Search Results (161)

The updated MODIS Collection 6.1 (C6.1) Dark Target (DT) aerosol optical depth (AOD) is extensively utilized in aerosol-climate studies in China. Nevertheless, the long-term accuracy of this data remains under-evaluated, especially for the forested areas. This study was undertaken to substantiate the accuracy of MODIS Terra (MOD04) and Aqua (MYD04) at 3 km resolution AOD retrievals at six forested sites in China from 2004 to 2022. The results revealed that MODIS C6.1 DT MOD04 and MYD04 datasets display good correlation (R = 0.75), low RMSE (0.20, 0.18), but significant underestimation, with only 53.57% (Terra) and 52.20% (Aqua) of retrievals within expected error (EE). Both the Terra and Aqua struggled in complex terrain (Gongga Mt.) and high aerosol loads (AOD > 1). In northern sites, MOD04 outperformed MYD04 with better correlation and a relatively high number of retrievals percentage within EE. In contrast, MYD04 outperformed MOD04 in central region with better R (0.69 vs. 0.62), and high percentage within EE (68.70% vs. 63.62%). Since both products perform well in the central region, MODIS C6.1 DT products are recommended for this region. In southern sites, MOD04 product performs relatively better than MYD04 with a marginally higher percentage within EE. However, MYD04 shows better correlation, although a higher number of retrievals fall below EE compared to MOD04. Seasonal biases, driven by snow and dust, were pronounced at northern sites during winter and spring. Southern sites faced issues during biomass burning seasons and complex terrain further degraded accuracy. MOD04 demonstrated a marginally superior performance compared to MYD04, yet both failed to achieve the global validation benchmark (66% within). The proposed results highlight critical limitations of current aerosol retrieval algorithms in forest and mountainous landscapes, necessitating methodological refinements to improve satellite-based derived AOD accuracy in ecological sensitive areas. Full article

Aerosols play a crucial role in air quality, climate regulation, and public health; their timely monitoring is hence fundamental. The aerosol optical depth (AOD) is the parameter used to investigate the spatial–temporal distribution of aerosols from space. Specifically, the AOD retrieved from the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm applied to a Moderate Resolution Imaging Spectroradiometer (MODIS) is suitable for aerosol investigation at a local scale by exploiting its high spatial resolution (1 km × 1 km). In this study, the MAIAC AOD retrieval over Rome (Italy) was validated for the first time, using ground-based data provided by an AERONET station operating in a semi-rural environment close to the city, over a time series from January 2001 to December 2022. Moreover, AOD trends were evaluated in a study area encompassing Rome and its surroundings, characterized by a transition zone between urban and rural environments. The results show a general underestimation of the MAIAC AOD; specifically, the validation process highlighted the less accurate performance of the algorithm under higher aerosol loading and with predominantly coarse mode aerosol. Interesting results were obtained concerning the influence of the geometrical configuration of satellite acquisition on the accuracy of the MAIAC product. In particular, the solar zenith angle, the relative azimuth and the scattering angle between the principal plane of the sun and satellite synergistically influence retrievals. Finally, the spatial distribution of the AOD shows a decreasing trend over the 2001–2022 period and a strong influence of the city of Rome over the whole study area. Full article

The satellite remote sensing of Aerosol Optical Depth (AOD) products is crucial in environmental monitoring and atmospheric pollution research. However, data gaps in AOD products from satellites like Fengyun significantly hinder continuous, seamless environmental monitoring capabilities, posing challenges for the long-term analysis of atmospheric pollution trends, responses to sudden ecological events, and disaster management. This study aims to develop a high-precision method to fill spatial AOD missing values and generate daily full-coverage AOD products for the Beijing–Tianjin–Hebei region in 2021 by integrating multi-dimensional data, including meteorological models, multi-source remote sensing, surface conditions, and nighttime light parameters, and applying machine learning methods. A comparison of five machine learning models showed that the random forest model performed optimally in AOD inversion, achieving a root mean square error (RMSE) of 0.11 and a coefficient of determination (R²) of 0.93. Seasonal evaluation further indicated that the model’s simulation was best in winter. Variable importance analysis identified relative humidity (RH) as the most critical factor influencing model results. The reconstructed full-coverage AOD product exhibited a spatial distribution trend of significantly higher values in the southern plain areas compared to mountainous regions, consistent with the actual aerosol distribution patterns in the Beijing–Tianjin–Hebei area. Moreover, the product demonstrated overall smoothness and high accuracy. This research lays the foundation for establishing a long-term, 1 km resolution, daily spatially continuous AOD product for the Beijing–Tianjin–Hebei region and beyond, providing more robust data support for addressing regional and larger-scale environmental challenges. Full article

