Parameterization of a Rising Smoke Plume for a Large Moving Ship Based on CFD

: The plume rising height of a ship will directly affect the maximum ground concentration and distance from the source caused by ﬂue gas emission. Ship movement has an important effect on plume rising, but it is often ignored in previous studies. We simulated the weakening effect caused by ship movement by considering the inﬂuence of four main parameters (wind speed, ship speed, ﬂue gas exit velocity, and ﬂue gas exit temperature) on the smoke plume rising height, using the computational ﬂuid dynamics (CFD) model (PHOENICS version 6.0 CHAM, London, UK). The main parameters affecting the difference in plume rising height between stationary and moving sources for the same parameter settings are the wind speed and the ship speed. Therefore, we established two simpliﬁed calculation methods that corrected the ﬂue gas exit velocity ( V (cid:48) exit ) and the ﬂue gas exit temperature ( T (cid:48) ) for approximately simulating the smoke plume rising height of the moving ship using the formula of a stationary ship. Veriﬁcation cases indicated that the corrected V (cid:48) exit (the average of relative error is 5.48%) and the corrected T (cid:48) (the average of relative error is 60.07%) not only saved calculation time but also improved the simulation accuracy compared with the uncorrected stationary source scheme (the average of relative error is 135.38%). Of these correction methods, the scheme with corrected V (cid:48) exit is more effective. The intention is to provide some references for the ﬁeld experimentation of moving ship plume rising in different ports in the future and to further study the mechanism of moving ship plume rising.


Introduction
Emissions from ships are increasing year by year and will increase in the future due to the growth in global trade. Air pollutant emissions from ships entering and leaving ports greatly affect the air quality in coastal areas [1][2][3] and inland areas hundreds of kilometers away [4]. Air pollutants also contribute to global atmospheric changes [5,6]. Ship emission pollutants range from conventional air pollutants, such as SO 2 [7], NO X [8], and PM [9,10], to organic pollutants [11] and some secondary inorganic ions [12]. These pollutants not only affect air quality directly but also pose a significant potential health risk [13][14][15][16], causing a certain number of premature deaths each year. It is therefore very important to study the dispersion of air pollutants emitted from ships to update the standards of air pollutants emitted from ships and to improve the air quality in the port areas in order to ultimately facilitate sustainable growth [17].
Model simulations are used to study the dispersion of ship exhaust plumes [18]. Models such as the weather research and forecasting with chemistry (WRF/Chem) model [19,20], the weather research and forecasting community multiscale air quality (WRF/CMAQ) model [21], and the California puff (CALPUFF) model [22][23][24][25], can obtain good simulation results. In these previous studies, ship pollution is often generalized as a non-point source to simulate its diffusion, and in the process of ship movement, moving pollution sources are often generalized as fixed line sources, which may cause some errors in the detection of ship pollutant concentration at port scale. Using the CALPUFF model as an example, the CALPUFF model is a three-dimensional unsteady air quality model developed on the basis of the Lagrange smoke cluster model. Based on similarity equation, turbulence, emission strengths, transformation, and removal, the CALPUFF model uses space and time varying meteorology to model gas and particle diffusion, considering buoyancy and momentum plume rise, stack effect, and building effect. It can simulate the transport of pollutants over a distance of 50 km and above, and has good simulation results for the diffusion of point sources, line sources, and unsteady conditions (quiet wind, smoke, coastal effect, etc.) [16]. A short-term field experiment was conducted at Yantian Port in Shenzhen, China in June 2018. The experimental results, however, show that the air pollutant concentration simulated by CALPUFF was lower than that observed on the shore. This underestimation may be related to the low estimation of ship source intensity or the failure of the simulations to account for emissions from gathering and transporting machinery in the port area. Some ship emission simulation studies also underestimated the actual concentrations of air pollutants [26,27]. The underestimation rate was related to the ratio of gas velocity to wind speed at funnel height (UR). The UR increased and the underestimation rate decreased. This was because an increase in UR means an increase in the pollutant momentum flux, which enhances the plume ascending effect and weakens the plume diffusion effect. The rise of the ship plume will therefore be affected by the flue gas exit velocity and wind speed.
The general underestimation mentioned focused attention on the ship exhaust pollution source characteristics. We speculated that this may be due to the fact that the simulated effective source height is much higher than the actual plume height, which may be related to the layout of the ship chimneys and the ship's movements. Xu et al. [28] analyzed the influence of the ship chimney layout. Our study will consider the influence of ship movement on emission plumes dispersion. Plume rising is one of the important behaviors of plume dispersion, which directly affects the maximum ground concentration and distance from the source caused by flue gas emission. Our study, therefore, focuses on the influence of ship movement on plume rising height.
Plume rising is caused by two factors: dynamic uplift and buoyancy uplift [29]. Dynamic uplift means that the plume has upward kinetic energy, and will still be able to move after leaving the chimney. Buoyancy uplift refers to the density difference caused by the temperature difference, so that the atmosphere, other than the flue gas, produces a buoyancy effect on the flue gas. In the initial stage of plume rising, dynamic uplift is the main factor. With the flue gas mixing with the surrounding atmosphere gradually, the rising speed caused by the initial momentum gradually decreases and the buoyancy uplift starts to play a major role. After that, the turbulence causes the structure of the plume to collapse, and the plume gradually flattens until it no longer rose. Marine flue gas is a high-temperature flue gas, where the combustion exhaust of marine diesel engines contains mainly nitrogen, sulfur oxides, and other gases. The ship exhaust temperature must also be above the acid dew point of the flue gas (generally above 200 • C) to reduce corrosion. To avoid downwash of the flue gas stream, there is also a lower velocity limit on the flue gas exit velocity, where the ratio of the flue gas exit velocity to the wind speed is greater than 2 to inhibit downwash [30]. In the case of high temperatures and certain flue gas exit velocities, the ship emissions are a buoyant moving source [31]. With the gradual release of waste heat from the actual ship plume along the route, the ship's movement disperses the air mass rather than causing a fixed release of heat, as in the case of a buoyant stationary source. If the plume rising is modeled using a Briggs lift equation that is similar to that in the CALPUFF model, where the source is equivalent to a row of buoyant point sources, enhanced plume rising will be observed due to point source clustering, which will likely cause high modeled plume rising heights. The actual thermal rising of the ship source is however lower, and the plume rising from the moving line source of the ship should be attenuated compared to the point source plume rising, because the duration of the emission at a specific location is short. This indicates that ship movement is not negligible for plume rising, because it can reflect the emission characteristics of the ship as a source of buoyancy movement.
Computational fluid dynamics (CFD) models use finite difference and finite volume methods to solve the Navier-Stokes equations in 3D space, providing complex analyses of fluid flows based on the conservation of mass and momentum [32]. The CFD model can perform more refined modeling of ports and ships, and can well simulate the influence of the hull itself on the flow field due to refined simulation. It is therefore one of the more commonly used methods in environmental pollution research and ship design research. In ship design research, it is used to simulate the flow field of ships and compares well with the actual measurement results [33][34][35]. The CFD model also simulates atmospheric convection conditions that take into account dynamic and thermal effects [36]. In addition, it can also simulate ship emission data with higher temporal resolution and reduce the uncertainty caused by ignoring the hourly fluctuations of ship emissions [37] in coastal urban areas and ports where ship activities are frequent. These applications convinced the authors that rising smoke plumes during ship movement could also be simulated by using the CFD software PHOENICS version 6.0 in this study. This study adopted the CFD model of ship buoyancy source as established by Xu et al. [28]. The ship movement was considered on this basis. The main parameters that affect rising smoke plumes from ships include ship speed, wind speed, flue gas exit velocity, and flue gas exit temperature [28,[38][39][40][41][42][43][44]. Wind direction may also be an important factor. When the direction of ship movement is not consistent with the environmental wind direction, it will affect the direction of plume dispersion. However, this influence is local, because the environmental wind covers the whole simulation area, while the hull movement is only local. Kulkarni et al. [45] considered the yaw angle of the ambient wind relative to the ship's heading, and turned the ship's heading and the ambient wind into a "synthetic wind" to consider the influence of the yaw angle. This is a simplified simulation method commonly used to observe whether the plume washing around the chimney will cause smoke damage on the deck. However, such results are inaccurate, because it amplifies the local influence of the ship's navigation. This may not be the main reason why the simulated concentration in our observation experiment, and references [26] and [27], were lower than the observed concentration. The distance between the shoreline observation point and the chimney in our observation experiment is more than one kilometer, and the actual environmental wind speed, at such a distance away from the ship, is closer to the regional background wind speed when the ship travels upwind. The influence of ship navigation on the actual environmental wind speed at the observation point is much smaller than that near the chimney. Therefore, the low simulated concentration at distant observation points should not be caused entirely by the influence of ship navigation on the environmental flow field. We speculated that the more likely reason is that the lifting force of the exhaust plume decreases during sailing.
In this paper, we used the CFD model to simulate the degree of influence of four parameters, namely wind speed, ship speed, flue gas exit velocity, and flue gas exit temperature, on the plume rising height of ships with moving sources. By analyzing the difference in the plume rising height between the stationary source and the moving source under the same parameter setting, new formulas for calculating the plume rising height, including the ship movement, were established. Section 2 presents the numerical simulation scheme and its parameter values for the transport and diffusion of the ship's smoke plume. Section 3 shows the analyses of the rising smoke plume, which was simulated for both the stationary source ship and the moving ship. The simulation results of the moving source ship scheme were analyzed relative to the stationary scheme. The results from this analysis were used to establish simplified correction methods to approximate the smoke plume rising heights of moving ships by the relative changes in the two simulation schemes. Section 4 concludes the study.

