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12 pages, 4072 KiB  
Article
Saharan Dust Contributions to PM10 Levels in Hungary
by Anita Tóth and Zita Ferenczi
Air 2024, 2(3), 325-336; https://doi.org/10.3390/air2030019 - 5 Sep 2024
Viewed by 1406
Abstract
There are meteorological situations when huge amounts of Saharan dust are transported from Africa to Europe. These natural dust events may have a significant impact on particulate matter concentrations at monitoring sites. This phenomenon affects mainly the countries in Southern Europe; however, some [...] Read more.
There are meteorological situations when huge amounts of Saharan dust are transported from Africa to Europe. These natural dust events may have a significant impact on particulate matter concentrations at monitoring sites. This phenomenon affects mainly the countries in Southern Europe; however, some strong advections can bring Saharan dust to higher latitudes too. The number of Saharan dust events in the Carpathian Basin is believed to increase due to the changing patterns in the atmospheric circulation over the Northern Hemisphere’s mid-latitudes. The jet stream becomes more meandering if the temperature difference between the Arctic areas and the lower latitudes decreases. This favours the northward transport of the North African dust. The European regulation makes it possible to subtract the concentration of Saharan-originated aerosol from the measured PM10 concentration. This manuscript describes the methodology used by the HungaroMet to calculate the amount of natural dust contributing to measured PM10 concentrations. Full article
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18 pages, 4152 KiB  
Article
Distinguishing Saharan Dust Plume Sources in the Tropical Atlantic Using Elemental Indicators
by Daniel E. Yeager and Vernon R. Morris
Atmosphere 2024, 15(5), 554; https://doi.org/10.3390/atmos15050554 - 30 Apr 2024
Viewed by 2305
Abstract
The Sahara Desert is the largest contributor of global atmospheric dust aerosols impacting regional climate, health, and ecosystems. The climate effects of these dust aerosols remain uncertain due, in part, to climate model uncertainty of Saharan source region contributions and aerosol microphysical properties. [...] Read more.
The Sahara Desert is the largest contributor of global atmospheric dust aerosols impacting regional climate, health, and ecosystems. The climate effects of these dust aerosols remain uncertain due, in part, to climate model uncertainty of Saharan source region contributions and aerosol microphysical properties. This study distinguishes source region elemental signatures of Saharan dust aerosols sampled during the 2015 Aerosols Ocean Sciences Expedition (AEROSE) in the tropical Atlantic. During the 4-week campaign, cascade impactors size-dependently collected airborne Saharan dust particulate upon glass microfiber filters. Inductively Coupled Plasma Mass Spectrometry (ICP-MS) analysis differentiated metal isotope concentrations within filter samples from various AEROSE dust sampling periods. Back-trajectory analysis and NOAA satellite aerosol optical depth retrievals confirmed source regions of AEROSE ’15 dust samples. Pearson correlational statistics of source region activity and dust isotope concentrations distinguished the elemental signatures of North African potential source areas (PSAs). This study confirmed that elemental indicators of these PSAs remain detectable within dust samples collected far into the marine boundary layer of the tropical Atlantic. Changes detected in dust elemental indicators occurred on sub-weekly timescales across relatively small sampling distances along the 23W parallel of the tropical Atlantic. PSA-2 emissions, covering the western coast of the Sahara, were very strongly correlated (R2 > 0.79) with Ca-44 isotope ratios in AEROSE dust samples; PSA-2.5 emissions, covering eastern Mauritania and western Mali, were very strongly correlated with K-39 ratios; PSA-3 emissions, spanning southwestern Algeria and eastern Mali, were very strongly correlated with Fe-57 and Ti-48 ratios. The abundance of Ca isotopes from PSA-2 was attributed to calcite minerals from dry lakebeds and phosphorous mining activities in Western Sahara, based on source region analysis. The correlation between K isotope ratios and PSA-2.5 was a likely indicator of illite minerals near the El Djouf Desert region, according to corroboration with mineral mapping studies. Fe and Ti ratio correlations with PSA-3 observed in this study were likely indicators of iron and titanium oxides from Sahelian sources still detectable in Atlantic Ocean observations. The rapid changes in isotope chemistry found in AEROSE dust samples provide a unique marker of Saharan source regions and their relative contributions to desert outflows in the Atlantic. These elemental indicators provide source region apportionments of Sahara Desert aerosol flux and deposition into the Atlantic Ocean, as well as a basis for model and satellite validation of Saharan dust emissions for regional climate assessments. Full article
