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Keywords = bismuth iron garnet

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9 pages, 1798 KiB  
Article
Magnetoplasmonic Resonators Designed with Hexagonally Arrayed Au/BIG Bilayer Nanodisks on Au Thin Film Layers for Enhanced MOKE and Refractive Index Sensing
by Ziqi Wang, Xiaojian Cui and Yujun Song
Coatings 2025, 15(5), 601; https://doi.org/10.3390/coatings15050601 - 18 May 2025
Viewed by 396
Abstract
A kind of magnetoplasmonic resonators is numerically designed with hexagonally arrayed Au/bismuth iron garnet (BIG) bilayer nanodiscks on Au thin film layers. Multi-physics coupling calculation on their magnetoplasmonic resonance features suggest that there exists a strong resonant coupling between the surface plasmon excited [...] Read more.
A kind of magnetoplasmonic resonators is numerically designed with hexagonally arrayed Au/bismuth iron garnet (BIG) bilayer nanodiscks on Au thin film layers. Multi-physics coupling calculation on their magnetoplasmonic resonance features suggest that there exists a strong resonant coupling between the surface plasmon excited by the hexagonal grating and the waveguide modes induced by Au-BIG-Au, which can significantly enhance the transverse magneto-optical Kerr effect. Interestingly, a new type of circular oscillating can be induced in the optical-transparent BIG layers as the thickness of BIG layers is between 2 nm and 22 nm. This circular oscillating exhibits a distinct thickness-dependent feature, which can be attributed to the near field interference of the excited localized plasmon resonance between the two interfaces formed by the middle BIG nanodiscs in the top Au nanodisks and the bottom Au thin film layers according to the simulation. These unique magnetoplasmonic features endow this kind of magnetoplasmonic resonators with a greatly enhanced refractive index sensing property, with a calculated figure of merit (FOM) value of up to 7527 RIU−1. Full article
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18 pages, 3847 KiB  
Review
Bi-Substituted Ferrite Garnet Type Magneto-Optic Materials Studied at ESRI Nano-Fabrication Laboratories, ECU, Australia
by Mohammad Nur-E-Alam, Mikhail Vasiliev and Kamal Alameh
Coatings 2022, 12(10), 1471; https://doi.org/10.3390/coatings12101471 - 5 Oct 2022
Cited by 6 | Viewed by 2965
Abstract
Since 2007, at the Electron Science Research Institute (ESRI) nano-fabrication laboratories, Edith Cowan University, Australia, we have devoted research efforts to the synthesis and characterization of bismuth-containing ferrite-garnet-type thin-film magneto-optic (MO) materials of different compositions. We report on the growth and characteristics of [...] Read more.
Since 2007, at the Electron Science Research Institute (ESRI) nano-fabrication laboratories, Edith Cowan University, Australia, we have devoted research efforts to the synthesis and characterization of bismuth-containing ferrite-garnet-type thin-film magneto-optic (MO) materials of different compositions. We report on the growth and characteristics of radio frequency (RF) magnetron sputtered bismuth-substituted iron-garnet thin films. We study the process parameters associated with the RF magnetron sputter deposition technique and investigate the results of optimizing process parameters. To achieve the best MO properties, we employ a few unique techniques, such as co-sputtered nanocomposite films and all-garnet multilayer structures, as well as the application of oxygen plasma treatment to amorphous garnet layers immediately following the deposition process. We demonstrated a remarkable enhancement in the MO properties of Bi-containing ferrite-type garnet thin-film materials, including record-high MO figures of merit and improved conventional and unconventional hysteresis loops of Faraday rotation. Previously unpublished research results on the forward-looking applications of magnetic garnet coatings applied to microparticles of advanced luminescent materials are reported. In the context of developing the next-generation ultra-fast optoelectronic devices, such as light intensity switches and modulators, high-speed flat panel displays, and high-sensitivity sensors, it is important to consider the desirable optical, magnetic, and magneto-optic properties that are found in highly bismuth-substituted iron garnet thin-film materials of various composition types. Full article
(This article belongs to the Special Issue New Advances in Novel Optical Materials and Devices)
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13 pages, 14406 KiB  
Article
Enhanced Magneto-Optic Properties in Sputtered Bi- Containing Ferrite Garnet Thin Films Fabricated Using Oxygen Plasma Treatment and Metal Oxide Protective Layers
by V. A. Kotov, M. Nur-E-Alam, M. Vasiliev, K. Alameh, D. E. Balabanov and V. I. Burkov
Materials 2020, 13(22), 5113; https://doi.org/10.3390/ma13225113 - 12 Nov 2020
Cited by 6 | Viewed by 2515
Abstract
Magneto-optic (MO) imaging and sensing are at present the most developed practical applications of thin-film MO garnet materials. However, in order to improve sensitivity for a range of established and forward-looking applications, the technology and component-related advances are still necessary. These improvements are [...] Read more.
