Majorana Zero Modes in Ferromagnetic Wires without Spin-Orbit Coupling

We present a novel controllable platform for engineering Majorana zero modes. The platform consists of a ferromagnetic metallic wire placed among conventional superconductors, which are in proximity to ferromagnetic insulators. We demonstrate that Majorana zero modes emerge localised at the edges of the ferromagnetic wire, due to the interplay of the applied supercurrents and the induced by proximity exchange fields with conventional superconductivity. Our mechanism does not rely on the pairing of helical fermions by combining conventional superconductivity with spin-orbit coupling, but rather exploits the misalignment between the magnetization of the ferromagnetic insulators and that of the ferromagnetic wire.


Introduction
The development of quantum computers promises a new technological revolution [1]. However, a fundamental obstacle hindering the development of quantum computation is quantum decoherence, the loss of quantum mechanical phase coherence and, therefore, of information encoded in qubits. Attempts to deal with this problem through quantum error correction algorithms lead to elaborate schemes consuming a highly disproportional amount of qubits. On the contrary, topological quantum computers suppress quantum decoherence at the hardware level. Qubits in these devices are realized from topologically protected entities, which are immune to environmental noise and, therefore, decoherence [2][3][4].
Such topological protected entities are Majorana zero modes-massless neutral particles that constitute their own antiparticles. Characterised by their particle-antiparticle symmetry, MZMs emerge as quasiparticles bound to defects or boundaries of topological superconductors [5]. The simplest topological superconductor is the effectively spinless superconducting phase of p-wave symmetry [6,7]. Although a topological p-wave state is proposed for the superconducting phase of Sr 2 RuO 4 [8], experimental results are yet inconclusive [9].
Instead, several proposals have been put forward for engineering topological p-wave superconductivity out of more trivial materials. Among them, we distinguish conventional superconductor/topological insulator heterostructures [10], semiconductors in proximity to conventional superconductors [11], non-centrosymmetric superconductors [12] and planar Josephson junctions [13]. All these proposals effectuate the pairing of helical fermions by combining conventional superconductivity with spin orbit coupling in the presence of a spin-splitting field, in order to realize an effectively spinless superconducting state.

Majorana Zero Modes in Superconductor/Ferromagnet Heterostructures
As aforementioned, realising MZMs using conventional superconductors requires the presence of a spin-splitting field. The simplest way to satisfy this requirement is by arXiv:2111.15260v1 [cond-mat.supr-con] 30 Nov 2021 applying an external magnetic field. However, magnetic fields are detrimental to conventional superconductivity; thereby, many proposals for realising MZMs are based on heterostructures among superconductors with ferromagnetic materials. Superconductorferromagnet heterostructures do not require the application of an external magnetic field and, therefore, are advantageous with respect to other platforms. Following this line of argument, topological superconductivity and MZMs have been demonstrated to emerge in half-metal/superconductor [14] or ferromagnet/unconventional superconductor [15] heterostructures, in ferromagnetic wires proximised to conventional superconductors [16][17][18] and in ferromagnetically aligned chains of magnetic impurities embedded in conventional superconductors [19][20][21][22][23][24][25][26]. Spin-orbit coupling is an essential component in all of these proposals.

A Novel Platform
Here, we put forward a novel platform for engineering topological superconductivity and Majorana zero modes, which does not require spin orbit coupling. The platform, as presented in Figure 1, consists of a ferromagnetic metallic wire, which is placed between two conventional superconducting layers where supercurrents flow in opposite directions. A ferromagnetic metallic wire placed among two conventional superconductors where supercurrents flow in opposite directions (blue arrows). The superconducting layers are deposited upon ferromagnetic insulators with opposite magnetisations (black arrows), which are perpendicular to the magnetisation of the ferromagnetic wire (white arrow). (Right) The energy bands, E s,± where s refers to spin components and ± to hole and particles, respectively, of a conventional superconductor when a supercurrent and an exchange field are applied. Supercurrent breaks inversion symmetry (k , −k momenta are not equivalent) and the exchange field breaks spin symmetry (s and s are not equivalent) leading to the emergence of p-wave superconducting correlations. Arrows indicate the pairing components of conventional superconductivity.
localised at the edges of the FM, due to the synergy between the externally applied supercurrents with the emergent in the SCs exchange fields [27]. We remark that several works have demonstrated both theoretically [28,29] and experimentally [30][31][32] the emergence of exchange fields in conventional SCs proximised by FIs. Moreover, developments in the fabrication of SC-FI heterostructures [33] and ferromagnetic metallic nanonwires embedded in conventional SCs [34][35][36], enhance the experimental feasibility of the proposed platform.

