Multi-Objective Optimization for Selecting and Siting the Cost-Effective BMPs by Coupling Revised GWLF Model and NSGAII Algorithm

Best management practices (BMPs) are an effective way to control water pollution. However, identification of the optimal distribution and cost-effect of BMPs provides a great challenge for watershed policy makers. In this paper, a semi-distributed, low-data, and robust watershed model, the Revised Generalized Watershed Loading Function (RGWLF), is improved by adding the pollutant attenuation process in the river channel and a bank filter strips reduction function. Three types of pollution control measures—point source wastewater treatment, bank filter strips, and converting farmland to forest—are considered, and the cost of each measure is determined. Furthermore, the RGWLF watershed model is coupled with a widely recognized multi-objective optimization algorithm, the non-dominated sorting genetic algorithm II (NSGAII), the combination of which is applied in the Luanhe watershed to search for spatial BMPs for dissolved nitrogen (DisN). Fifty scenarios were finally selected from numerous possibilities and the results indicate that, at a minimum cost of 9.09 × 107 yuan, the DisN load is 3.1 × 107 kg and, at a maximum cost of 1.77 × 108 yuan, the total dissolved nitrogen load is 1.31 × 107 kg; with the no-measures scenario, the DisN load is 4.05 × 107 kg. This BMP optimization model system could assist decision-makers in determining a scientifically comprehensive plan to realize cost-effective goals for the watershed.


Introduction
Water pollution has received increasing attention, and many countries have increased their investments into water pollution control and water resources protection [1]. Designing scientific, reasonable, and efficient management measures to control or reduce pollutants at the watershed scale has become one of the most challenging problems for policy researchers and decision makers [2]. Many policies for the selection of best management practice (BMPs) have been created and applied to specific cases all around the world. For example, the United States and Europe have developed the corresponding Total Maximum Daily Loads and European Water Framework Directive for such purposes [3,4]. The implementation of these plans has provided a sufficient theoretical basis for subsequent watershed governance research [5].
BMPs are the most effective measure for controlling watershed pollution, including vegetative filter strips, land-use transformation, reducing the amount of fertilizer, terraces, and so on [6]. In general, BMP implementation plans should consist of a combination of maximum pollution reduction and

Study Area and Data Sources
The Luanhe River watershed, which is located in North China (Figure 1), was selected in this study. It is a major component of one of the nine main river watersheds in China: the Haihe River watershed. It has been listed by the Chinese government as an important ecological conservation area in the Beijing-Tianjin-Hebei region. At the same time, its downstream reservoir is an important source of drinking water. The study watershed covers an area of about 30,000 km 2 . According to the 2010 national Land Cover Data set, the watershed consists of 39.2% forest, 33.3% grassland, 21.6% agricultural area, and 1% water bodies. The climate is dominated by temperate semiarid monsoon climate. From 2000-2014, the annual average temperature for this area was 5.7 • C and the mean annual precipitation was 422 mm. Most of the precipitation was concentrated between April and August.
Water 2020, 12, x FOR PEER REVIEW 3 of 12

Study Area and Data Sources
The Luanhe River watershed, which is located in North China (Figure 1), was selected in this study. It is a major component of one of the nine main river watersheds in China: the Haihe River watershed. It has been listed by the Chinese government as an important ecological conservation area in the Beijing-Tianjin-Hebei region. At the same time, its downstream reservoir is an important source of drinking water. The study watershed covers an area of about 30,000 km 2 . According to the 2010 national Land Cover Data set, the watershed consists of 39.2% forest, 33.3% grassland, 21.6% agricultural area, and 1% water bodies. The climate is dominated by temperate semiarid monsoon climate. From 2000-2014, the annual average temperature for this area was 5.7 °C and the mean annual precipitation was 422 mm. Most of the precipitation was concentrated between April and August. QGIS3 (https://qgis.org/en/site/index.html) and TauDEM (http://hydrology.usu.edu/taudem) were used to divide the Luanhe River Watershed into 62 sub-basins. Climate data were obtained from the Annual Hydrological Report P. R. China for precipitation data and the China Meteorological Data Service Center for temperature data. Thirty-meter resolution digital elevation models (DEMs) were downloaded from the Geospatial Data Cloud (http://www.gscloud.cn). Furthermore, a land-use map (in vector format) was provided by the National Earth System Science Data Center (http://www.geodata.cn). Observed flow data were gathered from the Annual Hydrological Report P. R. China. The hydrological monitoring station and the water quality monitoring station are located in sub-basin 62, which is at the outlet of the whole watershed. The above-mentioned data for the model setup are summarized in Table 1. QGIS3 (https://qgis.org/en/site/index.html) and TauDEM (http://hydrology.usu.edu/taudem) were used to divide the Luanhe River Watershed into 62 sub-basins. Climate data were obtained from the Annual Hydrological Report P. R. China for precipitation data and the China Meteorological Data Service Center for temperature data. Thirty-meter resolution digital elevation models (DEMs) were downloaded from the Geospatial Data Cloud (http://www.gscloud.cn). Furthermore, a land-use map (in vector format) was provided by the National Earth System Science Data Center (http://www.geodata.cn). Observed flow data were gathered from the Annual Hydrological Report P. R. China. The hydrological monitoring station and the water quality monitoring station are located in sub-basin 62, which is at the outlet of the whole watershed. The above-mentioned data for the model setup are summarized in Table 1.

