects during a Combined Smoke–Dust Event. Environ. Sci. Proc. 2023, 26, 26. https://doi.org/10.3390/environsciproc2023026026
Fountoulakis I, Siomos N, Raptis I-P, Eleftheratos K, Kouklaki D, Psiloglou BE, Amiridis V, Kazadzis S. Using Radiometric Measurements to Separate Dust and Smoke Radiative Effects during a Combined Smoke–Dust Event. Environmental Sciences Proceedings. 2023; 26(1):26. https://doi.org/10.3390/environsciproc2023026026
Chicago/Turabian StyleFountoulakis, Ilias, Nikolaos Siomos, Ioannis-Panagiotis Raptis, Kostas Eleftheratos, Dimitra Kouklaki, Basil E. Psiloglou, Vassilis Amiridis, and Stelios Kazadzis. 2023. "Using Radiometric Measurements to Separate Dust and Smoke Radiative Effects during a Combined Smoke–Dust Event" Environmental Sciences Proceedings 26, no. 1: 26. https://doi.org/10.3390/environsciproc2023026026