Special Issue "Advances in Studies of Atmospheric Aerosol and Clouds Using Remote Sensing Techniques"
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A special issue of Atmosphere (ISSN 2073-4433).
Deadline for manuscript submissions: closed (31 October 2012)
Special Issue Editor
Guest Editor
Dr. Alexander A. Kokhanovsky
Institute of Environmental Physics, University of Bremen, Otto Hahn Allee 1, D-28234 Bremen, Germany
Website: http://www.iup.physik.uni-bremen.de/~alexk
E-Mail: alexk@iup.physik.uni-bremen.de
Interests: remote sensing; light scattering; radiative transfer; inverse problems; atmospheric optics; retrieval of aerosol and cloud properties from spaceborne observations
Special Issue Information
Dear Colleagues,
Various solid and liquid macroscopic particles (including cloud droplets and crystals) reside in atmosphere.
They interact with atmospheric gases and influence both climate and human health. Therefore, it is of importance to develop new instrumentation and improve existing techniques for the determination of particulate matter vertical columns in atmosphere. The chemical composition of aerosol particles is also of a great interest.
The main subject of this issue is to discuss recent trends and results in the area of remote sensing of atmospheric aerosol and clouds using ground, airborne, shipborne, and satellite optical instrumentation (in particular, spectrometers and radiometers). This requires the solution of inverse problem of the radiative transfer theory. Therefore, the papers dealing with various aspects of light scattering and radiative transfer in atmosphere are particularly welcome.
Dr. Alexander A. Kokhanovsky
Guest Editor
Submission
Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. Papers will be published continuously (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.
Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are refereed through a peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Atmosphere is an international peer-reviewed Open Access quarterly journal published by MDPI.
Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 300 CHF (Swiss Francs).
English correction and/or formatting fees of 250 CHF (Swiss Francs) will be charged in certain cases for those articles accepted for publication that require extensive additional formatting and/or English corrections.
Keywords
- aerosol
- cloud
- remote sensing
- light scattering
- radiative transfer
- inverse problem
- underlying surface reflectance
- atmospheric correction
Published Papers (7 papers)
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Received: 1 August 2012; in revised form: 20 September 2012 / Accepted: 26 September 2012 / Published: 10 October 2012
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Abstract: This paper presents a new version of radiative transfer model called the Fast Line-by-Line Model (FLBLM), which is based on the Line-by-Line (LbL) and Monte Carlo (MC) methods and rigorously treats particulate and molecular scattering alongside absorption. The advantage of this model consists in the use of the line-by-line model that allows for the computing of high-resolution spectra quite quickly. We have developed the model by taking into account the polarization state of light and carried out some validations by comparison against benchmark results. FLBLM calculates the Stokes parameters spectra of shortwave radiation in vertically inhomogeneous atmospheres. This update makes the model applicable for the assessment of cloud and aerosol influence on radiances as measured by the SW high-resolution polarization spectrometers. In sample results we demonstrate that the high-resolution spectra of the Stokes parameters contain more detailed information about clouds and aerosols than the medium- and low-resolution spectra wherein lines are not resolved. The presented model is rapid enough for many practical applications (e.g., validations) and might be useful especially for the remote sensing. FLBLM is suitable for development of the reliable technique for retrieval of optical and microphysical properties of clouds and aerosols from high-resolution satellites data.
