Numerical and Experimental Characterization of Fiber-Reinforced Thermoplastic Composite Structures with Embedded Piezoelectric Sensor-Actuator Arrays for Ultrasonic Applications †

The paper presents preliminary numerical and experimental studies of active textile-reinforced thermoplastic composites with embedded sensor-actuator arrays. The goal of the investigations was the assessment of directional sound wave generation capability using embedded sensor-actuator arrays and developed a wave excitation procedure for ultrasound measurement tasks. The feasibility of the proposed approach was initially confirmed in numerical investigations assuming idealized mechanical and geometrical conditions. The findings were validated in real-life conditions on specimens of elementary geometry. Herein, the technological aspects of unique automated assembly of thermoplastic films containing adapted thermoplastic-compatible piezoceramic modules and conducting paths were described.


Introduction
Textile-reinforced thermoplastic composites (TRTC) show a high potential for serial manufacturing of innovative function-integrating lightweight constructions.Due to the textile structure, the layered construction, and the associated specific production processes, such materials enable the possibility for a matrix-homogeneous integration of functional elements such as sensors, actuators, or even electronic circuit boards [1][2][3][4][5][6][7].The matrix-homogeneity is achieved by the utilization of identical thermoplastic materials both for the functional elements and the matrix of the composite component.Signals from integrated systems can be favorably utilized to broaden the application scope of TRTC through the implementation of auxiliary functions, e.g., active vibration damping, condition, or structural health monitoring [8,9].State of the art solutions utilize conventional piezoelectric transducers, e.g., macro-fiber composites, or active fiber composites, which are mainly adhesively bonded to the structural components [10,11].The associated assembly and bonding processes are characterized by several labor-extensive work steps.To successfully transform the current manual production process of active textile-reinforced thermoplastic composites into a fully automated mass production process, novel piezoelectric modules and adapted manufacturing technologies are necessary [12].In the following studies an assembly method is presented, which is based on an automated thermal or ultrasonic fixing of functional elements on thermoplastic carrier films.The assembly process has been named ePreforming and the respective outcome-a functionalized film-is called the ePreform [12,13].The ePreforming technology enables a direct coupling of the piezoceramic transducer to the host structure, which reduces deformation losses compared to adhesively-bonded transducers [10].Therefore, the coupling efficiency should be higher for integrated than bonded piezoceramic actuators.
A vital prerequisite for this process is the use of thermoplastic-compatible piezoceramic modules (TPMs).These modules are based on a piezoceramic functional layer (wafer or fiber composite) enclosed between two thermoplastic carrier films that are metallized with electrode structures.Thereby, the TPM-carrier films and the matrix of the fiber-reinforced composite components are made from identical materials.The possibility for ePreforming the whole arrays of actuators and sensors enables new application fields of these active structures with a high potential for ultrasonic measuring tasks, like the measurement of flow rate or distance.

Phenomenological Description
Embedded piezoelectric transducer arrays are suitable for transmission of mechanical waves into adjacent media (radiation of sound) and reception of sound waves.This property can be used for ultrasound-based measuring tasks, condition monitoring, or structural health monitoring (SHM) applications [14][15][16].For condition monitoring or SHM the influence of flaws, defects, or damage on the plate wave propagation characteristics is applied [17,18].For ultrasound measurement tasks the plate waves are used for an efficient radiation of sound waves into the adjacent media, e.g., water or air [19].This effect can also be reversed in order to receive the sound waves [20].

Ultrasound Radiation and Reception
The sound radiation and reception is based on the interaction of fluid and solid waves.Especially the flexural wave, also known as the first asymmetric Lamb wave mode (A 0 -mode), can be efficiently used for sound radiation due to the high out-of-plane displacement amplitudes.An exemplary interaction between the waves in the plate and acoustic waves is shown in Figure 1.
Appl.Sci.2016, 6, 55 2 of 13 thermoplastic carrier films.The assembly process has been named ePreforming and the respective outcome-a functionalized film-is called the ePreform [12,13].The ePreforming technology enables a direct coupling of the piezoceramic transducer to the host structure, which reduces deformation losses compared to adhesively-bonded transducers [10].Therefore, the coupling efficiency should be higher for integrated than bonded piezoceramic actuators.
A vital prerequisite for this process is the use of thermoplastic-compatible piezoceramic modules (TPMs).These modules are based on a piezoceramic functional layer (wafer or fiber composite) enclosed between two thermoplastic carrier films that are metallized with electrode structures.Thereby, the TPM-carrier films and the matrix of the fiber-reinforced composite components are made from identical materials.The possibility for ePreforming the whole arrays of actuators and sensors enables new application fields of these active structures with a high potential for ultrasonic measuring tasks, like the measurement of flow rate or distance.

Phenomenological Description
Embedded piezoelectric transducer arrays are suitable for transmission of mechanical waves into adjacent media (radiation of sound) and reception of sound waves.This property can be used for ultrasound-based measuring tasks, condition monitoring, or structural health monitoring (SHM) applications [14][15][16].For condition monitoring or SHM the influence of flaws, defects, or damage on the plate wave propagation characteristics is applied [17,18].For ultrasound measurement tasks the plate waves are used for an efficient radiation of sound waves into the adjacent media, e.g., water or air [19].This effect can also be reversed in order to receive the sound waves [20].