(This article belongs to the Section Aerosols)
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7 pages, 5367 KiB  
Proceeding Paper
Effect of Dust Events on Photovoltaics Electricity Production in the European and North African Regions
by Davender Sethi and Panagiotis G. Kosmopoulos
Environ. Sci. Proc. 2023, 26(1), 8; https://doi.org/10.3390/environsciproc2023026008 - 23 Aug 2023
Cited by 3 | Viewed by 1190
Abstract
The effect of two dust events on solar energy has been studied in Europe and North Africa. For analysis, total aerosol and dust optical depth (AOD) in conjunction with solar irradiation and energy data were utilized from Copernicus Atmosphere Monitoring Service (CAMS). The [...] Read more.
The effect of two dust events on solar energy has been studied in Europe and North Africa. For analysis, total aerosol and dust optical depth (AOD) in conjunction with solar irradiation and energy data were utilized from Copernicus Atmosphere Monitoring Service (CAMS). The AOD reached ~2.8 and ~1.7 during the dust events (16–19 April 2021 and 15–18 March 2022), respectively. Both events originated in North Africa, reaching the northern parts of Europe and the Black Sea. The energy production of solar photovoltaics in the affected regions was reduced by almost 18–36 GWh, followed by an estimated financial loss of close to 4 million euros. Full article
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22 pages, 13693 KiB  
Article
Machine Learning-Based Improvement of Aerosol Optical Depth from CHIMERE Simulations Using MODIS Satellite Observations
by Farouk Lemmouchi, Juan Cuesta, Mathieu Lachatre, Julien Brajard, Adriana Coman, Matthias Beekmann and Claude Derognat
Remote Sens. 2023, 15(6), 1510; https://doi.org/10.3390/rs15061510 - 9 Mar 2023
Cited by 9 | Viewed by 4278
Abstract
We present a supervised machine learning (ML) approach to improve the accuracy of the regional horizontal distribution of the aerosol optical depth (AOD) simulated by the CHIMERE chemistry transport model over North Africa and the Arabian Peninsula using Moderate Resolution Imaging Spectroradiometer (MODIS) [...] Read more.
We present a supervised machine learning (ML) approach to improve the accuracy of the regional horizontal distribution of the aerosol optical depth (AOD) simulated by the CHIMERE chemistry transport model over North Africa and the Arabian Peninsula using Moderate Resolution Imaging Spectroradiometer (MODIS) AOD satellite observations. Our method produces daily AOD maps with enhanced precision and full spatial domain coverage, which is particularly relevant for regions with a high aerosol abundance, such as the Sahara Desert, where there is a dramatic lack of ground-based measurements for validating chemistry transport simulations. We use satellite observations and some geophysical variables to train four popular regression models, namely multiple linear regression (MLR), random forests (RF), gradient boosting (XGB), and artificial neural networks (NN). We evaluate their performances against satellite and independent ground-based AOD observations. The results indicate that all models perform similarly, with RF exhibiting fewer spatial artifacts. While the regression slightly overcorrects extreme AODs, it remarkably reduces biases and absolute errors and significantly improves linear correlations with respect to the independent observations. We analyze a case study to illustrate the importance of the geophysical input variables and demonstrate the regional significance of some of them. Full article
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20 pages, 5325 KiB  
Review
Impact of North African Sand and Dust Storms on the Middle East Using Iraq as an Example: Causes, Sources, and Mitigation
by Salih Muhammad Awadh
Atmosphere 2023, 14(1), 180; https://doi.org/10.3390/atmos14010180 - 13 Jan 2023
Cited by 47 | Viewed by 9911
Abstract
This study aims to determine the reasons for the increase in the frequency of sand and dust storms in the Middle East and to identify their sources and mitigate them. A set of climatic data from 60 years (1960–2022) was analyzed. Sand storms [...] Read more.