The Watershed Model
The RGWLF model is a semi-distributed simulation model, which includes sub-basin calculation and the channel routing process, in contrast to the original model (GWLF) [25]. Detailed improvements and verification can be referred to in the author's previous article [24]. However, the original study did not include a description of the pollutant transport process in the channel. In this study, we added nutrient channel routing algorithms and made several references to the equations of the Sparrow models. Its main assumption is that contaminant flux along the stream satisfies a first-order decay process and the fraction of contaminant removed over a given stream distance is estimated as an exponential function of a first-order reaction rate coefficient and the cumulative water time of travel over this distance [26]: where NtrStore i,t represents the amount of nutrient load in reach i at day t; UpNtr i,t represents the amount of nutrient load from upstream in reach i at day t; LandNtr i,t represents the amount of nutrient load from local land area in reach i at day t; PntNtr i,t represents the amount of nutrient load from a point source in reach i at day t; NtrOut i,t represents the amount of nutrient load to an outflow before attenuation in reach i at day t; NtrOut i,t ' represents the amount of nutrient load to an outflow after attenuation in reach i at day t; θ i represent the nutrient attenuation exponent in reach i; and TravelTime i,t represents the flow travel time in reach i at day t.

BMPs and Costs
Three management practices were selected in this study: point source wastewater treatment, bank filter strips, and converting farmland to forest. The cost information for each practice is summarized in Table 2, which was based on published data and reports for this region.
According to the characteristics of point source wastewater in the study area, the sequencing batch reactor (SBR) treatment process was selected as the treatment method. This process is suitable for treating starch plant wastewater [27,28]. The cost of wastewater treatment consists of two parts: the construction of a wastewater treatment plant and wastewater treatment per unit volume: where 2.978 × Q i 0.9427 represents the construction costs of the sewage treatment plant [29], where Q i (m 3 ·day −1 ) represents the scale of sewage treatment in sub-basin i; T represents the total number of days during the simulation; q i,k (m 3 ) represents the actual treatment flow of the sewage treatment plant in sub-basin i at day t; and Ce (yuan/m 3 ) represents the costs of treating wastewater per cubic meter.
The cost of land-use conversion refers to the policy documents of the Chinese Ministry of Finance on returning farmland to forests. The bank filter strip trapping efficiency for nutrients is calculated using the following equations: where trap surface is the fraction of the constituent loading trapped by the filter strip, trap subsurf is the fraction of the subsurface flow constituent loading trapped by the filter strip, and width filtstrip is the width of the filter strip (m).