Physical Model and Governing Equations
A typical large container ship at the Yantian Port in Shenzhen was selected as the research sample for modeling in June 2018. Figure 1 shows the ship model, the domain, and the grids in the CFD model. rising smoke plume, which was simulated for both the stationary source ship an moving ship. The simulation results of the moving source ship scheme were ana relative to the stationary scheme. The results from this analysis were used to est simplified correction methods to approximate the smoke plume rising heights of m ships by the relative changes in the two simulation schemes. Section 4 conclud study.

Physical Model and Governing Equations
A typical large container ship at the Yantian Port in Shenzhen was selected research sample for modeling in June 2018. Figure 1 shows the ship model, the do and the grids in the CFD model. Equations were set up for the CFD (PHOENICS version 6.0) model after the p cal model of the ship was imported into the model. A standard k-ε turbulence m which is a two-equation model, was chosen for the simulation. The differential m was chosen as a hybrid model that combines the central differencing scheme wi first-order upwind. It applies the central differencing scheme when | | 2 and a the first-order upwind when | | 2, where is the Peclet number, indicating t tio of convective velocity to diffusive velocity. The Boussinesq assumption was al troduced, which is about the density being constant (incompressible flow), allowing for change due to temperature variations (which induces buoyancy).
Xu et al. [28] validated the above model using wind tunnel experimental data the literature. The simulation results agree well with the wind tunnel test results cating that using the CFD model for the simulation of ship plume behavior is feasib

Experimental Case Simulation Parameter Scheme
This study is a parametric simulation of the plume characteristics of a single ing ship. The parameters that influence the rising plume of a ship include the speed, wind speed, flue gas exit velocity, and flue gas exit temperature. For actual the ship speed is closely related to the flue gas exit velocity and flue gas temper The reference ship sample research data, however, only had the flue gas exit ve data that changed with ship speed, but not the flue gas exit temperature data. On flue gas exit velocity was therefore associated with the working condition in the p eter setting.
Near-surface wind speed statistics from meteorological stations in the Dapen sea area of Shenzhen from 2009 to 2018 [46] indicated that the wind speed varie tween 1.5 and 15 m/s. We subdivided this wind speed segment further into fou ments and took the representative wind speed values of each segment for the num simulations in this study. Table 1 shows the detailed values. The ship speed values Equations were set up for the CFD (PHOENICS version 6.0) model after the physical model of the ship was imported into the model. A standard k-ε turbulence model, which is a two-equation model, was chosen for the simulation. The differential model was chosen as a hybrid model that combines the central differencing scheme with the first-order upwind. It applies the central differencing scheme when |P e | < 2 and applies the first-order upwind when |P e | ≥ 2, where P e is the Peclet number, indicating the ratio of convective velocity to diffusive velocity. The Boussinesq assumption was also introduced, which is about the density being constant (incompressible flow), allowing only for change due to temperature variations (which induces buoyancy).
Xu et al. [28] validated the above model using wind tunnel experimental data from the literature. The simulation results agree well with the wind tunnel test results, indicating that using the CFD model for the simulation of ship plume behavior is feasible.