Ultrasound Radiation and Reception
The sound radiation and reception is based on the interaction of fluid and solid waves.Especially the flexural wave, also known as the first asymmetric Lamb wave mode (A0-mode), can be efficiently used for sound radiation due to the high out-of-plane displacement amplitudes.An exemplary interaction between the waves in the plate and acoustic waves is shown in Figure 1.The radiation of the Lamb waves into the adjacent fluid takes place at an angle φ which results from the ratio of the wavelength in the fluid λF to the wavelength of the Lamb wave λP.This angle can be calculated either from the wavelengths or from the velocities of the waves using the following equation: wherein cF is the speed of sound in the fluid and cP is the phase velocity of the flexural wave in the plate.Since the phase velocity is not only a function of the mechanical material properties but also of the excitation frequency, the radiation angle can be set by modifying the excitation signal characteristics of the structure-integrated actuators.In order to scrutinize the procedure to set the The radiation of the Lamb waves into the adjacent fluid takes place at an angle ϕ which results from the ratio of the wavelength in the fluid λ F to the wavelength of the Lamb wave λ P .This angle can be calculated either from the wavelengths or from the velocities of the waves using the following equation: wherein c F is the speed of sound in the fluid and c P is the phase velocity of the flexural wave in the plate.Since the phase velocity is not only a function of the mechanical material properties but also of the excitation frequency, the radiation angle can be set by modifying the excitation signal characteristics of the structure-integrated actuators.In order to scrutinize the procedure to set the radiation angle a case study employing the mechanical properties of the analyzed material is presented below.Glass fiber-reinforced polyamide 6 (GF/PA6) plate with the thickness of 2 mm is studied.The dispersion curves-describing the relation between the wave speed and the excitation frequency-can be calculated analytically based on mathematical relation presented in various textbooks (see e.g., [21]) by assuming isotropic material properties (Young's modulus E = 20 GPa, mass density ρ = 1800 kg/m³, Poisson's ratio ν = 0.3). Figure 2 shows the dispersion curves with the phase velocities and the group velocities of the A 0 -and the S 0 -modes.radiation angle a case study employing the mechanical properties of the analyzed material is presented below.Glass fiber-reinforced polyamide 6 (GF/PA6) plate with the thickness of 2 mm is studied.The dispersion curves-describing the relation between the wave speed and the excitation frequency-can be calculated analytically based on mathematical relation presented in various textbooks (see e.g., [21]) by assuming isotropic material properties (Young's modulus E = 20 GPa, mass density ρ = 1800 kg/m³, Poisson's ratio ν = 0.3). Figure 2 shows the dispersion curves with the phase velocities and the group velocities of the A0and the S0-modes.The wavelength calculated from the phase velocity of the A0-mode is shown in Figure 3A as a function of the excitation frequency.For the radiation in the air (cF = 340 m/s), the radiation angle is shown in Figure 3B.For example, at a frequency of 35 kHz the A0 Lamb wave phase velocity is 640 m/s and the resulting wavelength of the flexural wave is 18.2 mm.The wavelength in air is 9.7 mm which leads to a radiation angle of 58°.As Figure 3 shows, this angle increases with increasing frequency.The angle can be adjusted to specific applications either by adapting the material and the thickness of the plate or by changing the excitation frequency.

Transducer Arrays for the Generation of Directional Waves in a Plate
For some measurement applications, especially when localization of obstacles is of key interest, it is advantageous to directionally send or receive sound waves.The first step to obtain directional ultrasound radiation is the generation of directional flexural waves in the plate.This can be achieved by using transducer arrays instead of a single transducer.Through adaptation of the actuator array configuration, the mainly excited or received wave mode can be precisely controlled [22].The wavelength calculated from the phase velocity of the A 0 -mode is shown in Figure 3A as a function of the excitation frequency.For the radiation in the air (c F = 340 m/s), the radiation angle is shown in Figure 3B.radiation angle a case study employing the mechanical properties of the analyzed material is presented below.Glass fiber-reinforced polyamide 6 (GF/PA6) plate with the thickness of 2 mm is studied.The dispersion curves-describing the relation between the wave speed and the excitation frequency-can be calculated analytically based on mathematical relation presented in various textbooks (see e.g., [21]) by assuming isotropic material properties (Young's modulus E = 20 GPa, mass density ρ = 1800 kg/m³, Poisson's ratio ν = 0.3). Figure 2 shows the dispersion curves with the phase velocities and the group velocities of the A0and the S0-modes.The wavelength calculated from the phase velocity of the A0-mode is shown in Figure 3A as a function of the excitation frequency.For the radiation in the air (cF = 340 m/s), the radiation angle is shown in Figure 3B.For example, at a frequency of 35 kHz the A0 Lamb wave phase velocity is 640 m/s and the resulting wavelength of the flexural wave is 18.2 mm.The wavelength in air is 9.7 mm which leads to a radiation angle of 58°.As Figure 3 shows, this angle increases with increasing frequency.The angle can be adjusted to specific applications either by adapting the material and the thickness of the plate or by changing the excitation frequency.

Transducer Arrays for the Generation of Directional Waves in a Plate
For some measurement applications, especially when localization of obstacles is of key interest, it is advantageous to directionally send or receive sound waves.The first step to obtain directional ultrasound radiation is the generation of directional flexural waves in the plate.This can be achieved by using transducer arrays instead of a single transducer.Through adaptation of the actuator array configuration, the mainly excited or received wave mode can be precisely controlled [22].For example, at a frequency of 35 kHz the A 0 Lamb wave phase velocity is 640 m/s and the resulting wavelength of the flexural wave is 18.2 mm.The wavelength in air is 9.7 mm which leads to a radiation angle of 58 ˝.As Figure 3 shows, this angle increases with increasing frequency.The angle can be adjusted to specific applications either by adapting the material and the thickness of the plate or by changing the excitation frequency.

