Sign in to use this feature.

Years

Between: -

Subjects

remove_circle_outline
remove_circle_outline
remove_circle_outline

Journals

Article Types

Countries / Regions

Search Results (3)

Search Parameters:
Keywords = Bi2Te3 nanoflakes

Order results
Result details
Results per page
Select all
Export citation of selected articles as:
10 pages, 4453 KiB  
Article
Bi2Te3/Carbon Nanotube Hybrid Nanomaterials as Catalysts for Thermoelectric Hydrogen Peroxide Generation
by Chunlei Li, Shun Li, Long Zhao and Jianming Zhang
Molecules 2024, 29(22), 5242; https://doi.org/10.3390/molecules29225242 - 6 Nov 2024
Viewed by 1222
Abstract
Harnessing waste heat from environmental or industrial sources presents a promising approach to eco-friendly and sustainable chemical synthesis. In this study, we introduce a thermoelectrocatalytic (TECatal) system capable of utilizing even small amounts of heat for hydrogen peroxide (H2O2) [...] Read more.
Harnessing waste heat from environmental or industrial sources presents a promising approach to eco-friendly and sustainable chemical synthesis. In this study, we introduce a thermoelectrocatalytic (TECatal) system capable of utilizing even small amounts of heat for hydrogen peroxide (H2O2) production. We developed a nanohybrid structure, combining carbon nanotubes (CNTs) and Bi2Te3 nanoflakes (Bi2Te3/CNTs), through a one-pot synthesis method. Bi2Te3, as a thermoelectric (TE) material, generates charge carriers under a temperature gradient via the Seebeck effect, enabling them to participate in surface redox reactions. However, the rapid recombination of these charge carriers greatly limits the TECatal activity. In the Bi2Te3/CNTs nanohybrid system, the introduction of CNTs substantially enhances the efficiency of H2O2 production, as the strong bonding between CNTs and Bi2Te3, along with the excellent conductivity of CNTs, facilitates charge carrier separation and transport, as confirmed by TE electrochemical tests. This study underscores the significant potential of thermoelectric nanomaterials for converting waste heat into green chemical synthesis. Full article
Show Figures

Figure 1

14 pages, 4927 KiB  
Article
Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi2Se3 Nanoflakes
by Zicheng Yuan, Xueke Zhao, Canhui Wang, Shuang Hang, Mengyao Li and Yu Liu
Nanomaterials 2023, 13(13), 1937; https://doi.org/10.3390/nano13131937 - 26 Jun 2023
Cited by 4 | Viewed by 1964
Abstract
Environmental heat-to-electric energy conversion presents a promising solution for powering sensors in wearable and portable devices. However, the availability of near-room temperature thermoelectric (TE) materials is highly limited, posing a significant challenge in this field. Bi2Se3, as a room-temperature [...] Read more.
Environmental heat-to-electric energy conversion presents a promising solution for powering sensors in wearable and portable devices. However, the availability of near-room temperature thermoelectric (TE) materials is highly limited, posing a significant challenge in this field. Bi2Se3, as a room-temperature TE material, has attracted much attention. Here, we demonstrate a large-scale synthesis of Bi2Se3 nanoflakes used for the microflexible TE generator. A high-performance micro-TE generator module, utilizing a flexible printed circuit, has been designed and fabricated through the process of screen printing. The TE generator configuration comprises five pairs of PN TE legs. The p-type TE leg utilizes commercially available Sb2Te3 powder, while the n-type TE leg employs Bi2Se3 nanoflakes synthesized in this study. For comparative purposes, we also incorporate commercially available Bi2Se3 powder as an alternative n-type TE leg. The optimal performance of the single-layer microflexible TE generator, employing Bi2Se3 nanoflakes as the active material, is achieved when operating at a temperature differential of 109.5 K, the open-circuit voltage (VOC) is 0.11 V, the short circuit current (ISC) is 0.34 mA, and the maximum output power (PMAX) is 9.5 μW, much higher than the generator consisting of commercial Bi2Se3 powder, which is expected to provide an energy supply for flexible electronic devices. Full article
Show Figures

Figure 1

8 pages, 2745 KiB  
Article
Plasmonic Emission of Bullseye Nanoemitters on Bi2Te3 Nanoflakes
by Qigeng Yan, Xiaoli Li and Baolai Liang
Materials 2020, 13(7), 1531; https://doi.org/10.3390/ma13071531 - 26 Mar 2020
Cited by 4 | Viewed by 2944
Abstract
Topological insulators, such as Bi2Te3, have been confirmed to exhibit plasmon radiation over the entire visible spectral range. Herein, we fabricate bullseye nanoemitters, consisting of a central disk and concentric gratings, on the Bi2Te3 nanoflake. Due [...] Read more.
Topological insulators, such as Bi2Te3, have been confirmed to exhibit plasmon radiation over the entire visible spectral range. Herein, we fabricate bullseye nanoemitters, consisting of a central disk and concentric gratings, on the Bi2Te3 nanoflake. Due to the existence of edge plasmon modes, Bi2Te3 bullseye nanostructures are possible to converge light towards the central disk. Taking advantage of the excellent spatial resolution of cathodoluminescence (CL) characterization, it has been observed that plasmonic behaviors depend on the excitation location. A stronger plasmonic intensity and a wider CL spectral linewidth can be obtained at the edge of the central disk. In order to further improve the focusing ability, a cylindrical Pt nanostructure has been deposited on the central disk. Additionally, the finite element simulation indicates that the electric-field enhancement originates from the coupling process between the plasmonic emission from the Bi2Te3 bullseye and the Pt nanostructure. Finally, we find that enhancement efficiency depends on the thickness of the Pt nanostructure. Full article
Show Figures

Figure 1

Back to TopTop