Experimental Case Simulation Parameter Scheme
This study is a parametric simulation of the plume characteristics of a single moving ship. The parameters that influence the rising plume of a ship include the ship speed, wind speed, flue gas exit velocity, and flue gas exit temperature. For actual ships, the ship speed is closely related to the flue gas exit velocity and flue gas temperature. The reference ship sample research data, however, only had the flue gas exit velocity data that changed with ship speed, but not the flue gas exit temperature data. Only the flue gas exit velocity was therefore associated with the working condition in the parameter setting.
Near-surface wind speed statistics from meteorological stations in the Dapeng Bay sea area of Shenzhen from 2009 to 2018 [46] indicated that the wind speed varied between 1.5 and 15 m/s. We subdivided this wind speed segment further into four segments and took the representative wind speed values of each segment for the numerical simulations in this study. Table 1 shows the detailed values. The ship speed values were referenced to the inbound and outbound ship speeds of a sample of ships in Dapeng Bay, Shenzhen in June 2018 (shown in Table A1 in the Appendix A). The ship speeds that were used varied from 0 to 16 knots. These ship speed segments were also further subdivided into four segments. Table 1 shows the representative ship speed value of each segment of the numerical simulation.  The flue gas exit velocities at the representative ship speeds in Table 1 were taken with reference to the range of variation in actual emission data from a sample of ships at Yantian Port, Dapeng Bay, Shenzhen in June 2018 (shown in Table A2 in the Appendix A). Table 2 shows that the flue gas exit velocities of the ship samples that correspond to the four representative ship speeds varied between 0.26 and 1.26 m/s, 0.46 and 2.35 m/s, 1.94 and 10.37 m/s, as well as 5.01 and 26.15 m/s, respectively. The flue gas exit velocity varies considerably with the ship sample for the same ship speed. The influence of flue gas exit velocity on the plume rising for different ship speeds was analyzed. To understand the differences in the plume characteristics between the different ship samples, three flue gas exit velocities were set up based on the exit velocity sample characteristics for each ship speed. The exit velocities were low, medium, and high, representing low, medium, and high emission samples (which are represented by V1, V2, and V3, respectively). The analysis of the flue gas exit velocity effect on the rising plume only considers the difference in the flue gas exit velocities between ship samples for the same ship speed to avoid duplicate analyses. Table 2 shows the simulated emission velocity scenario settings. Based on the actual ship sample research results, the flue gas exit temperature of the ship varied between 60 and 400 • C (shown in Table A1 in the Appendix A). Since the flue gas exit temperature of the ship is generally higher than 200 • C to prevent acid corrosion, three cases of 200 • C, 300 • C, and 400 • C were therefore taken for this study (represented by T1, T2, and T3). The ship parameter settings were further considered for the three aforementioned flue gas temperature values (T1, T2, and T3), of which the combinations are shown in Table 2. This resulted in the full emission scenario for the actual simulation.
In both the moving source ship simulation and the stationary source ship simulation schemes, all the simulation parameters are the same, except for the movement of the ship. The stationary source ship simulation schemes will therefore also involve the simulation of the emission conditions at different ship speeds, even though the ship is stationary during the simulation. For the stationary source ship simulation, the ship speed changes during the simulation cause the change in the flue gas exit velocity, and are still treated as an effect of the change in ship speed in the analysis of the results to facilitate comparison with the results of the moving source ship schemes.
The area of high air pollutant concentrations contributed by the ship emissions is mainly concentrated close to the coast [21,47], specifically within 1-2 km from the ship track [48]. The air pollutant plume behavior 1 km behind the ship chimney is of specific interest in this study. The smoke plume rising heights of the maximum plume concentration at the 1 km downwind direction of the ship chimney in the X-Z plane was compared after completing the numerical simulations. The cubic spline interpolation of the meshing concentration given by numerical simulation was used to determine the smoke plume rising height.

Computational Domains, Boundary Conditions, and Simulation Settings
The computing grid and computing domain vary based on the ship speed (see Table 3). The grid setup mainly takes into account the dispersed simulation requirements of emissions. Given the dispersed nature of emissions, we would like to be able to set up at least one grid that has an outlet so that the actual impact of outlet dispersion can be simulated as finely as possible. The software sets the minimum time step for transient simulation to 1 s, so each outlet continues to discharge for at least 1 s. We actually set the duration of a single outlet to be 2~15 s, where 2 s is the discharge outlet duration at the highest ship speed (14 knots). The distance of 2 s from the ship at this ship speed is 14.392 m, so the grid spacing is 15 m. With smaller grids, the emission duration per grid would need to be less than 1 s, a time step setting that cannot be implemented in the software. In order to facilitate the comparison of the simulation results at various ship speeds, the grid spacing in this study is uniformly set as 15 m, that is, each grid on the ship route has at least one discharge outlet. This study determined the emission parameters for different working conditions based on the ship speed. These emission parameters applied to both the moving and stationary source simulation schemes. All the surfaces of the computational domain and the ship wall were non-slip boundary conditions. The exponential law wind profile was chosen in the vertical direction as the wind blew from the bow to the stern. The ambient fluid air was at 1 atmosphere pressure and the temperature was 20 • C.
The MOFOR function of PHOENICS was used to simulate the ship's movement. Transient simulations were used for the moving source ship simulation scheme and steadystate simulations were used for the stationary source simulation scheme. A series of INLET objects located in the path of the ship movement was used to simulate pollutant emissions. The INLET properties were used to set the flue gas exit velocity and flue gas exit temperature. The total simulation time for each moving source ship simulation case was 360 s and the results were taken for the period after the flow field stabilized.