Magneto-optic (MO) imaging and sensing are at present the most developed practical applications of thin-film MO garnet materials. However, in order to improve sensitivity for a range of established and forward-looking applications, the technology and component-related advances are still necessary. These improvements are expected to originate from new material system development. We propose a set of technological modifications for the RF-magnetron sputtering deposition and crystallization annealing of magneto-optic bismuth-substituted iron-garnet films and investigate the improved material properties. Results show that standard crystallization annealing for the as-deposited ultrathin (sputtered 10 nm thick, amorphous phase) films resulted in more than a factor of two loss in the magneto-optical activity of the films in the visible spectral region, compared to the liquid-phase grown epitaxial films. Results also show that an additional 10 nm-thick metal-oxide (Bi2O3) protective layer above the amorphous film results in ~2.7 times increase in the magneto-optical quality of crystallized iron-garnet films. On the other hand, the effects of post-deposition oxygen (O2) plasma treatment on the magneto-optical (MO) properties of Bismuth substituted iron garnet thin film materials are investigated. Results show that in the visible part of the electromagnetic spectrum (at 532 nm), the O2 treated (up to 3 min) garnet films retain higher specific Faraday rotation and figures of merit compared to non-treated garnet films. Full article
(This article belongs to the Special Issue Photoactive Materials: Synthesis, Applications and Technology)
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8 pages, 2099 KiB  
Article
Influence of Sputtered ZnO and Al:ZnO Top Layers on Magneto-Optic Responses of Yttrium Iron Garnet Films
by Shinichiro Mito, Satsuki Kikuchi, Yasutoshi Ito, Nana Ota and Mitsuteru Inoue
Crystals 2018, 8(10), 396; https://doi.org/10.3390/cryst8100396 - 22 Oct 2018
Viewed by 3590
Abstract
Zinc oxide (ZnO) is a promising material for combining with magneto-optic (MO) materials because it can propagate stable exciton-polaritons, with velocities considerably lower than that of photons in a vacuum. This study investigated the influence of sputtered ZnO and Al:ZnO top layers on [...] Read more.
Zinc oxide (ZnO) is a promising material for combining with magneto-optic (MO) materials because it can propagate stable exciton-polaritons, with velocities considerably lower than that of photons in a vacuum. This study investigated the influence of sputtered ZnO and Al:ZnO top layers on MO responses of a bismuth-substituted yttrium iron garnet (Bi:YIG) film. The ZnO top layer modulated the Faraday rotation and magnetic circular dichroism (MCD) of the Bi:YIG around the exciton resonance wavelength of ZnO at 369 nm. Furthermore, Al-substituted ZnO, which is a conductive ZnO, also changed the MO effects around the exciton resonance wavelength. These results imply that the exciton-polaritons in ZnO affect the MO interaction, because of their considerably low group velocity. The results suggest potential for controlling the MO response via excitons. Full article
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12 pages, 1866 KiB  
Article
Influence of Substrate Stage Temperature and Rotation Rate on the Magneto-Optical Quality of RF-Sputtered Bi2.1Dy0.9Fe3.9Ga1.1O12 Garnet Thin Films
by M. Nur-E-Alam, Mikhail Vasiliev and Kamal Alameh
Appl. Sci. 2018, 8(3), 456; https://doi.org/10.3390/app8030456 - 16 Mar 2018
Cited by 4 | Viewed by 4276
Abstract
Highly bismuth-substituted iron garnet thin films are prepared on quartz substrates by using a radio frequency (RF) magnetron sputtering technique. We study the factors (process parameters associated with the RF magnetron sputter deposition technique) affecting the magneto-optical (MO) properties of ferrite garnet films [...] Read more.