Multi-Objective Functions and NSGAII Optimization Processes
NSGAII generates offspring using a specific type of crossover and mutation and selects the next generation according to non-dominated sorting and crowding distance comparison. Figure 2 illustrates the genetic encoding of the various measure's structures for arrangement of conservation practices in the optimization algorithm. The sub-basins delineated by RGWLF and the configurations of management practices in each sub-basin form the basic chromosome units. The length of each chromosome is equal to the total number of sub-basins.
Water 2020, 12, x FOR PEER REVIEW 5 of 12 According to the characteristics of point source wastewater in the study area, the sequencing batch reactor (SBR) treatment process was selected as the treatment method. This process is suitable for treating starch plant wastewater [27,28]. The cost of wastewater treatment consists of two parts: the construction of a wastewater treatment plant and wastewater treatment per unit volume: where 2.978 * Qi 0.9427 represents the construction costs of the sewage treatment plant [29], where Qi (m 3 ·day −1 ) represents the scale of sewage treatment in sub-basin i; T represents the total number of days during the simulation; qi,k (m 3 ) represents the actual treatment flow of the sewage treatment plant in sub-basin i at day t; and Ce (yuan/m 3 ) represents the costs of treating wastewater per cubic meter.
The cost of land-use conversion refers to the policy documents of the Chinese Ministry of Finance on returning farmland to forests. The bank filter strip trapping efficiency for nutrients is calculated using the following equations: where trapsurface is the fraction of the constituent loading trapped by the filter strip, trapsubsurf is the fraction of the subsurface flow constituent loading trapped by the filter strip, and widthfiltstrip is the width of the filter strip (m).

Multi-Objective Functions and NSGAII Optimization Processes
NSGAII generates offspring using a specific type of crossover and mutation and selects the next generation according to non-dominated sorting and crowding distance comparison. Figure 2 illustrates the genetic encoding of the various measure's structures for arrangement of conservation practices in the optimization algorithm. The sub-basins delineated by RGWLF and the configurations of management practices in each sub-basin form the basic chromosome units. The length of each chromosome is equal to the total number of sub-basins. The analytical flow chart for this research is outlined in Figure 3. The watershed model was created to provide the nutrient load; the cost of management practices will be calculated by referring to the policy literature and actual surveys. To obtain the most cost-effective set of BMPs, the operation must satisfy two objective functions-the minimization of net total cost and the lowest dissolved nitrogen load-which are expressed by the equations: The analytical flow chart for this research is outlined in Figure 3. The watershed model was created to provide the nutrient load; the cost of management practices will be calculated by referring to the policy literature and actual surveys. To obtain the most cost-effective set of BMPs, the operation must satisfy two objective functions-the minimization of net total cost and the lowest dissolved nitrogen load-which are expressed by the equations: where Cost pns,i , Cost lu,i , and Cost strip,I are the costs of wastewater treatment plant, converting land-use, and bank filter strisp in sub-basin i; and DisN i,BMPs is the total dissolved nitrogen load in sub-basin i.
Water 2020, 12, x FOR PEER REVIEW 6 of 12 where Costpns,i, Costlu, i, and Coststrip,I are the costs of wastewater treatment plant, converting land-use, and bank filter strisp in sub-basin i; and DisNi,BMPs is the total dissolved nitrogen load in sub-basin i. The optimization process consists of several procedures, as follows: (1) Initialize the population and read the watershed model input data. Then, simulate the baseline scenario. (2) For the two objective functions, obtain the pollutant load of the basin model and the net cost of each management measure combination. (3) Through a series of processes, including non-dominated sorting, calculation of crowded distance, selection, crossover, and mutation, NSGAII obtains the Pareto-optimal result set of the current generation. (4) Repeat the second process, determine whether it is the last generation, and then perform the third process.

RGWLF Model Calibration and Validation
Nine years of monthly records of observed streamflow and dissolved nitrogen data were used for model calibration and verification at the outlet of the watershed. The simulation period was from 2005-2014, in which the first year (2005) was used as a warming-up period, the data from 2006-2011 were used for the calibration process, and the rest were used for model validation.
The generalized likelihood uncertainty estimation (GLUE), a frequently used Bayesian parameter estimation method, was used for calibration analysis in terms of both hydrology and pollutants for the watershed model [30,31]. Table 3 lists the uniform prior distribution range and best value for each calibrated parameter after 10,000 iterations. The Nash-Sutcliffe efficiency (NES) and the coefficient of determination (R 2 ) were selected as the simulation evaluation criteria [32]. NSE can range from minus infinity to 1 and an efficiency of 1 indicates a perfect performance. R 2 ranges from 0 to 1, with higher values indicating a better fit for the model. The optimization process consists of several procedures, as follows: (1) Initialize the population and read the watershed model input data. Then, simulate the baseline scenario. (2) For the two objective functions, obtain the pollutant load of the basin model and the net cost of each management measure combination. (3) Through a series of processes, including non-dominated sorting, calculation of crowded distance, selection, crossover, and mutation, NSGAII obtains the Pareto-optimal result set of the current generation. (4) Repeat the second process, determine whether it is the last generation, and then perform the third process.