The Underlying Mechanism
According to our mechanism, a topological superconducting state is stabilized over the FM wire, when charge supercurrents are applied in conventional SCs where finite exchange fields are present. The supercurrent and the exchange field break inversion and spin symmetries, respectively, and, therefore, partially convert conventional superconductivity to a p-wave superconducting field. This emergent p-wave superconducting field still pairs electrons of different energy bands of the superconductor, while MZMs require intraband superconductivity.
However, in an FM wire with magnetisation perpendicular to the magnetisation of the ferromagnetic insulators, the induced p-wave superconducting field pairs electrons of the same energy band of the FM. An intraband superconducting component emerges when the d-vector of p-wave superconductivity [37] is misaligned to the exchange field of the FM wire [38]. Thus, when this p-wave superconducting field mediates into the FM wire, due to the proximity effect, an effectively spinless superconducting state is stabilised, and MZMs emerge. In the next section, we present analytically how the triplet superconducting component emerges, due to the coexistence of the exchange field and the supercurrents with conventional superconductivity.

Induced p-Wave Superconductivity
In order to demonstrate how triplet p-wave superconductivity is induced, we consider a superconducting wire with order parameter ∆, where a supercurrent J is applied in the presence of an exchange field h z . We consider the following Hamiltonian where Ψ † = (ψ † ↑ , ψ † ↓ , ψ ↑ , ψ ↓ ) the extended Nambu spinor and τ and σ are the Pauli matrices acting on particle-hole and spin space, respectively, ψ ( †) s (x) the operator destroying(creating) an electron with spin s at coordinate x, h z the exchange field and ∆ = |∆|e iJxτ z the singlet superconducting field. Under the gauge transformation kinetic term ∂ 2 x 2m transforms to x is a current term and − J 2 8m τ z can be absorbed in the chemical potential µ. Thus, Hamiltonian Equation (1) takes the form Considering a translationally invariant wire Hamiltonian Equation (3) takes the following form upon the Fourier transformation The energy bands of the wire where s = ± corresponds to ↓ and ↑ bands respectively, derive from the transformation and and The induced p-wave correlations derive from the equation where n F (E m ) the Fermi distribution andσ = (σ x , τ z σ y , σ z ). For d = d z = (0, 0, 1), we find Therefore, and apparently the < ∆ p z > correlations emerge from the imbalance between singlet pairing (14) it is straightforward that, for h = 0, < ∆ p z >= 0 since, in this case, n F (E −,+ ) = n F (E +,+ ) and n F (E −,− ) = n F (E +,− ), and therefore ∑ s,± ∓sn F (E s,± ) = 0. Moreover, for J = 0 expression ∑ s,± ∓sn F (E s,± ) is even in momenta, and therefore < ∆ p z >= 0, due to the multiplication with momenta k. Thus, pwave correlations are induced only when both h = 0 and J = 0.
For the other two components of the d vector, d y = (0, 1, 0) and d x = (1, 0, 0), there are no p-wave correlations induced. Particularly, for d y = (0, 1, 0) we get Therefore, Therefore, has no diagonal terms. Thus, we conclude that only p-wave correlations with < d h > emerge, due to the imbalance among the two spin configurations of interband conventional pairing.

Intraband p-Wave Superconductivity in the Ferromagnetic Wire
As demonstrated in the previous section, triplet p-wave correlations are induced in a conventional superconductor when a supercurrent and an exchange or Zeeman field are applied. However, topological superconductivity and Majorana zero modes cannot be engineered in a superconducting wire simply by applying a supercurrent and a magnetic field. The triplet p-wave correlations induced in this setup still connect different energy bands of the wire, while MZMs require intraband or effectively spinless superconductivity. Nevertheless, when these correlations mediate to a material with magnetisation perpendicular to the exchange field induced in the superconductors, an intraband superconducting state that hosts MZMs is realised.
Considering the particular setup presented in Figure 1, the induced ∆ p correlations in the SCs correspond to Cooper pairs of electrons with opposite spin, i.e., p z ≡ τ x σ x correlations. These correlations, for which d = d z , mediate in the ferromagnet with polarisation along the x-axis, i.e., perpendicular to the d vector of the induced correlations, described by the following Hamiltonian The energy bands of the FM wire derive from the following transformation where U is the matrix that diagonalises the Hamiltonian H FM . In this eigenbasis, the induced p z triplet correlations are expressed as From Equation (23), it becomes apparent that, in the eigenbasis of the FM, the induced by proximity p-wave field ∆ p pairs electrons from the same energy band, i.e., we obtain intraband pairing. The Hamiltonian Equation (21) upon the U transformation acquires the form which can be reduced into two copies of the Kitaev's Hamiltonian where Ψ † s = (ψ † s , ψ s ), s = ± the band index and µ FM,s = µ FM + sh FM . Based on the above analysis, it becomes clear that the optimal configuration for the emergence of MZMs in the particular platform, is that of anti-parallel supercurrents in the SCs and anti-parallel magnetisations in the FIs. This configuration guarantees that no supercurrent or exchange fields parallel to the magnetisation of the FIs are induced in the FM wire. Thus, the d-vector of the induced p-wave superconducting correlations remains perpendicular to the magnetisation of the FM wire and an intraband superconducting state is realised. However, as we will elaborate in a future work, MZMs are robust against significant deviations from this optimal configuration for the supercurrents and the FIs magnetisations.