Highly bismuth-substituted iron garnet thin films are prepared on quartz substrates by using a radio frequency (RF) magnetron sputtering technique. We study the factors (process parameters associated with the RF magnetron sputter deposition technique) affecting the magneto-optical (MO) properties of ferrite garnet films of composition Bi2.1Dy0.9Fe3.9Ga1.1O12. All films show high MO response across the visible range of wavelengths after being annealed. In particular, the effects of substrate stage temperature and rotation rate on the various properties of films are studied. Experimental results reveal that the characteristics of garnet films of this type can be tuned and optimized for use in various magnetic field-driven nanophotonics and integrated optics devices, and that, at a substrate stage rotation rate near 16 revolutions per minute, the MO quality of the developed MO films is the best, in comparison with films deposited at other rotation rates. To the best of our knowledge, this is the first report on the effects of deposition parameters on the properties of garnet films of this stoichiometry. Full article
(This article belongs to the Section Materials Science and Engineering)
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29 pages, 12097 KiB  
Article
Focused Ion Beam and Advanced Electron Microscopy for Minerals: Insights and Outlook from Bismuth Sulphosalts
by Cristiana L. Ciobanu, Nigel J. Cook, Christian Maunders, Benjamin P. Wade and Kathy Ehrig
Minerals 2016, 6(4), 112; https://doi.org/10.3390/min6040112 - 20 Oct 2016
Cited by 34 | Viewed by 7898
Abstract
This paper comprises a review of the rapidly expanding application of nanoscale mineral characterization methodology to the study of ore deposits. Utilising bismuth sulphosalt minerals from a reaction front in a skarn assemblage as an example, we illustrate how a complex problem in [...] Read more.
This paper comprises a review of the rapidly expanding application of nanoscale mineral characterization methodology to the study of ore deposits. Utilising bismuth sulphosalt minerals from a reaction front in a skarn assemblage as an example, we illustrate how a complex problem in ore petrology, can be approached at scales down to that of single atoms. We demonstrate the interpretive opportunities that can be realised by doing this for other minerals within their petrogenetic contexts. From an area defined as Au-rich within a sulphosalt-sulphide assemblage, and using samples prepared on a Focused Ion Beam–Scanning Electron Microscopy (SEM) platform, we identify mineral species and trace the evolution of their intergrowths down to the atomic scale. Our approach progresses from a petrographic and trace element study of a larger polished block, to high-resolution Transmission Electron Microscopy (TEM) and High Angle Annular Dark Field (HAADF) Scanning-TEM (STEM) studies. Lattice-scale heterogeneity imaged in HAADF STEM mode is expressed by changes in composition of unit cell slabs followed by nanoparticle formation and their growth into “veins”. We report a progressive transition from sulphosalt species which host lattice-bound Au (neyite, lillianite homologues; Pb-Bi-sulphosalts), to those that cannot accept Au (aikinite). This transition acts as a crystal structural barrier for Au. Fine particles of native gold track this progression over the scale of several hundred microns, leading to Au enrichment at the reaction front defined by an increase in the Cu gradient (several wt %), and abrupt changes in sulphosalt speciation from Pb-Bi-sulphosalts to aikinite. Atom-scale resolution imaging in HAADF STEM mode allows for the direct visualisation of the three component slabs in the neyite crystal structure, one of the largest and complex sulphosalts of boxwork-type. We show for the first time the presence of aikinite nanoparticles a few nanometres in size, occurring on distinct (111)PbS slabs in the neyite. This directly explains the non-stoichiometry of this phase, particularly with respect to Cu. Such non-stoichiometry is discussed elsewhere as defining distinct mineral species. The interplay between modular crystal structures and trace element behaviour, as discussed here for Au and Cu, has applications for other mineral systems. These include the incorporation and release of critical metals in sulphides, heavy elements (U, Pb, W) in iron oxides, the distribution of rare earth elements (REE), Y, and chalcophile elements (Mo, As) in calcic garnets, and the identification of nanometre-sized particles containing daughter products of radioactive decay in ores, concentrates, and tailings. Full article
(This article belongs to the Special Issue Advances in Mineral Analytical Techniques)
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