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Keywords = Asia-Pacific Economic Cooperation summit

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19 pages, 2469 KiB  
Article
Characteristics and Source Apportionment of Metallic Elements in PM2.5 at Urban and Suburban Sites in Beijing: Implication of Emission Reduction
by Miaoling Li, Zirui Liu, Jing Chen, Xiaojuan Huang, Jingyun Liu, Yuzhu Xie, Bo Hu, Zhongjun Xu, Yuanxun Zhang and Yuesi Wang
Atmosphere 2019, 10(3), 105; https://doi.org/10.3390/atmos10030105 - 26 Feb 2019
Cited by 18 | Viewed by 4284
Abstract
To gain insights into the impacts of emission reduction measures on the characteristics and sources of trace elements during the 2014 Asia-Pacific Economic Cooperation (APEC) summit, PM2.5 samples were simultaneously collected from an urban site and a suburban site in Beijing from [...] Read more.
To gain insights into the impacts of emission reduction measures on the characteristics and sources of trace elements during the 2014 Asia-Pacific Economic Cooperation (APEC) summit, PM2.5 samples were simultaneously collected from an urban site and a suburban site in Beijing from September 15th to November 12th, and fifteen metallic elements were analyzed, including five crustal elements (Mg, Al, K, Ca and Fe), nine trace metals (V, Cr, Mn, Co, Cu, Zn, Ag, Cd and Pb) and As. Most of the trace metals (V, Cr, Mn, As, Cd and Pb) decreased more than 40% due to the emission regulations during APEC, while the crustal elements decreased considerably (4–45%). Relative to the daytime, trace metals increased during the nighttime at both sites before the APEC summit, but no significant difference was observed during the APEC summit, suggesting suppressed emissions from anthropogenic activities. Five sources (dust, traffic exhaust, industrial sources, coal and oil combustion and biomass burning) were resolved using positive matrix factorization (PMF), which were collectively decreased by 30.7% at the urban site and 14.4% at the suburban site during the APEC summit. Coal and oil combustion regulations were the most effective for reducing the trace elements concentrations (urban site: 63.1%; suburban site: 52.0%), followed by measures to reduce traffic exhaust (52.8%) at the urban site and measures to reduce biomass burning (37.7%) at the suburban site. Our results signify that future control efforts of metallic elements in megacities like Beijing should prioritize coal and oil combustion, as well as traffic emissions. Full article
(This article belongs to the Special Issue Urban Atmospheric Aerosols: Sources, Analysis and Effects)
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