Rising Height of the Smoke Plume for the Stationary and Moving Source Simulation Schemes
The rising height of the smoke plume of both the stationary source and the moving source schemes varied significantly with wind speed and emission scenarios. Figure 2 shows that the smoke plume rising height (hereafter denoted as H + ) of the two schemes always decreases as the wind speed increases from 3 m/s to 12 m/s. This is because as the wind speed of the atmospheric transverse wind gradually increases, the turbulence degree of the flow field intensifies, which accelerates the mixing process of flue gas at the outlet of the chimney and the surrounding atmosphere, and reduces the plume rising height. Emission scenarios also have a significant impact on H + . In Figure 2 for the wind speed of 3 m/s for the S4 group, the H + gradually increases as the emission levels increase from V1 (5.01 m/s) to V3 (26.15 m/s). Figure 3 shows selected simulation results for the stationary and moving source schemes for different flue gas exit temperatures. At a wind speed of 3 m/s, the H + increased gradually for both schemes as the flue gas exit temperature increased from T1 (200 • C) to T3 (400 • C) in the S2-V2 group. The reason is that the larger the flue gas exit velocity and temperature, the larger the initial momentum and heat of the flue gas, and the stronger the anti-disturbance ability of the mixed air flow to the transversal wind above the outlet during the process of diffusing into the surrounding atmosphere, leading to the higher plume rising height. The effect of the ship speed on the H + for the two schemes is, however, significantly different. For the V2 group in Figure 3, the H + of the stationary source scheme gradually increased with an increase in the ship speed from S1 (2 knots) to S4 (14 knots), as the flue gas exit velocity of S1 is lower than that of S4. The H + decreased and then increased with the minimum value of H + at the ship speed S2 scenario (6 knots) for the moving source scheme.
Transient simulations were used for the moving source ship simulation scheme and steady-state simulations were used for the stationary source simulation scheme. A series of INLET objects located in the path of the ship movement was used to simulate pollutant emissions. The INLET properties were used to set the flue gas exit velocity and flue gas exit temperature. The total simulation time for each moving source ship simulation case was 360 s and the results were taken for the period after the flow field stabilized.

Rising Height of the Smoke Plume for the Stationary and Moving Source Simulation Schemes
The rising height of the smoke plume of both the stationary source and the moving source schemes varied significantly with wind speed and emission scenarios. Figure 2 shows that the smoke plume rising height (hereafter denoted as H+) of the two schemes always decreases as the wind speed increases from 3 m/s to 12 m/s. This is because as the wind speed of the atmospheric transverse wind gradually increases, the turbulence degree of the flow field intensifies, which accelerates the mixing process of flue gas at the outlet of the chimney and the surrounding atmosphere, and reduces the plume rising height. Emission scenarios also have a significant impact on H+. In Figure 2 for the wind speed of 3 m/s for the S4 group, the H+ gradually increases as the emission levels increase from V1 (5.01 m/s) to V3 (26.15 m/s). Figure 3 shows selected simulation results for the stationary and moving source schemes for different flue gas exit temperatures. At a wind speed of 3 m/s, the H+ increased gradually for both schemes as the flue gas exit temperature increased from T1 (200 °C) to T3 (400 °C) in the S2-V2 group. The reason is that the larger the flue gas exit velocity and temperature, the larger the initial momentum and heat of the flue gas, and the stronger the anti-disturbance ability of the mixed air flow to the transversal wind above the outlet during the process of diffusing into the surrounding atmosphere, leading to the higher plume rising height. The effect of the ship speed on the H+ for the two schemes is, however, significantly different. For the V2 group in Figure 3, the H+ of the stationary source scheme gradually increased with an increase in the ship speed from S1 (2 knots) to S4 (14 knots), as the flue gas exit velocity of S1 is lower than that of S4. The H+ decreased and then increased with the minimum value of H+ at the ship speed S2 scenario (6 knots) for the moving source scheme.  Different parameters affect H + to different degrees and the same parameter affects H + to different degrees for different ship source schemes. The relative rate of change (R H+ ) in H + with these parameters was therefore calculated for the two modeled schemes (Figure 4). The R H+ was obtained by dividing the difference between the H + of the simulated and the reference scenario by the H + of the reference scenario. The H + of the emission scenario S2-V2-T2 with a wind speed of 3 m/s was used for the reference scenario. The R H+ varied from −100% to 0% for the stationary source scheme and from −90% to 0% for the moving source scheme as the wind speed increased from 3 m/s to 12 m/s. The range of R H+ for the stationary source scheme was approximately −20% to 780% as the ship speed increased from S1 to S4. As described in Section 2.2, the ship is stationary during this simulation and only the change in emission characteristics due to the change in ship speed is simulated. For the moving source scheme, the R H+ varied from 0% to 140%. When the flue gas exit velocity changed from V1 to V3, the range of change in R H+ was approximately −30% to 50% for the stationary source scheme and −60% to 100% for the moving source scheme. With an increase in flue gas exit temperature from T1 to T3, the R H+ varied from −20% to 30% for the stationary source scheme and from −30% to 30% for the moving source scheme. When these parameters are taken together, within their actual range of values, their influence on the H + of the stationary source simulation scheme is, in descending order, the ship speed, wind speed, flue gas exit velocity, and flue gas exit temperature. The large effect of the ship speed is highlighted by the high ship speed (S4). The effects of the ship speed, the wind speed, and the flue gas exit velocity are all relatively large for the moving source simulation scheme. The effects of these three are similar and only slightly larger than the effects of the flue gas exit temperature. When considering the R H+ for the two simulation schemes, it can be seen that all the parameters, except ship speed, are very similar in magnitude in both scenarios. The only significant difference is the result for ship speed.  Different parameters affect H+ to different degrees and the same parameter affects H+ to different degrees for different ship source schemes. The relative rate of change (RH+) in H+ with these parameters was therefore calculated for the two modeled schemes (Figure 4). The RH+ was obtained by dividing the difference between the H+ of the simulated and the reference scenario by the H+ of the reference scenario. The H+ of the emission scenario S2-V2-T2 with a wind speed of 3 m/s was used for the reference scenario. The RH+ varied from −100% to 0% for the stationary source scheme and from −90% to 0% for the moving source scheme as the wind speed increased from 3 m/s to 12 m/s. The range of RH+ for the stationary source scheme was approximately −20% to 780% as the ship speed increased from S1 to S4. As described in Section 2.2, the ship is stationary during this simulation and only the change in emission characteristics due to the change in ship speed is simulated. For the moving source scheme, the RH+ varied from 0% to 140%. When the flue gas exit velocity changed from V1 to V3, the range of change in RH+ was approximately −30% to 50% for the stationary source scheme and −60% to 100% for the moving source scheme. With an increase in flue gas exit temperature from T1 to T3, the RH+ varied from −20% to 30% for the stationary source scheme and from −30% to 30% for the moving source scheme. When these parameters are taken together, within their actual range of values, their influence on the H+ of the stationary source simulation scheme is, in descending order, the ship speed, wind speed, flue gas exit velocity, and flue gas exit temperature. The large effect of the ship speed is highlighted by the high ship speed (S4). The effects of the ship speed, the wind speed, and the flue gas exit velocity are all relatively large for the moving source simulation scheme. The effects of these three are similar and only slightly larger than the effects of the flue gas exit temperature. When considering the RH+ for the two simulation schemes, it can be seen that all the parameters, except ship speed, are very similar in magnitude in both scenarios. The only significant difference is the result for ship speed.