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Received: 13 June 2012; in revised form: 27 August 2012 / Accepted: 21 September 2012 / Published: 17 October 2012
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Abstract: The possible interaction and modification of cloud properties due to aerosols is one of the most poorly understood mechanisms within climate studies, resulting in the most significant uncertainty as regards radiation budgeting. In this study, we explore direct ground based remote sensing methods to assess the Aerosol-Cloud Indirect Effect directly, as space-borne retrievals are not directly suitable for simultaneous aerosol/cloud retrievals. To illustrate some of these difficulties, a statistical assessment of existing multispectral imagers on geostationary (e.g., GOES)/Moderate Resolution Imaging Spectroradiometer (MODIS) satellite retrievals of the Cloud Droplet Effective Radius (Reff) showed significant biases especially at larger solar zenith angles, further motivating the use of ground based remote sensing approaches. In particular, we discuss the potential of using a combined Microwave Radiometer (MWR)—Multi-Filter Rotating Shadowband Radiometer (MFRSR) system for real-time monitoring of Cloud Optical Depth (COD) and Cloud Droplet Effective Radius (Reff), which are combined with aerosol vertical properties from an aerosol lidar. An iterative approach combining the simultaneous observations from MFRSR and MWR are used to retrieve the COD and Reff for thick cloud cases and are extensively validated using the DoE Southern Great Plains (SGP) retrievals as well as regression based parameterized model retrievals. In addition, we account for uncertainties in background aerosol, surface albedo and the combined measurement uncertainties from the MWR and MFRSR in order to provide realistic uncertainty estimates, which is found to be ~10% for the parameter range of interest in Aerosol-Cloud Interactions. Finally, we analyze a particular case of possible aerosol-cloud interaction described in the literature at the SGP site and demonstrate that aerosol properties obtained at the surface can lead to inconclusive results in comparison to lidar-derived aerosol properties near the cloud base.
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Received: 25 July 2012; in revised form: 17 September 2012 / Accepted: 9 October 2012 / Published: 24 October 2012
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Abstract: The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) being developed for airborne measurements will offer retrievals of aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. In this study, we assess the expected accuracy of the 4STAR-based aerosol retrieval and its sensitivity to major sources of anticipated perturbations in the 4STAR measurements. The major anticipated perturbations are (1) an apparent enhancement of sky radiance at small scattering angles associated with the necessarily compact design of the 4STAR and (2) an offset (i.e., uncertainty) of sky radiance calibration independent of scattering angle. The assessment is performed through application of the operational AERONET aerosol retrieval and constructed synthetic 4STAR-like data. Particular attention is given to the impact of these perturbations on the broadband fluxes and the direct aerosol radiative forcing. The results from this study suggest that limitations in the accuracy of 4STAR-retrieved particle size distributions and scattering phase functions have diminished impact on the accuracy of retrieved bulk microphysical parameters, permitting quite accurate retrievals of properties including the effective radius (up to 10%, or 0.03), and the radiatively important optical properties, such as the asymmetry factor (up to 4%, or ±0.02) and single-scattering albedo (up to 6%, or ±0.04). Also, the obtained results indicate that the uncertainties in the retrieved aerosol optical properties are quite small in the context of the calculated fluxes and direct aerosol radiative forcing (up to 15%, or 3 W∙m−2).
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Received: 25 October 2012; in revised form: 8 December 2012 / Accepted: 13 December 2012 / Published: 18 December 2012
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Abstract: Accurate characterization of surface reflection is essential for retrieval of aerosols using downward-looking remote sensors. In this paper, observations from the Ground-based Multiangle SpectroPolarimetric Imager (GroundMSPI) are used to evaluate a surface polarized bidirectional reflectance distribution function (PBRDF) model. GroundMSPI is an eight-band spectropolarimetric camera mounted on a rotating gimbal to acquire pushbroom imagery of outdoor landscapes. The camera uses a very accurate photoelastic-modulator-based polarimetric imaging technique to acquire Stokes vector measurements in three of the instrument’s bands (470, 660, and 865 nm). A description of the instrument is presented, and observations of selected targets within a scene acquired on 6 January 2010 are analyzed. Data collected during the course of the day as the Sun moved across the sky provided a range of illumination geometries that facilitated evaluation of the surface model, which is comprised of a volumetric reflection term represented by the modified Rahman-Pinty-Verstraete function plus a specular reflection term generated by a randomly oriented array of Fresnel-reflecting microfacets. While the model is fairly successful in predicting the polarized reflection from two grass targets in the scene, it does a poorer job for two manmade targets (a parking lot and a truck roof), possibly due to their greater degree of geometric organization. Several empirical adjustments to the model are explored and lead to improved fits to the data. For all targets, the data support the notion of spectral invariance in the angular shape of the unpolarized and polarized surface reflection. As noted by others, this behavior provides valuable constraints on the aerosol retrieval problem, and highlights the importance of multiangle observations.

