Table of Contents
Magnetochemistry, Volume 3, Issue 3 (September 2017)
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Cover Story (view full-size image) The local magnetic susceptibility tensor of the cubane cluster [Ni4(L)4(MeOH)4], where H2L = [...] Read more. The local magnetic susceptibility tensor of the cubane cluster [Ni4(L)4(MeOH)4], where H2L = salicylidene-2-ethanolamine; MeOH = methanol, was fully determined by Polarized Neutron Diffraction (PND) on single crystal. Two molecular orientations coexist in the monoclinic cell and therefore angular-resolved magnetometry cannot provide information on the local molecular anisotropy but on the crystal magnetic anisotropy only. In the weak magnetic exchange limit, PND also gives access to the local magnetic anisotropy of each Ni(II) ion and of the antiferromagnetic pairs they form. We show that one of the two antiferromagnetic pairs in the cluster presents stronger easy-axis type anisotropy than the other. View this paper