Topological Criteria for the Ferromagnetic Wire
where we also considered an induced by proximity conventional superconducting field ∆. We remark that Hamiltonian Equation (26) is expressed in lattice instead of continuum space, in order to connect with the numerical results presented in the next section. In the particular case, the reality conditions, ΘH(k)Θ −1 = H(−k) and ΞH(k)Ξ −1 = −H(−k) where Θ and Ξ anti-unitary operators [39], are satisfied for Ξ = τ x K with Ξ 2 = I and Θ = iτ z σ z K with Θ 2 = I. In addition, a unitary chiral symmetry operator S = Θ · Ξ = τ y σ z anticommutes with the Hamiltonian. Thus, the system belongs to the BDI symmetry class, characterised by an integer Z topological invariant, and Hamiltonian Equation (26) in the eigenbasis of the chiral operator S. Therefore, by z(k) [40] , where z(k) the unimodular complex number defined as z(k) = Det(A(k))/|Det(A(k))|. For the particular system, we find Since within each topological phase, the θ(k) is a continuous function of momentum k, the maximum possible value of the winding number relates to the number n of roots Det(A(k)) within the interval [0, 2π), max|N | = n/2. Notice that because Det(A(k)) = − Det((A(−k)), number n is always even. Next, we distinguish the two following cases. The first case holds for |µ| > 2t. In this case, Det(A(k)) = 0 only for k = 0, π, and therefore the maximum absolute value of the winding number is max|N | = 1. The topological N = 1 phase is realised when z(k = 0)z(k = π) = ∆ 2 + (2t FM < 0, which results in the following condition for the chemical potential or equivalently for the exchange field The second case holds for |µ FM | < 2t. When this condition holds, Det(A(k)) = 0 is realised also for another pair of momenta k * = ±cos −1 µ FM 2t . However, since for ∆ 2 + (2t − µ FM ) 2 < |h FM | < ∆ 2 + (2t + µ FM ) 2 , z(k = 0)z(k = π) < 0, it is straightforward that |N | = 1 within these limits, even in this case. In general, considering ∆ p << ∆, a |N | = 2 topological phase can be realised for for which z(k = 0)z(k = π) > 0 and z(k = k * )z(k = π) < 0.

Numerical Calculations for the FI-SC-FM-SC-FI Heterostructure
In order to verify the above arguments, we employ the following lattice Bogoliubov de Gennes equation, which describes the FI-SC-FM-SC-FI heterostructure presented in Figure 1, with the Hamiltonian of the superconductor, where a = l, r stand for left and right SC with h l,SC = −h r,SC , J l = −J r and a,s,i and φ ( †) s,i the operators destroying (creating) an electron with spin s of the a = l, r SC and FM, respectively, at lattice site i, τ and σ the Pauli matrices acting on particle-hole and spin space respectively, f i,j = δ j,i±x + δ j,i±ŷ and g i,j = (±iδ j,i±x , ±iδ j,i±ŷ ) the even and odd in spatial inversion, respectively, functions connecting nearest neighbours lattice points. Moreover, t is the hopping integral and J the supercurrent term. The proximity of the SCs to the FIs is modelled by the introduction of an exchange field term in the H SC Equation (32). The SCs are connected with the FM wire through the following Hamiltonian In general, we consider t c = t for simplicity. MZMs are anticipated to emerge localised at the edges of the wire for |2t − is the induced by proximity conventional superconducting field over the FM. In Figure 2a we present the phase diagram for the setup of Figure 1 considering ∆/2t = 1, µ SC /2t = 0, J/2t = 0.2 and h SC /2t = 0.2. Based on this diagram, we observe that for µ FM < 2t, the induced singlet superconducting field over the FM is ∆ /2t 0.25 while the hopping term along the wire is normalised to t 0.86t, due to the coupling of the wire to the SCs [41]. For µ FM > 2t, again, the hopping term along the wire is normalised to t 0.86t and the black lines h FM /2t µ FM /2t − 2t /2t and h FM /2t µ FM /2t + 2t /2t define the region of parameters for which N = 1 and a pair of MZMs emerge at the edges of the FM wire. Notice that the particular phase diagram is in accordance with the topological criteria for the N = 1 and N = 2 topological phases presented in the previous section. However, we remark that the particular results correspond to a fixed conventional order parameter, which has not been self-consistently determined over the SC regions.
Therefore, the effect of finite momentum Cooper pairs, which, in principle, can emerge due to the presence of the supercurrent and the exchange field in the conventional superconductor, on the phase diagram (Figure 2), has not been investigated and will be examined in a future work.