Transducer Arrays for the Generation of Directional Waves in a Plate
For some measurement applications, especially when localization of obstacles is of key interest, it is advantageous to directionally send or receive sound waves.The first step to obtain directional ultrasound radiation is the generation of directional flexural waves in the plate.This can be achieved by using transducer arrays instead of a single transducer.Through adaptation of the actuator array configuration, the mainly excited or received wave mode can be precisely controlled [22].Furthermore, the directivity of the waves can also be adjusted [23,24].The simplest setup is a one-dimensional array on the surface of the plate.Depending on the size and the distance between the individual transducers and the time-delays in the electrical driving signal, the directional characteristics can be adjusted, for example, to amplify the wave generation in one direction.It is also possible to use electronic beam-steering (see e.g., [25]) in order to vary the direction of the dominant wave generation.
For a one-dimensional array the optimal delay time for an additive superposition in the array longitudinal direction can be analytically calculated using the transducer offset ∆l and the phase velocity c p .In the case of a GF/PA6 plate and a 15 mm offset between the actuators the optimal time delay yields [26]:

Application of Integrated Transducer Arrays for Generation of Sound Waves
In order to confirm the capability to apply the integrated transducer arrays for effective generation of sound waves, firstly, a numerical model has been elaborated, where the possibility to generate a directional wave is analyzed.These investigations were followed by the experimental investigations where, firstly, the manufacturing process of the active composite is described, followed by the characterization of the waves in the plate using a laser scanning vibrometer and the measurement of the resulting sound waves in the air using a microphone.

Numerical Investigations
A three-dimensional parametrical model consisting of two sub-models: a free-free supported plate and attached to it four piezoelectric transducers (transducer array), was elaborated (see Figure 4).The model has been created using commercially available finite-element software [27].To realistically simulate the interaction between the electrical driving signal of the transducers and the resulting solid waves, a coupled electromechanical problem has to be solved.Therefore the transducers were modeled as 3-D, 20-node, coupled-field solid elements (SOLID 226).The elastic base structure has been meshed with 116,568 elements of type SOLID 186 with a maximum element size of 0.2 mm.
Furthermore, the directivity of the waves can also be adjusted [23,24].The simplest setup is a one-dimensional array on the surface of the plate.Depending on the size and the distance between the individual transducers and the time-delays in the electrical driving signal, the directional characteristics can be adjusted, for example, to amplify the wave generation in one direction.It is also possible to use electronic beam-steering (see e.g., [25]) in order to vary the direction of the dominant wave generation.
For a one-dimensional array the optimal delay time for an additive superposition in the array longitudinal direction can be analytically calculated using the transducer offset Δl and the phase velocity cp.In the case of a GF/PA6 plate and a 15 mm offset between the actuators the optimal time delay yields [26]:

Application of Integrated Transducer Arrays for Generation of Sound Waves
In order to confirm the capability to apply the integrated transducer arrays for effective generation of sound waves, firstly, a numerical model has been elaborated, where the possibility to generate a directional wave is analyzed.These investigations were followed by the experimental investigations where, firstly, the manufacturing process of the active composite is described, followed by the characterization of the waves in the plate using a laser scanning vibrometer and the measurement of the resulting sound waves in the air using a microphone.

Numerical Investigations
A three-dimensional parametrical model consisting of two sub-models: a free-free supported plate and attached to it four piezoelectric transducers (transducer array), was elaborated (see Figure 4).The model has been created using commercially available finite-element software [27].To realistically simulate the interaction between the electrical driving signal of the transducers and the resulting solid waves, a coupled electromechanical problem has to be solved.Therefore the transducers were modeled as 3-D, 20-node, coupled-field solid elements (SOLID 226).The elastic base structure has been meshed with 116,568 elements of type SOLID 186 with a maximum element size of 0.2 mm.
In order to capture the time-and space-dependent phenomena connected with the propagation of mechanical waves, a transient analysis with the time step of 2.5 µs has been performed.Herein, the termination time was set to 500 µs which results in 200 load steps per one simulation.The mechanical properties of the base structure are presented in Appendix A.  In order to capture the time-and space-dependent phenomena connected with the propagation of mechanical waves, a transient analysis with the time step of 2.5 µs has been performed.Herein, the termination time was set to 500 µs which results in 200 load steps per one simulation.The mechanical properties of the base structure are presented in Table A1.
The transducers were driven by a Hann-windowed sine signal with 35 kHz center frequency and amplitude A equal to 6 V (Figure 5).The signal characteristics have been selected based on the technical specifications of the existing devices, planned to be used in the experimental investigations.
predefined moments in order to amplify the desired plate mode as well as to shape the directional characteristics of the propagating wave.The geometrical configuration together with the material properties of the base structure governs the optimal time delay (Δt) which in the presented study equals 23.4 µs (see section 2).
Since the analyzed phenomena are time-and location-dependent, a simple and informative presentation of the results is greatly limited.In order to visualize the wave field, snapshots at some time step have been created.For the results presentation, the wave field for one time step namely at 20 µs has been selected based on the following criteria:  the wave has to propagate through some distance in order to reveal its directivity and plate mode character; and  the reflections of higher Lamb modes-if any present-from the plate edges should not interfere with the main wave front;   In order to generate directional waves in the plate, the transducers have to be activated in predefined moments in order to amplify the desired plate mode as well as to shape the directional characteristics of the propagating wave.The geometrical configuration together with the material properties of the base structure governs the optimal time delay (∆t) which in the presented study equals 23.4 µs (see Section 2).

