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Acidic Mesoporous Zeolite ZSM-5 Supported Cu Catalyst with Good Catalytic Performance in the Hydroxysulfurization of Styrenes with Disulfides

1
School of Chemical and Environmental Engineering, Jiangsu University of Technology, Changzhou 213001, China
2
School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China
*
Author to whom correspondence should be addressed.
Nanomaterials 2017, 7(12), 459; https://doi.org/10.3390/nano7120459
Received: 20 November 2017 / Revised: 10 December 2017 / Accepted: 13 December 2017 / Published: 19 December 2017
(This article belongs to the Special Issue Nanosized Zeolites and their Applications)
Development of highly active heterogeneous catalysts is an effective strategy for modern organic synthesis chemistry. In this work, acidic mesoporous zeolite ZSM-5 (HZSM-5-M), acidic-free mesoporous zeolite TS-1 (TS-1-M), and basic ETS-10 zeolite supported metal Cu catalysts were prepared to investigate their catalytic performances in the hydroxysulfurization of styrenes with diaryl disulfides. The effect of pore size and acidities of the supports, as well as the Cu species electronic properties of the catalysts on reaction activity were investigated. The results show that Cu+ and Cu2+ binded on HZSM-5-M show the highest activity and product selectivity for the desired β-hydroxysulfides compounds. View Full-Text
Keywords: mesoporous zeolite ZSM-5; copper; hydroxysulfurization; acidity mesoporous zeolite ZSM-5; copper; hydroxysulfurization; acidity
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MDPI and ACS Style

Hu, J.; Zhu, C.; Xia, F.; Fang, Z.; Yang, F.; Weng, J.; Yao, P.; Zheng, C.; Dong, H.; Fu, W. Acidic Mesoporous Zeolite ZSM-5 Supported Cu Catalyst with Good Catalytic Performance in the Hydroxysulfurization of Styrenes with Disulfides. Nanomaterials 2017, 7, 459.

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