This study investigated the dust storm observation data from the Taklimakan Desert in 2018, focusing on analyzing horizontal dust flux (Q), vertical dust flux (F), their relationships with aerosol optical depth (AOD), and the relationship between HYSPLIT backward trajectories and dust storm dispersion direction. Key findings include: (1) at the Xiaotang (XT) station, Q values at low heights (1–10 m) exceeded those at higher altitudes, highlighting the role of flat terrain in dust accumulation, while Q values at the Tazhong (TZ) station remained relatively stable, suggesting dust redistribution influenced by undulating topography; (2) vertical dust flux (F) decreased with height, with significant seasonal variations in spring linked to frequent dust events; (3) at station XT, the contribution of F at 5 m height is relatively strong to AOD and its peak precedes AOD by 24–72 h, although the direct correlation is weak; and (4) dust dispersion directions aligned with HYSPLIT trajectories and high Q values corresponded with remotely derived dust dispersion patterns. Full article

The Directional Polarimetric Camera (DPC) aboard the Chinese GaoFen-5 02 satellite is designed to monitor aerosols and particulate matter (PM). In this study, we retrieved the aerosol optical depth (AOD) over the Jing–Jin–Ji (JJJ) region using multi-angle data from the DPC, employing a combination of dark dense vegetation (DDV) and multi-angle retrieval methods. The added value of our method included novel hybrid methodology and good practical performance. The retrieval process involves three main steps: (1) deriving AOD from DPC data collected at the nadir angle using linear parameters of land surface reflectance between the blue and red bands from the MOD09 surface product; (2) after performing atmospheric correction with the retrieved AOD, calculating the variance of the normalized reflectance at all observation angles; and (3) leveraging the calculated variance to obtain the final AOD values. AOD images over the JJJ region were successfully retrieved from DPC data collected between January and June 2022. To validate the retrieval method, we compared our results with aerosol products from the AErosol RObotic NETwork (AERONET) Beijing-RADI site, as well as aerosol data from MODerate-resolution Imaging Spectroradiometer (MODIS) and the generalized retrieval of atmosphere and surface properties (GRASP)/models over the same site. In terms of validation metrics, the correlation coefficient (R²) and root mean square error (RMSE) indicated that our method achieved high accuracy, with an R² value greater than 0.9 and an RMSE below 0.1, closely aligning with the performance of GRASP. Full article

Having good replication of the soil moisture evolution is desirable to properly simulate the dust emissions and atmospheric dust load because soil moisture increases the cohesive forces of soil particles, modulating the wind erosion threshold above which emissions occur. To reduce errors, one can use soil moisture retrievals from space-borne microwave radiometers. Here, we explore the potential of inserting soil moisture retrievals from the Soil Moisture Active Passive (SMAP) satellite into the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to improve dust simulations. We focus our analysis on the contiguous U.S. due to the presence of important dust sources and good observational networks. Our analysis extends over the first year of SMAP retrievals (1 April 2015–31 March 2016) to cover the annual soil moisture variability and go beyond extreme events, such as dust storms, in order to provide a statistically robust characterization of the potential added value of the soil moisture retrievals. We focus on the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model from the Air Force Weather Agency (GOCART-AFWA) dust emission parameterization that represents soil moisture modulations of the wind erosion threshold with a parameterization developed by fitting observations. The dust emissions are overestimated by the GOCART-AFWA parameterization and result in an overestimation of the aerosol optical depth (AOD). Sensitivity experiments show that emissions reduced to 25% in the GOCART-AFWA simulations largely reduced the AOD bias over the Southwest and lead to better agreement with the standard WRF-Chem parameterization of dust emissions (GOCART) and with observations. Comparisons of GOCART-AFWA simulations with emissions reduced to 25% with and without SMAP soil moisture insertion show added value of the retrievals, albeit small, over the dust sources. These results highlight the importance of accurate dust emission parameterizations when evaluating the impact of remotely sensed soil moisture data on numerical weather prediction models. Full article

Methane (CH₄) emissions in coal-energy-rich regions are characterized by hidden emission point sources and highly variable emission rates. While the Matched Filter (MF) method for detecting the CH₄ point source using hyperspectral satellite sensors has been validated for high-emission concentrations, the accurate inversion of low-concentration emissions in complex environments remains challenging. In this study, an ‘end-to-end’ experiment—from emission simulations to satellite spectra and inversion results—has been designed to quantify the impact of internal payload parameters and environmental parameters for CH₄ emission inversions, and perform real-scenario calculations. The study reveals several key findings: (1) Under ideal conditions, 15% of satellite spectral noise contributes to a 13% bias in CH4 detection inversion, and a spectral resolution of 10–14 nm allows the detection of CH₄ emissions with concentrations as low as 350 ppb, above the background level of 1900 ppb. (2) For near-surface aerosols at 2100 nm, an aerosol optical depth (AOD) of 0.1 leads to a low bias of −51.6% with water-soluble aerosols and a strong bias of −69.2% with black carbon aerosols, while dust aerosols induce a medium bias of up to −60.7%. (3) The height of the aerosol layer affects the accuracy of methane inversion, which is up to 7.3% higher under aerosol conditions at 3 km than under aerosol conditions near the ground. (4) When the CH₄ emission source and its diffuse plume are located above a high-reflectance (bright) surface, while the background CH₄ concentration is associated with a low-reflectance (dark) surface, the significant reflectance contrast between the two surfaces leads to a rapid degradation in inversion accuracy. This contrast makes it impossible to effectively extract CH₄ signals when the reflectance difference reaches 0.2. (5) Under harsh conditions, where multiple parameters are present (AOD = 0.2, albedo = 0.2, aerosol layer height (ALH) = 2), the MF method is still able to detect CH₄ emissions, but with a significant error of 74.65%. (6) External environmental variables, particularly atmospheric pressure and water vapor content, significantly influence the inversion accuracy of methane (CH₄) concentrations. Variations in atmospheric pressure induce deviations in the CH₄ concentration distribution, resulting in an average inversion error of −12.06%. Similarly, elevated water vapor levels can lead to a maximum error of −16.2%. These findings highlight the substantial challenges in accurately detecting low-concentration CH₄ emissions. The results offer critical insights for refining CH₄ detection algorithms and enhancing the precision of satellite-based inversions for low-concentration CH₄ point-source emissions. Full article

Near-surface ozone is a secondary pollutant, and its high concentrations pose significant risks to human and plant health. Based on an Extra Tree (ET) model, this study estimated near-surface ozone concentrations with the high spatiotemporal resolution based on Himawari-8 aerosol optical depth (AOD) data and meteorological variables from 1 January 2016 to 31 December 2020. The SHapley Additive exPlanation (SHAP) method was employed to evaluate the contribution of AOD and meteorological factors on ozone concentration. The results indicate that (1) the ET model achieves a sample-based cross-validation R² of 0.75–0.87 and an RMSE (μg/m³) of 17.96–20.30. The coefficient of determination (R²) values of the model in spring, summer, autumn, and winter are 0.81, 0.80, 0.87, and 0.75, respectively. (2) Higher temperature and boundary layer heights were found to positively contribute to ozone concentration, whereas higher relative humidity exerted a negative influence. (3) From 11:00 to 15:00 (Beijing time, UTC+08:00), ozone concentration increases gradually, with the highest occurring in the summer, followed by spring. This study has obtained high spatial and temporal resolution ozone concentration data, offering valuable insights for the development of fine-scale ozone pollution prevention and control strategies. Full article