Smoke Plume Rising Height Difference between the Stationary Source and the Moving Source Simulation Schemes
The analysis initially revealed that the characteristics of the rising smoke plume in the case of a moving ship are significantly different from a stationary ship. The stationary source simulation scheme is taken as the reference in this section to further analyze the deviation between the results of the moving source scheme and the stationary source scheme. Here, the plume rising height of the stationary source scheme is subtracted from the moving source scheme for the same parameter settings (hereafter denoted as dH+). The following analysis remains combined with the results of typical scenarios due to the relatively large number of scenarios simulated. Figure 5 shows the dH+ at different wind speeds (for the V2-T2 group). The variation in

Smoke Plume Rising Height Difference between the Stationary Source and the Moving Source Simulation Schemes
The analysis initially revealed that the characteristics of the rising smoke plume in the case of a moving ship are significantly different from a stationary ship. The stationary source simulation scheme is taken as the reference in this section to further analyze the deviation between the results of the moving source scheme and the stationary source scheme. Here, the plume rising height of the stationary source scheme is subtracted from Atmosphere 2022, 13, 1507 9 of 21 the moving source scheme for the same parameter settings (hereafter denoted as dH + ). The following analysis remains combined with the results of typical scenarios due to the relatively large number of scenarios simulated. Figure 5 shows the dH + at different wind speeds (for the V2-T2 group). The variation in dH + with wind speed gradually increases as the ship speed increases. It shows that the difference between the two results at a 3 m/s wind speed becomes significant for S4, but this feature is not as prominent at higher wind speeds, especially at speeds of 12 m/s where the dH + is almost zero. In other words, the increase in ship speed would significantly increase the plume rising height at low wind speed, but when the wind speed is gradually increased, the promoting effect of the ship speed on the plume rising was weakened.

Smoke Plume Rising Height Difference between the Stationary Source and the Moving Source Simulation Schemes
The analysis initially revealed that the characteristics of the rising smoke plume in the case of a moving ship are significantly different from a stationary ship. The stationary source simulation scheme is taken as the reference in this section to further analyze the deviation between the results of the moving source scheme and the stationary source scheme. Here, the plume rising height of the stationary source scheme is subtracted from the moving source scheme for the same parameter settings (hereafter denoted as dH+). The following analysis remains combined with the results of typical scenarios due to the relatively large number of scenarios simulated. Figure 5 shows the dH+ at different wind speeds (for the V2-T2 group). The variation in dH+ with wind speed gradually increases as the ship speed increases. It shows that the difference between the two results at a 3 m/s wind speed becomes significant for S4, but this feature is not as prominent at higher wind speeds, especially at speeds of 12 m/s where the dH+ is almost zero. In other words, the increase in ship speed would significantly increase the plume rising height at low wind speed, but when the wind speed is gradually increased, the promoting effect of the ship speed on the plume rising was weakened. Figure 5. The rising height difference dH+ between the moving source scheme and the stationary source scheme at different wind speeds in the V2−T2 scenario. Figure 5. The rising height difference dH + between the moving source scheme and the stationary source scheme at different wind speeds in the V2−T2 scenario. Figure 6 shows the simulation results for the ship samples with different emission levels in the T2 scenario and low wind speed (3 m/s). Under the three ship speed scenarios S1, S2, and S3, dH + has a small variation with the increase in emission level. However, in the high ship speed scenario (S4), dH + decreases significantly with the increase in emission level, which means that the plume rising height of the moving source is significantly lower than that of the stationary source. Figure 7 shows the simulation results at different flue gas temperatures in the T2 scenario and low wind speed (3 m/s). It can be seen that the dH + variation in the T1 from T3 in the results from S1 to S3 are also similar, and only slightly different is the dH + of S3 from T2 to T3. In the results of group S4, the amplitude of dH + change with temperature increase is significantly different from that of the first three ship speeds.
The three dH + figures clearly show that wind speed and ship speed mainly influence dH + . At high wind speeds, specifically, the dH + is small for all emission scenarios; while at low wind speeds, the dH + is larger at high ship speeds and smaller at low ship speeds. All dH + values are small at low ship speeds, while at high ship speeds the dH + is larger at low wind speeds and small at high wind speeds. At both low wind speeds and high ship speeds, changes in the flue gas exit velocity or the flue gas exit temperature cause more significant changes in dH + . This is because the effects of the latter two parameters are effective at limited wind speeds and ship speeds, and are secondary influences. Figure 6 shows the simulation results for the ship samples with different emission levels in the T2 scenario and low wind speed (3 m/s). Under the three ship speed scenarios S1, S2, and S3, dH+ has a small variation with the increase in emission level. However, in the high ship speed scenario (S4), dH+ decreases significantly with the increase in emission level, which means that the plume rising height of the moving source is significantly lower than that of the stationary source.  Figure 7 shows the simulation results at different flue gas temperatures in the T2 scenario and low wind speed (3 m/s). It can be seen that the dH+ variation in the T1 from T3 in the results from S1 to S3 are also similar, and only slightly different is the dH+ of S3 from T2 to T3. In the results of group S4, the amplitude of dH+ change with temperature increase is significantly different from that of the first three ship speeds.  is significantly lower than that of the stationary source.  Figure 7 shows the simulation results at different flue gas temperatures in the T2 scenario and low wind speed (3 m/s). It can be seen that the dH+ variation in the T1 from T3 in the results from S1 to S3 are also similar, and only slightly different is the dH+ of S3 from T2 to T3. In the results of group S4, the amplitude of dH+ change with temperature increase is significantly different from that of the first three ship speeds.