This study aims to determine the reasons for the increase in the frequency of sand and dust storms in the Middle East and to identify their sources and mitigate them. A set of climatic data from 60 years (1960–2022) was analyzed. Sand storms in Iraq are a silty sand mature arkose composed of 72.7% sand, 25.1% silt, and 2.19% clay; the clay fraction in dust storms constitutes 70%, with a small amount of silt (20.6%) and sand (9.4%). Dust and sand storms (%) are composed of quartz (49.2, 67.1), feldspar (4.9, 20.9), calcite (38, 5), gypsum (4.8, 0.4), dolomite (0.8, 1.0), and heavy minerals (3.2, 6.6). Increasing temperatures in Iraq, by an average of 2 °C for sixty years, have contributed to an increase in the number of dust storms from 75 to 200 times annually. North African storms affect the Middle East, with a monthly average exceeding 300 g/m3 in peak dust seasons. To reduce the negative impacts on public health, property, and infrastructure, the study suggests solutions to mitigate them, including reducing carbon dioxide gas emissions to prevent the expansion of drought and the afforestation of the desert with plants adapted to drought using advanced techniques and avoiding land overuse. Full article
(This article belongs to the Special Issue Sand and Dust Storms: Impact and Mitigation Methods)
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22 pages, 9955 KiB  
Article
Quantitative Evaluation of Dust and Black Carbon Column Concentration in the MERRA-2 Reanalysis Dataset Using Satellite-Based Component Retrievals
by Lei Li, Huizheng Che, Xin Su, Xindan Zhang, Ke Gui, Yu Zheng, Hujia Zhao, Hengheng Zhao, Yuanxin Liang, Yadong Lei, Lei Zhang, Junting Zhong, Zhili Wang and Xiaoye Zhang
Remote Sens. 2023, 15(2), 388; https://doi.org/10.3390/rs15020388 - 8 Jan 2023
Cited by 14 | Viewed by 3154
Abstract
The aerosol optical property products of Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis dataset have been extensively investigated on a global or regional scale. However, the understanding of MERRA-2 aerosol component products on an extensive temporal and spatial scale [...] Read more.
The aerosol optical property products of Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis dataset have been extensively investigated on a global or regional scale. However, the understanding of MERRA-2 aerosol component products on an extensive temporal and spatial scale is inadequate. Recently, the aerosol component products have been derived from the observations of Polarization and Directionality of the Earth’s Reflectances/Polarization and Anisotropy of Reflectance for Atmospheric Science coupled with observations from a Lidar (POLDER/PARASOL). This study presents a quantitative evaluation of the MERRA-2 reanalysis dust and black carbon (BC) column concentration using independent satellite-based aerosol component concentration retrievals. Both GRASP/Component and MERRA-2 reanalysis products can capture well the temporal variation in dust column concentration over the dust emission resource and downwind dust-dominated regions with the correlation coefficient (R) varying from 0.80 to 0.98. MERRA-2 reanalysis dust products present higher column concentration than GRASP/Component dust retrievals with relative differences of about 20~70%, except in the Taklamakan Desert and Bay of Bengal, where the relative differences can be negative. The differences in dust column concentration over the African dust regions are larger than that over the Asian dust regions. Similar temporal variations in BC column concentration are characterized by both GRASP/Component BC retrievals and MERRA-2 BC products with R of about 0.70~0.90, except in the North China Plain region. We should pay more caution with the regional applicability of MERRA-2 component products when large differences and high correlation coefficients are obtained simultaneously. The results are favorable for identifying the behavior of MERRA-2 reanalysis component estimation in a new view and demonstrate a practical application of the satellite-based component retrievals, which could make more contributions to the improvement of model estimation in the near future. Full article
(This article belongs to the Special Issue Stereoscopic Remote Sensing of Air Pollutants and Applications)
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19 pages, 23208 KiB  
Article
Atmospheric Conditions for Uplift and Dust Transport in the Latitudinal 10° North–20° North Band in Africa
by Abdoulaye Bouya Diop, Malick Wade, Abdoulaye Sy, Abdoul Karim Mbodji, Abdou Karim Farota, El hadji Deme, Babacar Niang, Bouya Diop, Amadou Thierno Gaye and Aboubakary Diakhaby
Atmosphere 2022, 13(7), 1083; https://doi.org/10.3390/atmos13071083 - 8 Jul 2022
Cited by 1 | Viewed by 2135
Abstract
Desert aerosols suspended in the atmosphere are a very marked fact in West Africa with estimates of 400 to 1000 million tons produced annually and concentrations exceeding 50 µg·m³ in Burkina. In Bamako, the daily dust concentration can go up to reach 504 [...] Read more.
Desert aerosols suspended in the atmosphere are a very marked fact in West Africa with estimates of 400 to 1000 million tons produced annually and concentrations exceeding 50 µg·m³ in Burkina. In Bamako, the daily dust concentration can go up to reach 504 µg/m³. The Sahara and the Sahel are recognized as the primary desert aerosol producing regions. Source areas continue to be discovered as the desert advances. Previous studies have mainly focused on the spatial and temporal variability of aerosols. The current question is: What makes an area a source of dust emission? Our study brings together all the climatic parameters of the 10–20 band, as well as the soil types and their characteristics; it reveals 4 soils characteristic of fine sandy semi-arid soils in Chad. The Ouadaï plateau in Chad was identified as a source area for dust emissions. We noted for JFM (January, February, March) that the strongest wind intensities were located mainly towards Chad for average rmaximum temperatures around 34.7 °C. The statistical study reveals a correlation of 66.8% between direct and indirect links between the climatic factors of the 10–20 band and the source area. The presence of vortexes throughout the year and a vertical wind profile that is among the strongest in the 10–20 band, this gradient is strongly localized in the grid “10° North, 20° North and 20° East, 30° East” next to the Kapka massif. The study shows that the AEJ (African Easterly Jet) profile, which is a strong wind, associated with the harmattan circulation, allows the transport of aerosols from Ouadaï to the West African coast. In Senegal, a significant deposition was observed. Full article
(This article belongs to the Special Issue Statistical Methods in Atmospheric Research)
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21 pages, 6486 KiB  
Article
Modification of Temperature Lapse Rates and Cloud Properties during a Spatiotemporally Extended Dust Aerosol Episode (16–18 June 2016) over the Mediterranean Basin Based on Satellite and Reanalysis Data
by Maria Gavrouzou, Nikolaos Hatzianastassiou, Christos J. Lolis, Marios-Bruno Korras-Carraca and Nikolaos Mihalopoulos
Remote Sens. 2022, 14(3), 679; https://doi.org/10.3390/rs14030679 - 31 Jan 2022
Cited by 2 | Viewed by 2557
Abstract
A spatiotemporally extended dust aerosol episode that occurred over the Mediterranean Basin (MB) from 16 to 18 June 2016 is investigated using observational satellite and reanalysis data, focusing on the effects of high dust loads on cloud formation and temperature fields, including the [...] Read more.