RGWLF Model Calibration and Validation
Nine years of monthly records of observed streamflow and dissolved nitrogen data were used for model calibration and verification at the outlet of the watershed. The simulation period was from 2005-2014, in which the first year (2005) was used as a warming-up period, the data from 2006-2011 were used for the calibration process, and the rest were used for model validation.
The generalized likelihood uncertainty estimation (GLUE), a frequently used Bayesian parameter estimation method, was used for calibration analysis in terms of both hydrology and pollutants for the watershed model [30,31]. Table 3 lists the uniform prior distribution range and best value for each calibrated parameter after 10,000 iterations. The Nash-Sutcliffe efficiency (NES) and the coefficient of determination (R 2 ) were selected as the simulation evaluation criteria [32]. NSE can range from minus infinity to 1 and an efficiency of 1 indicates a perfect performance. R 2 ranges from 0 to 1, with higher values indicating a better fit for the model. As shown in Figure 4, during the calibration period, the NES was 0.93 for streamflow and 0.68 for DisN; moreover, the R 2 values were 0.93 and 0.68 for the simulated streamflow and DisN, respectively. At the same time, the model validation for the streamflow R 2 and NES were 0.77 and 0.78, respectively. Similar to streamflow, DisN had a lower validation value of 0.60 for R 2 and 0.58 for NES. Both streamflow and DisN simulations by the model had a good performance on a monthly time scale, which indicates robustness of the RGWLF model, according to previous research [33].  As shown in Figure 4, during the calibration period, the NES was 0.93 for streamflow and 0.68 for DisN; moreover, the R 2 values were 0.93 and 0.68 for the simulated streamflow and DisN, respectively. At the same time, the model validation for the streamflow R 2 and NES were 0.77 and 0.78, respectively. Similar to streamflow, DisN had a lower validation value of 0.60 for R 2 and 0.58 for NES. Both streamflow and DisN simulations by the model had a good performance on a monthly time scale, which indicates robustness of the RGWLF model, according to previous research [33].

Sensitivity Analysis of NSGAII Operational Parameters
To ensure accuracy of the NSGAII and optimization operational efficiency, sensitivity analyses were performed for the four key parameters, including population size, generations, crossover, and

Sensitivity Analysis of NSGAII Operational Parameters
To ensure accuracy of the NSGAII and optimization operational efficiency, sensitivity analyses were performed for the four key parameters, including population size, generations, crossover, and mutation probability, by the one-at-a-time sensitivity analysis method [16,34]. Table 4 lists the default and per-change values for the four NSGAII parameters.  Figure 5a-d illustrate the Pareto-optimal fronts under per-change for the four key parameters. It is apparent in Figure 5a that the improvement in the Pareto-optimal fronts was remarkable as the population size increased from 30 to 50, but there was little gap for Pareto-optimal fronts when the population size was increased from 80 to 200. The main reason for this case is possibly that a population size of 50 had enough convergence chance for the solution space's freedom of the whole optimization system. Furthermore, a value of 50 would considerably reduce the computation time, compared to the default values of 80, 100 and 200.
Water 2020, 12, x FOR PEER REVIEW 8 of 12 mutation probability, by the one-at-a-time sensitivity analysis method [16,34]. Table 4 lists the default and per-change values for the four NSGAII parameters.  Figure 5a that the improvement in the Pareto-optimal fronts was remarkable as the population size increased from 30 to 50, but there was little gap for Pareto-optimal fronts when the population size was increased from 80 to 200. The main reason for this case is possibly that a population size of 50 had enough convergence chance for the solution space's freedom of the whole optimization system. Furthermore, a value of 50 would considerably reduce the computation time, compared to the default values of 80, 100 and 200. As shown in Figure 5b, the number of generations also had an appreciable impact on the Paretooptimal fronts. A significant improvement in the Pareto-optimal front was noticed, with the number of generations increasing from 50 to 200. In stark contrast, increasing from 200 to 500 did not bring any improvement for the Pareto-optimal fronts.
Unlike the above two parameters, the Pareto-optimal front was not sensitive to changes in the crossover probability, which is displayed in Figure 5c. The Pareto-optimal front had an inconspicuous shift approaching the origin as the crossover probability increasing from 0.1 to 0.5. When the crossover probability reached a value of 0.7, the Pareto-optimal front was farther away from the origin. As shown in Figure 5b, the number of generations also had an appreciable impact on the Pareto-optimal fronts. A significant improvement in the Pareto-optimal front was noticed, with the number of generations increasing from 50 to 200. In stark contrast, increasing from 200 to 500 did not bring any improvement for the Pareto-optimal fronts. Unlike the above two parameters, the Pareto-optimal front was not sensitive to changes in the crossover probability, which is displayed in Figure 5c. The Pareto-optimal front had an inconspicuous shift approaching the origin as the crossover probability increasing from 0.1 to 0.5. When the crossover probability reached a value of 0.7, the Pareto-optimal front was farther away from the origin.
The trend of the Pareto-optimal front, as affected by the change of Mutation probability, is presented in Figure 5d. What stands out most in this figure is that mutation probability is a sensitive parameter, especially in the range from 0.001 to 0.03, where the Pareto-optimal front approached the origin with an increase of parameter value. However, there was no benefit for the Pareto-optimal front as the parameter increased from 0.03 to 0.08.
Considering all of the above analyses, the values 50, 200, 0.5 and 0.03 were used as population size, generations, crossover, and mutation probability, respectively, for the further optimization processes.