The Flow Field Characteristics That Cause Differences in the Smoke Plume Rising Height
The dH + is strongly affected by wind speed and ship speed, especially at low wind speeds and high ship speeds. In these cases, the rising height of the smoke from the moving source simulation scheme is significantly smaller than from the stationary source simulation scheme. This difference between the two is, however, small at high wind speeds. Wind speed is an important parameter affecting smoke plume rising [40,49,50], with smoke plumes rising higher due to buoyancy in the low wind scenario. When the wind speed is high, the dynamic and buoyancy mechanisms for smoke rising become weak, causing small smoke rising heights. This effect is applicable to both stationary and moving sources, only the degree of the effect may vary. Section 3.1, for example, shows that the H + is small for both the simulation schemes at high wind speeds and therefore the corresponding dH + at high wind speeds is also small. This is also reflected in the flow field characteristics obtained from the numerical simulations. Figure 8c,d shows that the vertical velocity fields for the stationary and moving sources are very similar for wind speeds of 12 m/s. With a decrease in the wind speed, the dynamic and buoyant effects of the rising smoke increase. The lower the wind speed, the more the smoke rises. The dynamic and buoyant effects of the rising smoke from the moving ship compared to the stationary ship are reduced due to the high dispersion of flue gas. The lack of experimental studies on these aspects makes it necessary to use numerical simulations to illustrate the rising smoke plume. The vertical velocity behind the ship has a high value in the plume's path, indicating that the plume has a tendency to rise in this area. The vertical velocity of the stationary source results in a wind speed of 3 m/s (Figure 8a), which is much larger than a wind speed of 12 m/s (Figure 8c), due to enhanced kinetic and thermal rising. The vertical velocity of the moving source at this wind speed (Figure 8b) is much smaller than that of the stationary source due to the dispersion of the momentum, the heat release along the course of the movement, and the weakened contribution to plume rising.
When the wind speed is high, the dynamic and buoyancy mechanisms for smoke rising become weak, causing small smoke rising heights. This effect is applicable to both stationary and moving sources, only the degree of the effect may vary. Section 3.1, for example, shows that the H+ is small for both the simulation schemes at high wind speeds and therefore the corresponding dH+ at high wind speeds is also small. This is also reflected in the flow field characteristics obtained from the numerical simulations. Figure  8c,d shows that the vertical velocity fields for the stationary and moving sources are very similar for wind speeds of 12 m/s. With a decrease in the wind speed, the dynamic and buoyant effects of the rising smoke increase. The lower the wind speed, the more the smoke rises. The dynamic and buoyant effects of the rising smoke from the moving ship compared to the stationary ship are reduced due to the high dispersion of flue gas. The lack of experimental studies on these aspects makes it necessary to use numerical simulations to illustrate the rising smoke plume. The vertical velocity behind the ship has a high value in the plume's path, indicating that the plume has a tendency to rise in this area. The vertical velocity of the stationary source results in a wind speed of 3 m/s (Figure 8a), which is much larger than a wind speed of 12 m/s (Figure 8c), due to enhanced kinetic and thermal rising. The vertical velocity of the moving source at this wind speed (Figure 8b) is much smaller than that of the stationary source due to the dispersion of the momentum, the heat release along the course of the movement, and the weakened contribution to plume rising.  The higher the ship speed, the greater the difference between the rising height of the plume for both the moving source scheme and the stationary source. These simulation results are in line with the results of the theoretical analysis, since the ship movement itself is the key factor causing the difference between the plume rising height of the two schemes, and since both the dynamic and thermal mechanisms of the rising smoke are weakened when the ship moves. The specific reasons for this characteristic of dH + can be analyzed together with the numerical simulation results of the flow field. Figure 9 shows that the vertical velocity and the extent of the region behind the moving ship where the smoke rises are much smaller than those behind the stationary ship at higher speeds (S3 and S4). The average height of the high-value area of the vertical velocity of the stationary source is also higher than that of the moving source, which leads to a larger dH + being statistically obtained at higher ship speeds as well. The difference between the two simulations is also the same for the lower ship speeds (S1 and S2). In this case, the difference is, however, much less significant than for the higher ship speeds. The higher the ship speed is, the greater the difference between the flow field behind the moving ship and the stationary ship, which causes a correspondingly greater dH + . speeds (S3 and S4). The average height of the high-value area of the vertical velocity of the stationary source is also higher than that of the moving source, which leads to a larger dH+ being statistically obtained at higher ship speeds as well. The difference between the two simulations is also the same for the lower ship speeds (S1 and S2). In this case, the difference is, however, much less significant than for the higher ship speeds. The higher the ship speed is, the greater the difference between the flow field behind the moving ship and the stationary ship, which causes a correspondingly greater dH+. Ship movement includes both exhaust outlet movement and hull movement that all influence the differences in results between the moving source scheme and the stationary source scheme. Numerical experiments were carried out to simulate these two factors separately to further understand the actual effect of these two factors on the dH+. Figure 10 shows the numerical simulation result of only the exhaust outlet movement. The patterns and values of the vertical velocity fields are relatively similar for both sets when comparing them with the simulation results for the moving source in Figure 9. This indicates that of the two movement-related factors, the central factor affecting the flue gas rising for the moving source scheme and the dH+ for both schemes is the movement of the exhaust outlet. Moving the exhaust outlet has a greater effect than moving the hull. Even though the exit velocity is greater at higher ship speeds, the initial Ship movement includes both exhaust outlet movement and hull movement that all influence the differences in results between the moving source scheme and the stationary source scheme. Numerical experiments were carried out to simulate these two factors separately to further understand the actual effect of these two factors on the dH + . Figure 10 shows the numerical simulation result of only the exhaust outlet movement. The patterns and values of the vertical velocity fields are relatively similar for both sets when comparing them with the simulation results for the moving source in Figure 9. This indicates that of the two movement-related factors, the central factor affecting the flue gas rising for the moving source scheme and the dH + for both schemes is the movement of the exhaust outlet. Moving the exhaust outlet has a greater effect than moving the hull. Even though the exit velocity is greater at higher ship speeds, the initial momentum and dispersive release of the initial heat due to exhaust outlet movement have a greater overall effect. The effect of the hull movement is however also noteworthy. The results in Section 3.1 show that the smoke rising height of a moving ship first decreases and then increases with an increase in ship speed (Figure 4b). Figures 9 and 10 show that the vertical velocity of S1 is overall slightly higher than that of S2. The vertical velocity field near the hull, however, (Figure 11), shows a negative region near the hull due to the movement of the ship, which increases with increasing ship speed. The smoke plume rising height decreases in this negative area. Even though the downwash of smoke near the hull is stronger at high ship speeds than at low ship speeds for the ship speeds S2 to S4, high ship speeds have a stronger rising effect in the area behind the ship. The smoke rising height, therefore, increases significantly due to the increase in ship speed (Figure 4b). The plume rising height of the S1 to S2 section in Figure 4b decreases, which may be due to the greater downwash caused by the hull at S2 than at S1 (Figure 11). speed. The smoke plume rising height decreases in this negative area. Even though the downwash of smoke near the hull is stronger at high ship speeds than at low ship speeds for the ship speeds S2 to S4, high ship speeds have a stronger rising effect in the area behind the ship. The smoke rising height, therefore, increases significantly due to the increase in ship speed (Figure 4b). The plume rising height of the S1 to S2 section in Figure 4b decreases, which may be due to the greater downwash caused by the hull at S2 than at S1 (Figure 11).  The effect of the dispersed release of the flue gas momentum and the heat in the moving source ship simulation scenario was mentioned several times in the previous analysis and discussion. Figures 12 and 13 show the relevant simulation results for the effects caused by heat dispersion. Figure 12 shows that the moving source heat release is dispersed, and that the moving source scheme achieves temperature equilibrium with near the hull due to the movement of the ship, which increases with increasing ship speed. The smoke plume rising height decreases in this negative area. Even though the downwash of smoke near the hull is stronger at high ship speeds than at low ship speeds for the ship speeds S2 to S4, high ship speeds have a stronger rising effect in the area behind the ship. The smoke rising height, therefore, increases significantly due to the increase in ship speed (Figure 4b). The plume rising height of the S1 to S2 section in Figure 4b decreases, which may be due to the greater downwash caused by the hull at S2 than at S1 (Figure 11).  The effect of the dispersed release of the flue gas momentum and the heat in the moving source ship simulation scenario was mentioned several times in the previous analysis and discussion. Figures 12 and 13 show the relevant simulation results for the effects caused by heat dispersion. Figure 12 shows that the moving source heat release is dispersed, and that the moving source scheme achieves temperature equilibrium with Figure 11. The vertical velocity contours near the hull in the V2−T2 scenario with wind speeds of 3 m/s: (a-d) are S1, S2, S3, and S4 scenarios, respectively.
The effect of the dispersed release of the flue gas momentum and the heat in the moving source ship simulation scenario was mentioned several times in the previous analysis and discussion. Figures 12 and 13 show the relevant simulation results for the effects caused by heat dispersion. Figure 12 shows that the moving source heat release is dispersed, and that the moving source scheme achieves temperature equilibrium with the ambient air within a relatively small range after the hot flue gas is emitted compared to the stationary source scenario. The contribution of the thermal buoyancy effects to the vertical velocity is, therefore, smaller in value ( Figure 13).

