Coordination-Driven Controlled Assembly of Polyphenol-Metal Green Coating on Wood Micro-Grooved Surfaces: A Novel Approach to Stable Superhydrophobicity
Abstract
:1. Introduction
2. Materials and Methods
2.1. Materials
2.2. Preparation of Superhydrophobic Surfaces on Wood Substrate
2.3. Characterizations
2.3.1. Micromorphology Analysis
2.3.2. Chemical Composition Analysis
2.3.3. Characterization of Superhydrophobic Properties
2.3.4. Characterization of Superhydrophobic Stabilities
3. Results and Discussion
3.1. Preparation Process and Reaction Mechanism
3.2. Micromorphology and Chemical Composition Analysis
3.3. Superhydrophobic Properties
3.4. Superhydrophobic Model Establishment
4. Conclusions
- The TA–FeIII complexes employed as a molecular building block for anchoring biomimetic coatings onto substrates also act as stable bridges between the substrate and hydrophobic groups. They also affect the reducibility of Ag nanoparticles, which endow the TA–FeIII complex coating with micro/nanostructure hierarchical roughness.
- The thickness and architecture of the TA–FeIII complex coating can be tailored by coordination-driven multistep assembly. The coating can fully cover the original substrate surface, even quite rugged surfaces with a large area, preventing any damage to the superhydrophobic performance due to uncoated hydrophilic substrates exposed on the surface.
- The whole procedure can be conducted under mild, eco-friendly conditions without destroying the substrate’s intrinsic structures or components.
- The TA–FeIII coordination process is fast, simple, versatile, and the raw materials are readily available and low in cost.
- The bionic-prepared superhydrophobic surfaces showed excellent stability and durability in harsh conditions.
Acknowledgments
Author Contributions
Conflicts of Interest
References
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Wang, K.; Wang, Z.; Dong, Y.; Zhang, S.; Li, J. Coordination-Driven Controlled Assembly of Polyphenol-Metal Green Coating on Wood Micro-Grooved Surfaces: A Novel Approach to Stable Superhydrophobicity. Polymers 2017, 9, 347. https://doi.org/10.3390/polym9080347
Wang K, Wang Z, Dong Y, Zhang S, Li J. Coordination-Driven Controlled Assembly of Polyphenol-Metal Green Coating on Wood Micro-Grooved Surfaces: A Novel Approach to Stable Superhydrophobicity. Polymers. 2017; 9(8):347. https://doi.org/10.3390/polym9080347
Chicago/Turabian StyleWang, Kaili, Zhong Wang, Youming Dong, Shifeng Zhang, and Jianzhang Li. 2017. "Coordination-Driven Controlled Assembly of Polyphenol-Metal Green Coating on Wood Micro-Grooved Surfaces: A Novel Approach to Stable Superhydrophobicity" Polymers 9, no. 8: 347. https://doi.org/10.3390/polym9080347