A spatiotemporally extended dust aerosol episode that occurred over the Mediterranean Basin (MB) from 16 to 18 June 2016 is investigated using observational satellite and reanalysis data, focusing on the effects of high dust loads on cloud formation and temperature fields, including the creation of temperature inversions. The atmospheric conditions before and during the 3-day dust aerosol episode case (DAEC) are also analyzed. The dust episode, which is identified using a contemporary satellite algorithm, consists of long-range transport of African dust to the western and central MB. The day to day, before and during the DAEC, atmospheric circulation, dust-cloud interactions, and dust effect on temperature are examined using a variety of Moderate Resolution Imaging Spectroradiometer (MODIS) Level-3 Collection 6.1 satellite and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) reanalysis data. According to the obtained results, the dust export from N. Africa, which occurs under the prevalence of a trough over the western MB, and a ridge over the central MB, extends from southwest to northeast along two axes, one in the western and another in the central Mediterranean, covering remote areas up to the coasts of southern Europe, including the Balearic and Tyrrhenian Seas, the Italian peninsula, the Ionian and Adriatic Seas, and the Balkan peninsula. The analysis provides evidence of the formation of mixed-phase clouds, with high cloud-top heights (CTH higher than 10 km) and low cloud-top temperatures (CTT as low as 230 K), which spatiotemporally coincide with the high dust loadings that provide the necessary CCN and IN. Dust aerosols are transported either in the boundary layer (within the first 1–2 km) of areas close to the North African dust source areas or in the free troposphere over the Mediterranean Sea and the Italian and Balkan peninsulas (between 2 and 8 km). Distinct and extended layers of remarkable temperature inversions (up to 20 K/km) are created below the exported dust layers in the boundary layer of Mediterranean Sea areas, while weak/reduced lapse rates are formed over continental areas of MB undergoing the dust transport. Such modifications of temperature fields are important for the dynamics of the atmosphere of MB. Full article
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25 pages, 6298 KiB  
Article
Model Sensitivity Study of the Direct Radiative Impact of Saharan Dust on the Early Stage of Hurricane Earl
by Jianyu Liang, Yongsheng Chen, Avelino F. Arellano and Abdulla Al Mamun
Atmosphere 2021, 12(9), 1181; https://doi.org/10.3390/atmos12091181 - 13 Sep 2021
Cited by 2 | Viewed by 2688
Abstract
Current studies report inconsistent results about the impacts of Saharan dust on the development of African Easterly Waves (AEWs), the African Easterly Jet (AEJ), and tropical cyclones (TCs). We present a modeling case study to further elucidate the direct radiative impacts of dust [...] Read more.
Current studies report inconsistent results about the impacts of Saharan dust on the development of African Easterly Waves (AEWs), the African Easterly Jet (AEJ), and tropical cyclones (TCs). We present a modeling case study to further elucidate the direct radiative impacts of dust on the early development stage of a TC. We conducted experiments using the Weather Research and Forecasting model coupled with chemistry (WRF-Chem-V3.9.1) to simulate Hurricane Earl (2010) which was influenced by the dusty Saharan Air Layer (SAL). We used the aerosol product from ECMWF MACC-II as the initial and boundary conditions to represent aerosol distribution, along with typical model treatment of its radiative and microphysical effects in WRF. Our simulations at 36-km resolution show that, within the first 36 h, the presence of dust weakens the low-pressure system over North Africa by less than 1 hPa and reduces its mean temperature by 0.03 K. Dust weakens and intensifies the AEJ at its core and periphery, respectively, with magnitudes less than 0.2 m/s. Dust slightly shifts the position of 600 hPa AEW to the south and reduces its intensity prior to impacting the TC. Finally, TC with dust remains weaker. Full article
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16 pages, 3945 KiB  
Article
Assessing Heatwaves and Their Association with North African Dust Intrusions in the Algarve (Portugal)
by Raquel Fernandes and Marcelo Fragoso
Atmosphere 2021, 12(9), 1090; https://doi.org/10.3390/atmos12091090 - 24 Aug 2021
Cited by 3 | Viewed by 2885
Abstract
Heatwaves are an extreme meteorological event in which affected populations may also be exposed to deteriorated air quality conditions due to the increase in air pollutant concentrations, such as PM10 (particulate matter < 10 µg/m3). In order to identify heatwaves [...] Read more.