Local Density of States
The pursuit of functional platforms for topological quantum computation, requires the experimental verification of the theoretical proposals for engineering topological superconductivity, by detecting the emergent MZMs. A characteristic signature of MZMs in conductance spectroscopy measurements is the quantized zero-bias tunnelling conductance. Emanating from an Andreev reflection resonant at zero energy, the zero bias conductance in the presence of a single MZMs pair equals 2e 2 h , i.e., double the conductance quantum, irrespective of the tunnelling barrier [42,43].
Several tunnelling experiments have demonstrated such zero bias conductance peaks and therefore provided supporting evidence for the emergence of MZMs in the semiconductor nanowires [44], the topological insulator/conventional superconductor heterostructures [45,46], the magnetic adatoms embedded in conventional superconductor [47], the heavy metal surfaces [48], the quantum anomalous Hall insulator [49], the iron-based superconductors [50] and the planar Josephson junctions [51] platforms. However, the results are far from being conclusive, since in each case several deviations from the corresponding theoretical predictions are observed.
Since differential conductance measurements in scanning tunnelling spectroscopy experiments are proportional to the local density of states of the sample, when the scanning tunnelling junction can be approximated by a point contact and the tunnelling amplitude is small, we calculate the local density of states at characteristic positions in the FM wire in order to link our results with relevant experiments. To this end, we solve the following eigenvalue equationĤ whereĤ i,j the Hamiltonian matrix of the FI-SC-FM-SC-FI heterostructure (Equation (31)) and u n,↑ (j) u n,↓ (j) v n,↑ (j) v n,↓ (j) T the eigenstate corresponding to eigenenergy E n . Based on the eigenstates and eigenvalues of the Hamiltonian we calculate the local density of states for spin up and down components according to the following equations the retarded Green's function. In order to account for the presence of impurities in the system, we consider a scattering time τ, which corresponds to a mean free path l = u F τ, where u F the Fermi velocity. Including the scattering from impurities, the density of states derives from equation where the Dirac function δ(ω − E n ) has been substituted by a Cauchy-Lorentz function 1 π γ (ω−E n ) 2 +γ 2 , with γ = 1/τ. Taking the clean superconductor limit, we assume that l/ξ 1000, where ξ = u F π∆ the superconducting coherence length, and therefore γ ∆ = πξ l 0.003. In Figure 3, we present the local density of states N(ω) for three values of the exchange field h FM of the wire considering µ FM /2t = 0.4, which corresponds to diagram (c) of Figure 2. From Figure 3a we deduce that the singlet pairing field induced in the wire, due to proximity with the conventional SC, is ∆ /∆ 0.25. Since in this case h FM < ∆ the FM is in a non-topological phase with N = 0. When h FM > ∆ the wire is in a topological N = 2 (Figure 3b) or N = 1 (Figure 3c) phase, and a peak for ω = 0 emerges at the local density of states spectrum only at the edges of the wire, signifying the presence of localised zero energy states, the MZMs.
For h FM /2t = 0.36 where N = 2 the two MZMs localised at the beginning of the wire, acquire opposite spin polarisation. The difference in the two zero energy peaks in Figure 3b indicates the different localization of the two MZMs, due to the difference in the Fermi velocity, u F = 2tsin(cos −1 ( −(±h FM +µ FM ) 2t ), among the two spin bands. The localization length l M of the MZMs equals l M = u F ∆ p . For h FM /2t = 0.72, a single pair of MZMs with particular spin polarisation emerges localised at the FM wire as indicated from the zero energy peak, which is significant for the spin down component. However, the zero energy density of states is also finite for the other spin component, due to the finite h SC .