Aerosol vertical stratification significantly influences the Earth’s radiative balance and particulate-matter-related air quality. Continuous vertically resolved observations remain scarce compared to surface-level and column-integrated measurements. This work presents and makes available a novel, long-term (2016–2022) aerosol dataset derived from continuous (24/7) vertical profile observations from three selected stations (Aosta, Rome, Messina) of the Italian Automated Lidar-Ceilometer (ALC) Network (ALICENET). Using original retrieval methodologies, we derive over 600,000 quality-assured profiles of aerosol properties at the 15 min temporal and 15 metre vertical resolutions. These properties include the particulate matter mass concentration (PM), aerosol extinction and optical depth (AOD), i.e., air quality legislated quantities or essential climate variables. Through original ALICENET algorithms, we also derive long-term aerosol vertical layering data, including the mixed aerosol layer (MAL) and elevated aerosol layers (EALs) heights. Based on this new dataset, we obtain an unprecedented, fine spatiotemporal characterisation of the aerosol vertical distributions in Italy across different geographical settings (Alpine, urban, and coastal) and temporal scales (from sub-hourly to seasonal). Our analysis reveals distinct aerosol daily and annual cycles within the mixed layer and above, reflecting the interplay between site-specific environmental conditions and atmospheric circulations in the Mediterranean region. In the lower troposphere, mixing processes efficiently dilute particles in the major urban area of Rome, while mesoscale circulations act either as removal mechanisms (reducing the PM by up to 35% in Rome) or transport pathways (increasing the loads by up to 50% in Aosta). The MAL exhibits pronounced diurnal variability, reaching maximum (summer) heights of >2 km in Rome, while remaining below 1.4 km and 1 km in the Alpine and coastal sites, respectively. The vertical build-up of the AOD shows marked latitudinal and seasonal variability, with 80% (30%) of the total AOD residing in the first 500 m in Aosta-winter (Messina-summer). The seasonal frequency of the EALs reached 40% of the time (Messina-summer), mainly in the 1.5–4.0 km altitude range. An average (wet) PM > 40 μg m⁻³ is associated with the EALs over Rome and Messina. Notably, 10–40% of the EAL-affected days were also associated with increased PM within the MAL, suggesting the entrainment of the EALs in the mixing layer and thus their impact on the surface air quality. We also integrated ALC observations with relevant, state-of-the-art model reanalysis datasets (ERA5 and CAMS) to support our understanding of the aerosol patterns, related sources, and transport dynamics. This further allowed measurement vs. model intercomparisons and relevant examination of discrepancies. A good agreement (within 10–35%) was found between the ALICENET MAL and the ERA5 boundary layer height. The CAMS PM₁₀ values at the surface level well matched relevant in situ observations, while a statistically significant negative bias of 5–15 μg m⁻³ in the first 2–3 km altitude was found with respect to the ALC PM profiles across all the sites and seasons. Full article