Heatwaves are an extreme meteorological event in which affected populations may also be exposed to deteriorated air quality conditions due to the increase in air pollutant concentrations, such as PM10 (particulate matter < 10 µg/m3). In order to identify heatwaves (1973–2019) in the region of Faro (Algarve) during the hot season (April–September), the Excess Heat Factor (EHF) index was applied. The Mann–Kendall test revealed an upward trend in three heatwave metrics in Faro, and the trend of accumulated heat load (EHF load) was also positive as would be expected, but its signal was not statistically significant. An inventory of North African dust events (2006–2019) was made, and their simultaneous occurrence with heatwaves was assessed, pointing to only 20% of dust events of the Sahara occurring simultaneously with heatwave days. A cluster analysis was conducted on daily geopotential height fields at 850 hPa level over the 2006–2019 period, and four distinct patterns were identified as the most prominent synoptic circulations promoting both heatwave conditions and North African dust over the Algarve. Full article
(This article belongs to the Special Issue Climate Change and Air Pollution in Portugal)
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17 pages, 1814 KiB  
Article
Housing Quality in a Rural and an Urban Settlement in South Africa
by Angela Mathee, Jocelyn Moyes, Thulisa Mkhencele, Jackie Kleynhans, Brigitte Language, Stuart Piketh, Elias Moroe, Floidy Wafawanaka, Neil Martinson, Meredith McMorrow, Stefano Tempia, Kathleen Kahn and Cheryl Cohen
Int. J. Environ. Res. Public Health 2021, 18(5), 2240; https://doi.org/10.3390/ijerph18052240 - 24 Feb 2021
Cited by 12 | Viewed by 4290
Abstract
During 2016 to 2018, a prospective household cohort study of influenza and respiratory syncytial virus community burden and transmission dynamics (the PHIRST study) was undertaken to examine the factors associated with influenza and other respiratory pathogen transmissions in South Africa. We collected information [...] Read more.
During 2016 to 2018, a prospective household cohort study of influenza and respiratory syncytial virus community burden and transmission dynamics (the PHIRST study) was undertaken to examine the factors associated with influenza and other respiratory pathogen transmissions in South Africa. We collected information on housing conditions in the PHIRST study sites: Rural villages near Agincourt, Bushbuckridge Municipality, Mpumalanga Province, and urban Jouberton Township in North West Province. Survey data were collected from 159 and 167 study households in Agincourt and Jouberton, respectively. Multiple housing-related health hazards were identified in both sites, but particularly in Agincourt. In Agincourt, 75% (119/159) of households reported daily or weekly interruptions in water supply and 98% (154/159) stored drinking water in miscellaneous containers, compared to 1% (1/167) and 69% (115/167) of households in Jouberton. Fuels other than electricity (such as wood) were mainly used for cooking by 44% (70/159) and 7% (11/167) of Agincourt and Jouberton households, respectively; and 67% (106/159) of homes in Agincourt versus 47% (79/167) in Jouberton were located on unpaved roads, which is associated with the generation of dust and particulate matter. This study has highlighted housing conditions in Agincourt and Jouberton that are detrimental to health, and which may impact disease severity or transmission in South African communities. Full article
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19 pages, 1708 KiB  
Article
PM10 Chemical Profile during North African Dust Episodes over French West Indies
by Philippe Quénel, Jade Vadel, Céline Garbin, Séverine Durand, Olivier Favez, Alexandre Albinet, Christina Raghoumandan, Stéphanie Guyomard, Laurent Yves Alleman and Fabien Mercier
Atmosphere 2021, 12(2), 277; https://doi.org/10.3390/atmos12020277 - 19 Feb 2021
Cited by 1 | Viewed by 3303
Abstract
The French West Indies are periodically affected by North African dust episodes (NADE) resulting in PM10 concentrations exceeding air quality standards. The aim of the present study was to decipher the PM10 chemical profile during NADE over Guadeloupe. PM10 samples [...] Read more.
