Study of Air Pollution Based on Remote Sensing

Two severe dust storm (DS) events (15–17 March and 28–29 March) hit northern China in 2021 consecutively. The lower atmospheric vertical dynamic and thermal structures during the two cases were compared using the ground-based sensor data from the microwave radiometer and radar wind profiler, combined with the environmental and meteorological observations data in Jinan, China. It was found that both cases occurred under the background of cold vortexes over northeastern China. The dust was transported through the cold air on the northwest route. During the dust period, 2–3 km was the west or northwest airflow, and below 2 km was the northeast wind. The variation in the dynamic structure determined the duration of the DS. During the DS maintenance phase, the vertical wind shear (VWS) below 3 km measured approximately 10 m∙(s∙km)⁻¹. The increased VWS during the dust intrusion period facilitated the transportation of dust. In contrast, the more significant VWS was not conducive to the maintenance of DS, and the shift to south wind control in the upper middle layer indicated the weakening of DS. In both cases, we observed a cliff-like decrease in relative humidity as a prominent indicator of dust outbreaks, occurring approximately 2–5 h beforehand. The diurnal difference between the vertical temperature and relative humidity during the dust maintenance period was found to be insignificant. Full article

Aerosol optical depth (AOD) is an important physical variable used to characterize atmospheric turbidity for the management and control of air pollution. This study aims to analyze the factors influencing the spatial and temporal variability in AOD across the arid region of Northwest China (ARNC) using MODIS Aqua C006 aerosol product data from 2008 to 2017. In terms of natural and socioeconomic factors, the correlation coefficient (R) was used to identify the most influential factor in the AOD changes. The results show that AOD values in spring and summer were much higher than those in autumn and winter, especially in spring. In general, AOD had an insignificant decreasing trend, with a small overall changing range. Spatial analysis revealed a significantly decreasing trend, mostly across the Gobi Desert area, which is located in the western region of the ARNC. From the perspective of natural factors, AOD was positively correlated with air temperature (AT), wind speed (WP), land surface temperature (LST), and the digital elevation model (DEM) and negatively correlated with precipitation, relative humidity (RH), and the normalized difference vegetation index (NDVI). The greatest positive correlation, with a maximum R value of 0.8, was found between AOD and wind speed. By contrast, AOD and relative humidity had the strongest negative correlation, with R values of −0.77. In terms of anthropogenic factors, gross domestic product (GDP), secondary industry, and population density were the three major anthropogenic factors that influenced the changes in AOD changes in this region. In general, the effects of anthropogenic factors on AOD are more significant in areas with high urban population densities. Full article

A long-term vertical ozone observational dataset has been provided during 2001–2019 by ozonesonde measurements in Beijing on the North China Plain. Previous studies using this dataset primarily focused on the vertical characteristics of climatological ozone and its variation; however, the driving factors of ozone variation have not been well discussed. In this study, by applying the wavelet analysis method (including continuous wavelet transform and cross wavelet) and sliding correlation coefficients to ~20 years of ozonesonde measurements collected in Beijing, we analyzed the dominant modes of ozone column variability within three height ranges over Beijing (total column ozone: TOT; stratospheric column ozone: SCO; and tropospheric column ozone: TCO). Moreover, we also preliminarily discussed the relationship between these three ozone columns and the El Niño Southern Oscillation (ENSO), Quasi-biennial Oscillation (QBO), and 11-year solar activity cycle. The results revealed that the ozone columns within the three height ranges predominantly adhered to interannual variability patterns, and the short-term variabilities in TOT and SCO may have been related to eruptive volcanic activity. In comparison to the TOT and SCO, the TCO was more susceptible to the forcing influences of high-frequency factors such as pollutant transport. Similar to the results in other mid-latitude regions, strong ENSO and QBO signals were revealed in the interannual ozone column variability over Beijing. The TOT and SCO showed positive anomalous responses to ENSO warm-phase events, and the peak of the ENSO warm phase led the winter peaks of the TOT and SCO by approximately 3–6 months. During the strong cold–warm transition phase in 2009–2012, the TOT and SCO showed a significant positive correlation with the ENSO index. The strong seasonality of the meridional circulation process driven by the QBO led to a significant positive correlation between the QBO index and the TOT and SCO in the interannual cycle, except for two periods of abnormal QBO fluctuations in 2010–2012 and 2015–2017, whereas the TCO showed a time-lagged correlation of approximately 3 months in the annual cycle relative to the QBO due to the influence of the thermodynamic tropopause. In addition, analysis of the F10.7 index and the ozone columns revealed that the ozone columns over Beijing exhibited lagged responses to the peaks of sunspot activity, and there was no obvious correlation between ozone columns and 11-year solar activity cycle. Given the complex driving mechanism of the climatic factors on local ozone variability, the preliminary results obtained in this study still require further validation using longer time series of observational data and the combination of chemical models and more auxiliary data. Full article

In recent years, the concentration of surface ozone (O₃) has increased in China. The formation regime of ozone is closely related to the ratio of volatile organic compounds (VOCs) to nitrogen oxides (NO_x). To explain this increase in ozone, we determined the sensitivity of ozone generation by determining the regional threshold of the ratio of formaldehyde to nitrogen dioxide (HCHO/NO₂) in the satellite troposphere. The different FNR(HCHO/NO₂) ratio ranges indicate three formation regimes: VOC limited, transitional, and NO_x limited. Polynomial fitting models were used to determine the threshold range for the transitional regime in the BTH region (2.0, 3.1). The ozone formation regime in the BTH (Beijing–Tianjin–Hebei) region mainly exhibited a transitional and NO_x-limited regime. VOC-limited regimes are mainly distributed in urban agglomeration areas, transitional regimes are mainly concentrated in urban expansion areas, and non-urban areas are mainly controlled by NO_x. The concentrations of HCHO and NO₂ in the BTH region showed a trend of urban agglomeration areas > urban expansion areas > non-urban areas in different land types from 2019 to 2022, whereas the FNR showed an opposite trend. Full article

Imported air pollution has a significant impact on urban air quality. Relevant studies have shown that many urban air pollution events are not resourced by local emissions but are imported by air pollution from surrounding areas transported across regions. The prevention and control of air pollution is very necessary. However, the existing supervision of urban air quality mostly relies on ground monitoring stations, which are extremely limited in time and space, and cannot satisfy continuous time-space air pollution research. Therefore, aiming at the problem of urban air pollution control, this paper used MERRA-2 reanalysis data and ground monitoring data to establish a “Time-Longitude-Latitude” three-dimensional pollution curve, and then a genetic algorithm was used to optimize its fitting. This study finally reconstructed the imported air pollution transmission route. This paper takes an air pollution event that occurred in Xuzhou City, China, on 12 January 2020, as an example. Through the analysis of aerosol optical depth (AOD), particulate matter (PM), wind speed, and other factors, we found the source, transmission route, and impact time of this pollution. We have verified the correctness and accuracy of the reconstructed contamination transport paths. It is proved that the method is universal and it can quickly and accurately restore the air pollution transmission route and identify the urban imported air pollution transmission entrance. This method will also provide strong data support for the division of responsibilities of environmental protection departments in various regions for severe air pollution transmission events and provide effective governance ideas for the prevention and control of imported air pollution in recipient cities. Full article