Lidar is the primary tool used to determine the vertical distribution of aerosol optical characteristics. Based on the observation characteristics of the mountain’s gradient, a validation analysis of the remote sensing and in situ observations of the aerosol optical characteristics and research on seasonal, monthly, and daily variations in aerosol optical depth (AOD) were performed using the dual-wavelength Lidar deployed at the foot of Mt. Lu and the aerosol particle-size spectrometer at the top of Mt. Lu. The validation results show that at the comparison heights, under cloudy-sky conditions with strong winds (>3.4 m/s) and high relative humidity (RH) (>70%), the aerosol extinction coefficients between the two sites are in good agreement; thus, the observations at the top of the mountain are more suitable for in situ validation under cloudy-sky conditions; however, the local circulations under clear-sky conditions lead to large differences in the aerosol properties at the same altitude between the two sites and are unsuitable for validation. An analysis of the AOD data from Mt. Lu reveals the following: (1) The AOD seasonal distribution frequencies under both clear-sky and cloudy-sky conditions are unimodal, with a values of 0.2∼0.6, and the inhomogeneity of the aerosol distribution in winter is evident; the seasonal difference in the AOD under clear-sky conditions is more significant, following the order of spring > summer > winter > autumn, and the AOD seasonal difference under cloudy-sky conditions is not obvious. (2) In the analysis of the AOD monthly variations, due to the influence of the meteorological conditions (high humidity, low wind speed) and pollutant transport, the AOD reached its peak in February (clear-sky: 0.63, cloudy-sky: 0.82). (3) Under clear-sky conditions, the negative correlation between the daily variations in AOD, and visibility is more significant during the daytime, and after 12:00, the AOD is positively correlated with $P{M}_{2.5}$; these results indicate that the AOD is affected mainly by pollutants and the boundary layer height. Under cloudy-sky conditions, the peaks in the daytime AOD are related to the morning and evening rush hours, the correlations with the visibility and $P{M}_{2.5}$ are low, and the accumulation of pollutants during the nighttime. And (4) overall, the AOD is greater under cloudy-sky conditions than under clear-sky conditions; this result is likely related to the more favorable subcloud humidity conditions for aerosol hygroscopic growth. Full article

Air quality is directly related to people’s health and quality of life and has a profound impact on the sustainable development of cities. Good air quality is the foundation of sustainable development. To solve the current problem of air quality for sustainable development, we used high-resolution (1 km) satellite-retrieved aerosol optical depth (AOD), meteorological, nighttime light and vegetation data to develop a spatiotemporal convolution feature random forest (SCRF) model to predict the PM_2.5 concentration in Shandong from 2016 to 2019. We evaluated the performance of the SCRF model and compared the results of other models, including neural network (BPNN), gradient boosting (GBDT), and random forest (RF) models. The results show that compared with the other models, the improved SCRF model performs best. The coefficient of determination (R²) and root mean square error (RMSE) are 0.83 and 9.87 µg/m³, respectively. Moreover, we discovered that the characteristic variables AOD and air temperature (TEM) data improved the accuracy of the model in Shandong Province. The annual average PM_2.5 concentrations in Shandong Province from 2016 to 2019 were 74.44 µg/m³, 65.01 µg/m³, 58.32 µg/m³, and 59 µg/m³, respectively. The spatial distribution of air pollution increases from northeastern and southeastern to western Shandong inland. In general, our research has significant implications for the sustainable development of various cities in Shandong Province. Full article

In this study, the spatial–temporal characteristics of AOD in the Yellow River Basin (YRB) and urban agglomerations within the basin were analyzed at a 1 km scale from 2011 to 2020 based on the MCD19A2 AOD dataset. This study shows the following: (1) From 2011 to 2020, the AOD value of the YRB showed a declining trend, with 96.011% of the zones experiencing a decrease in AOD. The spatial distribution of AOD displayed a pattern of high in the east, low in the west, high in the south, and low in the north. The rate of decline showed a distribution pattern of fast in the southeast and slow in the northwest. (2) The AOD in the YRB showed similar characteristics in different seasons: the south and east were consistently higher than the north and west. The seasonal AOD values in the YRB showed the following pattern: summer > spring > autumn > winter. The AOD values of urban agglomeration were basically larger in spring and summer. (3) The SDE and mean center of the yearly AOD were located in the southeast and Shanxi Province, with the movement from southeast to northwest. It can be divided into three stages based on the movement trajectory: northeast–southwest round-trip movement (2011–2014), one-way movement to the northwest (2014–2018), and southeast–northwest round-trip movement (2018–2020). Full article