Simplified Calculation Methods for Simulating the Rising Smoke Plume of a Moving Ship with a Stationary Source Scheme
The effective height of the rising source plume is an important factor affecting the ambient concentration and distribution of pollutants. The uplift formula commonly used in the dispersion simulations is only applicable to stationary sources and not to moving sources [19,51]. The influence of the ship movement is therefore usually not considered in modeling studies of exhaust pollutants from moving sources on ships [20,52,53]. To obtain more accurate simulation results with limited computational cost, this study, therefore, attempts to establish a simplified method for approximating the rising plume from a moving ship using a stationary source simulation scheme. the ambient air within a relatively small range after the hot flue gas is emitted compared to the stationary source scenario. The contribution of the thermal buoyancy effects to the vertical velocity is, therefore, smaller in value ( Figure 13).

Simplified Calculation Methods for Simulating the Rising Smoke Plume of a Moving Ship with a Stationary Source Scheme
The effective height of the rising source plume is an important factor affecting the ambient concentration and distribution of pollutants. The uplift formula commonly used in the dispersion simulations is only applicable to stationary sources and not to moving sources [19,51]. The influence of the ship movement is therefore usually not considered in modeling studies of exhaust pollutants from moving sources on ships [20,52,53]. To obtain more accurate simulation results with limited computational cost, this study, therefore, attempts to establish a simplified method for approximating the rising plume from a moving ship using a stationary source simulation scheme.
When the ship is in motion, especially at high speeds, both the dynamic rising effect and the thermal rising effect are weaker due to the dispersed release of the momentum and heat from the flue gases. This results in lower plume rising for moving ships than for stationary sources. The kinetic and thermal effects of the flue gas emissions are directly related to the flue gas exit velocity and the flue gas exit temperature of the ships. the ambient air within a relatively small range after the hot flue gas is emitted compared to the stationary source scenario. The contribution of the thermal buoyancy effects to the vertical velocity is, therefore, smaller in value ( Figure 13).