The French West Indies are periodically affected by North African dust episodes (NADE) resulting in PM10 concentrations exceeding air quality standards. The aim of the present study was to decipher the PM10 chemical profile during NADE over Guadeloupe. PM10 samples were collected daily at a rural site and an urban site during five episodes between April and October in 2017. During these events, the median PM10 mass concentrations were, on average, 2 to 5 times higher than in the post-episode baseline period. Sampled filters were analyzed for their quantification of chemical constituents including carbonaceous fractions (elemental and organic carbon, EC/OC), anions/cations and levoglucosan, 51 elements, and 57 selected organic species. An orthogonal partial least squares discriminant analysis (OPLS-DA) was conducted to identify the specific chemical profile of PM10 during NADE: 16 elements were identified as the most discriminant between the NADE and the control samples with mass concentration levels twice as high during a NADE. Among them, only two (Mn and V) are classified as emerging pollutant while no limit values exist for the other ones. The extensive characterization of the NADE PM10 chemical profile we performed is a key step to assess the chemical exposure of French West Indies populations during such events. Full article
(This article belongs to the Special Issue Air Pollution and Environment in France)
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18 pages, 5789 KiB  
Article
Estimation of Particulate Matter Contributions from Desert Outbreaks in Mediterranean Countries (2015–2018) Using the Time Series Clustering Method
by Álvaro Gómez-Losada and José C. M. Pires
Atmosphere 2021, 12(1), 5; https://doi.org/10.3390/atmos12010005 - 23 Dec 2020
Cited by 2 | Viewed by 3047
Abstract
North African dust intrusions can contribute to exceedances of the European PM10 and PM2.5 limit values and World Health Organisation standards, diminishing air quality, and increased mortality and morbidity at higher concentrations. In this study, the contribution of North African dust [...] Read more.
North African dust intrusions can contribute to exceedances of the European PM10 and PM2.5 limit values and World Health Organisation standards, diminishing air quality, and increased mortality and morbidity at higher concentrations. In this study, the contribution of North African dust in Mediterranean countries was estimated using the time series clustering method. This method combines the non-parametric approach of Hidden Markov Models for studying time series, and the definition of different air pollution profiles (regimes of concentration). Using this approach, PM10 and PM2.5 time series obtained at background monitoring stations from seven countries were analysed from 2015 to 2018. The average characteristic contributions to PM10 were estimated as 11.6 ± 10.3 µg·m−3 (Bosnia and Herzegovina), 8.8 ± 7.5 µg·m−3 (Spain), 7.0 ± 6.2 µg·m−3 (France), 8.1 ± 5.9 µg·m−3 (Croatia), 7.5 ± 5.5 µg·m−3 (Italy), 8.1 ± 7.0 µg·m−3 (Portugal), and 17.0 ± 9.8 µg·m−3 (Turkey). For PM2.5, estimated contributions were 4.1 ± 3.5 µg·m−3 (Spain), 6.0 ± 4.8 µg·m−3 (France), 9.1 ± 6.4 µg·m−3 (Croatia), 5.2 ± 3.8 µg·m−3 (Italy), 6.0 ± 4.4 µg·m−3 (Portugal), and 9.0 ± 5.6 µg·m−3 (Turkey). The observed PM2.5/PM10 ratios were between 0.36 and 0.69, and their seasonal variation was characterised, presenting higher values in colder months. Principal component analysis enabled the association of background sites based on their estimated PM10 and PM2.5 pollution profiles. Full article
(This article belongs to the Special Issue Air Quality and Health in the Mediterranean)
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15 pages, 3794 KiB  
Article
Snow Impurities in the Central Pyrenees: From Their Geochemical and Mineralogical Composition towards Their Impacts on Snow Albedo
by Jorge Pey, Jesús Revuelto, Natalia Moreno, Esteban Alonso-González, Miguel Bartolomé, Jesús Reyes, Simon Gascoin and Juan Ignacio López-Moreno
Atmosphere 2020, 11(9), 937; https://doi.org/10.3390/atmos11090937 - 2 Sep 2020
Cited by 16 | Viewed by 3571
Abstract
The aim of this work is to understand aerosol transfers to the snowpack in the Spanish Pyrenees (Southern Europe) by determining their episodic mass-loading and composition, and to retrieve their regional impacts regarding optical properties and modification of snow melting. Regular aerosol monitoring [...] Read more.