Optimization Result and Cost-Effectiveness Analysis
The baseline scenario for this watershed was no management practice and 4.05 × 10 7 kg for the total dissolved nitrogen load over nine years. Figure 6 provides the final optimization progress with two objectives, minimizing the net cost and dissolved nitrogen load by scattering four Pareto-optimal fronts belonging to four generations (1, 50, 100 and 200). The overall trend for the four scatter diagrams was that the dissolved nitrogen decreased as the net cost increased. Each new generation's chromosomes were initialized by random numbers without no optimization process (such as non-dominance, selection, crossover, and so on), so it was regarded as the 0th generation and not shown in the figure. In the first generation, the distribution of points was more concentrated, indicating that the solutions were less differentiated. As the number of generations increased, the solution became more and more scalable, and came closer to the origin. For the final generation, the most widespread solution set, which was closest to the origin, can be seen. Thus, the best quality and broadest decision supports were supplied to the policy researchers and decision-makers.
Water 2020, 12, x FOR PEER REVIEW 9 of 12 The trend of the Pareto-optimal front, as affected by the change of Mutation probability, is presented in Figure 5d. What stands out most in this figure is that mutation probability is a sensitive parameter, especially in the range from 0.001 to 0.03, where the Pareto-optimal front approached the origin with an increase of parameter value. However, there was no benefit for the Pareto-optimal front as the parameter increased from 0.03 to 0.08.
Considering all of the above analyses, the values 50, 200, 0.5 and 0.03 were used as population size, generations, crossover, and mutation probability, respectively, for the further optimization processes.

Optimization Result and Cost-Effectiveness Analysis
The baseline scenario for this watershed was no management practice and 4.05 × 10 7 kg for the total dissolved nitrogen load over nine years. Figure 6 provides the final optimization progress with two objectives, minimizing the net cost and dissolved nitrogen load by scattering four Pareto-optimal fronts belonging to four generations (1, 50, 100 and 200). The overall trend for the four scatter diagrams was that the dissolved nitrogen decreased as the net cost increased. Each new generation's chromosomes were initialized by random numbers without no optimization process (such as non-dominance, selection, crossover, and so on), so it was regarded as the 0th generation and not shown in the figure. In the first generation, the distribution of points was more concentrated, indicating that the solutions were less differentiated. As the number of generations increased, the solution became more and more scalable, and came closer to the origin. For the final generation, the most widespread solution set, which was closest to the origin, can be seen. Thus, the best quality and broadest decision supports were supplied to the policy researchers and decision-makers. The set of solutions was divided into three segments with four endpoints, which were: the lowest cost, the lower tertile cost point, the higher tertile cost point, and the highest cost. The values of cost, dissolved nitrogen load, and spatial distribution of corresponding management measures for the four scenarios are shown in Figure 7. For the lowest cost scenario (Figure 7a), the scale of treatment of polluted water plants is small and the measures are mainly bank filter strips and converting farmland to forest. As cost increased, the intensity and scale of management practices also increased, which is illustrated in Figure 7b,c. At the point of maximum cost (Figure 7d), the load of dissolved nitrogen reached its minimum value, where the designed daily treatment capacity of the sewage plant was The set of solutions was divided into three segments with four endpoints, which were: the lowest cost, the lower tertile cost point, the higher tertile cost point, and the highest cost. The values of cost, dissolved nitrogen load, and spatial distribution of corresponding management measures for the four scenarios are shown in Figure 7. For the lowest cost scenario (Figure 7a), the scale of treatment of polluted water plants is small and the measures are mainly bank filter strips and converting farmland to forest. As cost increased, the intensity and scale of management practices also increased, which is illustrated in Figure 7b,c. At the point of maximum cost (Figure 7d), the load of dissolved nitrogen reached its minimum value, where the designed daily treatment capacity of the sewage plant was extremely high and there was no conversion of farmland to forests in some upstream sub-basins. The majority of management practices are concentrated in middle and lower regions of the watershed.