Manufacturing Process
Since the analyzed phenomena are time-and location-dependent, a simple and informative presentation of the results is greatly limited.In order to visualize the wave field, snapshots at some time step have been created.For the results presentation, the wave field for one time step namely at 20 µs has been selected based on the following criteria:

‚
the wave has to propagate through some distance in order to reveal its directivity and plate mode character; and ‚ the reflections of higher Lamb modes-if any present-from the plate edges should not interfere with the main wave front; The obtained results (Figure 6) confirmed that through application deliberately-activated structure-integrated transducers organized into a linear array the generation of directional wave is possible.It is clearly visible that the wave amplitudes along the main wave propagation direction are amplified in comparison with those propagating in the other direction.It can be observed that some side lobes are also present.In order to confirm these observations experimental investigations on nominally-identical structures have been conducted.The transducers were driven by a Hann-windowed sine signal with 35 kHz center frequency and amplitude A equal to 6 V (Figure 5).The signal characteristics have been selected based on the technical specifications of the existing devices, planned to be used in the experimental investigations.
In order to generate directional waves in the plate, the transducers have to be activated in predefined moments in order to amplify the desired plate mode as well as to shape the directional characteristics of the propagating wave.The geometrical configuration together with the material properties of the base structure governs the optimal time delay (Δt) which in the presented study equals 23.4 µs (see section 2).
Since the analyzed phenomena are time-and location-dependent, a simple and informative presentation of the results is greatly limited.In order to visualize the wave field, snapshots at some time step have been created.For the results presentation, the wave field for one time step namely at 20 µs has been selected based on the following criteria:  the wave has to propagate through some distance in order to reveal its directivity and plate mode character; and  the reflections of higher Lamb modes-if any present-from the plate edges should not interfere with the main wave front;   For the animation of the wave field please refer to supplementary material.

Manufacturing Process
For investigations regarding the application of structure-integrated transducers for sound wave generation, manufacturing of the active textile-reinforced thermoplastic composites (TRTC), the application of thermoplastic-compatible piezoceramic modules (TPMs) on the surface of a fiber-reinforced semi-finished plate (organic sheet) was necessary.The organic sheet consists of a glass fiber-reinforced polyamide 6 (type: 102-RG600(x)/47% Roving Glass-PA 6 Consolidated Composite Laminate produced by Bond-Laminates GmbH).The ePreform consists of a polyamide 6 (PA 6) film with a thickness of 100 µm.In regard to the built up of the TPM, commercially available monolithic wafers (type: PZT 5A1, electromechanical properties can be found in Table A2) with a square area of 100 mm² and a thickness of 0.2 mm were used (see Figure 7B).The outer surfaces of the wafers were metallized by silver printed electrodes and contacted by conductive copper tapes.This layup was embedded into two PA 6 carrier films with a thickness of 100 µm (see Figure 7A).The TPMs are polarized in the thickness direction and work in the d 31 mode, which means a principal deflection normal to the polarization direction.For investigations regarding the application of structure-integrated transducers for sound wave generation, manufacturing of the active textile-reinforced thermoplastic composites (TRTC), the application of thermoplastic-compatible piezoceramic modules (TPMs) on the surface of a fiberreinforced semi-finished plate (organic sheet) was necessary.The organic sheet consists of a glass fiber-reinforced polyamide 6 (type: 102-RG600(x)/47% Roving Glass-PA 6 Consolidated Composite Laminate produced by Bond-Laminates GmbH).The ePreform consists of a polyamide 6 (PA 6) film with a thickness of 100 µm.In regard to the built up of the TPM, commercially available monolithic wafers (type: PZT 5A1) with a square area of 100 mm² and a thickness of 0.2 mm were used (see Figure 7B).The outer surfaces of the wafers were metallized by silver printed electrodes and contacted by conductive copper tapes.This layup was embedded into two PA 6 carrier films with a thickness of 100 µm (see Figure 7A).The TPMs are polarized in the thickness direction and work in the d31 mode, which means a principal deflection normal to the polarization direction.A major precondition for the embedding of the TPMs into the composite structures is the use of identical thermoplastic materials for the TPM carrier films and the matrix of the fiber-reinforced structure.During the consolidation, the module will be matrix homogeneous integrated into the composite structure.Compared to adhesively-bonded modules the integration of TPM enables an efficient coupling of the piezoceramic layer to the reinforcement as shown in Figure 8.The conceptual manufacturing process for active TRTC, which bases on a press technology, starts with the first process step, the so-called ePreforming process.It comprises the rollup and cutting of a thermoplastic film, the precise positioning, and fixing of TPMs, the application of conductive paths and the accompanied electrical contacting (see Figure 9).A major precondition for the embedding of the TPMs into the composite structures is the use of identical thermoplastic materials for the TPM carrier films and the matrix of the fiber-reinforced structure.During the consolidation, the module will be matrix homogeneous integrated into the composite structure.Compared to adhesively-bonded modules the integration of TPM enables an efficient coupling of the piezoceramic layer to the reinforcement as shown in Figure 8.For investigations regarding the application of structure-integrated transducers for sound wave generation, manufacturing of the active textile-reinforced thermoplastic composites (TRTC), the application of thermoplastic-compatible piezoceramic modules (TPMs) on the surface of a fiberreinforced semi-finished plate (organic sheet) was necessary.The organic sheet consists of a glass fiber-reinforced polyamide 6 (type: 102-RG600(x)/47% Roving Glass-PA 6 Consolidated Composite Laminate produced by Bond-Laminates GmbH).The ePreform consists of a polyamide 6 (PA 6) film with a thickness of 100 µm.In regard to the built up of the TPM, commercially available monolithic wafers (type: PZT 5A1) with a square area of 100 mm² and a thickness of 0.2 mm were used (see Figure 7B).The outer surfaces of the wafers were metallized by silver printed electrodes and contacted by conductive copper tapes.This layup was embedded into two PA 6 carrier films with a thickness of 100 µm (see Figure 7A).The TPMs are polarized in the thickness direction and work in the d31 mode, which means a principal deflection normal to the polarization direction.A major precondition for the embedding of the TPMs into the composite structures is the use of identical thermoplastic materials for the TPM carrier films and the matrix of the fiber-reinforced structure.During the consolidation, the module will be matrix homogeneous integrated into the composite structure.Compared to adhesively-bonded modules the integration of TPM enables an efficient coupling of the piezoceramic layer to the reinforcement as shown in Figure 8.The conceptual manufacturing process for active TRTC, which bases on a press technology, starts with the first process step, the so-called ePreforming process.It comprises the rollup and cutting of a thermoplastic film, the precise positioning, and fixing of TPMs, the application of conductive paths and the accompanied electrical contacting (see Figure 9).The conceptual manufacturing process for active TRTC, which bases on a press technology, starts with the first process step, the so-called ePreforming process.It comprises the rollup and cutting of a thermoplastic film, the precise positioning, and fixing of TPMs, the application of conductive paths and the accompanied electrical contacting (see Figure 9).In the developed manufacturing process (see Figure 10) the ePreform is positioned in the pressing die and covered by a preheated and melted organic sheet and, subsequently, the press closes.During the consolidation the TPMs are simultaneously polarized [28].In regard to the manufacturing of the ePreform an especially-developed ePreforming unit was used in order to assure the automated assembly of thermoplastic films with TPM and the necessary conductors.The transfer of TPM from storage to the predefined position is realized by a vacuum gripper, whereas the fixation to the thermoplastic film can be realized by thermal stapling or ultrasonic welding.In this investigation the TPM were fixed by thermal stapling.The leads are automatically rolled up from the wire coil, fixed by thermal welding points, and cut at the end of the conductive paths.In these studies the leads consists of tin-coated copper wires with a diameter of 0.21 mm.Furthermore the TPMs, shown in Figure 11, are arranged to a linear pattern of six elements which have an offset of the piezoceramic wafers of 15 mm (see Figure 11).
For the initial prototypic tests the ePreform was positioned and fixed at the organic sheet plate manually using thermal resistant polyimide tape.The plate had dimensions of 1000 mm length, 600 mm width, and 2 mm thickness, and the TPM pattern was positioned 250 mm from the short side in the middle of the plate.In contrast to the introduced manufacturing process of such active parts, the consolidation of the investigated plate was performed by an autoclave process because of its prototypic configuration.The main process parameters are a maximum temperature of 230 °C, a dwell time at maximum temperature for 2 min, a consolidation pressure of 5 bar, and a vacuum of 20 mbar.In the developed manufacturing process (see Figure 10) the ePreform is positioned in the pressing die and covered by a preheated and melted organic sheet and, subsequently, the press closes.During the consolidation the TPMs are simultaneously polarized [28].In the developed manufacturing process (see Figure 10) the ePreform is positioned in the pressing die and covered by a preheated and melted organic sheet and, subsequently, the press closes.During the consolidation the TPMs are simultaneously polarized [28].In regard to the manufacturing of the ePreform an especially-developed ePreforming unit was used in order to assure the automated assembly of thermoplastic films with TPM and the necessary conductors.The transfer of TPM from storage to the predefined position is realized by a vacuum gripper, whereas the fixation to the thermoplastic film can be realized by thermal stapling or ultrasonic welding.In this investigation the TPM were fixed by thermal stapling.The leads are automatically rolled up from the wire coil, fixed by thermal welding points, and cut at the end of the conductive paths.In these studies the leads consists of tin-coated copper wires with a diameter of 0.21 mm.Furthermore the TPMs, shown in Figure 11, are arranged to a linear pattern of six elements which have an offset of the piezoceramic wafers of 15 mm (see Figure 11).
For the initial prototypic tests the ePreform was positioned and fixed at the organic sheet plate manually using thermal resistant polyimide tape.The plate had dimensions of 1000 mm length, 600 mm width, and 2 mm thickness, and the TPM pattern was positioned 250 mm from the short side in the middle of the plate.In contrast to the introduced manufacturing process of such active parts, the consolidation of the investigated plate was performed by an autoclave process because of its prototypic configuration.The main process parameters are a maximum temperature of 230 °C, a dwell time at maximum temperature for 2 min, a consolidation pressure of 5 bar, and a vacuum of 20 mbar.In regard to the manufacturing of the ePreform an especially-developed ePreforming unit was used in order to assure the automated assembly of thermoplastic films with TPM and the necessary conductors.The transfer of TPM from storage to the predefined position is realized by a vacuum gripper, whereas the fixation to the thermoplastic film can be realized by thermal stapling or ultrasonic welding.In this investigation the TPM were fixed by thermal stapling.The leads are automatically rolled up from the wire coil, fixed by thermal welding points, and cut at the end of the conductive paths.In these studies the leads consists of tin-coated copper wires with a diameter of 0.21 mm.Furthermore the TPMs, shown in Figure 11, are arranged to a linear pattern of six elements which have an offset of the piezoceramic wafers of 15 mm (see Figure 11).
For the initial prototypic tests the ePreform was positioned and fixed at the organic sheet plate manually using thermal resistant polyimide tape.The plate had dimensions of 1000 mm length, 600 mm width, and 2 mm thickness, and the TPM pattern was positioned 250 mm from the short side in the middle of the plate.In contrast to the introduced manufacturing process of such active parts, the consolidation of the investigated plate was performed by an autoclave process because of its prototypic configuration.The main process parameters are a maximum temperature of 230 ˝C, a dwell time at maximum temperature for 2 min, a consolidation pressure of 5 bar, and a vacuum of 20 mbar.

Experimental Investigations
The aim of the experimental studies was to characterize the generation of a directed acoustic wave using the integrated actuator array.Herein, two experimental techniques were utilized, i.e. laser Doppler vibrometry (LDV) and microphone measurements in order to identify the actuator-induced wave propagation of the investigated plate and the corresponding acoustic wave.

Laser Doppler Vibrometry
To assess the mechanical wave induced by the actuators, a series of experiments using the scanning laser Doppler vibrometer (type PSV-400 produced by Polytec GmbH, Waldbronn, Germany) were conducted.The application of a contactless measurement system guarantees that the mechanical properties of the investigated object are not distorted by the additional mass of typical vibration sensors.
Since the output signal of the laser scanning vibrometer is directly proportional to the velocity of the targeted surface along the laser beam direction, the LDV has been positioned normal to the analyzed plate.In order to assure to high reflection of the laser light and, hence, a high signal-to-noise ratio, a large section on the plate surface was covered with a reflective spray paint.A regular spatial distribution of 55 × 97 discrete measuring points in approximately 2 mm distance has been selected to guarantee reliable capturing of the wave's spatial and time development.The investigated plate was hung vertically using a thin light rope (Figure 12).The actuators were excited with a typical burst signal as it can be used for different measurement tasks.Based on the plate dimensions and the array setup a center frequency of 35 kHz was chosen.The signal consists of a four-periods-long sinusoidal signal which was windowed with a Hann

Experimental Investigations
The aim of the experimental studies was to characterize the generation of a directed acoustic wave using the integrated actuator array.Herein, two experimental techniques were utilized, i.e. laser Doppler vibrometry (LDV) and microphone measurements in order to identify the actuator-induced wave propagation of the investigated plate and the corresponding acoustic wave.

Laser Doppler Vibrometry
To assess the mechanical wave induced by the actuators, a series of experiments using the scanning laser Doppler vibrometer (type PSV-400 produced by Polytec GmbH, Waldbronn, Germany) were conducted.The application of a contactless measurement system guarantees that the mechanical properties of the investigated object are not distorted by the additional mass of typical vibration sensors.
Since the output signal of the laser scanning vibrometer is directly proportional to the velocity of the targeted surface along the laser beam direction, the LDV has been positioned normal to the analyzed plate.In order to assure to high reflection of the laser light and, hence, a high signal-to-noise ratio, a large section on the plate surface was covered with a reflective spray paint.A regular spatial distribution of 55 ˆ97 discrete measuring points in approximately 2 mm distance has been selected to guarantee reliable capturing of the wave's spatial and time development.The investigated plate was hung vertically using a thin light rope (Figure 12).

Experimental Investigations
The aim of the experimental studies was to characterize the generation of a directed acoustic wave using the integrated actuator array.Herein, two experimental techniques were utilized, i.e. laser Doppler vibrometry (LDV) and microphone measurements in order to identify the actuator-induced wave propagation of the investigated plate and the corresponding acoustic wave.

Laser Doppler Vibrometry
To assess the mechanical wave induced by the actuators, a series of experiments using the scanning laser Doppler vibrometer (type PSV-400 produced by Polytec GmbH, Waldbronn, Germany) were conducted.The application of a contactless measurement system guarantees that the mechanical properties of the investigated object are not distorted by the additional mass of typical vibration sensors.
Since the output signal of the laser scanning vibrometer is directly proportional to the velocity of the targeted surface along the laser beam direction, the LDV has been positioned normal to the analyzed plate.In order to assure to high reflection of the laser light and, hence, a high signal-to-noise ratio, a large section on the plate surface was covered with a reflective spray paint.A regular spatial distribution of 55 × 97 discrete measuring points in approximately 2 mm distance has been selected to guarantee reliable capturing of the wave's spatial and time development.The investigated plate was hung vertically using a thin light rope (Figure 12).The actuators were excited with a typical burst signal as it can be used for different measurement tasks.Based on the plate dimensions and the array setup a center frequency of 35 kHz was chosen.The signal consists of a four-periods-long sinusoidal signal which was windowed with a Hann The actuators were excited with a typical burst signal as it can be used for different measurement tasks.Based on the plate dimensions and the array setup a center frequency of 35 kHz was chosen.The signal consists of a four-periods-long sinusoidal signal which was windowed with a Hann window to limit the bandwidth.The triggered 2.5 ms long time series of out-of-plane velocities were recorded Appl.Sci.2016, 6, 55 9 of 13 20 times in every point and subsequently averaged to reduce the noise content in the acquired signals.
The time resolution of the LDV was set to 4.883 µs to assure at least five samples per measured signal period.

Microphone Measurements
Due to the excitation of the integrated actuator-array mechanical flexural plate waves were generated.In regard to the achievement of a directed radiation of plate waves, the excitations of the transducers were delayed 24 µs relatively to the previous transducer.In regard to the directional characteristic of the acoustic wave and the defined radiation angle, the spatial distribution of sound pressure was recorded.For this purpose a ¼" free-field microphone (MK301, Microtech Gefell, Gefell, Germany) was used and the sound pressure was determined at different heights (10 mm, 30 mm, 70 mm) over the plate.The raster of the discrete measuring points in each height was set to 20 mm. Figure 13 shows the planar coordinate system in the plate plane, whereupon the origin was set to the end of the first transducer element.
Appl.Sci.2016, 6, 55 9 of 13 window to limit the bandwidth.The triggered 2.5 ms long time series of out-of-plane velocities were recorded 20 times in every point and subsequently averaged to reduce the noise content in the acquired signals.The time resolution of the LDV was set to 4.883 µs to assure at least five samples per measured signal period.

Microphone Measurements
Due to the excitation of the integrated actuator-array mechanical flexural plate waves were generated.In regard to the achievement of a directed radiation of plate waves, the excitations of the transducers were delayed 24 µs relatively to the previous transducer.In regard to the directional characteristic of the acoustic wave and the defined radiation angle, the spatial distribution of sound pressure was recorded.For this purpose a ¼" free-field microphone (MK301, Microtech Gefell, Gefell, Germany) was used and the sound pressure was determined at different heights (10 mm, 30 mm, 70 mm) over the plate.The raster of the discrete measuring points in each height was set to 20 mm. Figure 13 shows the planar coordinate system in the plate plane, whereupon the origin was set to the end of the first transducer element.The recorded time series of out-of-plane velocities and sound pressures obtained using the laser Doppler velocimetry technique and microphone provide a basis for the subsequent analysis regarding the mechanical and acoustic wave propagation.The results of this analysis are presented in this section.

Propagation of Structural Mechanical Waves
Mainly, the impact of the time delay between the actuator initialization has been studied.The wavefront for cases with zero time delay and optimal time delay are presented in Figure 14.In this context, an optimal time delay of 24 µs was experimentally determined.The difference of 0.6 µs between theoretical and experimental delay times (see Section 2) is affected by uncertainties and tolerances of the geometry and the material properties of the experimental setup.The recorded time series of out-of-plane velocities and sound pressures obtained using the laser Doppler velocimetry technique and microphone provide a basis for the subsequent analysis regarding the mechanical and acoustic wave propagation.The results of this analysis are presented in this section.

Propagation of Structural Mechanical Waves
Mainly, the impact of the time delay between the actuator initialization has been studied.The wavefront for cases with zero time delay and optimal time delay are presented in Figure 14.In this context, an optimal time delay of 24 µs was experimentally determined.The difference of 0.6 µs between theoretical and experimental delay times (see Section 2) is affected by uncertainties and tolerances of the geometry and the material properties of the experimental setup.
Appl.Sci.2016, 6, 55 9 of 13 window to limit the bandwidth.The triggered 2.5 ms long time series of out-of-plane velocities were recorded 20 times in every point and subsequently averaged to reduce the noise content in the acquired signals.The time resolution of the LDV was set to 4.883 µs to assure at least five samples per measured signal period.

Microphone Measurements
Due to the excitation of the integrated actuator-array mechanical flexural plate waves were generated.In regard to the achievement of a directed radiation of plate waves, the excitations of the transducers were delayed 24 µs relatively to the previous transducer.In regard to the directional characteristic of the acoustic wave and the defined radiation angle, the spatial distribution of sound pressure was recorded.For this purpose a ¼" free-field microphone (MK301, Microtech Gefell, Gefell, Germany) was used and the sound pressure was determined at different heights (10 mm, 30 mm, 70 mm) over the plate.The raster of the discrete measuring points in each height was set to 20 mm. Figure 13 shows the planar coordinate system in the plate plane, whereupon the origin was set to the end of the first transducer element.The recorded time series of out-of-plane velocities and sound pressures obtained using the laser Doppler velocimetry technique and microphone provide a basis for the subsequent analysis regarding the mechanical and acoustic wave propagation.The results of this analysis are presented in this section.

Propagation of Structural Mechanical Waves
Mainly, the impact of the time delay between the actuator initialization has been studied.The wavefront for cases with zero time delay and optimal time delay are presented in Figure 14.In this context, an optimal time delay of 24 µs was experimentally determined.The difference of 0.6 µs between theoretical and experimental delay times (see Section 2) is affected by uncertainties and tolerances of the geometry and the material properties of the experimental setup.It is clearly observable that, while for the zero time delay the wave propagates equally in positive and negative y-direction, for the case with the optimized time delay, the wave propagates mainly in the positive y-direction.Additionally, the wave amplitude of the latter case was twice as much as in the first case.In order to generate evidence, that such wavefronts cause a directed sound wave, the signals recorded using the microphone were analyzed.

Propagation of Acoustic Waves
Figure 15 shows the maximum sound pressure of the received bursts for the scanned heights.Herein, the results for the plane 10 mm above the structure show an obvious maximum of about 90 dB at the end of the array.In a height of 70 mm the sound pressure level is about 82 dB to 84 dB and extended over a larger area.The measured data fits quite well to the expected radiation angle of approximately 60 ˝.
Appl.Sci.2016, 6, 55 10 of 13 It is clearly observable that, while for the zero time delay the wave propagates equally in positive and negative y-direction, for the case with the optimized time delay, the wave propagates mainly in the positive y-direction.Additionally, the wave amplitude of the latter case was twice as much as in the first case.In order to generate evidence, that such wavefronts cause a directed sound wave, the signals recorded using the microphone were analyzed.

Propagation of Acoustic Waves
Figure 15 shows the maximum sound pressure of the received bursts for the scanned heights.Herein, the results for the plane 10 mm above the structure show an obvious maximum of about 90 dB at the end of the array.In a height of 70 mm the sound pressure level is about 82 dB to 84 dB and extended over a larger area.The measured data fits quite well to the expected radiation angle of approximately 60°.On closer examination of the results, the lateral emission of ultrasound (side lobes) is recognizable.This is caused by the side lobes of the plate waves discussed in the previous section.These side lobes can be suppressed or prevented by a modified array design.

Conclusions and Outlook
The integration of sensors and actuators like piezoceramic modules exhibits a high potential to functionalize composite materials.Especially, a manufacturing technology ready for serial production can reduce the costs of active structures and, thus, lead to a wider range of possible applications.The developed ePreforming technology gives the possibility to integrate sensors and actuators into composites using established manufacturing technologies, like press processes.Furthermore, the process enables the integration of sensor-actuator arrays with reproducible positioning.Both possibilities could be validated in the performed manufacturing studies.Moreover, the robustness of the ePreforming technique, in terms of fatigue behavior in comparison with conventionally-bonded functional elements, will be analyzed in further studies.
Considering the functional testing, experimental studies were done, showing the high potential of piezoelectric transducer arrays for an angular radiation of ultrasound waves.In the future, this effect can be used to realize new material-integrated concepts for measuring distances or flow rates.Additionally, the developed concept can be applied for SHM applications based on the analysis of Lamb wave scatter on discontinuities or cracks.On closer examination of the results, the lateral emission of ultrasound (side lobes) is recognizable.This is caused by the side lobes of the plate waves discussed in the previous section.These side lobes can be suppressed or prevented by a modified array design.