The population of Senegal faces health challenges related to desert dust and heat waves (HWs). This study aims to (a) update the documentation of HWs in Senegal, expanding on the work of Sambou et al. (2019); (b) investigate the modulation of dust indicators during HWs; and (c) assess the distinct impacts of dust content on night-time and daytime HWs. We use [i] the daily maximum air temperature (Tx), minimum air temperature (Tn), and apparent temperature (Ta) from 12 stations in the Global Surface Summary of the Day (GSOD) database and [ii] the Dust Aerosol Optical Depth (Dust AOD), particulate matter (PM) concentrations, 925 hPa wind, and Mean Sea Level Pressure (MSLP) from the Copernicus Atmosphere Monitoring Service (CAMS) reanalysis. HWs are defined for each station in spring as periods when Tx, Tn, or Ta exceeds the 95th percentile for at least three consecutive days. Three homogeneous zones from the Atlantic coast to inland Senegal are identified using hierarchical cluster analysis: Zone 1 (Saint-Louis, Dakar-Yoff, Ziguinchor, and Cap Skirring), Zone 2 (Podor, Linguère, Diourbel, and Kaolack), and Zone 3 (Matam, Tambacounda, Kédougou, and Kolda). Our results show that Zone 1 records the highest number of HWs for Tx, Tn, and Ta, while Zone 3 experiences more HWs in terms of Tn and Ta than Zone 2. The influence of dust is notably stronger for HWs linked to Tn and Ta than for those related to Tx. Analysis of the mechanisms shows that the presence of dust in Senegal and its surrounding regions is detected up to four days before the onset of HWs. These findings suggest that dust conditions associated with spring HWs in Senegal may be better distinguished and predicted. Full article

Given the complex spatiotemporal variability of aerosols, high-frequency satellite observations are essential for accurately mapping their distribution. However, optical remote sensing encounters difficulties in detecting Aerosol Optical Depth (AOD) over cloud-covered regions, creating data gaps that limit comprehensive environmental analysis. This study introduces a spatial gap-filling method for Himawari-8/Advanced Himawari Imager (AHI) hourly AOD data, using a Random Forest (RF) model that integrates meteorological variables and model-based AOD data. Developed and validated over South Korea from 1 January to 31 December 2019, the model effectively improved data coverage from 6% to 100%. The approach demonstrated high performance in blind tests, achieving a root mean square error (RMSE) of 0.064 and a correlation coefficient (CC) of 0.966. Meteorological analysis indicated optimal model performance under cold, dry conditions (RMSE: 0.047, CC: 0.956), compared to humid conditions (RMSE: 0.105, CC: 0.921). Validation against Aerosol Robotic Network (AERONET) ground observations showed that, while the original Himawari-8 data exhibited higher accuracy (RMSE: 0.189, CC: 0.815, n = 346), the gap-filled dataset maintained reasonable precision (RMSE: 0.208, CC: 0.711) and significantly increased the number of valid data points (n = 4149). Furthermore, the gap-filled dataset successfully captured seasonal AOD patterns, with values ranging from 0.245–0.300 in winter to 0.381–0.391 in summer, providing a comprehensive view of aerosol dynamics across South Korea. Full article

Aerosol optical depth (AOD) serves as a significant parameter in aerosol research. With the increasing utilization of satellite data in AOD research, it is crucial to evaluate the satellite AOD data. Using Aerosol Robotic Network (AERONET) in situ measurements, this study investigates the accuracy and applicability of Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) AOD data in Asia from June 2006 to June 2023. By matching the CALIPSO AOD data in a 1° × 1° area around the selected AERONET sites, various statistical metrics were used to create a comprehensive evaluation system. The results show that: (1) There is a high correlation between the AODs of CALIPSO and AERONET (R = 0.636), and the AOD values of CALIPSO are only 1.7% higher than those of AERONET on average. The MAE (0.215) and RMSE (0.358) suggest that the error level of CALIPSO AOD is relatively low; (2) In most of the 25 sites throughout Asia CALIPSO AOD have high matching accuracies with the AERONET AOD, and only in three sites has a validation accuracy of ‘Poor’; (3) The accuracy varies across the four seasons, ranked as follows: winter demonstrates the highest accuracy, followed by autumn, spring, and summer; (4) The accuracy varies with surface elevation, with better matching in lowest altitude (<50 m) and high altitude (>500 m) areas, but slightly worse matching in medium altitude (200–500 m) areas and low altitude (50–200 m). The uncertainty in the CALIPSO AOD retrievals varies in seasons, altitudes, and aerosol characteristics. Full article