Conclusions
In this study, we supplemented the RGWLF model with the addition of a pollutant attenuation process in the river channel and a bank filter strips reduction function, based on our previous research. Meanwhile, taking into account the regional pollution source composition of the watershed studied and the characteristics of the models used, three types of pollution control measures-point source wastewater treatment, bank filter strips, and converting farmland to forest-were considered, and the cost of each measure was determined. Furthermore, the optimization algorithm NGSAII was linked with the RGWFL watershed model and the implemented measures to search for a Paretooptimal set of BMPs. Before the final optimization calculation, sensitivity analyses for the four key parameters of NGSAII were performed. According to the results of the sensitivity analysis, the entire coupled model system supplied 50 solutions which could provide managers with many pollution reduction options. In the end, depending on the cost, we chose four gradient solutions and demonstrated the geospatial distribution of their different management measure characteristics and briefly analyzed the differences and features of the four solutions.
The research results show that, with almost no increase in data requirements, dissolved nitrogen had an excellent simulation performance, expanding the spatial scope of pollutant simulation for the GWLF. Moreover, due to its robustness and semi-distribution, the RGWLF model was able to be coupled with NSGAII. The entire linkage system had good performance in the optimization process and provided a range of watershed implementation measures for DisN reduction and minimizing cost, which is a worthy reference for policy researchers and decision-makers to realize their watershed management goals. However, limited by the available data, funding, and researchers' capabilities, we did not consider other target indicators, such as sediment, phosphorus, and so on, which could be carried out in future research.
Author Contributions: Y.W. conceived and designed the framework; Z.Q. and G.K. wrote the paper; Z.Q. and X.W. conducted software and data analysis; Z.Q. and Y.S. Visualization; Y.W. contributed to improving the article. All authors have read and agreed to the published version of the manuscript.

Conclusions
In this study, we supplemented the RGWLF model with the addition of a pollutant attenuation process in the river channel and a bank filter strips reduction function, based on our previous research. Meanwhile, taking into account the regional pollution source composition of the watershed studied and the characteristics of the models used, three types of pollution control measures-point source wastewater treatment, bank filter strips, and converting farmland to forest-were considered, and the cost of each measure was determined. Furthermore, the optimization algorithm NGSAII was linked with the RGWFL watershed model and the implemented measures to search for a Pareto-optimal set of BMPs. Before the final optimization calculation, sensitivity analyses for the four key parameters of NGSAII were performed. According to the results of the sensitivity analysis, the entire coupled model system supplied 50 solutions which could provide managers with many pollution reduction options. In the end, depending on the cost, we chose four gradient solutions and demonstrated the geospatial distribution of their different management measure characteristics and briefly analyzed the differences and features of the four solutions.
The research results show that, with almost no increase in data requirements, dissolved nitrogen had an excellent simulation performance, expanding the spatial scope of pollutant simulation for the GWLF. Moreover, due to its robustness and semi-distribution, the RGWLF model was able to be coupled with NSGAII. The entire linkage system had good performance in the optimization process and provided a range of watershed implementation measures for DisN reduction and minimizing cost, which is a worthy reference for policy researchers and decision-makers to realize their watershed management goals. However, limited by the available data, funding, and researchers' capabilities, we did not consider other target indicators, such as sediment, phosphorus, and so on, which could be carried out in future research.