The aim of this work is to understand aerosol transfers to the snowpack in the Spanish Pyrenees (Southern Europe) by determining their episodic mass-loading and composition, and to retrieve their regional impacts regarding optical properties and modification of snow melting. Regular aerosol monitoring has been performed during three consecutive years. Complementarily, short campaigns have been carried out to collect dust-rich snow samples. Atmospheric samples have been chemically characterized in terms of elemental composition and, in some cases, regarding their mineralogy. Snow albedo has been determined in different seasons along the campaign, and temporal variations of snow-depth from different observatories have been related to concentration of impurities in the snow surface. Our results noticed that aerosol flux in the Central Pyrenees during cold seasons (from November to May, up to 12–13 g m−2 of insoluble particles overall accumulated) is much higher than the observed during the warm period (from June to October, typically around 2.1–3.3 g m−2). Such high values observed during cold seasons were driven by the impact of severe African dust episodes. In absence of such extreme episodes, aerosol loadings in cold and warm season appeared comparable. Our study reveals that mineral dust particles from North Africa are a major driver of the aerosol loading in the snowpack in the southern side of the Central Pyrenees. Field data revealed that the heterogeneous spatial distribution of impurities on the snow surface led to differences close to 0.2 on the measured snow albedo within very short distances. Such impacts have clear implications for modelling distributed energy balance of snow and predicting snow melting from mountain headwaters. Full article
(This article belongs to the Special Issue Interaction of Air Pollution with Snow and Seasonality Effects)
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30 pages, 8645 KiB  
Article
Analysis of the Transport of Aerosols over the North Tropical Atlantic Ocean Using Time Series of POLDER/PARASOL Satellite Data
by Hélène Fréville, Malik Chami and Marc Mallet
Remote Sens. 2020, 12(5), 757; https://doi.org/10.3390/rs12050757 - 25 Feb 2020
Cited by 4 | Viewed by 3623
Abstract
The time series of total, fine and coarse POLAC/PARASOL aerosol optical depth (AOD) satellite products (2005–2013) processed by the POLAC algorithm are examined to investigate the transport of aerosols over the North Tropical Atlantic Ocean, a region that is characterized by significant dust [...] Read more.
The time series of total, fine and coarse POLAC/PARASOL aerosol optical depth (AOD) satellite products (2005–2013) processed by the POLAC algorithm are examined to investigate the transport of aerosols over the North Tropical Atlantic Ocean, a region that is characterized by significant dust aerosols events. First, the comparison of satellite observations with ground-based measurements acquired by AERONET ground-based measurements shows a satisfactory consistency for both total AOD and coarse mode AOD (i.e., correlation coefficients of 0.75 and bias ranging from −0.03 to 0.03), thus confirming the robustness and performance of POLAC/PARASOL data to investigate the spatio-temporal variability of the aerosols over the study area. Regarding fine mode aerosol, POLAC/PARASOL data present a lower performance with correlation coefficient ranging from 0.37 to 0.73. Second, the analysis of POLAC/PARASOL aerosol climatology reveals a high contribution of the coarse mode of aerosols ( AOD c between 0.1 and 0.4) at long distance from the African sources, confirming previous studies related to dust transport. The POLAC/PARASOL data were also compared with aerosol data obtained over the North Tropical Atlantic Ocean from MACC and MERRA-2 reanalyses. It is observed that the total AOD is underestimated in both reanalysis with a negative bias reaching −0.2. In summary, our results thus suggest that satellite POLAC/PARASOL observations of fine and coarse modes of aerosols could provide additional constraints useful to improve the quantification of the dust direct radiative forcing on a regional scale but also the biogeochemical processes such as nutrient supply to the surface waters. Full article
(This article belongs to the Special Issue Active and Passive Remote Sensing of Aerosols and Clouds)
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