Simplified Calculation Methods for Simulating the Rising Smoke Plume of a Moving Ship with a Stationary Source Scheme
The effective height of the rising source plume is an important factor affecting the ambient concentration and distribution of pollutants. The uplift formula commonly used in the dispersion simulations is only applicable to stationary sources and not to moving sources [19,51]. The influence of the ship movement is therefore usually not considered in modeling studies of exhaust pollutants from moving sources on ships [20,52,53]. To obtain more accurate simulation results with limited computational cost, this study, therefore, attempts to establish a simplified method for approximating the rising plume from a moving ship using a stationary source simulation scheme.
When the ship is in motion, especially at high speeds, both the dynamic rising effect and the thermal rising effect are weaker due to the dispersed release of the momentum and heat from the flue gases. This results in lower plume rising for moving ships than for stationary sources. The kinetic and thermal effects of the flue gas emissions are directly related to the flue gas exit velocity and the flue gas exit temperature of the ships. When the ship is in motion, especially at high speeds, both the dynamic rising effect and the thermal rising effect are weaker due to the dispersed release of the momentum and heat from the flue gases. This results in lower plume rising for moving ships than for stationary sources. The kinetic and thermal effects of the flue gas emissions are directly related to the flue gas exit velocity and the flue gas exit temperature of the ships. To approximate the attenuating effect of the flue gas dynamic rising and the thermal rising, two correction schemes were considered. These included correcting the flue gas exit velocity or the flue gas exit temperature. The aim was to correct the smoke plume rising height of the stationary source simulation scheme at the flue gas exit velocity (V exit ) or the flue gas exit temperature (T ) equal to or close to the smoke plume rising height of the moving source simulation scheme at the actual flue gas exit velocity (V exit ) or the actual flue gas exit temperature (T).
The dH + results obtained in the above scenario of a higher ship speed and a lower wind speed (ship speed ≥ 10 knots and wind speed ≤ 6 m/s), were used in a stepwise regression fitting with wind speed (V wind ), ship speed (V ship ), flue gas exit velocity (V exit ), and flue gas exit temperature (T) as independent variables. This yielded the following correction equations for V exit (Equation (1)) or T (Equation (2)): (1) where V exit is the corrected flue gas exit velocity in m/s; V exit is the actual flue gas exit velocity in m/s; V wind is the wind speed in m/s; V ship is the ship speed in knots; T is the actual flue gas exit temperature in • C; and T is the corrected flue gas exit temperature in • C. For the last step of the stepwise regression fitting, the R 2 for Equation (1) is 0.77 and the R 2 for Equation (2) is 0.99. The effects of the two corrected methods were compared. To do this, the corrected parameter values were used to simulate the stationary source scheme for 20 CFD model cases in this study for the low wind speed and high ship speed scenarios. Then the modified stationary source scheme was compared with the moving source scheme for the plume's rising heights. Table 4 shows the case parameters, together with the corrected flue gas exit velocity and flue gas exit temperature. The tested cases cover different combinations of flue gas exit velocity and flue gas temperature for high ship speed and low wind speed conditions. Figure 14 shows the approximate simulated plume rising heights at 1 km downwind for the stationary source scheme compared to the moving source scheme. These cases were introduced in Section 2, therefore, the stationary source scheme results shown in Section 3.1 are also compared in Figure 14 (i.e., the group without correction).  The relative error (R dH+ ) between the moving source simulation and the stationary source simulation was calculated to quantitatively assess the effect of the correction methods. This was done by taking H + at 100 m intervals within 1 km behind the chimney for each simulation scheme, and was calculated as follows: where S i and M i are the stationary source ship plume rising height and the moving source ship plume rising height. Table 4 presents the statistical results, where R dH+ is the mean of 10 R dH+ values calculated for each simulation scheme using Equation (3). An R dH+ greater than 0 means that the H + of the stationary source simulation scheme is generally higher than the moving source simulation scheme, while the opposite is lower than the H + of the moving source simulation scheme. The closer the absolute value of R dH+ is to zero, the closer the H + of the stationary source simulation is to that of the moving source simulation. For 20 validation cases, the average of R dH+ for the three stationary source simulations (without correction, corrected V exit , and corrected T ) were 135.38%, 5.48%, and 60.07%, respectively. The average of R dH+ with both the corrected V exit and the T were lower than the R dH+ without correction, while the average of R dH+ with the corrected V exit was lower than that with the corrected T . For the results of the two correction schemes, the results with the V exit correction are slightly better than those with the T correction.
The simulation time of the simulation experiment was found to be greatly reduced by using the stationary source scheme to approximate the calculation of the smoke plume rising height of the moving source ship. The simulation results of the validation cases reveal that the approximate simulation results are similar to those from the moving source scheme. These simulation results are expected to be used to improve the problem of the underestimation of atmospheric pollutants in the mesoscale model simulations of ships, specifically the V exit correction scheme (shown in Equation (1)). By using this correction scheme, the simultaneous correction of the flue gas exit velocity and the flue gas exit temperature is also feasible. Since both these parameters affect the rising height of the smoke plume, there would be an infinite number of parameter combination options for a simultaneous correction. The simultaneous correction was therefore not considered in this study.

Conclusions
To understand the smoke plume rising characteristics of a moving ship, this study simulated the smoke plume characteristics of the moving ship by using parameterized values in the CFD software PHOENICS 6.0. The rising smoke plume characteristics were simulated and analyzed for the stationary source scheme and the moving source scheme. The relative variation in the simulation results of the moving source scheme was analyzed using the simulation results of the stationary source scheme. Finally, simplified calculation methods were established to approximate the rising smoke plume of the moving ship using the stationary source scheme parameters.
The main parameters affecting the rising smoke plume of the moving ships include the ship speed, the environmental wind speed, the flue gas exit velocity, and the flue gas exit temperature. For the two simulation schemes (stationary source and moving source), the plume rising height decreased with an increase in wind speed and increased with an increase in the flue gas exit velocity and the flue gas exit temperature. The difference between the two is reflected in the results of the different ship speeds. In the stationary source scheme, the plume's rising height increases with an increase in ship speed. In the moving source scheme, the plume's rising height first decreases and then increases with an increase in ship speed. The lowest value appears when the ship speed is 6 knots. The wind speed and the ship speed mainly influence the plume rising height difference between the stationary source and the moving source simulation schemes.
This study used simplified calculation methods to approximate the plume rising height of a moving ship using a stationary source simulation scheme. Stepwise regression fitting was used to determine the corrected flue gas exit velocity (V exit ) and the corrected flue gas exit temperature (T ). For the validation cases, the average relative error of the stationary source simulation scheme without correction, the stationary source scheme with corrected V exit , and the stationary source scheme with corrected T versus the moving source scheme were 135.38%, 5.48%, and 60.07%, respectively. These two correction methods can potentially improve the modeled underestimation of air pollutant emissions from moving ships in the mesoscale model, with the corrected V exit method being more effective.
Future work plans to carry out field experimentation in more different ports based on the results of this exploratory study on the plume rising height of moving ships, and use more ship cases to validate the plume rising height correction formulas proposed in this study. We plan to compare the simulation results with the field experimentation results to further study the mechanism of the plume rising of moving ships, hoping to provide some reference for the study of plume dispersion of moving ships at port.