As(V) and P Competitive Sorption on Soils, By-Products and Waste Materials
Abstract
:1. Introduction
2. Material and Methods
2.1. Materials
Parameter | Forest Soil | Vineyard Soil | Pyritic Material | Granitic Material | Coarse Shell | Fine Shell | Shell Ash | Pine-Sawdust | Slate Fines |
---|---|---|---|---|---|---|---|---|---|
C (%) | 4.22 | 2.94 | 0.26 | 0.11 | 12.67 | 11.43 | 13.21 | 46.13 | 0.2 |
N (%) | 0.33 | 0.23 | 0.04 | 0.04 | 0.36 | 0.21 | 1.13 | 0.03 | 0.02 |
pHwater | 5.65 | 4.48 | 2.97 | 5.72 | 9.11 | 9.39 | 12.54 | 4.91 | 8.61 |
Cae (cmol·kg−1) | 4.37 | 1.78 | 0.36 | 0.18 | 12.64 | 24.75 | 39.27 | 5.39 | 4.31 |
Mge (cmol·kg−1) | 0.66 | 0.24 | 0.29 | 0.13 | 0.58 | 0.72 | 7.47 | 1.37 | 0.31 |
Nae (cmol·kg−1) | 0.33 | 0.14 | 0.14 | 0.27 | 5.24 | 4.37 | 19.92 | 0.66 | 0.63 |
Ke (cmol·kg−1) | 0.60 | 0.83 | 0.24 | 0.31 | 0.31 | 0.38 | 2.61 | 1.55 | 0.31 |
Ale (cmol·kg−1) | 1.92 | 2.28 | 2.86 | 1.63 | 0.04 | 0.03 | 0 | 0.05 | 0.01 |
CICe (cmol·kg−1) | 7.88 | 5.27 | 3.89 | 2.53 | 18.82 | 30.25 | 69.28 | 9.02 | 5.57 |
POlsen (mg·kg−1) | 28.80 | 147.64 | 8.80 | 2.56 | 23.21 | 54.17 | 534.6 | 11.47 | 0.93 |
PT (mg·kg−1) | 423.9 | 679.3 | 606.3 | 88.62 | 186.5 | 101.5 | 1617 | 88.04 | 661.3 |
CaT (mg·kg−1) | 708.5 | 607.1 | 603 | <0.01 | 298,085 | 280,168 | 247,859 | 8088 | 2810 |
MgT (mg·kg−1) | 830.5 | 5003 | 8384 | 355 | 1020 | 980.6 | 5286 | 164.4 | 11,797 |
NaT (mg·kg−1) | 515.1 | 297.6 | 412 | 102 | 5508 | 5173 | 8074 | 98.35 | 53.72 |
KT (mg·kg−1) | 1544 | 5441 | 3186 | 1434 | 80.57 | 202.1 | 896 | 540.7 | 991.3 |
AsT (mg·kg−1) | 4.18 | 3.41 | 7 | 3 | 0.48 | 1.12 | 1.71 | 0.39 | 3.1 |
CdT (mg·kg−1) | 0.43 | 0.14 | 0.08 | <0.001 | 0.02 | 0.07 | 63.09 | 50.82 | 95.18 |
CrT (mg·kg−1) | 18.35 | 41.44 | 99 | 3 | 1.32 | 4.51 | 4596 | 234.2 | 54,010 |
CuT (mg·kg−1) | 15.72 | 521.1 | 773 | 7 | 3.20 | 6.72 | 31.75 | 14.87 | 30.95 |
NiT (mg·kg−1) | 10.69 | 21.73 | 5 | 1 | 5.64 | 8.16 | 3421 | 260.6 | 24,737 |
ZnT (mg·kg−1) | 36.74 | 49.57 | 58 | 18 | 7.71 | 7.66 | 18.75 | 0 | 36.89 |
MnT (mg·kg−1) | 92.99 | 305.4 | 296 | 24 | 5.70 | 33.75 | 18.67 | 5.19 | 28.46 |
AlT (mg·kg−1) | 22,676 | 25,664 | 9624 | 5981 | 93.89 | 433.2 | 3421 | 260.7 | 24,737 |
FeT (mg·kg−1) | 9486 | 21,284 | 135,157 | 3505 | 170.37 | 1855 | 4596 | 234.2 | 54,010 |
Alo (mg·kg−1) | 4275 | 2003 | 563 | 1425 | 85.00 | 178.3 | 1733 | 112.5 | 730.6 |
Feo (mg·kg−1) | 2333 | 1239 | 41,860 | 224 | 42.67 | 171.0 | 1659 | 15.62 | 1256 |
2.2. Methods
2.2.1. Characterization of the Materials Used
2.2.2. As(V) and P Competitive Sorption
3. Results
3.1. Sorbed As When a Constant P Concentration and Increasing As Concentrations Are Added, and Sorbed P When a Constant As Concentration and Increasing P Concentrations Are Added
3.2. As and P Sorbed in the Absence or in the Presence of Each Other
4. Discussion
4.1. As and P Competition
4.2. Implications of the Study
5. Conclusions
Acknowledgments
Author Contributions
Conflicts of Interest
References
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Rivas-Pérez, I.M.; Paradelo-Núñez, R.; Nóvoa-Muñoz, J.C.; Arias-Estévez, M.; Fernández-Sanjurjo, M.J.; Álvarez-Rodríguez, E.; Núñez-Delgado, A. As(V) and P Competitive Sorption on Soils, By-Products and Waste Materials. Int. J. Environ. Res. Public Health 2015, 12, 15706-15715. https://doi.org/10.3390/ijerph121215016
Rivas-Pérez IM, Paradelo-Núñez R, Nóvoa-Muñoz JC, Arias-Estévez M, Fernández-Sanjurjo MJ, Álvarez-Rodríguez E, Núñez-Delgado A. As(V) and P Competitive Sorption on Soils, By-Products and Waste Materials. International Journal of Environmental Research and Public Health. 2015; 12(12):15706-15715. https://doi.org/10.3390/ijerph121215016
Chicago/Turabian StyleRivas-Pérez, Ivana María, Remigio Paradelo-Núñez, Juan Carlos Nóvoa-Muñoz, Manuel Arias-Estévez, María José Fernández-Sanjurjo, Esperanza Álvarez-Rodríguez, and Avelino Núñez-Delgado. 2015. "As(V) and P Competitive Sorption on Soils, By-Products and Waste Materials" International Journal of Environmental Research and Public Health 12, no. 12: 15706-15715. https://doi.org/10.3390/ijerph121215016