Robustness of Emergent Majorana Zero Modes against Disorder
In realistic experimental setups, the presence of disorder is unavoidable. On this account, we demonstrate, in this section, the robustness of the emergent MZMs against disorder in the FM wire. In particular, we consider a random on-site potential δµ FM (x)τ z that derives from a normal distribution with mean value 0 and variance σ 2 corresponding to correlator < δµ FM The mean free path l along the wire is related to the variance through the following relation l = u F τ = u 2 f /σ 2 = u F /[πσ 2 N(µ)] where u F the Fermi velocity and N(µ) = 1/πu F the density of states at the Fermi level. In the lattice model described by Hamiltonian Equation (33), u F in the FM wire equals u F (µ) = 2tsin[cos −1 (−µ/2t)] considering a common Fermi velocity for the two spin components. We define the dimensionless parameter , where ξ = u F π∆ p is the coherence length of the p-wave superconductivity induced in the FM wire. In Figure 4, we present the low energy spectrum of the wire for µ FM /2t = 0.4 and h FM /2t = 0.36 for which N = 2 and h FM /2t = 0.72 for which N = 1.
For h FM /2t = 0.36, we observe that the energy gap essentially closes for l/ξ = 2, however, the spin up MZM remains at zero energy until 2l = ξ, which is the critical value of disorder for p-wave superconducting wires [52]. We attribute the difference in the critical mean free path for the two MZMs pairs in their different localization. For h FM /2t = 0.72 the energy gap closes at l ξ. We remark that in both cases, the energy gap is reduced by 50% with respect to that of a pristine wire when l 10ξ, signifying the robustness of the emergent MZMs against disorder of the chemical potential of the FM wire.
Finally, we investigate the robustness of the emergent MZMs against disorder in the exchange field h FM of the FM wire. We remark that our mechanism does not depend on the structural characteristics of the FM wire, which can therefore also be considered as an array of ferromagnetically aligned magnetic impurities. Magnetic impurities induce in the superconductor subgap bound states, the Yu-Shiba-Rusinov states [53][54][55]. Depending on the hopping integral among the impurities, these subgap states form an energy band, which may lie within the superconducting gap (Shiba limit), or extent above the superconducting energy gap (wire limit) [18]. Our mechanism is valid in both limits.
Considering this possible formation of the FM wire, it is worth examining the robustness of the emergent MZMs against disorder in the ferromagnetic alignment of the In both cases, the energy gap is reduced by 50% with respect to that of a pristine wire, for l 10ξ. (right) For h FM /2t = 0.72 the low energy spectrum with respect to magnetic disorder l m /ξ m . Although the energy gap is again reduced by approximately 50% for l m = 10ξ m , the MZMs appear to acquire finite energy only for l m < 3ξ m . Green and blue colours for the zero energy modes correspond to spin components as in Figure 3. E gap,0 is the energy gap in the pristine ferromagnetic wire. magnetic impurities and, therefore, in the corresponding orientation of the local exchange field, which otherwise is considered to have a fixed magnitude. In complete analogy to the previous case, we consider two normal distributions D θ = (0, σ m ) and D φ = (0, σ m ) for the angle θ of the local magnetisation with respect to the x-axis and for the angle φ in the y − z plane. We define a magnetic mean free path l m = u F σ 2 m N(µ) as a measure of disorder of the local exchange field and the magnetic coherence length ξ m = u F πh FM . In Figure 4, we present the low energy spectrum of the FM wire with respect to disorder strength l m /ξ m only for h FM /2t = 0.72. We note that for h FM /2t = 0.36 the two pairs of MZMs interact with each other and acquire finite energy even for infinitesimal magnetic disorder, since magnetic disorder breaks the spin symmetry that prevents the two MZMs from interacting with each other.

Conclusions
We present a novel platform for realising Majorana zero modes based on superconductor-ferromagnet heterostructures. The platform consists of a ferromagnetic wire placed among conventional superconductors, which are proximised by ferromagnetic insulators. Instead of spin-orbit coupling, the essential element of the physical mechanism underlying the proposed platform is the misalignment between the magnetisation of the ferromagnetic wire and that of the ferromagnetic insulators.
The robustness of the emergent MZMs against impurities disorder resembles that of a p superconducting wire, although the emergence of two pairs of MZMs and the observation of a zero bias conductance peak in the corresponding phase is hindered even for infinitesimal disorder in the magnetisation of the FM wire. We assert that recent developments in heterostructures fabrication renders our platform experimentally feasible, while the controllable application of the supercurrents in the superconductors provides an additional advantage with respect to other relevant proposals.

Abbreviations
The following abbreviations are used in this manuscript: