Study on Temporal and Spatial Distribution and Transport Characteristics of Dust in New Composite Spraying Slurry

: In view of the problems of traditional spraying technology, such as complex processes, high costs, large dust amounts, and poor air leakage effects, a new composite spraying slurry is proposed in this paper, which takes clay as the main base material and uses water pressure and wind pressure to ensure intrinsic safety. Firstly, the airtightness, bending resistance, and viscosity of the spraying material were measured in the laboratory; secondly, the gas–liquid–solid three-phase ﬂow process involved in the spraying process was simulated by using the CFD-DPM method, adopting the Eulerian two-ﬂuid model for continuous gas–water two-phases and the discrete phase DPM model for dust generation, and the transport, diffusion, and full space-time distribution characteristics of dust generation were studied. The research shows that: (1) the new composite slurry spraying material made of clay as the main material is made by adding a small proportion of cement and engineering ﬁber to increase the toughness of the material, and ﬁnally, determining the mass ratio of the composite material as follows: clay: cement: additive: engineering ﬁber = 84:14:1.85:0.15. It has good sealing and bending resistance and good adhesion; (2) the water phase distribution under the action of spray determines the distribution of solid-phase dust, and the distribution area of dust is similar to that of the water phase; (3) under the action of spray, the area at the bottom of the roadway is covered by dust ﬂow, and the dust in this area is obviously stratiﬁed. The particle size of the dust gradually decreases from bottom to top. The large particle size dust is deposited at the bottom, while the small particle size dust is suspended at a certain height, and the diffusion area gradually increases; (4) the effect of spray angle on dust is mainly manifested in the initial dust ﬂow shape and dust diffusion time. The larger the spray angle, the faster the diffusion; (5) when the water velocity at the nozzle outlet is large, the dust concentration is low in the whole area, but in areas higher than 1.5 m, the PM2.5 concentration also increases with the increase in water ﬂow. The dust suppression effect of larger a water ﬂow is mainly reﬂected in the bottom area, and the disturbed surrounding airﬂow can make PM2.5 diffuse to higher areas. The results show that the concentration of PM2.5 decreases with the increase in water ﬂow in the area below 0.7 m. For the area higher than 1.5 m, the concentration of PM2.5 also increases with the increase in water ﬂow, which indicates that a larger water ﬂow can effectively suppress dust, mainly in the bottom area. At the same time, the larger water ﬂow intensiﬁes the disturbance of the surrounding airﬂow, and the disturbed airﬂow carries dust diffusion, which makes the dust such as PM2.5 spread to a higher area.


Introduction
More than 90% of China's coal mines are facing a major threat of mine fire in the process of mining. Among them, coal spontaneous combustion is the main disaster in the process of coal safety production, which usually occurs in the air leakage channel areas, such as goafs, open ditches, production lines, geological structure zones, etc [1,2]. In addition, in many high gas mines, the development of coal pillar fractures will produce gas leakage channels between the roadways of the mining face and the adjacent goafs, which can easily cause an increase in gas concentration in the upper corner of the coal mining

Performance Analysis of a New Composite Spraying Slurry
On the basis of clay as the main material, a small proportion of cement and engineering fiber are added to increase the toughness of the material. Through comparative analysis, the final mass ratio of the composite material is Clay: cement: additive: engineering fiber = 84:14:1.85:0.15.
Compared with the traditional cement mortar spraying technology, the main material of the spraying material is changed from cement to clay. Combined with the air leakage situation of the tunnel walls, the air tightness, bending resistance, and viscosity of the material are tested.
(1) Air tightness analysis of paste materials In the mercury injection experiment, in order to overcome the internal surface tension, a certain pressure p needs to be provided before filling the pores with radius R. For cylindrical pores, p and R need to meet the Washburn relationship, as follows: where σ is the surface tension of mercury and θ is the contact angle between mercury and solid.
Through the analysis of the experimental data, the specific gravity and porosity of the slurry are shown in Table 1, the pore surface area and the distribution percentage of different types of slurry materials are shown in Table 2, and the volume and distribution percentage of different types of pores are shown in Table 3. According to Table 1, the porosity of the paste material is 32.71%; according to Table 2, the total surface area of micropores, pores, and mesopores accounts for 99.06% of the total surface area of pore structures, and the proportion of mesopores is close to 50%. It can be seen from Table 3 that in the basic distribution of the micropore structure of paste materials, the mesoporous pore (1.0 × 10 −4~1 .0 × 10 −3 mm) volume accounted for 75.82%. Table 1. Determination results of specific gravity and porosity of paste materials.

Test Specimen
True Specific Gravity (g/cm 3 )

Apparent Specific
Gravity (g/cm 3

) Porosity
Test block 1.2134 0.8165 32.71  The results show that the porosity of the slurry is 32.71%. The sum of the surface areas of the micropores, pores, and mesopores accounted for 99.06% of the total surface area of the pore structure, and the sum of their volumes accounted for 79.16% of the total pore volume.
The microfractures are characterized by the development and change from micropore to mesopore (pore size ≤ 1.0 × 10 −3 mm), which accounted for the majority of the paste materials, accounting for more than 80%. The coarse, large pores and fractures are not developed, and the actual proportion is relatively small.
According to the above conclusions, the slurry material is compact in structure and has good air tightness. However, the static pressure difference between the two sides of narrow coal pillars is generally less than 500 Pa, and the slurry material selected can basically block the airflow and prevent gas emission near the goaf.
(2) Analysis of the bending resistance of the slurry A 15 cm × 40 cm acrylic plate is used to glue the broken coal blocks with different particle sizes on it. After standing for one day, an experimental wall similar to the tunnel wall was obtained, as shown in Figure 1a. The slurry material was sprayed on the experimental wall of the roadway and left for 15 days, as shown in Figure 1b. A bending test was carried out on the spraying material, as shown in Figure 2. When obvious cracks appeared on the spray coating surface (as shown in Figure 3), the bending test was stopped. When there were obvious cracks, the arc length was 40 cm, the angle was 70 • , and the bending radius was r = 32.75 cm. The curvature of the experimental plate was ρ = 1/r = 0305 = 3.05%. The highest point of the arc was 5.92 cm higher than that before bending ε = 5.92/40 = 14.81%.
According to the experimental results, after the deformation of the underground roadway, the local area will produce bending deformations. When the bending curvature reaches about 3.05% or the ratio of the distance between the starting point of the local area and the horizontal distance of the overall deformation area is close to 14.81%, the spraying material will crack obviously, which may produce gas emission channels.   According to the experimental results, after the deformation of the underground roadway, the local area will produce bending deformations. When the bending curvature reaches about 3.05% or the ratio of the distance between the starting point of the local area and the horizontal distance of the overall deformation area is close to 14.81%, the spraying material will crack obviously, which may produce gas emission channels.
(3) Viscosity analysis of the slurry At normal temperatures, the viscosity of the wetted paste was measured by a mcr102 rheometer. Based on the different proportions of water, the shear frequency is 60 s −1 . Five groups were measured; each group was measured three times, and the average value was taken. The measurement curve is shown in Figure 4. It can be seen from Figure 4 that the viscosity of the paste material decreases with the increase in the water ratio.   According to the experimental results, after the deformation of the underground roadway, the local area will produce bending deformations. When the bending curvature reaches about 3.05% or the ratio of the distance between the starting point of the local area and the horizontal distance of the overall deformation area is close to 14.81%, the spraying material will crack obviously, which may produce gas emission channels.
(3) Viscosity analysis of the slurry At normal temperatures, the viscosity of the wetted paste was measured by a mcr102 rheometer. Based on the different proportions of water, the shear frequency is 60 s −1 . Five groups were measured; each group was measured three times, and the average value was taken. The measurement curve is shown in Figure 4. It can be seen from Figure 4 that the    According to the experimental results, after the defor roadway, the local area will produce bending deformations. reaches about 3.05% or the ratio of the distance between the s and the horizontal distance of the overall deformation area is material will crack obviously, which may produce gas emiss (3) Viscosity analysis of the slurry (3) Viscosity analysis of the slurry At normal temperatures, the viscosity of the wetted paste was measured by a mcr102 rheometer. Based on the different proportions of water, the shear frequency is 60 s −1 . Five groups were measured; each group was measured three times, and the average value was taken. The measurement curve is shown in Figure 4. It can be seen from Figure 4 that the viscosity of the paste material decreases with the increase in the water ratio.

Selection of the Two-Fluid Model
As shown in Figure 5, the slurry spraying process belongs to a typical three-phase flow. The feeding module continuously inhales the slurry base material particles into the spraying operation system through the negative pressure generated by the pneumatic suction device. After fully mixing the atomized water on the spray gun mouth and the nozzle, it moves to the spraying surface under the action of inertia. Based on the CFD-DPM method, the Eulerian two-fluid model is used to simulate the gas and water phases, and the Lagrange model is used to track dust particles. The dust migration process under various working conditions is studied, and the three-phase flow is analyzed in detail. The water spray and surrounding air belong to a continuous phase, and the Euler-Euler two-fluid model is used to simulate. The base material of the slurry belongs to a discrete particle phase, and the DPM model is used to track and simulate.
The particle size distribution of industrial dust is not uniform; it is randomly distributed, but the industrial dust particle size distribution generally presents certain regularity. The commonly used particle size distribution functions generally include the normal distribution, the logarithmic normal distribution, and the Rosin-Rammler distribution function.
The particle size distribution used in this paper is shown in the figure below, and the average particle size was taken as d = 100 μm. The particle distribution index n = 3.5, and the dust particle size distribution is shown in Figure 6.

Selection of the Two-Fluid Model
As shown in Figure 5, the slurry spraying process belongs to a typical three-phase flow. The feeding module continuously inhales the slurry base material particles into the spraying operation system through the negative pressure generated by the pneumatic suction device. After fully mixing the atomized water on the spray gun mouth and the nozzle, it moves to the spraying surface under the action of inertia.

Selection of the Two-Fluid Model
As shown in Figure 5, the slurry spraying process belongs to a typical three-phase flow. The feeding module continuously inhales the slurry base material particles into the spraying operation system through the negative pressure generated by the pneumatic suction device. After fully mixing the atomized water on the spray gun mouth and the nozzle, it moves to the spraying surface under the action of inertia. Based on the CFD-DPM method, the Eulerian two-fluid model is used to simulate the gas and water phases, and the Lagrange model is used to track dust particles. The dust migration process under various working conditions is studied, and the three-phase flow is analyzed in detail. The water spray and surrounding air belong to a continuous phase, and the Euler-Euler two-fluid model is used to simulate. The base material of the slurry belongs to a discrete particle phase, and the DPM model is used to track and simulate.
The particle size distribution of industrial dust is not uniform; it is randomly distributed, but the industrial dust particle size distribution generally presents certain regularity. The commonly used particle size distribution functions generally include the normal distribution, the logarithmic normal distribution, and the Rosin-Rammler distribution function.
The particle size distribution used in this paper is shown in the figure below, and the average particle size was taken as d = 100 μm. The particle distribution index n = 3.5, and the dust particle size distribution is shown in Figure 6. Based on the CFD-DPM method, the Eulerian two-fluid model is used to simulate the gas and water phases, and the Lagrange model is used to track dust particles. The dust migration process under various working conditions is studied, and the three-phase flow is analyzed in detail. The water spray and surrounding air belong to a continuous phase, and the Euler-Euler two-fluid model is used to simulate. The base material of the slurry belongs to a discrete particle phase, and the DPM model is used to track and simulate.
The particle size distribution of industrial dust is not uniform; it is randomly distributed, but the industrial dust particle size distribution generally presents certain regularity. The commonly used particle size distribution functions generally include the normal distribution, the logarithmic normal distribution, and the Rosin-Rammler distribution function.
The particle size distribution used in this paper is shown in the figure below, and the average particle size was taken as d = 100 µm. The particle distribution index n = 3.5, and the dust particle size distribution is shown in Figure 6.  As shown in Figure 6, the dust distribution basically presents a normal distribution, and the dust particle size is mostly concentrated below 150 μm.

Calculation Conditions and Parameters
In order to focus on discussing the dust generation and its distribution characteristics in the slurry spraying process, the actual situation is simplified as follows: the heat transfer between the air and the slurry is not considered in the numerical calculation of the spray dust generation process; that is, the related flow problems are studied under cold conditions. The overall model structure is shown in Figure 7a, and the simplified physical model diagram is given. The structured grid is adopted, and the grid opposites are verified, as shown in Figure 7b.  The spraying process of slurries belongs to a typical three-phase flow. Based on the CFD-DPM (computational fluid dynamics discrete particle method), this paper uses the Eulerian two-fluid model to simulate the gas phase and water phase and uses the Lagrangian model to track the dust particles to study the dust migration process under various working conditions. Among them, the water spray and the surrounding air belong to the continuous phase, and the Euler-Euler two-fluid model is used for simulation research; the base material of the slurry belongs to the discrete particle phase, and the DPM model As shown in Figure 6, the dust distribution basically presents a normal distribution, and the dust particle size is mostly concentrated below 150 µm.

Calculation Conditions and Parameters
In order to focus on discussing the dust generation and its distribution characteristics in the slurry spraying process, the actual situation is simplified as follows: the heat transfer between the air and the slurry is not considered in the numerical calculation of the spray dust generation process; that is, the related flow problems are studied under cold conditions. The overall model structure is shown in Figure 7a, and the simplified physical model diagram is given. The structured grid is adopted, and the grid opposites are verified, as shown in Figure 7b.  As shown in Figure 6, the dust distribution basically presents a normal distribution, and the dust particle size is mostly concentrated below 150 μm.

Calculation Conditions and Parameters
In order to focus on discussing the dust generation and its distribution characteristics in the slurry spraying process, the actual situation is simplified as follows: the heat transfer between the air and the slurry is not considered in the numerical calculation of the spray dust generation process; that is, the related flow problems are studied under cold conditions. The overall model structure is shown in Figure 7a, and the simplified physical model diagram is given. The structured grid is adopted, and the grid opposites are verified, as shown in Figure 7b.  The spraying process of slurries belongs to a typical three-phase flow. Based on the CFD-DPM (computational fluid dynamics discrete particle method), this paper uses the Eulerian two-fluid model to simulate the gas phase and water phase and uses the Lagrangian model to track the dust particles to study the dust migration process under various working conditions. Among them, the water spray and the surrounding air belong to the continuous phase, and the Euler-Euler two-fluid model is used for simulation research; the base material of the slurry belongs to the discrete particle phase, and the DPM model The spraying process of slurries belongs to a typical three-phase flow. Based on the CFD-DPM (computational fluid dynamics discrete particle method), this paper uses the Eulerian two-fluid model to simulate the gas phase and water phase and uses the Lagrangian model to track the dust particles to study the dust migration process under various working conditions. Among them, the water spray and the surrounding air belong to the continuous phase, and the Euler-Euler two-fluid model is used for simulation research; the base material of the slurry belongs to the discrete particle phase, and the DPM model is used for tracking and simulation calculation. See Table 4 for the two-fluid model and the related parameters and Table 5 for the DPM model and the related parameters. In order to discuss the dust production in the process of slurry spraying, the local roadway is taken as the research object. The length of the roadway is 3 m, the width is 4 m, and the distance between the vault and the ground is 4 m. Combined with the actual situation, the following physical model is simplified: the roadway is full of air, and there is airflow in the horizontal direction (along the x axis). The spray gun is perpendicular to the airflow direction and placed horizontally. The base material is ejected from the central nozzle. The diameter of the spray gun is about 0.03 m, and the length is 0.5 m. There are four nozzles around the nozzle for spray atomization.

Dust Distribution with or without Spray
The particle size range of the dust was 2 × 10 −6~3 × 10 −4 m. In order to observe the temporal and spatial distribution changes of the dust, when the dust is visualized, the dust should be enlarged to the appropriate size so that the spatiotemporal distribution information of dust with different particle sizes can be obtained intuitively.
(1) Dust distribution without spray When the velocity of the spray gun is lower than that of the spray gun, there is no dust in the exit of the tunnel. Due to the continuous outflow of dust from the spray gun, the dust gradually increases so that the cross-section of the dust mainstream increases gradually during the dust migration until it flows out from the outlet, as shown in Figure 8.
With the increase in the initial velocity of the base material ejected from the spray gun, the dust generated will move to the side under the action of inertia and diffuse around at the same time. With the continuous outflow of dust from the spray gun, the amount of dust increases gradually, and the dust diffusion area also gradually increases, as shown in Figure 9. At the same time, due to the influence of transverse airflow in the roadway, there is more dust at the downwind side; the amount of dust on the side where the spraying surface is located gradually increases, and the diffusion area gradually extends to the surrounding area, as shown in Figure 9 (t = 0.6 s). At this time, the dust has diffused to the bottom and top areas of the spraying side. The distribution of dust with different particle sizes (i.e., different colors in the figure) is different. For example, the top area is mostly fine dust (blue and green particles), and the large particle size dust is relatively small (red particles). The dust continues to diffuse under the action of airflow. With the increase in dust production, the diffusion area continues to increase until it diffuses to the whole calculation area; see t = 1.0 s. The dust has diffused to the whole roadway calculation area. With the continuous spraying process, more and more dust is in the whole calculation area, and the visibility gradually decreases until t = 20.0 s. At this time, the spraying is stopped; that is, the dust is no longer produced at the dust source. Under the carrying effect of the transverse airflow, the dust in the roadway area is gradually discharged from the outlet, the dust particles are rapidly reduced, the dust concentration is gradually reduced, and the visibility is also gradually improved.  With the increase in the initial velocity of the base material ejected from the spray gun, the dust generated will move to the side under the action of inertia and diffuse around at the same time. With the continuous outflow of dust from the spray gun, the amount of dust increases gradually, and the dust diffusion area also gradually increases, as shown in Figure 9. At the same time, due to the influence of transverse airflow in the roadway, there is more dust at the downwind side; the amount of dust on the side where the spraying surface is located gradually increases, and the diffusion area gradually extends to the surrounding area, as shown in Figure 9 (t = 0.6 s). At this time, the dust has diffused to the bottom and top areas of the spraying side. The distribution of dust with different particle sizes (i.e., different colors in the figure) is different. For example, the top area is mostly fine dust (blue and green particles), and the large particle size dust is relatively small (red particles). The dust continues to diffuse under the action of airflow. With the increase in dust production, the diffusion area continues to increase until it diffuses to the whole calculation area; see t = 1.0 s. The dust has diffused to the whole roadway calculation area. With the continuous spraying process, more and more dust is in the whole calculation area, and the visibility gradually decreases until t = 20.0 s. At this time, the spraying is stopped; that is, the dust is no longer produced at the dust source. Under the carrying effect of the transverse airflow, the dust in the roadway area is gradually discharged from the outlet, the dust particles are rapidly reduced, the dust concentration is gradually reduced, and the visibility is also gradually improved.   With the increase in the initial velocity of the base material ejected from the spray gun, the dust generated will move to the side under the action of inertia and diffuse around at the same time. With the continuous outflow of dust from the spray gun, the amount of dust increases gradually, and the dust diffusion area also gradually increases, as shown in Figure 9. At the same time, due to the influence of transverse airflow in the roadway, there is more dust at the downwind side; the amount of dust on the side where the spraying surface is located gradually increases, and the diffusion area gradually extends to the surrounding area, as shown in Figure 9 (t = 0.6 s). At this time, the dust has diffused to the bottom and top areas of the spraying side. The distribution of dust with different particle sizes (i.e., different colors in the figure) is different. For example, the top area is mostly fine dust (blue and green particles), and the large particle size dust is relatively small (red particles). The dust continues to diffuse under the action of airflow. With the increase in dust production, the diffusion area continues to increase until it diffuses to the whole calculation area; see t = 1.0 s. The dust has diffused to the whole roadway calculation area. With the continuous spraying process, more and more dust is in the whole calculation area, and the visibility gradually decreases until t = 20.0 s. At this time, the spraying is stopped; that is, the dust is no longer produced at the dust source. Under the carrying effect of the transverse airflow, the dust in the roadway area is gradually discharged from the outlet, the dust particles are rapidly reduced, the dust concentration is gradually reduced, and the visibility is also gradually improved.  (2) Dust distribution with spray When there is spray, the dust generation is directly affected by the surrounding four water mist streams and is forced to flow with the water mist to the side wall; see t = 0.10 s in Figure 10. With the spraying process going on, the dust production gradually increases; see t = 0.6 s. Under the action of water mist, the generated dust flows to and reaches the side wall and diffuses on the side wall; see t = 1.0 s. At this time, there are more red particles at the bottom and more blue-green particles at the top. This shows that the dust is gradually stratified in the flow process, and the large particle size dust tends to deposit, while the small particle size dust easily diffuses to the high places.
Due to the blocking effect of the side wall, the water generated in the spraying process will carry the dust to the ground and then flow along the ground to the opposite side, as shown in Figure 10. As a result, the dust carries downward to the opposite side. At the same time, affected by the transverse airflow in the roadway, the water mist diffuses to the opposite side and the outlet direction at the same time. The dust also diffuses to the opposite side and the outlet side under the carrying effect of the water mist. See T = 2.0 S in Figure 10.  The bottom area of the roadway has been covered by the dust flow. In this area, from the bottom up, it gradually changes from red particles to green particles, and then to a blue-green mixed particle area, while the top has more blue particles and fewer green particles. It can be seen that the dust stratification is obvious; the large particle size dust is deposited at the bottom, while the small particle size dust is suspended at a certain height. Compared with the simulation results in Figures 9 and 10, compared with the case without spray, the dust is mainly distributed in the bottom area under the action of water mist, and the effect of the spray dust reduction is obvious. The distribution of dust with large and small particle sizes changes under the action of spray, and the dust with a large particle size is easier to settle under the action of gravity. In Figure 10, no fine dust diffuses to the top area, which shows that the spray can effectively inhibit the diffusion of fine dust in the height direction.
As shown in Figure 11, the distribution of dust under spray is closely related to that of the water phase. Taking the vertical and horizontal section of the central point of the calculation area as an example, the water phase distribution in the gas-liquid-solid threephase is analyzed, and its development with time and space is observed. After the water mist is ejected from the nozzle, it carries the dust diameter directly to the spraying wall under the inertial action, which is blocked by the spraying wall, and forms a mist area with a large water phase concentration near the spraying wall. Under the action of gravity, the mist will flow to the bottom of the roadway and diffuse along the opposite side of the spraying surface. After the non-spraying surface, the diffusion area starts to extend Due to the blocking effect of the side wall, the water generated in the spraying process will carry the dust to the ground and then flow along the ground to the opposite side, as shown in Figure 10. As a result, the dust carries downward to the opposite side. At the same time, affected by the transverse airflow in the roadway, the water mist diffuses to the opposite side and the outlet direction at the same time. The dust also diffuses to the opposite side and the outlet side under the carrying effect of the water mist. See T = 2.0 S in Figure 10.
The bottom area of the roadway has been covered by the dust flow. In this area, from the bottom up, it gradually changes from red particles to green particles, and then to a blue-green mixed particle area, while the top has more blue particles and fewer green particles. It can be seen that the dust stratification is obvious; the large particle size dust is deposited at the bottom, while the small particle size dust is suspended at a certain height. Compared with the simulation results in Figures 9 and 10, compared with the case without spray, the dust is mainly distributed in the bottom area under the action of water mist, and the effect of the spray dust reduction is obvious. The distribution of dust with large and small particle sizes changes under the action of spray, and the dust with a large particle size is easier to settle under the action of gravity. In Figure 10, no fine dust diffuses to the top area, which shows that the spray can effectively inhibit the diffusion of fine dust in the height direction.
As shown in Figure 11, the distribution of dust under spray is closely related to that of the water phase. Taking the vertical and horizontal section of the central point of the calculation area as an example, the water phase distribution in the gas-liquid-solid threephase is analyzed, and its development with time and space is observed. After the water mist is ejected from the nozzle, it carries the dust diameter directly to the spraying wall under the inertial action, which is blocked by the spraying wall, and forms a mist area with a large water phase concentration near the spraying wall. Under the action of gravity, the mist will flow to the bottom of the roadway and diffuse along the opposite side of the spraying surface. After the non-spraying surface, the diffusion area starts to extend upward, thus forming a relatively continuous mist area with a small water compatibility and a small gradient on the two sides and bottom of the roadway.
Compared with the solid-phase dust distribution map of T = 20.0 s in Figure 10 and the water phase diagram in Figure 11a, it can be seen that the distribution area of dust is similar to that of the water phase, mainly distributed on the two sides and near the bottom of the roadway. In addition, under the action of transverse airflow in the roadway, the thin water mist will flow from the inlet side to the outlet side under the action of the airflow. The water volume at the outlet side is obviously more than that at the inlet side, as shown in Figure 11b. The dust in the outlet side is also more than that in the air-inlet side, as shown in the solid-phase dust distribution diagram with T = 5.0 s in Figure 10. This shows that the distribution of the solid phase can determine the effect of the water spray. The dust concentration on the site of the new spraying process and the traditional spraying process is significantly reduced, as shown in Figure 12. Compared with the solid-phase dust distribution map of T = 20.0 s in Figure 10 and the water phase diagram in Figure 11a, it can be seen that the distribution area of dust is similar to that of the water phase, mainly distributed on the two sides and near the bottom of the roadway. In addition, under the action of transverse airflow in the roadway, the thin water mist will flow from the inlet side to the outlet side under the action of the airflow. The water volume at the outlet side is obviously more than that at the inlet side, as shown in Figure 11b. The dust in the outlet side is also more than that in the air-inlet side, as shown in the solid-phase dust distribution diagram with T = 5.0 s in Figure 10. This shows that the distribution of the solid phase can determine the effect of the water spray. The dust concentration on the site of the new spraying process and the traditional spraying process is significantly reduced, as shown in Figure 12.

Temporal and Spatial Distribution of Dust
(1) Temporal and spatial distribution of total dust Under the working conditions of a spray angle of 70°, a material suction of 0.038 kg/s, a side air velocity of 0.5 m/s, and a water spray rate of 11 L/min, the dust migration process in the spraying process is simulated and the spatial and temporal distributions are as shown in Figure 13.  Compared with the solid-phase dust distribution map of T = 20.0 s in Figure 10 and the water phase diagram in Figure 11a, it can be seen that the distribution area of dust is similar to that of the water phase, mainly distributed on the two sides and near the bottom of the roadway. In addition, under the action of transverse airflow in the roadway, the thin water mist will flow from the inlet side to the outlet side under the action of the airflow. The water volume at the outlet side is obviously more than that at the inlet side, as shown in Figure 11b. The dust in the outlet side is also more than that in the air-inlet side, as shown in the solid-phase dust distribution diagram with T = 5.0 s in Figure 10. This shows that the distribution of the solid phase can determine the effect of the water spray. The dust concentration on the site of the new spraying process and the traditional spraying process is significantly reduced, as shown in Figure 12.

Temporal and Spatial Distribution of Dust
(1) Temporal and spatial distribution of total dust Under the working conditions of a spray angle of 70°, a material suction of 0.038 kg/s, a side air velocity of 0.5 m/s, and a water spray rate of 11 L/min, the dust migration process in the spraying process is simulated and the spatial and temporal distributions are as shown in Figure 13.

Temporal and Spatial Distribution of Dust
(1) Temporal and spatial distribution of total dust Under the working conditions of a spray angle of 70 • , a material suction of 0.038 kg/s, a side air velocity of 0.5 m/s, and a water spray rate of 11 L/min, the dust migration process in the spraying process is simulated and the spatial and temporal distributions are as shown in Figure 13. As shown in Figure 13, the dust concentration gradually decreases along the length direction. The dust concentration in most areas is less than 10 mg/m 3 . The dust concentration is higher in the downwind side, especially near the exit. With the increase in spraying time, the dust concentration on the downwind side increased significantly. Among them,       As shown in Figure 13, the dust concentration gradually decreases along the length direction. The dust concentration in most areas is less than 10 mg/m 3 . The dust concentration is higher in the downwind side, especially near the exit. With the increase in spraying time, the dust concentration on the downwind side increased significantly. Among them, 1.5 m is the location of the spray gun, which is the dust source, and the dust concentration is slightly higher than in other areas. The distribution of the dust concentration in the width direction showed a trend of being high at both ends, and in the middle of the dust source, the dust concentration increased. The width of 4.0 m corresponds to the sprayed wall, and the dust concentration near the wall increases with the spraying time. When the width is 0.0 m, the growth rate of the dust concentration is far greater than that of the sprayed side. This is mainly the result of spray, airflow, and wall obstruction. The dust concentration decreases with the increase in height, especially in the area near the ground (below 0.4 m). This shows that the dust, especially the dust with a large particle size, is mainly distributed in the bottom area of the roadway. In the area above 0.5 m, the rate of decrease in the dust concentration is greatly reduced, and it is all lower than 5 mg/m 3 and only slightly increased at the height of 1.5 m. There is almost no dust in the area above 2.0 m, and its concentration tends to 0. It is further explained that, compared with the case without spraying, spraying can effectively inhibit the dust diffusion in the height direction.
(2) Dust distribution with different particle sizes From the above analysis, it can be seen that the dust concentration decreases with the increase in height. Considering the different dust diffusion capacities of different particle sizes, three particle size ranges of PM2.5, PM40-100, and PM50-100 are selected to investigate the distribution and changes of the three groups of dust in the height direction, as shown in Figure 14a. As shown in Figure 13, the dust concentration gradually decreases along the length direction. The dust concentration in most areas is less than 10 mg/m 3 . The dust concentration is higher in the downwind side, especially near the exit. With the increase in spraying time, the dust concentration on the downwind side increased significantly. Among them, 1.5 m is the location of the spray gun, which is the dust source, and the dust concentration is slightly higher than in other areas. The distribution of the dust concentration in the width direction showed a trend of being high at both ends, and in the middle of the dust source, the dust concentration increased. The width of 4.0 m corresponds to the sprayed wall, and the dust concentration near the wall increases with the spraying time. When the width is 0.0 m, the growth rate of the dust concentration is far greater than that of the sprayed side. This is mainly the result of spray, airflow, and wall obstruction. The dust concentration decreases with the increase in height, especially in the area near the ground (below 0.4 m). This shows that the dust, especially the dust with a large particle size, is mainly distributed in the bottom area of the roadway. In the area above 0.5 m, the rate of decrease in the dust concentration is greatly reduced, and it is all lower than 5 mg/m 3 and only slightly increased at the height of 1.5 m. There is almost no dust in the area above 2.0 m, and its concentration tends to 0. It is further explained that, compared with the case without spraying, spraying can effectively inhibit the dust diffusion in the height direction.
(2) Dust distribution with different particle sizes From the above analysis, it can be seen that the dust concentration decreases with the increase in height. Considering the different dust diffusion capacities of different particle sizes, three particle size ranges of PM2.5, PM40-100, and PM50-100 are selected to investigate the distribution and changes of the three groups of dust in the height direction, as shown in Figure 14a.   Considering that the mass concentration of PM2.5 is relatively small (<0.001 mg/m 3 ), as shown in Figure 14b, the quantitative percentages of the three groups of dust at different heights are counted here, and it is found that the percentage of PM2.5 is relatively large, more than 40% in the bottom area. In addition, the number percentage of PM2.5 is large in the whole height direction, indicating that PM2.5 has strong diffusion ability in the height direction, and its concentration gradually decreases along the height direction, only slightly increasing at 1.5 m of the dust source (>15%). In contrast, the concentration of dust with a medium particle size, namely PM40-100, is relatively small, and it is almost 0 in areas higher than 2.0 m. For large particle size dust, the number percentage decreases significantly near the wall, indicating that the large particle size dust is mostly concentrated at the bottom. It can be seen from Figure 14b that the initial concentration of PM2.5 dust with a small particle size is very small, lower than 0.0002 mg/m 3 , and no PM2.5 is found in the top area. With the spraying process, the mass concentration of PM2.5 in the top area also gradually increases.

Influence of the Spray Angle of the Water Mist
(1) Temporal and spatial distribution of the total dust The spray angle is defined as the angle between the direction of the water jet and the cross-section of the outlet. In this paper, under the conditions of 0.038 kg/s of suction, 0.5 m/s of side air supply, and 11 L/min of water spray, three working conditions of 58 • , 64 • , and 70 • are selected to simulate and calculate, and the temporal and spatial distribution of the dust is analyzed. The temporal and spatial distribution of the dust is shown in Figures 15-17. The results show that at the initial moment, the influence of the water jet angle on the dust flow is obvious. The larger the jet angle is, the smaller the water mist area formed by the four water jets is. dust with a small particle size is very small, lower than 0.0002 mg/m 3 , and no PM found in the top area. With the spraying process, the mass concentration of PM2.5 top area also gradually increases.

Influence of the Spray Angle of the Water Mist
(1) Temporal and spatial distribution of the total dust The spray angle is defined as the angle between the direction of the water jet a cross-section of the outlet. In this paper, under the conditions of 0.038 kg/s of sucti m/s of side air supply, and 11 L/min of water spray, three working conditions of 5 °, and 70 ° are selected to simulate and calculate, and the temporal and spatial distri of the dust is analyzed. The temporal and spatial distribution of the dust is shown ures 15-17. The results show that at the initial moment, the influence of the water je on the dust flow is obvious. The larger the jet angle is, the smaller the water mi formed by the four water jets is.  dust with a small particle size is very small, lower than 0.0002 mg/m 3 , and no PM found in the top area. With the spraying process, the mass concentration of PM2.5 top area also gradually increases.

Influence of the Spray Angle of the Water Mist
(1) Temporal and spatial distribution of the total dust The spray angle is defined as the angle between the direction of the water jet a cross-section of the outlet. In this paper, under the conditions of 0.038 kg/s of sucti m/s of side air supply, and 11 L/min of water spray, three working conditions of 5 °, and 70 ° are selected to simulate and calculate, and the temporal and spatial distri of the dust is analyzed. The temporal and spatial distribution of the dust is shown ures 15-17. The results show that at the initial moment, the influence of the water je on the dust flow is obvious. The larger the jet angle is, the smaller the water mi formed by the four water jets is.  Due to the different spray angles, the velocity of the water jet perpendicular to the spraying surface is different. When the spraying angle is 70 • , the velocity perpendicular to the spraying surface is larger, so the time for water carrying dust to reach the spraying surface is shorter, and the dust diffusion to the surrounding area is faster.
In order to explore the influence of the different spray angles of water mist on the dust distribution, the total dust distribution along the length and width of the roadway was calculated, as shown in Figure 18.  Due to the different spray angles, the velocity of the water jet perpend spraying surface is different. When the spraying angle is 70 °, the velocity pe to the spraying surface is larger, so the time for water carrying dust to reach t surface is shorter, and the dust diffusion to the surrounding area is faster.
In order to explore the influence of the different spray angles of water dust distribution, the total dust distribution along the length and width of t was calculated, as shown in Figure 18. (1) In the length direction, the dust flows out from the air supply outlet, and its concentration gradually increases to 5 mg/m 3 (du cation). Then, the dust concentration gradually decreases and in idly near the outlet. Due to the different spray angles, the velocity of the water jet perpendicular to the spraying surface is different. When the spraying angle is 70 °, the velocity perpendicular to the spraying surface is larger, so the time for water carrying dust to reach the spraying surface is shorter, and the dust diffusion to the surrounding area is faster.
In order to explore the influence of the different spray angles of water mist on the dust distribution, the total dust distribution along the length and width of the roadway was calculated, as shown in Figure 18. (1) In the length direction, the dust flows out from the air supply outlet to the outlet, and its concentration gradually increases to 5 mg/m 3 (dust source location). Then, the dust concentration gradually decreases and increases rapidly near the outlet. (2) In the width direction, the dust concentration on both sides of the wall is higher, and the dust concentration near the spraying surface is significantly higher than that of the non-spraying surface. At the same time, the dust concentration near the two sides is larger when the spraying angle is 70 °. (3) PM2.5 distribution As shown in Figure 19, the distribution of the PM2.5 concentration under different injection angles is obtained by taking PM2. (1) In the length direction, the dust flows out from the air supply outlet to the outlet, and its concentration gradually increases to 5 mg/m 3 (dust source location). Then, the dust concentration gradually decreases and increases rapidly near the outlet. (2) In the width direction, the dust concentration on both sides of the wall is higher, and the dust concentration near the spraying surface is significantly higher than that of the non-spraying surface. At the same time, the dust concentration near the two sides is larger when the spraying angle is 70 • . (3) PM2.5 distribution As shown in Figure 19, the distribution of the PM2.5 concentration under different injection angles is obtained by taking PM2.5 as an example in the height direction. The concentration of PM2.5 decreased with the increase in height and fluctuated slightly at the position of the 1.5 m dust source. In the height range of 0.4 m to 1.5 m, the concentration of PM2.5 increased with the increase in injection angle. This is because when the spray angle is larger, the vertical velocity of the spray surface is larger, so the water carries the dust movement faster and the dust diffusion speed is faster. The diffusion rate decreases gradually along the way, so the injection angle has little effect on the PM2.5 concentration in the area higher than 1.6 m. This shows that the influence of the spray angle changes on PM2.5 diffusion is mainly in the initial stage and the middle and lower regions. spray surface is larger, so the water carries the dust movement faster a dust diffusion speed is faster. The diffusion rate decreases gradually alo way, so the injection angle has little effect on the PM2.5 concentration in t higher than 1.6 m. This shows that the influence of the spray angle chan PM2.5 diffusion is mainly in the initial stage and the middle and lower re

Effect of Spray Water Velocity
(1) Temporal and spatial distribution of the total dust When the spray angle is 58 degrees, the suction rate is 0.038 kg/s, the side air is 0.5 m/s, and the water spray rate is 3.0 L/min, 7.4 L/min, and 11.0 L/min, respe the dust spatial and temporal distribution is analyzed. The temporal and spatial d tion of the dust is shown in Figure 20.

Effect of Spray Water Velocity
(1) Temporal and spatial distribution of the total dust When the spray angle is 58 degrees, the suction rate is 0.038 kg/s, the side air supply is 0.5 m/s, and the water spray rate is 3.0 L/min, 7.4 L/min, and 11.0 L/min, respectively; the dust spatial and temporal distribution is analyzed. The temporal and spatial distribution of the dust is shown in Figure 20. angle. This is because when the spray angle is larger, the vertical velocity of the spray surface is larger, so the water carries the dust movement faster and the dust diffusion speed is faster. The diffusion rate decreases gradually along the way, so the injection angle has little effect on the PM2.5 concentration in the area higher than 1.6 m. This shows that the influence of the spray angle changes on PM2.5 diffusion is mainly in the initial stage and the middle and lower regions.

Effect of Spray Water Velocity
(1) Temporal and spatial distribution of the total dust When the spray angle is 58 degrees, the suction rate is 0.038 kg/s, the side air supply is 0.5 m/s, and the water spray rate is 3.0 L/min, 7.4 L/min, and 11.0 L/min, respectively; the dust spatial and temporal distribution is analyzed. The temporal and spatial distribution of the dust is shown in Figure 20. It can be seen from Figure 20 that when the water velocity at the nozzle outlet is large, the surrounding airflow is also driven. Under the action of fast velocity, the dust diffuses rapidly in the roadway area. When the diffusion rate is t = 1.0 s, the growth is the fastest. At t = 5.0 s, comparing the dust distribution map of the three groups of flow, it can be found that the velocity of dust migration to the spraying surface is slow due to the low velocity.
In the process of migration, due to the different particle sizes and the different gravity and fluid-carrying effects, there is an obvious stratification phenomenon. For example, when t = 1.0 s in Figure 20a and T = 5.0 s in Figure 20b, there is more red dust with a larger particle size in the lower area of the nozzle frontend. When t = 5.0 s in Figure 20b, the particle size of the dust gradually decreases from right to left, followed by red dust, green dust, and blue dust. This shows that when the water velocity at the nozzle outlet is small, the water flow carrying effect is limited, and the large particle size dust easily separates from the dust flow under the action of gravity and gradually settles to the bottom.
When the water velocity at the outlet of the nozzle is large, the phenomenon of stratification also exists, as shown in Figure 20c, but it is not as obvious as that when the water velocity at the outlet of the nozzle is small. At t = 10.0 s, comparing the dust distribution map of the three groups of flow, it can be found that when the velocity is high, the dust diffuses rapidly in the bottom area of the roadway, and the diffusion space is also large.
As shown in Figure 21, the distribution of dust along the length, width, and height of roadway is counted under different water velocities at the nozzle outlet. When the nozzle outlet water velocity is large, the dust concentration is low in the length, width, and height directions; that is, when the nozzle outlet water velocity is large, the dust concentration is low in the whole calculation area. As shown in Figure 21a, when the nozzle outlet water velocity is small, the dust diffusion is slow, and the dust distribution in the length direction is not stable. In addition to the high concentration at the dust source position, a high concentration area also appears in the front of the outlet. When the nozzle outlet water velocity is large, the dust distribution in the length direction is more than 5 mg/ m 3 . The dust concentration near the dust source and outlet increases rapidly. Compared with the nozzle outlet water of 7.4 L/min, the dust concentration near the outlet of 11.0 L/min is lower.
It can be seen from Figure 20 that when the water velocity at the nozzle outlet is large, the surrounding airflow is also driven. Under the action of fast velocity, the dust diffuses rapidly in the roadway area. When the diffusion rate is t = 1.0 s, the growth is the fastest. At t = 5.0 s, comparing the dust distribution map of the three groups of flow, it can be found that the velocity of dust migration to the spraying surface is slow due to the low velocity. In the process of migration, due to the different particle sizes and the different gravity and fluid-carrying effects, there is an obvious stratification phenomenon. For example, when t = 1.0 s in Figure 20a and T = 5.0 s in Figure 20b, there is more red dust with a larger particle size in the lower area of the nozzle frontend. When t = 5.0 s in Figure 20b, the particle size of the dust gradually decreases from right to left, followed by red dust, green dust, and blue dust. This shows that when the water velocity at the nozzle outlet is small, the water flow carrying effect is limited, and the large particle size dust easily separates from the dust flow under the action of gravity and gradually settles to the bottom.
When the water velocity at the outlet of the nozzle is large, the phenomenon of stratification also exists, as shown in Figure 20c, but it is not as obvious as that when the water velocity at the outlet of the nozzle is small. At t = 10.0 s, comparing the dust distribution map of the three groups of flow, it can be found that when the velocity is high, the dust diffuses rapidly in the bottom area of the roadway, and the diffusion space is also large.
As shown in Figure 21, the distribution of dust along the length, width, and height of roadway is counted under different water velocities at the nozzle outlet. When the nozzle outlet water velocity is large, the dust concentration is low in the length, width, and height directions; that is, when the nozzle outlet water velocity is large, the dust concentration is low in the whole calculation area. As shown in Figure 21a, when the nozzle outlet water velocity is small, the dust diffusion is slow, and the dust distribution in the length direction is not stable. In addition to the high concentration at the dust source position, a high concentration area also appears in the front of the outlet. When the nozzle outlet water velocity is large, the dust distribution in the length direction is more than 5 mg/ m 3 . The dust concentration near the dust source and outlet increases rapidly. Compared with the nozzle outlet water of 7.4 L/min, the dust concentration near the outlet of 11.0 L/min is lower. As shown in Figure 21b, from the dust concentration distribution in the width direction, the dust concentration is generally high when the outlet water flow is small. When the outlet water flow rate is small, the dust concentration on the opposite side of the spraying surface exceeds that on the spraying side, which indicates that more dust is separated from the main stream along the way, depositing and diffusing. However, when the outlet flow is large, the dust concentration is relatively low in the whole width direction.
As shown in Figure 21c, the dust concentration decreases rapidly in the near-ground area, then decreases slowly with the increase in height and only slightly increases at the As shown in Figure 21b, from the dust concentration distribution in the width direction, the dust concentration is generally high when the outlet water flow is small. When the outlet water flow rate is small, the dust concentration on the opposite side of the spraying surface exceeds that on the spraying side, which indicates that more dust is separated from the main stream along the way, depositing and diffusing. However, when the outlet flow is large, the dust concentration is relatively low in the whole width direction.
As shown in Figure 21c, the dust concentration decreases rapidly in the near-ground area, then decreases slowly with the increase in height and only slightly increases at the height of the dust source. When the dust concentration is higher than 1.5 m, the dust concentration under the three working conditions almost tends to 0. In addition, the decreasing speed of the dust concentration in the bottom area decreases with the increase in water flow.
(2) Temporal and spatial distribution of PM2.5 Taking PM2.5 as an example, the change of the PM2.5 concentration under different water flow conditions was observed. The measurement results are shown in Figure 22. The results show that the concentration of PM2.5 decreases with the increase in water flow in the area below 0.7 m. For the area higher than 1.5 m, the concentration of PM2.5 also increases with the increase in water flow, which indicates that a larger water flow can effectively suppress dust, mainly in the bottom area. At the same time, the larger water flow intensifies the disturbance of the surrounding airflow, and the disturbed airflow carries dust diffusion, which makes the dust such as PM2.5 spread to a higher area.
ing speed of the dust concentration in the bottom area decreases with the increase in flow.
(2) Temporal and spatial distribution of PM2.5 Taking PM2.5 as an example, the change of the PM2.5 concentration under d water flow conditions was observed. The measurement results are shown in Fig  The results show that the concentration of PM2.5 decreases with the increase in wat in the area below 0.7 m. For the area higher than 1.5 m, the concentration of PM2 increases with the increase in water flow, which indicates that a larger water fl effectively suppress dust, mainly in the bottom area. At the same time, the large flow intensifies the disturbance of the surrounding airflow, and the disturbed airfl ries dust diffusion, which makes the dust such as PM2.5 spread to a higher area.

Conclusions
(1) The composite spraying slurry with clay as the main base material has sealing performance, certain bending resistance, and good adhesion, wh be used for the air leakage plugging technology of spraying in roadways. (2) The distribution of solid dust is determined by the distribution of the wate under the action of spray. The distribution area of dust is similar to tha water phase, mainly at the two sides and near the bottom of the roadway pared with the non-spray condition, the effect of the spray dust reduction vious. (3) Under the action of spraying, the bottom area of the roadway is covered b flow, and the dust stratification phenomenon is obvious in this area. Th particle size gradually decreases from the bottom to the top, and the large p size dust is deposited at the bottom, while the small particle size dust pended at a certain height; the diffusion area is gradually increased. (4) The influence of spray angle on dust is mainly reflected in the initial du shape and dust diffusion time. The larger the spray angle is, the faster th sion is. The influence of spray angle on the diffusion of dust, especially PM mainly concentrated in the middle and lower regions. (5) When calculating the velocity, the dust concentration is larger in the whole area. However, in the area higher than 1.5 m, the concentration of PM2.5 in with the increase in water flow, which indicates that the dust suppressio of a larger water flow is mainly reflected in the bottom area, and the dis surrounding airflow can make PM2.5 diffuse to higher areas.

Conclusions
(1) The composite spraying slurry with clay as the main base material has a good sealing performance, certain bending resistance, and good adhesion, which can be used for the air leakage plugging technology of spraying in roadways. (2) The distribution of solid dust is determined by the distribution of the water phase under the action of spray. The distribution area of dust is similar to that of the water phase, mainly at the two sides and near the bottom of the roadway. Compared with the non-spray condition, the effect of the spray dust reduction is obvious. (3) Under the action of spraying, the bottom area of the roadway is covered by dust flow, and the dust stratification phenomenon is obvious in this area. The dust particle size gradually decreases from the bottom to the top, and the large particle size dust is deposited at the bottom, while the small particle size dust is suspended at a certain height; the diffusion area is gradually increased. (4) The influence of spray angle on dust is mainly reflected in the initial dust flow shape and dust diffusion time. The larger the spray angle is, the faster the diffusion is. The influence of spray angle on the diffusion of dust, especially PM2.5, is mainly concentrated in the middle and lower regions. (5) When calculating the velocity, the dust concentration is larger in the whole nozzle area.
However, in the area higher than 1.5 m, the concentration of PM2.5 increases with the increase in water flow, which indicates that the dust suppression effect of a larger water flow is mainly reflected in the bottom area, and the disturbed surrounding airflow can make PM2.5 diffuse to higher areas. Funding: This research received no external funding.

Data Availability Statement:
The Microsoft Excel Worksheet data used to support the findings of this study are available from the corresponding author (18342833697@163.com) upon request.