Preparation of Long-Term Antibacterial SiO2-Cinnamaldehyde Microcapsule via Sol-Gel Approach as a Functional Additive for PBAT Film
Abstract
:1. Introduction
2. Materials and Methods
2.1. Materials and Regents
2.2. Preparation and Characterization of Microcapsules
2.2.1. Preparation of Microcapsules
2.2.2. Characterizations of Microcapsules
2.2.3. Encapsulation Efficiency
2.2.4. Sustained-Release Performance of Microcapsules
2.2.5. Antibacterial Assay of Microcapsules
2.3. Preparation and Characterization of Microcapsules Loaded Films
2.3.1. Preparation of Films
2.3.2. Characterization of Films
2.3.3. Antibacterial Assay of Films
2.4. Statistical Analysis
3. Results and Discussion
3.1. Preparation of Microcapsules
3.1.1. Preparation
3.1.2. Effect of CA Concentration on Encapsulation Efficiency
3.2. Structural and Morphological Properties of Microcapsules
3.2.1. Functional Structure
3.2.2. Crystallography
3.2.3. Surface Morphology
3.3. Sustained-Release Performance Analysis
3.4. Antibacterial Activity Analysis
3.5. Modification Effect of Microcapsule on Films
3.5.1. Physical Properties of Films
3.5.2. Thermodynamic Properties of Films
3.5.3. Surface Morphology of Films
3.5.4. Antibacterial Properties of Films
4. Conclusions
Supplementary Materials
Author Contributions
Funding
Acknowledgments
Conflicts of Interest
References
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Equation Model | Release Condition | Fitting Equation | R2 | |
---|---|---|---|---|
90%RH | 4 °C | Q = 55.1637 (1 × 10−0.0555t) | 0.9835 | |
23 °C | Q = 74.1331 (1× 10−0.0618t) | 0.9438 | ||
40 °C | Q = 87.7758 (1 × 10−0.08t) | 0.9751 | ||
40 °C | 50%RH | Q = 75.7937 (1 × 10−0.0465t) | 0.9867 | |
70%RH | Q = 84.2127 (1 × 10−0.0480t) | 0.9934 | ||
90%RH | Q = 87.7758 (1 × 10−0.08t) | 0.9751 |
Concentration (mg·mL−1) | Inhibition Zone Diameter (mm) | |
---|---|---|
ListeriaMonocytogenes | E. coli | |
Blank control | -- | -- |
Negative control | -- | -- |
40 | 12.55 | -- |
50 | 12.70 | -- |
60 | 12.74 | -- |
70 | 12.89 | -- |
80 | 13.26 | 11.08 |
90 | 13.95 | 11.99 |
Sample | Tonset (°C) | Tc (°C) | Tm (°C) | Xc (%) |
---|---|---|---|---|
PBAT film | 92.91 | 61.54 | 123.13 | 11.12 |
PSC-0.5% film | 94.20 | 66.44 | 124.06 | 11.22 |
PSC-2.5% film | 94.65 | 70.25 | 123.49 | 11.67 |
PSC-4.5% film | 92.67 | 70.21 | 123.28 | 10.10 |
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Xu, Y.; Huang, C.; Dang, X.; Khan, M.R.; Huang, H.; Zhao, Y.; Wang, S. Preparation of Long-Term Antibacterial SiO2-Cinnamaldehyde Microcapsule via Sol-Gel Approach as a Functional Additive for PBAT Film. Processes 2020, 8, 897. https://doi.org/10.3390/pr8080897
Xu Y, Huang C, Dang X, Khan MR, Huang H, Zhao Y, Wang S. Preparation of Long-Term Antibacterial SiO2-Cinnamaldehyde Microcapsule via Sol-Gel Approach as a Functional Additive for PBAT Film. Processes. 2020; 8(8):897. https://doi.org/10.3390/pr8080897
Chicago/Turabian StyleXu, Yangfan, Chongxing Huang, Xiujie Dang, Muhammad Rafiullah Khan, Haohe Huang, Yuan Zhao, and Shuangfei Wang. 2020. "Preparation of Long-Term Antibacterial SiO2-Cinnamaldehyde Microcapsule via Sol-Gel Approach as a Functional Additive for PBAT Film" Processes 8, no. 8: 897. https://doi.org/10.3390/pr8080897