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Received: 31 October 2012; in revised form: 4 February 2013 / Accepted: 19 February 2013 / Published: 28 February 2013
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Abstract: A smoke plume originating from the massive wildfires near Moscow was clearly detected in northern Finland on 30 July 2010. Measurements made with remote sensing instruments demonstrated how the biomass burning aerosols affected the chemical and optical characteristics of the atmosphere in regions hundreds of kilometers away from the actual fires. In this study, we used MODIS, AIRS, CALIOP, PFR, ceilometers, FTS and Brewer data to quantify the properties of the transported smoke plume. In addition, in situ measurements of aerosol concentration (DMPS), absorption (aethalometer) and scattering (nephelometer) are presented. We found that due to the smoke plume in northern Finland, the daily averaged optical thickness of aerosols increased fourfold, and MODIS retrieved AOD as high as 4.5 for the thickest part of the plume. FTS measurements showed that CO concentration increased by 100% during the plume. CALIOP and ceilometer measurements revealed that the smoke plume was located close to the surface, below 3 km, and that the plume was not homogeneously mixed. In addition, in situ measurements showed that the scattering and absorption coefficients were almost 20 times larger in the smoke plume than on average, and that the number of particles larger than 320 nm increased 14-fold. Moreover, a comparison with in situ measurements recorded in eastern Finland on the previous day showed that the transport from eastern to northern Finland decreased the scattering coefficient, black carbon concentration, and total number concentration 0.5%/h, 1.5%/h and 2.0%/h, respectively.
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Received: 2 November 2012; in revised form: 26 February 2013 / Accepted: 26 February 2013 / Published: 5 March 2013
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Abstract: Thanks to its observational frequency of 15 min, the Meteosat Second Generation (MSG) geostationary satellite offers a great potential to monitor dust storms. To explore this potential, an algorithm for the detection and the retrieval of dust aerosol optical properties has been tested. This is a multispectral algorithm based on visible and infrared data which has been applied to 15 case studies selected between 2007 and 2011. The algorithm has been validated in the latitude–longitude box between 30 and 50 degrees north, and −10 and 20 degrees east, respectively. Hereafter we present the obtained results that have been validated against Aerosol Robotic Network (AERONET) ground-based measurements and compared with the retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) on NASA’s Terra and Aqua satellites. The dust aerosol optical depth variations observed at the AERONET sites are well reproduced, showing good correlation of about 0.77, and a root mean square difference within 0.08, and the spatial patterns retrieved by using the algorithm developed are in agreement with those observed by MODIS.

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Received: 19 December 2012; in revised form: 7 March 2013 / Accepted: 13 March 2013 / Published: 19 March 2013
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Abstract: This paper presents an approach using the GEneralized Nonlinear Retrieval Analysis (GENRA) tool and general inverse theory diagnostics including the maximum likelihood solution and the Shannon information content to investigate the performance of a new spectral technique for the retrieval of cloud optical properties from surface based transmittance measurements. The cumulative retrieval information over broad ranges in cloud optical thickness (τ), droplet effective radius (re), and overhead sun angles is quantified under two conditions known to impact transmitted radiation; the variability in land surface albedo and atmospheric water vapor content. Our conclusions are: (1) the retrieved cloud properties are more sensitive to the natural variability in land surface albedo than to water vapor content; (2) the new spectral technique is more accurate (but still imprecise) than a standard approach, in particular for τ between 5 and 60 and re less than approximately 20 μm; and (3) the retrieved cloud properties are dependent on sun angle for clouds of from 5 to 10 and re < 10 μm, with maximum sensitivity obtained for an overhead sun.

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Last update: 25 September 2012