Conclusions and Outlook
The integration of sensors and actuators like piezoceramic modules exhibits a high potential to functionalize composite materials.Especially, a manufacturing technology ready for serial production can reduce the costs of active structures and, thus, lead to a wider range of possible applications.The developed ePreforming technology gives the possibility to integrate sensors and actuators into composites using established manufacturing technologies, like press processes.Furthermore, the process enables the integration of sensor-actuator arrays with reproducible positioning.Both possibilities could be validated in the performed manufacturing studies.Moreover, the robustness of the ePreforming technique, in terms of fatigue behavior in comparison with conventionally-bonded functional elements, will be analyzed in further studies.
Considering the functional testing, experimental studies were done, showing the high potential of piezoelectric transducer arrays for an angular radiation of ultrasound waves.In the future, this effect can be used to realize new material-integrated concepts for measuring distances or flow rates.Additionally, the developed concept can be applied for SHM applications based on the analysis of Lamb wave scatter on discontinuities or cracks.

Figure 1 .
Figure 1.Radiation of the ultrasound wave from the functionalized Textile-reinforced thermoplastic composites (TRTC) plate at an angle φ.

Figure 1 .
Figure 1.Radiation of the ultrasound wave from the functionalized Textile-reinforced thermoplastic composites (TRTC) plate at an angle ϕ.

Figure 3 .
Figure 3. Determination of the radiation angle.(A) Wavelength of the A0-mode in a 2 mm thick GF/PA6 plate; (B) Radiation angle of sound waves in air.

Figure 3 .
Figure 3. Determination of the radiation angle.(A) Wavelength of the A0-mode in a 2 mm thick GF/PA6 plate; (B) Radiation angle of sound waves in air.

Figure 3 .
Figure 3. Determination of the radiation angle.(A) Wavelength of the A 0 -mode in a 2 mm thick GF/PA6 plate; (B) Radiation angle of sound waves in air.

Figure 4 .
Figure 4. General overview of the elaborated model with geometrical interpretation of the modifiable parameters.

Figure 4 .
Figure 4. General overview of the elaborated model with geometrical interpretation of the modifiable parameters.

Figure 5 .
Figure 5. Transducer driving signals.(A) For the first transducer within the array.(B) For the second transducer within the array.(C) For the third transducer within the array.(D) For the fourth transducer within the array.The obtained results (Figure6) confirmed that through application deliberately-activated structure-integrated transducers organized into a linear array the generation of directional wave is possible.It is clearly visible that the wave amplitudes along the main wave propagation direction are amplified in comparison with those propagating in the other direction.It can be observed that some side lobes are also present.In order to confirm these observations experimental investigations on nominally-identical structures have been conducted.

Figure 6 .
Figure 6.Out-of-plane displacements of the plate wave generated by a transducer array at t = 20 µs.

Figure 5 .
Figure 5. Transducer driving signals.(A) For the first transducer within the array.(B) For the second transducer within the array.(C) For the third transducer within the array.(D) For the fourth transducer within the array.

Figure 5 .
Figure 5. Transducer driving signals.(A) For the first transducer within the array.(B) For the second transducer within the array.(C) For the third transducer within the array.(D) For the fourth transducer within the array.The obtained results (Figure6) confirmed that through application deliberately-activated structure-integrated transducers organized into a linear array the generation of directional wave is possible.It is clearly visible that the wave amplitudes along the main wave propagation direction are amplified in comparison with those propagating in the other direction.It can be observed that some side lobes are also present.In order to confirm these observations experimental investigations on nominally-identical structures have been conducted.

Figure 6 .
Figure 6.Out-of-plane displacements of the plate wave generated by a transducer array at t = 20 µs.

Figure 6 .
Figure 6.Out-of-plane displacements of the plate wave generated by a transducer array at t = 20 µs.For the animation of the wave field please refer to supplementary material.

Figure 8 .
Figure 8. Micrograph of a matrix homogeneous integrated TPM.

Figure 8 .
Figure 8. Micrograph of a matrix homogeneous integrated TPM.

Figure 8 .
Figure 8. Micrograph of a matrix homogeneous integrated TPM.

Figure 12 .
Figure 12.Experimental setup for the determination of propagation of induced mechanical and acoustical waves.

Figure 12 .
Figure 12.Experimental setup for the determination of propagation of induced mechanical and acoustical waves.

Figure 12 .
Figure 12.Experimental setup for the determination of propagation of induced mechanical and acoustical waves.

Figure 13 .
Figure 13.Coordinate system for the microphone measurement (origin at the first transducer of the array).

Figure 14 .
Figure 14.Out-of-plane velocities at t = 20 µs for different time delays.(A) for zero seconds; (B) for 24 ms.

Figure 13 .
Figure 13.Coordinate system for the microphone measurement (origin at the first transducer of the array).

Figure 13 .
Figure 13.Coordinate system for the microphone measurement (origin at the first transducer of the array).

Figure 14 .
Figure 14.Out-of-plane velocities at t = 20 µs for different time delays.(A) for zero seconds; (B) for 24 ms.

Figure 14 .
Figure 14.Out-of-plane velocities at t = 20 µs for different time delays.(A) for zero seconds; (B) for 24 ms.

Figure 15 .
Figure 15.Measured maximum sound pressure level of the radiated ultrasound burst at different heights.(A) 10 mm above the plate; (B) 30 mm above the plate; (C) 70 mm above the plate.

Figure 15 .
Figure 15.Measured maximum sound pressure level of the radiated ultrasound burst at different heights.(A) 10 mm above the plate; (B) 30 mm above the plate; (C) 70 mm above the plate.

Table A2 .
[30]rial parameters of the PIC181 calculated on the basis of the manufacturer data[30].