Scanning Probe Spectroscopy: From Radio- to Terahertz Frequencies

A special issue of Nanomaterials (ISSN 2079-4991).

Deadline for manuscript submissions: closed (1 May 2019) | Viewed by 3519

Special Issue Editors


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Guest Editor
Institute of Semiconductor and Solid State Physics, Johannes Kepler University Linz, 4040 Linz, Austria
Interests: radio-frequency scanning tunneling microscopy; electron and nuclear spin excitation in single molecules; functional molecules ferromagnet/semiconductor hetero-and nanostructures; magnetologic; stress and magnetostriction of thin epitaxial films; self organization of surfaces and heterostructures

E-Mail Website
Guest Editor
Institute of Semiconductor and Solid State Physics, Johannes Kepler University Linz, 4040 Linz, Austria
Interests: radio-frequency scanning tunneling spectroscopy (rf-STS); molecule-based hybrid nanostructures; experimental nanophysics

Special Issue Information

Dear Colleagues,

With the increasing importance of nanosciences in daily life and technology, there is a strong demand for new investigation tools that have the precision needed for studying and controlling the quantum physical and chemical properties of nanoscale objects. Since the early 1980s, a variety of scanning probe techniques have been established as leading experimental tools in their fields of research. This has enabled the determination and control of, for example, the geometric, electronic, magnetic, and chemical structure of single-crystal surfaces and adsorbates, artificial quantum dots, nanowires and -islands with atomic-scale spatial resolution, and, more recently, even of single atoms and molecules.  

The energy-resolution limit of the established scanning probe spectroscopy techniques—presently ≈0.1 meV—remains among the biggest challenges. Recent spectroscopic resonance experiments utilize either high-frequency AC voltages or THz-laser irradiation. The respective resonance energies range between about 40 neV and a few meV. These novel approaches have revolutionized the field of scanning probe spectroscopy by improving the energy resolution up to 104 times and the sensitivity down to the detection-limit of single spins. Recent studies demonstrate, e.g., the electron and nuclear spin resonance (ESR, NMR), as well as electron-nuclear double resonance (ENDOR) of single atoms and molecules, the excitation of mechanical vibrations in molecules, molecular chains and surface layers, or the detection of subsurface dopants in semiconductors.  

This Special Issue of Nanomaterials attempts to cover the most recent advances in the field of scanning probe spectroscopy operating at resonance frequencies of MHz to THz. Submissions of regular as well as review articles are appreciated.

Prof. Dr. Reinhold Koch
Prof. Dr. Stefan Müllegger
Guest Editors

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Keywords

  • Single-spin excitation and detection 
  • Mechanical excitation of nanoscale objects (atoms, molecules, clusters, surfaces) 
  • Noise spectroscopy and stochastic resonance 
  • (Sub)surface material characterization 
  • Advances of instrumentation

Published Papers (1 paper)

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Research

10 pages, 1863 KiB  
Article
Towards Laterally Resolved Ferromagnetic Resonance with Spin-Polarized Scanning Tunneling Microscopy
by Marie Hervé, Moritz Peter, Timofey Balashov and Wulf Wulfhekel
Nanomaterials 2019, 9(6), 827; https://doi.org/10.3390/nano9060827 - 31 May 2019
Cited by 3 | Viewed by 3273
Abstract
We used a homodyne detection to investigate the gyration of magnetic vortex cores in Fe islands on W(110) with spin-polarized scanning tunneling microscopy at liquid helium temperatures. The technique aims at local detection of the spin precession as a function of frequency using [...] Read more.
We used a homodyne detection to investigate the gyration of magnetic vortex cores in Fe islands on W(110) with spin-polarized scanning tunneling microscopy at liquid helium temperatures. The technique aims at local detection of the spin precession as a function of frequency using a radio-frequency (rf) modulation of the tunneling bias voltage. The gyration was excited by the resulting spin-polarized rf current in the tunneling junction. A theoretical analysis of different contributions to the frequency-dependent signals expected in this technique is given. These include, besides the ferromagnetic resonance signal, also signals caused by the non-linearity of the I ( U ) characteristics. The vortex gyration was modeled with micromagnetic finite element methods using realistic parameters for the tunneling current, its spin polarization, and the island shape, and simulations were compared with the experimental results. The observed signals are presented and critically analyzed. Full article
(This article belongs to the Special Issue Scanning Probe Spectroscopy: From Radio- to Terahertz Frequencies)
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