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One-Step Chemical Vapor Deposition Synthesis of 3D N-doped Carbon Nanotube/N-doped Graphene Hybrid Material on Nickel Foam

1
Institute for Advanced Study, Nanchang University, Nanchang 330031, China
2
School of Resources Environmental & Chemical Engineering, Nanchang University, Nanchang 330031, China
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Key Laboratory of Poyang Lake Environment and Resource Utilization, Nanchang University, Ministry of Education, Nanchang 330031, China
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School for Engineering of Matter, Transport and Energy, Arizona State University, Tempe, AZ 85287, USA
5
Department of Physics, North Carolina Central University, Durham, NC 27707, USA
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Department of Chemistry and Biochemistry, North Carolina Central University, Durham, NC 27707, USA
*
Authors to whom correspondence should be addressed.
Nanomaterials 2018, 8(9), 700; https://doi.org/10.3390/nano8090700
Received: 26 July 2018 / Revised: 31 August 2018 / Accepted: 4 September 2018 / Published: 7 September 2018
3D hybrid nanostructures connecting 1D carbon nanotubes (CNTs) with 2D graphene have attracted more and more attentions due to their excellent chemical, physical and electrical properties. In this study, we firstly report a novel and facile one-step process using template-directed chemical vapor deposition (CVD) to fabricate highly nitrogen doped three-dimensional (3D) N-doped carbon nanotubes/N-doped graphene architecture (N-CNTs/N-graphene). We used nickel foam as substrate, melamine as a single source for both carbon and nitrogen, respectively. The morphology and microstructure were characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, isothermal analyses, X-ray photoelectron microscopy and Raman spectra. The obtained 3D N-CNTs/N-graphene exhibits high graphitization, a regular 3D structure and excellent nitrogen doping and good mesoporosity. View Full-Text
Keywords: N-doped CNTs; N-doped graphene; 3D hybrid; melamine; CVD synthesis N-doped CNTs; N-doped graphene; 3D hybrid; melamine; CVD synthesis
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MDPI and ACS Style

Li, H.-F.; Wu, F.; Wang, C.; Zhang, P.-X.; Hu, H.-Y.; Xie, N.; Pan, M.; Zeng, Z.; Deng, S.; Wu, M.H.; Vinodgopal, K.; Dai, G.-P. One-Step Chemical Vapor Deposition Synthesis of 3D N-doped Carbon Nanotube/N-doped Graphene Hybrid Material on Nickel Foam. Nanomaterials 2018, 8, 700.

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